Abstract
We show that the principle of coherent control of chemical reactions can be implemented, in a two pulse sequence, to control the relative yield of reaction products in unimolecular dissociation. Experimental control parameters in this implementation are seen to be the intensity of the pulses and the delay time between them, with required delay times in the experimentally accessible picosecond range. As an example, application is made to control the production of D+H2 vs HD+H in the dissociation of a model collinear molecule with DH2 masses. In addition, plots of the evolving superposition state are presented in order to emphasize relevant characteristics of excitation with slow pulses.
Sign-in/Register to access full text options 
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a callDisclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.
