Impacts of atmospheric transport and biomass burning on the inter-annual variation in black carbon aerosols over the Tibetan Plateau

Abstract

<p>Atmospheric black carbon (BC) in the Tibetan Plateau (TP) can largely impact regional and global climate. Applying a backward-trajectory method that combines BC concentrations from a global chemical transport model, GEOS-Chem, and trajectories from the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model, we assess the contributions of worldwide source regions to surface BC in the TP. We estimate that on a 20-year average (1995-2014), 77% of surface BC in the TP comes from South Asia (43%) and East Asia (35%). In terms of the amount of BC imported, South Asia and East Asia are dominant source regions in winter and summer, respectively. However, in terms of affected areas in the TP, South Asia is the dominant contributor throughout the year. Inter-annually, surface BC over the TP is largely modulated by atmospheric transport of BC from non-local regions year-round and by biomass burning in South Asia, mostly in spring. We find that the extremely strong biomass burning in South Asia in the spring of 1999 greatly enhanced surface BC concentrations in the TP (31% relative to the climatology). The strength of the Asian monsoon correlates significantly with the inter-annual variation in the amount of BC transported to the TP from non-local regions. In summer, a stronger East Asian summer monsoon and a South Asian summer monsoon tend to, respectively, lead to more BC transport from central China and north-eastern South Asia to the TP. In winter, BC transport from central China is enhanced in years with a strong East Asian winter monsoon or a Siberian High.</p>