Abstract
A novel pump-probe method has been developed to study anisotropic relaxation and energy transfer in excited states of polyatomic molecules excited by femtosecond laser pulses. The method was used to study the rotational diffusion of NADH with a temporal resolution of about 0.6 ps. For the first time, absorption from the excited state of biological molecules pumped by laser pulses with energies of 1 nJ was detected
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