For the safety of the wound-rotor synchronous machine (WRSM) in aircraft applications, the overvoltage at the motor terminals, electromagnetic interference (EMI) performance, and bearing currents as well as the loss analysis are the core areas to be addressed. The high-frequency (HF) modeling method of the WRSM, which has a strong relationship with all these core areas, is a very critical theme. In this paper, a measurement-based wide-frequency (WF) modeling method to characterize the impedance of the WRSM is proposed to build a straightforward correlation between fundamental models and HF parasitic circuit elements. In this paper, the voltage-behind-reactance method is applied to demonstrate the rotor-angle-dependent characters in the low-frequency domain, while the vector fitting method is used to parameterize the HF branch for high-accuracy consideration. By doing this, a WF electrical model with multistage RLC units is formed, which comprehensively considers both the saliency character of the machine and frequency range. The WF model is also compatible with the circuit-based simulation. Finally, the EMI prediction orientated simulation and experimental results are implemented on a 10 kVA WRSM prototype to verify the correctness and advantages of the proposed modeling method.