Zero-point Fluctuations Research Articles

Optomechanical sideband asymmetry explained by stochastic electrodynamics

Within the framework of stochastic electrodynamics we derive the noise spectrum of a laser beam reflected from a suspended mirror. The electromagnetic field follows Maxwell's equations and is described by a deterministic part that accounts for the laser field and a stochastic part that accounts for thermal and zero-point background fluctuations.Likewise, the mirror motion satisfies Newton's equation of motion and is composed of deterministic and stochastic parts, similar to a Langevin equation. We consider a photodetector that records the power of the field reflected from the mirror interfering with a frequency-shifted reference beam (heterodyne interferometry). We theoretically show that the power spectral density of the photodetector signal is composed of four parts: (i) a deterministic term with beat notes, (ii) shot noise, (iii) the actual heterodyne signal of the mirror motion and (iv) a cross term resulting from the correlation between measurement noise (shot noise) and backaction noise (radiation pressure shot noise). The latter gives rise to the Raman sideband asymmetry observed with ultracold atoms, cavity optomechanics and with levitated nanoparticles. Our classical theory fully reproduces experimental observations and agrees with the results obtained by a quantum theoretical treatment.

Spontaneous symmetry breaking in frustrated triangular atom arrays due to cooperative light scattering

We demonstrate the presence of an optical phase transition with frustration-induced spontaneous symmetry breaking in a triangular planar atomic array due to cooperative light-mediated interactions. We show how the array geometry of triangle unit cells at low light intensities leads to degenerate collective radiative excitations forming nearly flat bands. We drive degenerate pairs of collective excitations to be equally populated in both cases of the atomic polarization in the lattice plane and perpendicular to it. At higher intensities, above specific threshold values, this symmetry in the populations is spontaneously broken. We also develop an effective few-mode model that provides semianalytic descriptions of the symmetry-breaking threshold and infinite-lattice limit phase transition. Surprisingly, we find how excitations due to dipolar interactions correspond to optical analogs of those found in frustrated magnets and superfluids, with closely related symmetry-breaking mechanisms despite the significant physical differences between these systems, opening potential for simulating even quantum magnetism. Transmitted light through the array conveys information about symmetry breaking in the hysteresis behavior of the spectrum. Moreover, in a Mott-insulator state, the atomic positions are subject to zero-point quantum fluctuations. Interpreting each stochastic realization as a light-induced quantum measurement of the atomic position configuration, we find how strong nonlinearities and even weak position uncertainties lead to considerable measurement-induced symmetry breaking, while ensemble-averaging over many realizations restores the original symmetry and the unbroken state. Larger position uncertainty results in the formation of domains of different broken symmetries.

Bubble nucleation and quantum initial conditions in classical statistical simulations

Classical-statistical lattice simulations provide a useful approximation to out-of-equilibrium quantum field theory, but only for systems exhibiting large occupation numbers, and only for phenomena that are not intrinsically quantum mechanical in nature. In certain special circumstances, it can be appropriate to initialize such real-time simulations with quantum-like zero-point fluctuations. We will revisit these points, and investigate reports that quantum bubble nucleation rates in 1+1 dimensions can be computed through the classical evolution of such a quantum-like initial condition [1]. We find that although intriguing, the reported numerical agreement between classical-statistical simulations and the quantum nucleation rate in 1+1 dimensions is a coincidence, which is not specific to this choice of initialisation, is parameter and lattice cut-off dependent and disappears as the number of space-dimensions increases from 1+1 to 2+1.

Analyzing quantum synchronization through Bohmian trajectories

We analyze quantum effects involved in continuous variable synchronization between two self-sustaining resonators in the framework of Bohmian mechanics. Bohmian trajectories provide visual descriptions of significant nonclassical dynamics, which allow us to characterize the level of quantum synchronization more intuitively compared with only utilizing some designed synchronization measures. It is found that in the quantum limit, the Bohmian trajectories will deviate from their corresponding semiclassical limit cycle behavior after they are distorted by the quantum potential. We explore the roles of zero-point fluctuation, superposition, and nonlocal correlation in synchronization dynamics, corresponding to the oscillators in a coherent state, superposition state, and entanglement state, respectively. We also explore the influence of squeezed Hamiltonian on spontaneous synchronization.

Recent developments on the Casimir torque

The Casimir force acts on nearby surfaces due to zero-point fluctuations of the quantum electromagnetic field. In the nonretarded limit, the interaction is also known as the van der Waals force. When the electromagnetic response of the surfaces is anisotropic, a torque may act on the surfaces. Here, we review the literature and recent developments on the Casimir torque. The theory of the Casimir torque is discussed in an explicit example for uniaxial birefringent plates. Recent theoretical predictions for the Casimir torque in various configurations are presented. A particular emphasis is made on experimental setups for measuring the Casimir torque.

Coarse-grained intermolecular interactions on quantum processors

Variational quantum algorithms (VQAs) are increasingly being applied in simulations of strongly bound (covalently bonded) systems using full molecular orbital basis representations. The application of quantum computers to the weakly bound intermolecular and noncovalently bonded regime, however, has remained largely unexplored. In this work, we develop a coarse-grained representation of the electronic response that is ideally suited for determining the ground state of weakly interacting molecules using a VQA. We require qubit numbers that grow linearly with the number of molecules and derive scaling behavior for the number of circuits and measurements required, which compare favorably to traditional variational quantum eigensolver methods. We demonstrate our method on IBM superconducting quantum processors and show its capability to resolve the dispersion energy as a function of separation for a pair of nonpolar molecules---thereby establishing a means by which quantum computers can model Van der Waals interactions directly from zero-point quantum fluctuations. Within this coarse-grained approximation, we conclude that current-generation quantum hardware is capable of probing energies in this weakly bound but nevertheless chemically ubiquitous and biologically important regime. Finally, we perform experiments on simulated and real quantum computers for systems of three, four, and five oscillators as well as oscillators with anharmonic onsite binding potentials; the consequences of the latter are unexamined in large systems using classical computational methods but can be incorporated here with low computational overhead.

Vortex lattices in binary Bose–Einstein condensates: collective modes, quantum fluctuations, and intercomponent entanglement

We study binary Bose–Einstein condensates subject to synthetic magnetic fields in mutually parallel or antiparallel directions. Within the mean-field theory, the two types of fields have been shown to give the same vortex-lattice phase diagram. We develop an improved effective field theory to study properties of collective modes and ground-state intercomponent entanglement. Here, we point out the need to introduce renormalized coupling constants for coarse-grained densities. We show that the low-energy excitation spectra for the two types of fields are related to each other by suitable rescaling with the renormalized coupling constants. By calculating the entanglement entropy, we find that for an intercomponent repulsion (attraction), the two components are more strongly entangled in the case of parallel (antiparallel) fields, in qualitative agreement with recent studies for a quantum (spin) Hall regime. We also find that the entanglement spectrum exhibits an anomalous square-root dispersion relation, which leads to a subleading logarithmic term in the entanglement entropy. All of these are confirmed by numerical calculations based on the Bogoliubov theory with the lowest-Landau-level approximation. Finally, we investigate the effects of quantum fluctuations on the phase diagrams by calculating the correction to the ground-state energy due to zero-point fluctuations in the Bogoliubov theory. We find that the boundaries between rhombic-, square-, and rectangular-lattice phases shift appreciably with a decrease in the filling factor.

Chemistry under Vibrational Strong Coupling.

Over the past decade, the possibility of manipulating chemistry and material properties using hybrid light-matter states has stimulated considerable interest. Hybrid light-matter states can be generated by placing molecules in an optical cavity that is resonant with a molecular transition. Importantly, the hybridization occurs even in the dark because the coupling process involves the zero-point fluctuations of the optical mode (a.k.a. vacuum field) and the molecular transition. In other words, unlike photochemistry, no real photon is required to induce this strong coupling phenomenon. Strong coupling in general, but vibrational strong coupling (VSC) in particular, offers exciting possibilities for molecular and, more generally, material science. Not only is it a new tool to control chemical reactivity, but it also gives insight into which vibrations are involved in a reaction. This Perspective gives the underlying fundamentals of light-matter strong coupling, including a mini-tutorial on the practical issues to achieve VSC. Recent advancements in "vibro-polaritonic chemistry" and related topics are presented along with the challenges for this exciting new field.

Particle creation in the spin modes of a dynamically oscillating two-component Bose-Einstein condensate

We investigate the parametric amplification of the zero-point fluctuations in the spin modes of a two-component Bose-Einstein condensate, triggered by the dynamical evolution of the condensate density. We first make use of a Thomas-Fermi approximation to develop a tractable theoretical model of the quantum dynamics of the Bogoliubov excitations in a harmonically trapped condensate with a time-dependent trapping frequency. The predictions of this model are then compared to an ab-initio numerical study of the correlation functions of density and spin fluctuations for general spatially inhomogeneous configurations. Results are shown for the two cases of expanding and oscillating condensates: while the quantum excitation of spin modes remains weak and relatively featureless in the case of an expanding condensate, clear and experimentally promising signatures of particle creation are anticipated for the oscillating case under suitable resonance conditions between the density and the spin modes.

Sub-Kelvin Feedback Cooling and Heating Dynamics of an Optically Levitated Librator.

Rotational optomechanics strives to gain quantum control over mechanical rotors by harnessing the interaction of light and matter. We optically trap a dielectric nanodumbbell in a linearly polarized laser field, where the dumbbell represents a nanomechanical librator. Using measurement-based parametric feedback control in high vacuum, we cool this librator from room temperature to 240mK and investigate its heating dynamics when released from feedback. We exclude collisions with residual gas molecules as well as classical laser noise as sources of heating. Our findings indicate that we observe the torque fluctuations arising from the zero-point fluctuations of the electromagnetic field.

Real-time optimal quantum control of mechanical motion at room temperature.

The ability to accurately control the dynamics of physical systems by measurement and feedback is a pillar of modern engineering1. Today, the increasing demand for applied quantum technologies requires adaptation of this level of control to individual quantum systems2,3. Achieving this in an optimal way is a challenging task that relies on both quantum-limited measurements and specifically tailored algorithms for state estimation and feedback4. Successful implementations thus far include experiments on the level of optical and atomic systems5-7. Here we demonstrate real-time optimal control of the quantum trajectory8 of an optically trapped nanoparticle. We combine confocal position sensing close to the Heisenberg limit with optimal state estimation via Kalman filtering to track the particle motion in phase space in real time with a position uncertainty of 1.3times the zero-point fluctuation. Optimal feedback allows us to stabilize the quantum harmonic oscillator to a mean occupation of 0.56±0.02quanta, realizing quantum ground-state cooling from room temperature. Our work establishes quantum Kalman filtering as a method to achieve quantum control of mechanical motion, with potential implications for sensing on all scales. In combination with levitation, this paves the way to full-scale control over the wavepacket dynamics of solid-state macroscopic quantum objects in linear and nonlinear systems.

Quantum analysis of second-order effects in superconducting travelling-wave parametric amplifiers

We have performed a quantum mechanical analysis of travelling-wave parametric amplifiers (TWPAs) in order to investigate five experimental phenomena related to their operations, namely the effect of impedance mismatch, the presence of upper idler modes, the presence of quantum and thermal noise, the generation of squeezed states, and the preservation of pre-squeezed states during amplification. Our analysis uses momentum operators to describe the spatial evolution of quantised modes along a TWPA. We calculate the restriction placed on pump amplitude as well as amplifier gain as a result of impedance mismatch between a TWPA and its external system. We apply our analysis to upper idler modes and demonstrate that they will result in suppressed gain. We show that an ideal TWPA is indeed quantum-limited—i.e. it introduces a half-quantum of zero-point fluctuation which is the minimum possible noise contribution for a phase-preserving linear amplifier. We analyse the thermal noise associated with a TWPA by considering the effect of distributed sources along an amplifier transmission line. Our analysis predicts a doubling of thermal noise in the high gain limit as a result of wave-mixing between signal and idler modes. We study the operation of a TWPA in the presence of a DC bias current, and have shown that highly squeezed states can in principle be generated. However, amplifying a pre-squeezed state using a non-degenerate TWPA generally reduces the squeezing advantage.

Bremsstrahlung of Light through Spontaneous Emission of Gravitational Waves

Zero-point fluctuations are a universal consequence of quantum theory. Vacuum fluctuations of electromagnetic field have provided crucial evidence and guidance for QED as a successful quantum field theory with a defining gauge symmetry through the Lamb shift, Casimir effect, and spontaneous emission. In an accelerated frame, the thermalisation of the zero-point electromagnetic field gives rise to the Unruh effect linked to the Hawking effect of a black hole via the equivalence principle. This principle is the basis of general covariance, the symmetry of general relativity as the classical theory of gravity. If quantum gravity exists, the quantum vacuum fluctuations of the gravitational field should also lead to the quantum decoherence and dissertation of general forms of energy and matter. Here we present a novel theoretical effect involving the spontaneous emission of soft gravitons by photons as they bend around a heavy mass and discuss its observational prospects. Our analytic and numerical investigations suggest that the gravitational bending of starlight predicted by classical general relativity should also be accompanied by the emission of gravitational waves. This in turn redshifts the light causing a loss of its energy somewhat analogous to the bremsstrahlung of electrons by a heavier charged particle. It is suggested that this new effect may be important for a combined astronomical source of intense gravity and high-frequency radiation such as X-ray binaries and that the proposed LISA mission may be potentially sensitive to the resulting sub-Hz stochastic gravitational waves.

Casimir-cavity-induced conductance changes

The authors show the effect of adjoining a Casimir cavity to one side of metal/insulator/metal device on its conductance, as a consequence of modifying a balance in injection of hot electrons excited by zero-point fluctuations.

Mapping the Cavity Optomechanical Interaction with Subwavelength-Sized Ultrasensitive Nanomechanical Force Sensors

In a canonical optomechanical system, mechanical vibrations are dynamically encoded on an optical probe field which reciprocally exerts a backaction force. Due to the weak single photon coupling strength achieved with macroscopic oscillators, most of existing experiments were conducted with large photon numbers to achieve sizeable effects, thereby causing a dilution of the original optomechanical non-linearity. Here, we investigate the optomechanical interaction of an ultrasensitive suspended nanowire inserted in a fiber-based microcavity mode. This implementation allows to enter far into the hitherto unexplored ultrastrong optomechanical coupling regime, where one single intracavity photon can displace the oscillator by more than its zero point fluctuations. To fully characterize our system, we implement nanowire-based scanning probe measurements to map the vectorial optomechanical coupling strength, but also to reveal the intracavity optomechanical force field experienced by the nanowire. This work establishes that the single photon cavity optomechanics regime is within experimental reach.

Optical-Cavity-Induced Current

The formation of a submicron optical cavity on one side of a metal–insulator–metal (MIM) tunneling device induces a measurable electrical current between the two metal layers with no applied voltage. Reducing the cavity thickness increases the measured current. Eight types of tests were carried out to determine whether the output could be due to experimental artifacts. All gave negative results, supporting the conclusion that the observed electrical output is genuinely produced by the device. We interpret the results as being due to the suppression of vacuum optical modes by the optical cavity on one side of the MIM device, which upsets a balance in the injection of electrons excited by zero-point fluctuations. This interpretation is in accord with observed changes in the electrical output as other device parameters are varied. A feature of the MIM devices is their femtosecond-fast transport and scattering times for hot charge carriers. The fast capture in these devices is consistent with a model in which an energy ∆E may be accessed from zero-point fluctuations for a time ∆t, following a ∆E∆t uncertainty-principle-like relation governing the process.

PAT for Continuous Chromatography Integrated into Continuous Manufacturing of Biologics towards Autonomous Operation

This study proposes a reliable inline PAT concept for the simultaneous monitoring of different product components after chromatography. The feed for purification consisted of four main components, IgG monomer, dimer, and two lower molecular weight components of 4.4 kDa and 1 kDa molecular weight. The proposed measurement setup consists of a UV–VIS diode-array detector and a fluorescence detector. Applying this system, a R2 of 0.93 for the target component, a R2 of 0.67 for the dimer, a R2 of 0.91 for the first side component and a R2 of 0.93 for the second side component is achieved. Root mean square error for IgG monomer was 0.027 g/L, for dimer 0.0047 g/L, for side component 1 0.016 g/L and for the side component 2 0.014 g/L. The proposed measurement concept tracked component concentration reliably down to 0.05 g/L. Zero-point fluctuations were kept within a standard deviation of 0.018 g/L for samples with no IgG concentration but with side components present, allowing a reliable detection of the target component. The main reason inline concentration measurements have not been established yet, is the false-positive measurement of target components when side components are present. This problem was eliminated using the combination of fluorescence and UV–VIS data for the test system. The use of this measurement system is simulated for the test system, allowing an automatic fraction cut at 0.05 g/L. In this simulation a consistent yield of >99% was achieved. Process disturbances for processed feed volume, feed purity and feed IgG concentration can be compensated with this setup. Compared to a timed process control, yield can be increased by up to 12.5%, if unexpected process disturbances occur.

What if Planck had known about these calculations?

Here we present some results that would possibly have attracted the attention of the physics community in the early days of quantum mechanics in such a way that its development could have been different from what we see today. We will first present a derivation of Planck's blackbody spectrum radiation without the hypothesis of quantized energy levels of the oscillator, the only additional hypothesis to the classical theory being the existence of zeropoint fluctuations in the electromagnetic field, and this would stand as a nontrivial vacuum which could be inferred by classical means. After doing this, we derive the Unruh-Hawking effect for the electromagnetic field in a purely undulatory context, without dualities and without photons, and one question, among many others, arises after these statements: What would be the development of quantum mechanics if Planck was aware of these possibilities?

Quantum annealed criticality: A scaling description

Experimentally there exist many materials with first-order phase transitions at finite temperature that display quantum criticality. Classically, a strain-energy density coupling is known to drive first-order transitions in compressible systems, and here we generalize this Larkin-Pikin mechanism to the quantum case. We show that if the T=0 system lies above its upper critical dimension, the line of first-order transitions ends in a "quantum annealed critical point" where zero-point fluctuations restore the underlying criticality of the order parameter. The generalized Larkin-Pikin phase diagram is presented and experimental consequences are discussed.

Ultrastrong plasmon–phonon coupling via epsilon-near-zero nanocavities

Vibrational ultrastrong coupling (USC), where the light-matter coupling strength is comparable to the vibrational frequency of molecules, presents new opportunities to probe the interactions of molecules with zero-point fluctuations, harness cavity-enhanced chemical reactions, and develop novel devices in the mid-infrared regime. Here we use epsilon-near-zero nanocavities filled with a model polar medium (SiO$_2$) to demonstrate USC between phonons and gap plasmons. We present classical and quantum mechanical models to quantitatively describe the observed plasmon-phonon USC phenomena and demonstrate a splitting of up to 50% of the resonant frequency. Our wafer-scale nanocavity platform will enable a broad range of vibrational transitions to be harnessed for USC applications.