Whispering-gallery Resonators Research Articles

Polarization-entangled photons from a whispering gallery resonator

Crystalline whispering gallery mode resonators (WGMRs) have been shown to facilitate versatile sources of quantum states that can efficiently interact with atomic systems. These features make WGMRs an efficient platform for quantum information processing. Here, we experimentally show that it is possible to generate polarization entanglement from WGMRs by using an interferometric scheme. Our scheme gives us the flexibility to control the phase of the generated entangled state by changing the relative phase of the interferometer. The S value of Clauser–Horne–Shimony–Holt’s inequality in the system is 2.45 ± 0.07, which violates the inequality by more than six standard deviations.

Frequency-tunable single-photon router based on a microresonator containing a driven three-level emitter

We propose a frequency-tunable router of single photons with high routing efficiency, which is constructed by two waveguides mediately linked by a single-mode whispering gallery resonator with a driven three-level emitter. Quantum routing probability in the output port is obtained via the real-space Hamiltonian. By adjusting the resonator–emitter coupling and the drive, the desired continuous central frequencies for the resonance peaks of routing photons can be manipulated nearly linearly, with the assistance of Rabi splitting effect and optical Stark shift. The proposed routing system may provide potential applications in designing other frequency-modulation quantum optical devices, such as multiplexers, filters, and so on.

Low Part-Per-Trillion, Humidity Resistant Detection of Nitric Oxide Using Microtoroid Optical Resonators.

The nitric oxide radical plays pivotal roles in physiological as well as atmospheric contexts. Although the detection of dissolved nitric oxide in vivo has been widely explored, highly sensitive (i.e., low part-per-trillion level), selective, and humidity-resistant detection of gaseous nitric oxide in air remains challenging. In the field, humidity can have dramatic effects on the accuracy and selectivity of gas sensors, confounding data, and leading to overestimation of gas concentration. Highly selective and humidity-resistant gaseous NO sensors based on laser-induced graphene were recently reported, displaying a limit of detection (LOD) of 8.3 ppb. Although highly sensitive (LOD = 590 ppq) single-wall carbon nanotube NO sensors have been reported, these sensors lack selectivity and humidity resistance. In this report, we disclose a highly sensitive (LOD = 2.34 ppt), selective, and humidity-resistant nitric oxide sensor based on a whispering-gallery mode microtoroid optical resonator. Excellent analyte selectivity was enabled via novel ferrocene-containing polymeric coatings synthesized via reversible addition-fragmentation chain-transfer polymerization. Utilizing a frequency locked optical whispering evanescent resonator system, the microtoroid's real-time resonance frequency shift response to nitric oxide was tracked with subfemtometer resolution. The lowest concentration experimentally detected was 6.4 ppt, which is the lowest reported to date. Additionally, the performance of the sensor remained consistent across different humidity environments. Lastly, the impact of the chemical composition and molecular weight of the novel ferrocene-containing polymeric coatings on sensing performance was evaluated. We anticipate that our results will have impact on a wide variety of fields where NO sensing is important such as medical diagnostics through exhaled breath, determination of planetary habitability, climate change, air quality monitoring, and treating cardiovascular and neurological disorders.

Ultrahigh-sensitivity temperature sensor based on an elastic TPU capillary whispering gallery resonator.

An ultrahigh sensitivity temperature sensor based on an elastic thermoplastic urethane (TPU) capillary whispering-gallery mode (WGM) microcavity is proposed. The temperature sensor comprises a dye-doped TPU capillary and two sealed fused silica capillaries covered at both ends and is fabricated via a thin film assembly and wet etching. The fused silica capillaries limit the thermal volume expansion of the air within it. The volume of the exposed part of the elastic TPU capillary, which has an ultrahigh sensitivity to temperature compared with the thermal volume expansion of material, is increased; the designed elastic TPU capillary WGM microcavity exhibited an ultrahigh sensitivity of 11.28 nm/°C.

Analysis and optimization of optical frequency comb spectra of magnesium fluoride microbottle resonator

<sec>Optical frequency comb has shown great potential applications in many areas including molecular spectroscopy, RF photonics, millimeter wave generation, frequency metrology, atomic clock, and dense/ultra-dense wavelength division multiplexed high speed optical communications. Optical frequency comb in the microresonator supporting whispering-gallery mode has attracted widespread interest because of its advantages such as flexible repetition rate, wide bandwidth, and compact size. The exceptionally long photon lifetime and small modal volume enhance light-matter interaction, which enables us to realize intracavity nonlinear frequency conversions with low pump threshold. With the advantages of small size, low power consumption, wide spectral coverage and adjustable dispersion, the magnesium fluoride microresonator optical frequency comb has potential applications in optical communication and mid-infrared spectroscopy.</sec><sec>In this work, the spectral characteristics of the optical frequency comb generated by a magnesium fluoride whispering-gallery mode microbottle resonator platform are investigated. In order to optimize the spectral distribution of the optical frequency comb of the magnesium fluoride microbottle resonator, the second-order dispersion and higher-order dispersion of the bottle resonator structure under different curvatures and axial modes are solved iteratively by the finite element method, and the spectral evolutions of the optical frequency comb under different axial mode excitations are simulated by solving the nonlinear Schrödinger equation through the split-step Fourier method. The results show that near-zero anomalous dispersion tuning can be achieved in a wide bandwidth range by exciting low-order axial mode at an optimal radius of curvature, while the high-order axial mode will lead the microbottle resonator to present the weak normal dispersion. The weaker anomalous dispersion in the lower-order axial mode broadens the bandwidth of the optical comb, demonstrating that the third-order dispersion and the negative fourth-order dispersion can broaden the Kerr soliton optical comb; the weak normal dispersion in the higher-order axial mode suppresses the generation of the Kerr optical comb, and the Raman optical comb dominates. The selective excitation of Kerr soliton combs and Raman combs can be achieved by modulating the axial mode of the microbottle resonator under suitable pumping conditions. The present work provides guidance for designing the dispersion in magnesium fluoride microresonator and the experimental tuning of broadband Kerr soliton optical combs and Raman optical combs.</sec>

Whispering-Gallery Mode Micro-Ring Resonator Integrated with a Single-Core Fiber Tip for Refractive Index Sensing

A micro-ring resonator structure was fabricated via the two-photon polymerization technique directly on a single-mode fiber tip and tested for refractive index sensing application. The micro-ring structure was used to excite whispering-gallery modes, and observations of the changes in the resonance spectrum introduced by changes in the refractive index of the environment served as the sensing principle. The proposed structure has the advantages of a very simple design, allowing for measurements in reflection mode, relatively easy and fast fabrication and integration with a single tip of a standard single-mode fiber, which allowed for quick and convenient measurements in the optical setup. The performance of the structure was characterized, and the resonant spectrum giving high potential for refractive index sensing was measured. Future perspectives of the research are addressed.

Automatic Alignment Method for Controlled Free-Space Excitation of Whispering-Gallery Resonances.

Whispering-gallery mode microresonators have gained wide popularity as experimental platforms for different applications, ranging from biosensing to nonlinear optics. Typically, the resonant modes of dielectric microresonators are stimulated via evanescent wave coupling, facilitated using tapered optical fibers or coupling prisms. However, this method poses serious shortcomings due to fabrication and access-related limitations, which could be elegantly overcome by implementing a free-space coupling approach; although additional alignment procedures are needed in this case. To address this issue, we have developed a new algorithm to excite the microresonator automatically. Here, we show the working mechanism and the preliminary results of our experimental method applied to a home-made silica microsphere, using a visible laser beam with a spatial light modulator and a software control.

Multi-mode microcavity frequency engineering through a shifted grating in a photonic crystal ring.

Frequency engineering of whispering-gallery resonances is essential in microcavity nonlinear optics. The key is to control the frequencies of the cavity modes involved in the underlying nonlinear optical process to satisfy its energy conservation criterion. Compared to the conventional method that tailors dispersion by cross-sectional geometry, thereby impacting all cavity mode frequencies, grating-assisted microring cavities, often termed as photonic crystal microrings, provide more enabling capabilities through mode-selective frequency control. For example, a simple single period grating added to a microring has been used for single frequency engineering in Kerr optical parametric oscillation (OPO) and frequency combs. Recently, this approach has been extended to multi-frequency engineering by using multi-period grating functions, but at the cost of increasingly complex grating profiles that require challenging fabrication. Here, we demonstrate a simple approach, which we term as shifted grating multiple mode splitting (SGMMS), where spatial displacement of a single period grating imprinted on the inner boundary of the microring creates a rotational asymmetry that frequency splits multiple adjacent cavity modes. This approach is easy to implement and presents no additional fabrication challenges compared to an unshifted grating, and yet is very powerful in providing multi-frequency engineering functionality for nonlinear optics. We showcase an example where SGMMS enables OPO across a wide range of pump wavelengths in a normal-dispersion device that otherwise would not support OPO.

Single-photon router utilizing whispering-gallery resonator coupled with atoms

Single-photon router utilizing whispering-gallery resonator coupled with atoms

Ambipolar charge-transfer graphene plasmonic cavities.

Plasmon polaritons in van der Waals materials hold promise for various photonics applications1-4. The deterministic imprinting of spatial patterns of high carrier density in plasmonic cavities and nanoscale circuitry can enable the realization of advanced nonlinear nanophotonic5 and strong light-matter interaction platforms6. Here we demonstrate an oxidation-activated charge transfer strategy to program ambipolar low-loss graphene plasmonic structures. By covering graphene with transition-metal dichalcogenides and subsequently oxidizing the transition-metal dichalcogenides into transition-metal oxides, we activate charge transfer rooted in the dissimilar work functions between transition-metal oxides and graphene. Nano-infrared imaging reveals ambipolar low-loss plasmon polaritons at the transition-metal-oxide/graphene interfaces. Further, by inserting dielectric van der Waals spacers, we can precisely control the electron and hole densities induced by oxidation-activated charge transfer and achieve plasmons with a near-intrinsic quality factor. Using this strategy, we imprint plasmonic cavities with laterally abrupt doping profiles with nanoscale precision and demonstrate plasmonic whispering-gallery resonators based on suspended graphene encapsulated in transition-metal oxides.

Subnanometer-Resolution Nanoparticle Sensing through the Strong Coupling between Surface Plasmon Polariton Whispering Gallery Resonances and Localized Surface Plasmon

High-resolution nanoparticle sensing is very important, and many schemes have been proposed to achieve this goal. Circular nanocavities in which surface plasmon polariton (SPP) whispering gallery mode (WGM) resonances were excited were designed to sense particles of ultra-small size and with high resolution. Localized surface plasmon resonances (LSPRs) were excited when a metal particle was set in the circular cavity. The SPP WGM split into symmetric mode (SM) and antisymmetric mode (ASM) due to the LSPRs scattering into the SPPs. The strong coupling between SM resonance and LSPRs generated positive and opposite modes, which were sensitive to the variation in nanoparticle size and position. Even a small nanometer-sized metal particle introduced LSPRs and produced mode splitting. The WGM mode splitting induced by LSPRs reduced the sensing limit. The simulation results show that 1 nm changes in nanoparticle radius and position led to SM 11.8 nm and 10.2 nm wavelength shifts, respectively. This means that variations of 0.09 nm in size and 0.1 nm in position can be sensed with a 1 nm spectral resolution. The strong coupling between SPP WGM and LSPRs can be applied to sense at a subnanometer resolution.

Pump tuning of a mid-infrared whispering gallery optical parametric oscillator.

Optical parametric oscillators (OPOs) constitute an important coherent, narrow-linewidth and widely tunable light source with applications in spectroscopy and many other fields. Their realizations based on whispering gallery resonators (WGRs) provide a small footprint and ultra-low thresholds, with demonstrations of tunability typically done via temperature variation. In this work, we show the pump tuning capabilities of a mm-sized WGR mid-infrared OPO made of CdSiP2. By tuning a telecom wavelength diode laser by 16 nm, we generate tunable light from 2708 to 3575 nm. Furthermore, we show controlled tuning in steps of 1 free spectral range (FSR) and the possibility of 12 GHz of continuous tuning. All these features are in good agreement with the theoretical predictions. We conclude that tuning from 2.4 to 4.9 µm is even possible, while still using commercially available near-infrared diode lasers. This work highlights the advantages of pump tuning of WGR OPOs and provides valuable insights for their precise control.

Trapezoidal Angled Fiber Coupler for Microsphere Resonator With Enhancement of Fano Resonance

We propose and demonstrate a trapezoidal angled fiber coupler for excitation of whispering-gallery mode microsphere resonator, with enhanced Fano resonance. The reflection from the angled fiber is enhanced when the oblique angle is greater than critical angle, which is obtained as 30° theoretically for angled fiber. To enhance the endface reflection, the front tip of the angled fiber is polished flat to achieve the trapezoidal angled fiber. Compared with angled fiber, the proportion of Fano lineshape in spectra for trapezoidal angled fiber is nearly doubled and the slope is greatly improved, which reaches 304.55 dB/nm. Moreover, through the coupling of dual microspheres, the <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">${Q}$ </tex-math></inline-formula> factor is improved severalfold and the thermal tuning efficiency is increased by 50%. With the advantage of low cost, easy fabrication procedure and reflection mode operation, the proposed device shows a great potential for sensing, optical tuning and optical switching applications.

Experimental and Numerical Validation of Whispering Gallery Resonators as Optical Temperature Sensors.

This study experimentally and numerically validates the commonly employed technique of laser-induced heating of a material in optical temperature sensing studies. Furthermore, the Er3+-doped glass microspheres studied in this work can be employed as remote optical temperature sensors. Laser-induced self-heating is a useful technique commonly employed in optical temperature sensing research when two temperature-dependent parameters can be correlated, such as in fluorescence intensity ratio vs. interferometric calibration, allowing straightforward sensor characterization. A frequent assumption in such experiments is that thermal homogeneity within the sensor volume, that is, a sound hypothesis when dealing with small volume to surface area ratio devices such as microresonators, but has never been validated. In order to address this issue, we performed a series of experiments and simulations on a microsphere supporting whispering gallery mode resonances, laser heating it at ambient pressure and medium vacuum while tracking the resonance wavelength shift and comparing it to the shift rate observed in a thermal bath. The simulations were done starting only from the material properties of the bulk glass to simulate the physical phenomena of laser heating and resonance of the microsphere glass. Despite the simplicity of the model, both measurements and simulations are in good agreement with a highly homogeneous temperature within the resonator, thus validating the laser heating technique.

Electro-optically tunable single-frequency lasing from neodymium-doped lithium niobate microresonators.

Tunable light sources are a key enabling technology for many applications such as ranging, spectroscopy, optical coherence tomography, digital imaging and interferometry. For miniaturized laser devices, whispering gallery resonator lasers are a well-suited platform, offering low thresholds and small linewidths, however, many realizations suffer from the lack of reliable tuning. Rare-earth ion-doped lithium niobate offers a way to solve this issue. Here we present a single-frequency laser based on a neodymium-doped lithium niobate whispering gallery mode resonator that is tuned via the linear electro-optic effect. Using a special geometry, we suppress higher-order transverse modes and hence ensure single-mode operation. With an applied voltage of just 68 V, we achieve a tuning range of 3.5 GHz. The lasing frequency can also be modulated with a triangular control signal. The freely running system provides a frequency and power stability of better than Δ ν=20MHz and 6 %, respectively, for a 30-minute period. This concept is suitable for full integration with existing photonic platforms based on lithium niobate.

Coaxial Micro Ring Arrays Fabricated on Self‐Assembled Microtube Cavities for Resonant Light Modulation

AbstractComposite optical microcavities, as a versatile platform for light manipulation, have been theoretically revealed that the configuration of concentrically coupled resonant trajectories can significantly enhance the coupling strength, which is however challenging in experimental preparation. Here coaxial whispering gallery resonator chains were designed and fabricated with optically coupled modes split apart by more than the free spectral range (FSR) of the cavity itself. Because such three dimensional (3D) coupled optical systems are extremely difficult to obtain with traditional processing techniques an approach is developed to release and roll‐up pre‐strained, nanostructured silicon nitride membranes into microtubular optical cavities. Parallel nano‐ridges modified on the patterned membranes form into coaxial micro ring arrays after the membrane rolls up into a microtubular structure. Energetic degeneracy, as a consequence of mode splitting exceeding the FSR, leads to interference between bonding and antibonding modes with different mode identities (mode number), resulting in novel light modulation in the form of hybrid super wave modes, which display a distinct hopping behavior resembling linear stretch modes of an oscillator chain.

Polarization Dependent Scattering in Cavity Optomagnonics.

The polarization dependence of magnon-photon scattering in an optical microcavity is reported. Because of the short cavity length, the longitudinal mode-matching conditions found in previously explored, large path-length whispering gallery resonators are absent. Nonetheless, for cross-polarized scattering a strong and broadband suppression of one sideband is observed. This arises due to an interference between the Faraday and second-order Cotton-Mouton effects. To fully account for the suppression of the cross-polarized scattering, it is necessary to consider the squeezing of magnon modes intrinsic to thin-film geometry. A copolarized scattering due to Cotton-Mouton effect is also observed. In addition, the magnon modes involved are identified as Damon-Eshbach surface modes, whose nonreciprocal propagation could be exploited in device applications. This Letter experimentally demonstrates the important role of second-order Cotton-Mouton effect for optomagnonic devices.

Nanolasers based on whispering‐gallery resonances in graphene cavities with hyperbolic dispersion

<p indent=0mm>We theoretically propose a novel nanolaser based on whispering-gallery resonances (WGRs) in spherical cavities with hyperbolic dispersion, composed of a dielectric core alternately wrapped by graphene and dielectric layers. First, we showed that the multilayer graphene‐dielectric core‐shell cavities have a negative dielectric constant in at least one direction and exhibit an unusual hyperbolic dispersion. Such cavities can support the whispering-gallery modes with resonance wavelengths much larger than the cavity sizes and can strongly confine the electromagnetic fields in deep subwavelength regions. Moreover, multiple dipole WGR modes with different orders can be excited by such cavities, accompanied by high Purcell factors and strong confinement electric fields within different dielectric layers. Therefore, by introducing gain into these different dielectric layers, lasing at different resonance wavelengths can be realized with a low lasing threshold. For the cavity with a diameter of <sc>404 nm,</sc> the lasing threshold at a wavelength of 32.3 μm is only<sc>80.6 cm⁻¹.</sc> Furthermore, we demonstrated that by manipulating the refractive index of the dielectric layers, graphene Fermi energy, or the number of pairs of graphene and dielectric layers, the lasing wavelengths in a wide spectral range could be easily adjusted. Finally, even for the relatively simple core-shell cavity with only two pairs of graphene and dielectric layers, the ratio of resonant wavelength and cavity diameter for the TM_1,1 mode is approximately 50, and the lasing threshold is only <sc>90.74 cm⁻¹.</sc> This type of nanolasers has the characteristics of deep subwavelength, low threshold, and wide-band tunability. Hence, these lasers have great potential for applications in integrated terahertz devices.

A Whispering-Gallery Mode Microsphere Resonator Based on Optical Fiber With an Open Microcavity

A whispering-gallery mode microsphere resonator based on optical fiber with an open microcavity is demonstrated, which is created by use of femtosecond laser micromachining and fusion splicing techniques. When a microsphere is placed into the open microcavity, whispering-gallery mode can be excited through evanescent field coupling. The device can be constructed in either single-mode fiber or multimode fiber, with the insertion loss of ~13.2 and ~21.0 dB, and the quality factor of 4.81X10 <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sup> and 2 X10 <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">5</sup> respectively. Because of its features of compact structure, low cost, easy fabrication, convenient operation and high durability, the device is expected to have many photonics applications.

Packaged whispering gallery resonator device based on an optical nanoantenna coupler.

In this work, we present a packaged whispering gallery mode (WGM) device based on an optical nanoantenna as the coupler and a glass microsphere as the resonator. The microspheres were fabricated from either SiO2 fiber or Er3+-doped fiber, the latter creating a WGM laser with a threshold of 93 µW at 1531 nm. The coupler-resonator WGM device was packaged in a glass capillary. The performance of the packaged microlaser was characterized, with lasing emission both excited in and collected from the WGM cavity via the nanoantenna. The packaged system provides isolation from environmental contamination, a small size, and unidirectional coupling while maintaining a high quality (Q-) factor (∼108).