Abstract
A comparison of the molecular structures of the five-co-ordinate bis(imido) and imido alkylidene molybdenum complexes [Mo(NC6H3Pri2-2,6)(L)(L′)], where L is a tridentate pyridinediolato ligand and L′ is either NC6H3Pri2-2,6 or CHCMe2Ph, strongly supports the notion that the nitrogen of the bent imido ligand in the bis(imido) complex is sp2-hybridised.
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