Abstract

We measured black carbon (BC) with a seven-wavelength aethalometer (AE-31) at the Nam Co Lake (NCL), the hinterland of the Tibetan Plateau (TP) from May 2015 to April 2016. The daily average concentration of BC was 145 ± 85 ng m−3, increasing by 50% since 2006. The seasonal variation of BC shows higher concentrations in spring and summer and lower concentrations in autumn and winter, dominated by the adjacent sources and meteorological conditions. The diurnal variation of BC showed that its concentrations peaked at 9:00–16:00 (UTC + 8), significantly related to local human activities (e.g., animal-manure burning and nearby traffic due to the tourism industry). The concentration-weighted trajectory (CWT) analysis showed that the long-distance transport of BC from South Asia could also be a potential contributor to BC at the NCL, as well as the biomass burning by the surrounding residents. The analyses of the absorption coefficient and absorption Ångström exponent show the consistency of sourcing the BC at the NCL. We suggest here that urgent measures should be taken to protect the atmospheric environment at the NCL, considering the fast-increasing concentrations of BC as an indicator of fuel combustion.

Highlights

  • Black carbon (BC) has a vital role in the earth’s climate system and energy budget

  • Compared with a decade ago [12], the average concentration of BC increased by 50%

  • BC was measured by a seven-wavelength aethalometer (AE-31) at the Nam Co Lake (NCL), the Tibetan Plateau (TP)

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Summary

Introduction

Black carbon (BC) has a vital role in the earth’s climate system and energy budget. BC is produced by the incomplete combustion of biomass, coal, and diesel fuels. BC causes atmospheric heating and alters cloud formation processes [1], which is estimated to be the second most important agent of global warming after CO2 [2,3]. BC deposited on ice and snow surfaces has been proven to reduce surface albedo by absorbing more solar radiation, which may accelerate glacier melting and result in changes in glaciers [4,5]. BC plays a major role in climate change, and has negative influences on human health [6]

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