Whispering Gallery Mode Resonators Research Articles

Suppression of the plasmon-quenching effect on light amplification in 20-μm-diameter plasmonic whispering gallery mode resonators fabricated from bowl-shaped organic/metal thin films.

Bowl-shaped plasmonic whispering gallery mode (WGM) resonators were fabricated from a 10-nm-thick metal (Al, Ag, or Au) plasmonic layer that was covered with a 100-nm-thick 4,4'-bis(N-carbazolyl)-1,1'-biphenyl spacer layer and a 250-nm-thick 2,7-bis[9,9-di(4-methylphenyl)-fluoren-2-yl]-9,9-di(4-methylphenyl)fluorene light-emitting layer; the layer structure was grown on a 20-μm-diameter silica microsphere. When compared with a reference structure without the plasmonic layer, the resonators, which included either Al or Ag, showed almost the same threshold excitation intensities for generation of amplified spontaneous emission (ASE). This result indicates that the ease of light amplification in the plasmonic resonators was comparable to that in the reference structure. Excitons that exist in the vicinity of metal thin films are generally easy to quench because propagating surface plasmon polaritons (SPPs) absorb the exciton energy. Therefore, the observed comparability demonstrates that the plasmonic WGM resonators overcome this quenching effect on ASE via localization of the SPPs in the vicinity of the excitons.

Device parameter to evaluate exciton energy transfer in organic whispering-gallery-mode microresonators and its dependence on the amplified spontaneous emission threshold.

Exciton energy transfer in organic whispering-gallery-mode (WGM) resonators and its effect on the amplified spontaneous emission (ASE) threshold have been investigated using the stilbene-based energy donor 4,4'-bis[(N-carbazole)styryl]biphenyl (BSB-Cz) and the coumarin-based energy acceptor 2,3,6,7-tetrahydro-1,1,7,7,-tetramethyl-1H,5H,11H-10-(2-benzothiazolyl)quinolizino[9,9a,1gh]coumarin (C545T). Using the stacked-layer structure of BSB-Cz/C545T/BSB-Cz, we fabricated bowl-shaped microresonators on silica microspheres with a total thickness of 250 nm fixing the thickness of the C545T layer to 1 nm. The ASE threshold depended on the thicknesses of the top and bottom BSB-Cz layers, which affect the magnitude of the energy transfer. To assess the relationship between the ASE threshold and energy transfer, we developed a device parameter to evaluate the magnitude of the energy transfer by formulating the rate equations. We found that ASE easily occurs under the condition that the C545T molecules become unable to accept energy from the BSB-Cz excitons owing to the high exciton density of C545T, and that the ASE threshold decreases with decreasing device parameter. The device parameter is useful for optimizing microresonator structures in multi-component organic WGM resonators that utilize energy transfer.

Functionalization of Phosphate and Tellurite Glasses and Spherical Whispering Gallery Mode Microresonators.

Active whispering gallery mode resonators made as spherical microspheres doped with quantum dots or rare earth ions achieve high quality factors and are excellent candidates for biosensors capable of detecting biomolecules at low concentrations. However, to produce quantum dot-doped microspheres, new low melting temperature glasses are sought, which require surface functionalization and antibody immobilization for biosensor development. Here, we demonstrate the successful functionalization of three low melting point glasses and microspheres made of them. The glasses were made from sodium borophosphate, sodium aluminophosphate, and tellurite, and then, they were functionalized using (3-glycidyloxypropyl)trimethoxysilane in ethanol- and toluene-based protocols. Proper silanization was confirmed by energy-dispersive X-ray spectroscopy and fluorescence microscopy of an amino-modified luminescent oligonucleotide probe. Fluorescence imaging showed successful silanization for all tested samples and no degradation for aluminophosphate and tellurite glasses. The strongest signal was registered for tellurite glass samples functionalized using the toluene-based silanization protocol. This conclusion implies that this functionalization method is the most efficient and is highly recommended for future antibody immobilization and biosensing application.

Fano resonance in whispering gallery mode microcavities and its sensing applications

With the advantages of high quality factor (Q) and small mode volume, whispering gallery mode (WGM) microcavities obtain lower detection limits and have been increasingly applied to the detection in physics, chemistry, and biology. The Fano resonance phenomenon, which could further improve the sensing performance in the sensitivity and detection limits because of its sharp change in phase and amplitude, has attracted wide attention and demonstrated that it could be achieved in whispering gallery mode resonators (WGMRs). Fano effect is caused by the interference between the discrete mode and the continuous mode and then shows it in the spectrum. In this paper, first, the relevant knowledge of the WGM resonator and the resonance phenomenon are introduced in detail. Second, the theory of Fano resonance is analyzed. Third, the generation methods and sensing applications of Fano resonance in WGMR in current are summarized. Finally, the existing problems and development prospects of this sensor are discussed.

Alignment-Free Coupling in Whispering Gallery Mode Resonator Based on a Tapered Capillary

Alignment-Free Coupling in Whispering Gallery Mode Resonator Based on a Tapered Capillary

Bogoliubov polaritons mediated strong indirect interaction between distant whispering-gallery-mode resonators.

We propose a method to achieve a strong indirect interaction between two distant whispering-gallery-mode (WGM) resonators in a hybrid quantum system at room temperature, even when the distance between them exceeds 40 wavelengths. By exploiting the quantum critical point, we can greatly enhance both the effective damping rate and the coupling strengths between a WGM resonator and a low-frequency polariton. We introduce a large effective frequency detuning to suppress the effective damping rate while maintaining the enhanced coupling strength. The strong indirect interaction between separated WGM resonators is mediated by a far-off-resonant low-frequency polariton through virtual excitations in a process similar to Raman process. This proposal provides a viable approach to building a quantum network based on strongly coupled WGM resonators.

Waveguide-integrated chip-scale optomechanical magnetometer.

Optomechanical magnetometers enable highly sensitive magnetic field sensing. However, all such magnetometers to date have been optically excited and read-out either via free space or a tapered optical fiber. This limits their scalability and integrability, and ultimately their range of applications. Here, we present an optomechanical magnetometer that is excited and read-out via a suspended optical waveguide fabricated on the same silicon chip as the magnetometer. Moreover, we demonstrate that thermomechanical noise limited sensitivity is possible using portable electronics and laser. The magnetometer employs a silica microdisk resonator selectively sputtered with a magnetostrictive film of galfenol (FeGa) which induces a resonant frequency shift in response to an external magnetic field. Experimental results reveal the retention of high quality-factor optical whispering gallery mode resonances whilst also demonstrating high sensitivity and dynamic range in ambient conditions. The use of off-the-shelf portable electronics without compromising sensor performance demonstrates promise for applications.

Label free optofluidic DNA hybridization detection based on suspended core fiber whispering gallery mode resonator

An optofluidic DNA biosensor based on a suspended core fiber (SCF) has been proposed for the detection of specific DNA sequence fragments. The sensor is formed by coupling a micro/nano tapered optical fiber to the cladding of an SCF, producing a whispering gallery mode (WGM) effect. The WGM resonance is sensitive to samples within the channels of the SCF. The diameter of the SCF is reduced by etching to increase refractive index sensitivity, up to 274 nm/RIU. Biomarkers are captured on the inner surface of the microfluidic channel leading to a change in the local refractive index. The experimental results show that the sensor can quantitatively detect complementary DNA (cDNA) by immobilizing probe DNA (pDNA) on the surface of the microfluidic channel with a limit of detection of 1.5 nM. The proposed DNA biosensor provides a label-free method for DNA detection, which has great potential for multiplexed detection and realizing disease diagnostics.

Forward Brillouin Scattering Spectroscopy in Optical Fibers with Whispering‐Gallery Modes

AbstractOpto‐mechanical interactions in different photonic platforms as optical fibers and optical microresonators are raising great attention, and new exciting achievements have been reported in the last few years. Transverse acoustic mode resonances (TAMRs) in optical fibers –which can be excited optically via electrostriction and generate forward Brillouin scattering (FBS)– are being promoted as the physical mechanism for new fiber‐sensing concepts. Here, the study reports a novel approach to detect and characterize opto‐excited TAMRs of an optical fiber based on the interplay with optical surface wave resonances, i.e., optical whispering‐gallery mode (WGM) resonances. TAMRs induce perturbations in the geometry and the dielectric permittivity of the fiber over the entire cross‐section. It is shown that these perturbations couple the acoustic with the optical resonances and affect WGMs in a noticeable way. The study proposes and demonstrates the use of WGMs for probing opto‐excited TAMRs in optical fibers. This probing technique provides the narrowest linewidths ever reported for the TAMRs and demonstrates an optimum efficiency for the detection of low‐order TAMRs. The interplay between sensitivity, bandwidth, and Q factor of the WGM resonance is discussed.

Development and analysis of whispering gallery mode model for refractive index sensing

A refractive index sensor based on a whispering gallery mode resonator is numerically investigated in this paper. Whispering gallery mode resonators confine light and can be used in sensing applications, and this work presents the model built using COMSOL software to analyze their sensing performance. This work has investigated the WGM resonators’ response to refractive index changes numerically using 2D models in the refractive index ranges 1.000 and 1.333. The resonator showed a sensitivity of 167 nm/RIU in the refractive index range of 1.3331.4 and a sensitivity of 95 nm/RIU in the refractive index range of 1.000-1.010. The sensing resonator has potential applications for biological and chemical analytes.

Soliton microcomb-assisted microring photonic thermometer with ultra-high resolution and broad range

Whispering gallery mode resonators (WGMRs) have proven their advantages in terms of sensitivity and precision in various sensing applications. However, when high precision is pursued, the WGMR demands a high-quality factor usually at the cost of its free spectral range (FSR) and corresponding measurement range. In this article, we propose a high-resolution and wide-range temperature sensor based on chip-scale WGMRs, which utilizes a Si3N4 ring resonator as the sensing element and a MgF2-based microcomb as a broadband frequency reference. By measuring the beatnote signal of the WGM and microcomb, the ultra-high resolution of 58 micro-Kelvin (μK) was obtained. To ensure high resolution and broad range simultaneously, we propose an ambiguity-resolving method based on the gradient of feedback voltage and combine it with a frequency-locking technique. In a proof-of-concept experiment, a wide measurement range of 45 K was demonstrated. Our soliton comb-assisted temperature measurement method offers high-resolution and wide-range capabilities, with promising advancements in various sensing applications.

Gallium arsenide whispering gallery mode resonators for terahertz photonics.

As the field of terahertz (THz) photonics advances, we present a monolithic gallium arsenide (GaAs) disk-shaped whispering gallery mode resonator that has potential as a component in THz nonlinear optics. GaAs is a material with significant optical nonlinearity which can be enhanced when the crystal is shaped into a microdisk resonator. A 4-mm-disk-resonator was fabricated using single-point diamond turning and was characterized to obtain a quality (Q) factor of 2.21k at ∼150 GHz and 1.41k at ∼300 GHz. We also demonstrated the blue-shifting of up to ∼0.3 GHz of the THz modes using a block of metal. This post-fabrication degree of freedom could be useful for phase-matching requirements for nonlinear optical processes, such as detection based on optical up-conversion of THz radiation. This proof-of-concept demonstration can pave the way for the implementation of a compact, tunable and efficient device which could be integrated into nonlinear photonic platforms for THz generation, manipulation and detection.

Thermo-optomechanically induced optical frequency comb in a whispering-gallery-mode resonator.

We present a theoretical study that combines thermal and optomechanical effects to investigate their influences on the formation of the optical frequency comb (OFC) in whispering-gallery-mode (WGM) microcavities. The results show that the cut-off order and center frequency of OFC affected by thermal effects exhibit an overall redshift by varying the power and detuning of the pump field, which provides the possibility of tuning the offset frequency of OFC. Our study demonstrates a method to characterize the effect on the generation of OFC and the tuning of its offset frequency in a WGM resonator with opto-thermo-mechanical properties and pave the way for the future development of OFC in thermo-optomechanical environments.

Design of terahertz plasmonic wavelength division multiplexer assisted by whispering gallery mode resonators

Design of terahertz plasmonic wavelength division multiplexer assisted by whispering gallery mode resonators

Encaved optical fiber nano-probe exciting whispering gallery mode resonance with focused far off-axis beam.

This paper demonstrates whispering gallery mode (WGM) resonance with the help of an encaved optical nano-probe developed inside an optical fiber tip cavity. The nano-probe generates a tightly focused beam with a spot-size of ∼3 µm. A barium titanate microsphere is placed besides the optical axis inside the cavity. The focused beam remains off-axis of the microresonator and excites the WGM. The off-axis excitation shows unique resonating properties depending on the location of the resonator. A resonant peak with quality factor as high as Q ∼7 × 104 is achieved experimentally. Another design with a shorter cavity length for a bigger resonator is also demonstrated by embedding a bigger microsphere on the cleaved fiber tip surface. The optical probe holds great potential for photonic devices and is ideal for studying morphology-based scattering problems.

Quantum-Dot-Induced Modification of Surface Functionalization for Active Applications of Whispering Gallery Mode Resonators.

Quantum dots can modify the properties of the whispering gallery mode resonators (WGMRs) used in various potential applications. A deposition of a suitable nanomaterial for the surface functionalization of WGMRs allows for the achievement of high quality (Q) factors. Here, we show that the WGMR surface can be functionalized using quantum dots. We demonstrate that WGMRs covered with thin layers of HgS and PbS quantum dots are suitable for third-harmonic generation due to the high Q factor of the developed microresonators, thus significantly lowering the pumping power required for nonlinear optical interactions.

Whispering Gallery Mode Microresonator Sensor Integrated in Exposed Core Fiber for Label-Free DNA Hybridization Detection

A novel optical fiber sensor using exposed-core fiber (ECF) to excite whispering gallery modes (WGMs) within a high refractive index barium titanate glass microsphere is proposed for achieving label-free real-time specific DNA detection. The microsphere is encapsulated into the exposed channel of the ECF allowing for physical stability while excited WGMs via the evanescent field. The structure enables the sensing area to be exposed to a large amount of aqueous solution and better contact with the sample to be analyzed. Using a transmission measurement, a high Q-factor in the order of 10 <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">4</sup> is obtained in an aqueous environment. To the best of our knowledge, this is the best Q-factor level obtained by the in fiber WGM sensor in an aqueous environment. Specific sequences of probe DNA are then bound to the surface of the microsphere so that specific detection of complementary DNA can be realized by tracking the wavelength shift the WGM resonance. Experimental results show a red shift of 5.6 pm for complementary DNA hybridization detection and less than 1 pm fluctuation for non-complementary DNA detection. The portable integrated sensor with miniature size has great potential for aqueous environmental sensing applications in the fields of diseases diagnostics, chemical analysis, and environmental protection.

From Whispering Gallery Mode Resonators to Biochemical Sensors.

Optical biosensors are frontrunners for the rapid and real-time detection of analytes, particularly for low concentrations. Among them, whispering gallery mode (WGM) resonators have recently attracted a growing focus due to their robust optomechanical features and high sensitivity, measuring down to single binding events in small volumes. In this review, we provide a broad overview of WGM sensors along with critical advice and additional "tips and tricks" to make them more accessible to both biochemical and optical communities. Their structures, fabrication methods, materials, and surface functionalization chemistries are discussed. We propose this reflection under a pedagogical approach to describe and explain these biochemical sensors with a particular focus on the most recent achievements in the field. In addition to highlighting the advantages of WGM sensors, we also discuss and suggest strategies to overcome their current limitations, leaving room for further development as practical tools in various applications. We aim to provide new insights and combine different knowledge and perspectives to advance the development of the next generation of WGM biosensors. With their unique advantages and compatibility with different sensing modalities, these biosensors have the potential to become major game changers for biomedical and environmental monitoring, among many other relevant target applications.

Large measurement range temperature sensor based on WGM and MMI in an offset structure fiber coupler

In this paper, a coupler based on a single-mode fiber (SMF)- no-core fiber (NCF)- SMF offset structure was proposed and demonstrated, which can generate the evanescent field to excite whispering gallery mode (WGM) of a microsphere cavity. By reasonably controlling the length and offset distance of NCF, the multimode interference (MMI) and WGMs can be generated at the same time. The experimental results show that the temperature measurement with a large measurement range and low detection limit can be realized simultaneously with the assistance of the interference envelope, which solves the problem of large range measurement difficulty caused by the dense dips of WGM to some extent. In the range of 22 ℃-80 ℃, the sensitivity of WGM resonant dips is ∼10.5 pm/℃. On the other hand, symmetric Lorenz lines with a quality factor of 8.2 × 103 and asymmetric Fano lines with a slope of -21.94 dB/nm were obtained under the modulation of interference. The coupler proposed in this paper has the advantages of simple preparation and strong structural robustness, and shows good potential in applications such as sensors and filters.

Spatial Multiplexing of Whispering Gallery Mode Sensors.

Whispering gallery mode resonators have proven to be robust and sensitive platforms for the trace detection of chemical and/or biological analytes. Conventional approaches using serially addressed resonators face challenges in simultaneous multi-channel (i.e., multi-species) detection. We present an alternative monitoring scheme that allows for the spatial multiplexing of whispering gallery mode resonators with the simultaneous observation of the resonance spectra from each of them. By imaging arrays of microspheres and monitoring the glare spot intensities through image processing routines, resonance spectra from multiple resonators may be simultaneously recorded without interference or confounding effects of serial excitation/detection. We demonstrate our multiplexed imaging approach with bulk refractive index variations and virus-antibody binding.