Abstract

Traditional real-time air quality monitoring instruments are expensive to install and maintain; therefore, such existing air quality monitoring networks are sparsely deployed and lack the measurement density to develop high-resolution spatiotemporal air pollutant maps. More recently, low-cost sensors have been used to collect high-resolution spatial and temporal air pollution data in real-time. In this paper, for the first time, Envirowatch E-MOTEs are employed for air quality monitoring as a case study in Sheffield. Ten E-MOTEs were deployed for a year (October 2016 to September 2017) monitoring several air pollutants (NO, NO2, CO) and meteorological parameters. Their performance was compared to each other and to a reference instrument installed nearby. E-MOTEs were able to successfully capture the temporal variability such as diurnal, weekly and annual cycles in air pollutant concentrations and demonstrated significant similarity with reference instruments. NO2 concentrations showed very strong positive correlation between various sensors. Mostly, correlation coefficients (r values) were greater than 0.92. CO from different sensors also had r values mostly greater than 0.92; however, NO showed r value less than 0.5. Furthermore, several multiple linear regression models (MLRM) and generalised additive models (GAM) were developed to calibrate the E-MOTE data and reproduce NO and NO2 concentrations measured by the reference instruments. GAMs demonstrated significantly better performance than linear models by capturing the non-linear association between the response and explanatory variables. The best GAM developed for reproducing NO2 concentrations returned values of 0.95, 3.91, 0.81, 0.005 and 0.61 for factor of two (FAC2), root mean square error (RMSE), coefficient of determination (R2), normalised mean biased (NMB) and coefficient of efficiency (COE), respectively. The low-cost sensors offer a more affordable alternative for providing real-time high-resolution spatiotemporal air quality and meteorological parameter data with acceptable performance.

Highlights

  • With an increasing trend towards urbanisation due to better job opportunities and greater access to amenities and facilities in cities, urban areas are expanding rapidly globally

  • The best generalised additive models (GAM) developed for reproducing NO2 concentrations returned values of 0.95, 3.91, 0.81, 0.005 and 0.61 for factor of two (FAC2), root mean square error (RMSE), coefficient of determination (R2), normalised mean biased (NMB) and coefficient of efficiency (COE), respectively

  • Various air pollutant concentrations showed a similar pattern at different monitoring sites during different seasons, for instance, NO2 concentration was higher in winter months and lower in summer

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Summary

Introduction

With an increasing trend towards urbanisation due to better job opportunities and greater access to amenities and facilities in cities, urban areas are expanding rapidly globally. The low-cost sensors use the latest microsensing technology and are considered the innovative tools for air quality monitoring in the future (Castell et al 2015; Snyder et al 2013; Kumar et al 2015; Stojanovic et al 2015) Data collected by these sensors can be used for detailed spatial and temporal mapping of air pollution, especially over distinct areas such as city or an urban district, for atmospheric model validation and assessing population exposure; the data need to be handle with caution and several corrections need to be applied first

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