Zero Magnetic Field Research Articles

Why the pyrochlore-like antiferromagnet NaCu3F7 is magnetically non-frustrated

We present a theoretical study of the magnetic properties for the pyrochlore-like NaCu3F7 compound, which surprisingly experience little or no frustration. The magnetic effective exchange interactions were calculated using ab-initio methods explicitly treating the electronic correlation. A model Hamiltonian (quantum Heisenberg Hamiltonian, and for comparison a spin 1/2 Ising Hamiltonian) was built from these interactions and used to determine the zero temperature magnetic order versus magnetic field. The magnetic order at zero magnetic field is non frustrated and associated with the propagation vector q→=(0,0,0) . The magnetization versus magnetic field reveals the existence of a 1/3 plateau that could be observed in high-pulsed magnetic field experiments. Analyzing the magnetic interactions, we highlight the importance of the magnetic ion nature, and the lattice distortion, in the non-frustrated nature of the NaCu3F7 magnetic structure, despite its triangular/Kagome subnetworks. We believe that this non-frustrated behavior could also take place in other triangular copper-based systems.

Imaging the Breakdown and Restoration of Topological Protection in Magnetic Topological Insulator MnBi2Te4.

Quantum anomalous Hall (QAH) insulators transport charge without resistance along topologically protected chiral 1D edge states. Yet, in magnetic topological insulators to date, topological protection is far from robust, with zero-magnetic field QAH effect only realized at temperatures an order of magnitude below the Néel temperature TN, though small magnetic fields can stabilize QAH effect. Understanding why topological protection breaks down is therefore essential to realizing QAH effect at higher temperatures. Here a scanning tunneling microscope is used to directly map the size of exchange gap (Eg,ex) and its spatial fluctuation in the QAH insulator 5-layer MnBi2Te4. Long-range fluctuations of Eg,ex are observed, with values ranging between 0 (gapless) and 70 meV, appearing to be uncorrelated to individual surface point defects. The breakdown of topological protection is directly imaged, showing that the gapless edge state, the hallmark signature of a QAH insulator, hybridizes with extended gapless regions in the bulk. Finally, it is unambiguously demonstrated that the gapless regions originate from magnetic disorder, by demonstrating that a small magnetic field restores Eg,ex in these regions, explaining the recovery of topological protection in magnetic fields. The results indicate that overcoming magnetic disorder is the key to exploiting the unique properties of QAH insulators.

Magnetoinduced spin Nernst effect in topological nodal-line semimetals

The spin Nernst effect (SNE) of a topological nodal-line semimetals (TNLSMs) nanowire in a four-terminal cross-bar device is studied. Based on the nonequilibrium Green’s function method combining with the tight-binding Hamiltonian, the spin Nernst coefficients Ns3z, Ns3x and Ns3y of the two thermal transport models (kz-y case and kx-y case) under a perpendicular magnetic field are obtained. The traditional SNE describes the transverse voltage and spin current caused by the longitudinal thermal gradient. The transverse spin current is generated by the spin–orbit interaction rather than the perpendicular magnetic field. Here we find that the spin Nernst coefficients are equal to zero at the zero-magnetic field, but have finite values for non-zero magnetic fields in TNLSMs. The spin Nernst coefficient is closely related to the strength of the magnetic field and temperature. With the increase of the magnetic field strength, the peak height of the spin Nernst coefficient increases. These results indicate that the SNE is induced by the perpendicular magnetic field in the present TNLSMs system, which can be considered as an anomalous spin Nernst phenomenon. In addition, we find that Ns3z displays a series of peaks when the transmission coefficient TLR jumps from one integer plateau to another, and the spin Nernst coefficient Ns3i (i=x,y,z) is an odd function of the Fermi energy EF with Ns3z/x/y(−EF)=−Ns3z/x/y(EF) in connection mode kz-y. For the kx-y connection mode, due to the presence of the mass term m opening the energy gap, a sudden jump of the transmission coefficient TLR in the vicinity of the energy gap edge causes a very larger peak for the spin Nernst coefficient Ns3z/x/y, and the symmetrical properties of the spin Nernst coefficient Ns3z/x/y are completely broken in the strong magnetic field. These results indicate that the spin Nernst coefficient in TNLSMs strongly depends on the thermal gradient direction and the transverse lead connection direction. The spin Nernst coefficient in TNLSMs has strongly spatial anisotropy, which can be used as the characterization of the experimental detection of TNLSMs.

Perpendicular magnetic anisotropy in Bi-substituted yttrium iron garnet films

Magnetic garnet thin films exhibiting perpendicular magnetic anisotropy (PMA) and ultra-low damping have recently been explored for applications in magnonics and spintronics. Here, we present a systematic study of PMA and magnetic damping in bismuth-substituted yttrium iron garnet (Bi-YIG) films grown on sGGG (111) substrates by pulsed laser deposition. Films with thicknesses ranging from 5 to 160 nm are investigated. Structural characterization using x-ray diffraction and reciprocal space mapping demonstrates the pseudomorphic growth of the films. The films exhibit perpendicular magnetic anisotropy up to 160 nm thickness, with the zero-magnetic field state changing from fully saturated for low thicknesses to a dense magnetic stripe pattern for thicker films. The films show a ferromagnetic resonance (FMR) linewidth of 100–200 MHz with a Gilbert damping constant of the order of 4×10−3. The broad FMR linewidth is caused by inhomogeneities of magnetic properties on micrometer length scales.

Possible zero-magnetic field fractional quantization in In0.75Ga0.25As heterostructures

In this Letter, we report a systematic study of a structure found in zero magnetic field at or near 0.2 ×(e2/h) in In0.75Ga0.25As heterostructures, where e is the fundamental unit of charge and h is Planck's constant. This structure has been observed in many samples and stays at near constant conductance despite a large range of external potential changes, the stability indicating a quantum state. We have also studied the structure in the presence of high in-plane magnetic fields and find an anisotropy which can be related to the Rashba spin–orbit interaction and agrees with a recent theory based on the formation of coherent back-scattering. A possible state with conductance at 0.25 ×(e2/h) has also been found. The quantum states described here will help with the fundamental understanding of low-dimensional electronic systems with strong spin–orbit coupling and may offer new perspectives for future applications in quantum information schemes.

Composite Fermi Liquid at Zero Magnetic Field in Twisted MoTe_{2}.

The pursuit of exotic phases of matter outside of the extreme conditions of a quantizing magnetic field is a long-standing quest of solid state physics. Recent experiments have observed spontaneous valley polarization and fractional Chern insulators in zero magnetic field in twisted bilayers of MoTe_{2}, at partial filling of the topological valence band (ν=-2/3 and -3/5). We study the topological valence band at half filling, using exact diagonalization and density matrix renormalization group calculations. We discover a composite Fermi liquid (CFL) phase even at zero magnetic field that covers a large portion of the phase diagram near twist angle ∼3.6°. The CFL is a non-Fermi liquid phase with metallic behavior despite the absence of Landau quasiparticles. We discuss experimental implications including the competition between the CFL and a Fermi liquid, which can be tuned with a displacement field. The topological valence band has excellent quantum geometry over a wide range of twist angles and a small bandwidth that is, remarkably, reduced by interactions. These key properties stabilize the exotic zero field quantum Hall phases. Finally, we present an optical signature involving "extinguished" optical responses that detects Chern bands with ideal quantum geometry.

Tailoring Zero‐Field Magnetic Skyrmions in Chiral Multilayers by a Duet of Interlayer Exchange Couplings

AbstractMagnetic skyrmions have emerged as promising elements for encoding information toward biomimetic computing applications due to their pseudoparticle nature and efficient coupling to spin currents. A key hindrance for skyrmionic devices is their instability against elongation at zero magnetic field (ZF). Prevailing materials approaches focused on tailoring skyrmion energetics have found ZF configurations to be highly sensitive, which imposes significant growth constraints and limits their device scalability. This work demonstrates that designer ZF skyrmion configurations can be robustly stabilized within chiral multilayer stacks by exploiting a duet of interlayer exchange couplings (IECs). Microscopic imaging experiments show that varying the two IECs enables the coarse and fine‐tuning of ZF skyrmion stability and density. Micromagnetic simulations reveal that the duo‐IEC approach is distinguished by its influence on the kinetics of skyrmion nucleation, in addition to the ability to tailor energetics, resulting in a substantially expanded parameter space, and enhanced stability for individual ZF skyrmions. This study underscores the importance of IEC as a means of stabilizing and controlling ZF skyrmions, paving the way to scalable skyrmion‐based devices.

DC magnetic field-assisted improvement of textile dye degradation efficiency with multi-capillary air bubble discharge plasma jet.

Axial DC magnetic field-assisted multi-capillary underwater air bubble discharge plasma jet has been used to study the productions of reactive oxygen species. Analyses of optical emission data revealed that the rotational (Tr) and vibrational temperatures (Tv) of plasma species slightly increased with magnetic field strength. The electron temperature (Te) and density (ne) increased almost linearly with magnetic field strength. Te increased from 0.53 to 0.59eV, whereas ne increased from 1.03 × 1015cm-3 to 1.33 × 1015cm-3 for B = 0 to B = 374 mT, respectively. Analytical results from the plasma treated water provided that the electrical conductivity (EC), oxidative reduction potential (ORP), and the concentrations of O3 and H2 O2 enhanced from 155 to 229 µS cm-1, 141 to 17mV, 1.34 to 1.92mg L-1, and 5.61 to 10.92mg L-1 due to the influence of axial DC magnetic field, while [Formula: see text] reduced from 5.10 to 3.93 for 30min treatment of water with B = 0 and B = 374 mT, respectively. The model wastewater prepared with Remazol brilliant blue textile dye and the plasma treated wastewater studied by optical absorption spectrometer, Fourier transform infrared spectrometer, and gas chromatography mass spectrometer. The results show that the decolorization efficiency increased ~ 20% after 5min treatment for the maximum B = 374 mT with respect to zero-magnetic field and, power consumption, and electrical energy cost reduced ~ 6.3% and ~ 4.5%, respectively, due to the maximum assisted axial DC magnetic field strength of 374 mT.

Enabling ambulatory movement in wearable magnetoencephalography with matrix coil active magnetic shielding

The ability to collect high-quality neuroimaging data during ambulatory participant movement would enable a wealth of neuroscientific paradigms. Wearable magnetoencephalography (MEG) based on optically pumped magnetometers (OPMs) has the potential to allow participant movement during a scan. However, the strict zero magnetic field requirement of OPMs means that systems must be operated inside a magnetically shielded room (MSR) and also require active shielding using electromagnetic coils to cancel residual fields and field changes (due to external sources and sensor movements) that would otherwise prevent accurate neuronal source reconstructions. Existing active shielding systems only compensate fields over small, fixed regions and do not allow ambulatory movement. Here we describe the matrix coil, a new type of active shielding system for OPM-MEG which is formed from 48 square unit coils arranged on two planes which can compensate magnetic fields in regions that can be flexibly placed between the planes. Through the integration of optical tracking with OPM data acquisition, field changes induced by participant movement are cancelled with low latency (25 ms). High-quality MEG source data were collected despite the presence of large (65 cm translations and 270° rotations) ambulatory participant movements.

Radio-wave Effect on Singlet Fission in Polycrystalline Tetracene near Zero Magnetic Field.

A triplet-triplet pair is a key intermediate in singlet fission (SF), which has the potential to overcome the theoretical limit of solar cell efficiency. Here, we report a new spectroscopy to directly detect a short-lived triplet-triplet pair via the effects of radio-wave (RF) irradiation near zero magnetic field at room temperature. The fluorescence of polycrystalline powder of tetracene is reduced by RF irradiation at zero field, which is caused by a quasi-static RF field effect on spin mixing and electron-spin resonance among zero-field-splitting sublevels of the triplet-triplet pair. The curve for the quasi-static RF field effect can be reproduced numerically from that for the observed magnetophotoluminescence (MPL) effect. The simultaneous simulation of the RF and MPL effects using the density matrix formalism estimates rate constants of 1.2 × 108 and 6.0 × 108 s-1 for the fusion and dissociation, respectively, of the triplet-triplet pair.

Spin-wave nonreciprocity at the spin-flop transition region in synthetic antiferromagnets

We investigate the frequency nonreciprocity in CoFeB/Ru/CoFeB synthetic antiferromagnets near the spin-flop transition region, where the magnetic moments in the two ferromagnetic layers are noncollinear. Using conventional Brillouin light scattering, we perform systematic measurements of the frequency nonreciprocity as a function of an external magnetic field. At near zero magnetic field, where the antiparallel alignment of the magnetic moments in the two layers is established, we observe a significant frequency nonreciprocity of up to a few GHz, which vanishes when the relative magnetization orientation switches into the parallel configuration at a large magnetic field. For the intermediate values of the magnetic field, where the system transitions from the antiparallel to the parallel orientation, a nonmonotonous dependence of the frequency nonreciprocity is found, with a maximum frequency shift around the spin-flop critical point. This nontrivial dependence of the nonreciprocity versus field is attributed to the nonmonotonous dependence of the dynamic dipolar interaction, which is the main factor that causes asymmetry in the dispersion relation. Furthermore, we found that the sign of the frequency shift changes even without switching the polarity of the bias field. These results show that one can precisely control the nonreciprocal propagation of spin waves via field-driven magnetization reorientation.

Magnetically controlled bio-inspired elastomeric actuators with high mechanical energy storage.

Many biological systems are made to operate more quickly, efficiently, and with more power by storing elastic energy. This work introduces a straightforward bioinspired design for the quick manufacture of pre-stressed soft magnetic actuators. The actuator requires a lower magnetic field strength to be activated and can regain its original shape without the need for external stimuli. These characteristics are demonstrated in this work through the creation of actuators with round and helical shape structures inspired by the tendril plant and chameleon's tongue. Both the final form of the actuator and its actuation sequence may be programmed by controlling the direction and strength of the force utilised to pre-stress the elastomeric layer. Analytical models are presented to trace the actuators' energy storage, radius, and pitch. High-speed shape recovery after releasing the magnetic force and a strong grasping force are achieved due to the stored mechanical elastic energy. Experiments are conducted to analyse the shape changes, grasping action, and determine the actuation force. The manufacture of the grippers with zero-magnetic field strength holding capacities of up to 20 times their weight is made possible by the elastic energy that actuators store in their pre-stressed elastomeric layer. The outcomes of our research show that a unique magnetic field-controlled soft actuator can be created in different shapes and designs based on requirements.

Current-Induced Nucleation and Motion of Skyrmions in Zero Magnetic Field

We study the stabilization and electrical manipulation of skyrmions in magnetic ultrathin films in the absence of an applied magnetic field. We show that this requires an increased magnetic anisotropy, controlled by the sample thickness, as compared to usual skyrmionic samples, so that the uniform state corresponds to the zero-field ground state and the skyrmions to metastable excitations. Although skyrmion stabilization at zero field is demonstrated over a broad range of thicknesses, electrical control appears to be more demanding to avoid skyrmion deformation. In the thinnest samples, the large magnetic anisotropy prevents skyrmion deformations and we show that they can be nucleated progressively by current pulses, which underlines that the only possible transition occurs between uniform and skyrmion states. The solitonic skyrmions in zero applied magnetic field have the same properties as compared to field-stabilized ones, with a long-term stability and high mobility when excited by a spin-orbit torque.

On the Reasons for Reversible Aggregation of Magnetite Ferrofluids during Their Dilution with a Pure Carrier in Zero Magnetic Field

On the Reasons for Reversible Aggregation of Magnetite Ferrofluids during Their Dilution with a Pure Carrier in Zero Magnetic Field

Robust superconductivity and fragile magnetism induced by the strong Cu impurity scattering in the high-pressure phase of FeSe

Superconductivity in FeSe is strongly enhanced under applied pressure and it is proposed to emerge from anomalously coupled structural and magnetic phases. Small impurities inside the Fe plane can strongly disrupt the pair formation in FeSe at ambient pressure and can also reveal the interplay between normal and superconducting phases. Here, we investigate how an impurity inside the Fe plane induced by the Cu substitution can alter the balance between competing electronic phases of FeSe at high pressures. In the absence of an applied magnetic field, at low pressures the nematic and superconducting phases are suppressed by a similar factor. On the other hand, at high pressures, above 10 kbar, the superconductivity remains unaltered despite the lack of any signature in transport associated to a magnetic phase in zero-magnetic field. However, by applying a magnetic field, the resistivity displays an anomaly preceding the activated behaviour in temperature, assigned to a magnetic anomaly. We find that the high-pressure superconducting phase of FeSe is robust and remains enhanced in the presence of Cu impurity, whereas the magnetic phase is not. This could suggest that high-$T_{\rm c}$ superconductivity has a sign-preserving order parameter in a presence of a rather glassy magnetic phase.

Erratum to: Formation of Gapless Z2 Spin Liquid Phase Manganites in the (Sm1 – yGdy)0.55Sr0.45MnO3 System in Zero Magnetic Field: Topological Phase Transitions to States with Low and High Density of 2D-Vortex Pairs Induced by the Magnetic Field

Erratum to: Formation of Gapless Z2 Spin Liquid Phase Manganites in the (Sm1 – yGdy)0.55Sr0.45MnO3 System in Zero Magnetic Field: Topological Phase Transitions to States with Low and High Density of 2D-Vortex Pairs Induced by the Magnetic Field

Enhanced d−p hybridization intertwined with anomalous ground state formation in the van der Waals itinerant magnet Fe5GeTe2

${\mathrm{Fe}}_{5}{\mathrm{GeTe}}_{2}$ is a van der Waals (vdW)-coupled unconventional ferromagnetic metal with a high Curie temperature (${T}_{\mathrm{C}}$) exceeding 300 K. The formation of an anomalous ground state significantly below ${T}_{\mathrm{C}}$ has received considerable attention, resulting in increased interest in understanding the spin-polarized electronic state evolution near the Fermi energy (${E}_{\mathrm{F}}$) as a function of temperature. Despite recent extensive studies, a microscopic understanding of the spin-polarized electronic structure around ${E}_{\mathrm{F}}$ has not yet been established owing to the intrinsic complexity of both the crystal and band structures. In this study, we investigate the temperature dependence of element-specific soft x-ray magnetic circular dichroism (XMCD). A systematic temperature evolution in the XMCD signal from both magnetic Fe and its ligand Te is clearly observed. More importantly, the enhancement in the hybridization between the Fe $3d$ and Te $5p$ states at low temperature in the zero-magnetic field limit is revealed. We discuss the implications of our observation in line with possible emergence of an exotic magnetic ground state in ${\mathrm{Fe}}_{5}{\mathrm{GeTe}}_{2}$.

Phonon-drag thermopower and thermoelectric performance of MoS2 monolayer in quantizing magnetic field

We present a theory of phonon-drag thermopower, , in MoS2 monolayer at a low-temperature regime in the presence of a quantizing magnetic field B. Our calculations for consider the electron–acoustic phonon interaction via deformation potential (DP) and piezoelectric (PE) couplings for longitudinal (LA) and transverse (TA) phonon modes. The unscreened TA-DP is found to dominate over other mechanisms. The is found to oscillate with the magnetic field where the lifting effect of the valley and spin degeneracies in MoS2 monolayer has been clearly observed. An enhanced with a peak value of mV K−1 at about T = 10 K is predicted, which is closer to the zero field experimental observation. In the Bloch–Grüneisen regime the temperature dependence of gives the power-law , where δ e varies marginally around 3 and 5 for unscreened and screened couplings, respectively. In addition, is smaller for larger electron density n e . The power factor PF is found to increase with temperature T, decrease with n e , and oscillate with B. The prediction of an increase of thermal conductivity with temperature and the magnetic field is responsible for the limit of the figure of merit (ZT). At a particular magnetic field and temperature, ZT can be maximized by optimizing electron density. By fixing cm−2, the highest ZT is found to be 0.57 at T = 5.8 K and B = 12.1 T. Our findings are compared with those in graphene and MoS2 for the zero-magnetic field.

Enhancement of giant magnetoelectric effect in Ni-doped CaBaCo4O7

The polar ferrimagnet CaBaCo${}_{4}$O${}_{7}$ exhibits the largest magnetic field driven electric polarization change \ensuremath{\Delta}$P$ reported so far in a narrow temperature range. Here, the authors demonstrate that only 2.5% of Ni substitution for Co increases the magnitude of \ensuremath{\Delta}$P$ by about 30%, as well as expanding the temperature range in which the giant \ensuremath{\Delta}$P$ appears down to a low temperature. This is attributable to the switching of the low-temperature zero magnetic field state from a ferrimagnetic to an antiferromagnetic state.

Zero Magnetic Field Plateau Phase Transition in Higher Chern Number Quantum Anomalous Hall Insulators.

The plateau-to-plateau transition in quantum Hall effect under high magnetic fields is a celebrated quantum phase transition between two topological states. It can be achieved by either sweeping the magnetic field or tuning the carrier density. The recent realization of the quantum anomalous Hall (QAH) insulators with tunable Chern numbers introduces the channel degree of freedom to the dissipation-free chiral edge transport and makes the study of the quantum phase transition between two topological states under zero magnetic field possible. Here, we synthesized the magnetic topological insulator (TI)/TI pentalayer heterostructures with different Cr doping concentrations in the middle magnetic TI layers using molecular beam epitaxy. By performing transport measurements, we found a potential plateau phase transition between C=1 and C=2 QAH states under zero magnetic field. In tuning the transition, the Hall resistance monotonically decreases from h/e^{2} to h/2e^{2}, concurrently, the longitudinal resistance exhibits a maximum at the critical point. Our results show that the ratio between the Hall resistance and the longitudinal resistance is greater than 1 at the critical point, which indicates that the original chiral edge channel from the C=1 QAH state coexists with the dissipative bulk conduction channels. Subsequently, these bulk conduction channels appear to self-organize and form the second chiral edge channel in completing the plateau phase transition. Our study will motivate further investigations of this novel Chern number change-induced quantum phase transition and advance the development of the QAH chiral edge current-based electronic and spintronic devices.