Abstract
Elastomers provide excellent damping performance owing to their unique viscoelasticity, which are widely used as vibration and noise reduction materials. However, conventional rubber-based elastomers with a low glass transition temperature (Tg) and narrow damping range are difficult to adapt to room-temperature conditions. Additionally, most of petroleum-based elastomers hinder the sustainable development. In this work, a series of novel polyurethane elastomers was synthesized using carbon-fixed CO2-based polycarbonate propylene diol (PPCD). The impact of hard segment (HS) content on the thermal, mechanical, and damping properties of CO2-based polyurethane (PU) was comprehensively investigated. Increasing the HS content from 16 % to 44 % increased the Tg from −3.8 °C to 21.7 °C, covering the entire damping range at room temperature with an adjustable damping performance. Furthermore, the tensile strength increased from 7.2 MPa to 27.0 MPa. The synthesis of CO2-based PU can propel the utilization of PU in damping applications, enabling sustainable advancement of the PU industry.
Published Version
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