Abstract

HighlightsPrecise exfoliation and modification of nano-Tellurium was realized by adopting a room-temperature ionic liquid as the electrolyte.Nano-Tellurium with high-entropy morphology can offer greater solar absorption and more kinds of surface chemical groups, giving rise to superior photothermal properties.Nano-Tellurium-poly(vinyl alcohol)-based photothermal foam hydrogels, with high compressibility, excellent water transport rate and low evaporation enthalpy of water, combined with a new heat-supply model, achieve an evaporation rate of 4.11 kg m−2 h−1 with energy efficiencies up to 128% under 1 sun irradiation, which are the highest values for semiconductor-based nanocomposites reported so far.

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