Wavelength Regime Research Articles

Measurement of interstellar extinction for classical T Tauri stars using far-UV H_2 line fluxes

Understanding the interstellar and potentially circumstellar extinction in the sight lines of classical T Tauri stars is an important ingredient for constructing reliable spectral energy distributions, which catalyze protoplanetary disk chemistry, for example. Therefore, some attempts of measuring $A_ V $ toward individual stars have been made using partly different wavelength regimes and different underlying assumptions. We used strong lines of Lyalpha fluorescent H$_ and derived the extinction based on the assumption of optically thin transitions. We investigated a sample of 72 classical T Tauri stars observed with the Hubble Space Telescope in the framework of the ULLYSES program. We computed $A_V$ and $R_V$ values for the 34 objects with sufficient data quality and an additionally $A_V$ value for the canonical $R_V=3.1$ value. Our results agree largely with values obtained from optical data. Moreover, we confirm the degeneracy between $A_ V $ and $R_ V $ and present possibilities to break this. Finally, we discuss whether the assumption of optical thin lines is valid.

PEPSI’s non-detection of escaping hydrogen and metal lines adds to the enigma of WASP-12 b

ABSTRACT WASP-12 b is an ultra-hot Jupiter of special interest for atmospheric studies since it is on an inspiraling orbit in an extreme environment of intense radiation and circumstellar gas. Previously claimed detections of active mass-loss from this planet are controversial across the literature. To address this controversy, we obtain two new transit observations of WASP-12 b with the optical high-resolution PEPSI spectrograph on the Large Binocular Telescope. Contrary to previous work, we do not observe planetary H$\alpha$ absorption and rule out the amplitude of previously reported detections. Our non-detection may be limited by the sensitivity of our data or could indicate weaker mass-loss than suggested by previous studies. We conduct injection-recovery experiments to place constraints on the radial extent of WASP-12 b’s escaping atmosphere as probed by Balmer lines, but find that our data do not have the sensitivity to probe down to the planet’s Roche lobe. Using physically motivated models of atmospheric escape, we explore upper limit constraints on the planet’s mass-loss rate and deem the data quality in the wavelength regime of Balmer lines insufficient to determine a physically meaningful constraint. We also conduct a spectral survey of other optical absorbers to trace atmospheric circulation but detect no additional absorption. We conclude that previous claims of H$\alpha$ absorption from the atmosphere of WASP-12 b should be reevaluated. Given the anticipated line strength of Balmer/optical features, observing the atmosphere of this faint target will require stacking more observations even with the largest telescope facilities available.

MANTA-Ray: Supercharging speeds for calculating the optical properties of fractal aggregates in the long-wavelength limit

Abstract Correctly modelling the absorptive properties of dust and haze particles is of great importance for determining the abundance of solid matter within protoplanetary disks and planetary atmospheres. Rigorous analyses such as the discrete dipole approximation (DDA) can be used to obtain accurate absorption cross-sections, but these require significant computing time and are often impractical to use in models. A simple analytical equation exists for spherical particles in the long-wavelength limit (where the wavelength is much larger than the size of the dust particle), but we demonstrate that this can significantly underestimate the absorption. This effect is found to depend strongly on refractive index, with values of m = 1 + 11i corresponding to an underestimate in absorption by a factor of 1,000. Here we present MANTA-Ray (Modified Absorption of Non-spherical Tiny Aggregates in the RAYleigh regime): a simple model that can calculate absorption efficiencies within 10-20% of the values predicted by DDA, but 1013 times faster. MANTA-Ray is very versatile and works for any wavelength and particle size in the long wavelength regime. It is also very flexible with regards to particle shape, and can correctly model structures ranging from long linear chains to tight compact clusters, composed of any material with refractive index 1+0.01i ≤m ≤ 11+11i. The packaged model is provided as publicly-available code for use by the astrophysical community.

Four-Wave Mixing Bragg Scattering for small frequency shift from Silicon Coupled Microrings

Abstract Frequency conversion is pivotal in nonlinear optics and quantum optics for manipulating and translating light signals across different wavelength regimes. Achieving frequency conversion between two light beams with small frequency interval is a central challenge. In this work, we design a pair of coupled silicon microrings wherein coupled-induced mode-splitting exists to achieve a small frequency shift by the process of four-wavemixing Bragg scattering. As an example, the signal can be up or down converted to the idler which is 15.5 GHz spaced when two pumps align with another pair of splitted resonances. The results unveil the potential of coupled microring resonators for small interval frequency conversion in the fields of high-fidelity all-optical signal processing quantum frequency interface.

Expanding the scope of resonance Raman spectroscopy in hydrogenase research: New observable states and reporter vibrations

Oxygen-tolerant [NiFe] hydrogenases are valuable blueprints for the activation and evolution of molecular hydrogen under application-relevant conditions. Vibrational spectroscopic techniques play a key role in the investigation of these metalloenzymes. For instance, resonance Raman spectroscopy has been introduced as a site-selective approach for probing metal-ligand coordinates of the [NiFe] active site and FeS clusters. Despite its success, this approach is still challenged by a limited number of detectable active-site states – due to missing resonance enhancement or intrinsic light sensitivity – and difficulties in their assignment. Utilizing two oxygen-tolerant [NiFe] hydrogenases as model systems, we illustrate how these challenges can be met by extending excitation and detection wavelength regimes in resonance Raman spectroscopic studies. Specifically, we observe that this technique does not only probe low-frequency metal-ligand vibrations but also high-frequency intra-ligand modes of the diatomic CO/CN− ligands at the active site of [NiFe] hydrogenases. These reporter vibrations are routinely probed by infrared absorption spectroscopy, so that direct comparison of spectra from both techniques allows an unambiguous assignment of states detected by resonance Raman spectroscopy. Moreover, we find that a previously undetected state featuring a bridging hydroxo ligand between Ni and Fe can be probed using higher excitation wavelengths, as photoconversion occurring at lower wavelengths is avoided. In summary, this study expands the applicability of resonance Raman spectroscopy to hydrogenases and other complex metalloenzymes by introducing new strategies for probing and assigning redox-structural states of the active site.

Giant Optical Anisotropy in 2D Metal-Organic Chalcogenates.

Optical anisotropy is a fundamental attribute of some crystalline materials and is quantified via birefringence. A birefringent crystal gives rise to not only asymmetrical light propagation but also attenuation along two distinct polarizations, a phenomenon called linear dichroism (LD). Two-dimensional (2D) layered materials with high in-plane and out-of-plane anisotropy have garnered interest in this regard. Mithrene, a 2D metal-organic chalcogenate (MOCHA) compound, exhibits strong excitonic resonances due to its naturally occurring multiquantum well (MQW) structure and in-plane anisotropic response in the blue wavelength (∼400-500 nm) regime. The MQW structure and the large refractive indices of mithrene allow the hybridization of the excitons with photons to form self-hybridized exciton-polaritons in mithrene crystals with appropriate thicknesses. Here, we report the giant birefringence (∼1.01) and the tunable in-plane anisotropic response of mithrene, which stem from its low symmetry crystal structure and strong excitonic properties. We show that the LD in mithrene can be tuned by leveraging the anisotropic exciton-polariton formation via the cavity coupling effect, exhibiting giant in-plane LD (∼77.1%) at room temperature. Our results indicate that mithrene is a polaritonic birefringent material for polarization-sensitive nanophotonic applications in the short wavelength regime.

Experimental Observation of Raman Assisted and Kerr Optical Frequency Comb in a 4H-Silicon-Carbide on Insulator Microresonator

Kerr nonlinear microcavities have garnered significant interest owing to their rich dynamics of nonlinear optical phenomena and compatibility with on-chip photonic integration. Recently, silicon carbide has emerged as a compelling platform due to its unique optical properties. In this study, we demonstrate Raman-assisted and Kerr optical frequency generation in a 4H-silicon carbide-on-insulator microresonator. By pumping the transverse electric (TE00) mode within the device, we observe a stimulated Raman scattering (SRS) Stokes with the Raman shift at approximately 775 cm-1, achieved with an on-chip power of 350 mW. Furthermore, by red-tuning the TE00 pump wavelength, we have achieved the coexistence of Raman and Kerr frequency combs. Using another device on the same chip with light variation of the taper we can observe the Raman and Kerr frequency combs within a spectral bandwidth ranging from ∼ 1440 to 1960 nm. The inclusion of the Raman-assisted comb extends the comb’s coverage into longer wavelength regimes, making it highly desirable for spectroscopy applications.

Key parameters to optimize the photothermoelectric effect of thermoelectric materials

Recently, photothermoelectric effect of thermoelectric materials has been hotly explored to develop self-powered and large bandwidth photodetectors working at ambient conditions. However, the key parameters for optimized photothermoelectric effect are still elusive. Here, based on the two-temperature model under static condition, we theoretically studied the key parameters to optimize the photothermoelectric performance of thermoelectric materials. Results verify that when the incident electromagnetic wave only generates electronic intra-band excitation, there is an ideal carrier concentration to optimize the photothermoelectric voltage; when the wavelength of a detected electromagnetic wave can resonantly excite quasi-particle (like phonons) except electrons, the photothermoelectric voltage can be enhanced significantly around the resonant wavelength regime; and when the electronic inter-band transition can be excited by an electromagnetic wave, photothermoelectric voltage is significantly increased due to the high optical absorption. As an example, the theoretical dependence of the photothermoelectric voltage of SnSe on wavelength is in line with the experimental result. This work elucidates the crucial parameters of thermoelectric materials to achieve the ideal photothermoelectric performance.

Nonlinear wave propagation in large extra spatial dimensions and the blackbody thermal laws

Abstract Nonlinear wave propagation in large extra spatial dimensions (on and above d = 2) is investigated in the context of nonlinear electrodynamics theories that depend exclusively on the invariant F ( = − ( 1 / 4 ) F μ ν F μ ν ) . In this vein, we consider propagating waves under the influence of external uniform electric and magnetic fields. Features related to the blackbody radiation in the presence of a background constant electric field such as the generalization of the spectral energy density distribution and the Stefan–Boltzmann law are obtained. Interestingly enough, anisotropic contributions to the frequency spectrum appear in connection to the nonlinearity of the electromagnetic field. In addition, the long wavelength regime and Wien’s displacement law in this situation are studied. The corresponding thermodynamics quantities at thermal equilibrium, such as energy, pressure, entropy, and heat capacity densities are contemplated as well.

Octave‐Spanning Second‐Harmonic Generation in Dispersion‐Engineered Lithium Niobate‐on‐Insulator Microwaveguide

Broadband lasers, e.g., ultrashort lasers, optical supercontinuum, and frequency combs, are revolutionary coherent light sources, which enable a plethora of state‐of‐the‐art applications ranging from precision spectroscopy to optical clocks. However, the spectral broadening of these coherent light sources mainly relies on the third‐order nonlinearity () and is difficult to extend to the visible or shorter wavelength regime. Second‐order nonlinearity (), which is orders of magnitude larger than , becomes a powerful tool for the frequency translation if its broadband operation is well addressed. Herein, an octave‐spanning second‐harmonic generation scheme is experimentally demonstrated beyond an extremely large frequency range of 135 THz and high conversion efficiency of 1% for sub‐100 pJ for the near‐infrared picosecond supercontinuum in a fiber–waveguide–fiber configuration. The process relies on ultrabroadband birefringence phase matching in the dispersion‐engineered lithium niobate‐on‐insulator ridge microwaveguide. The mode area of microwaveguide well matches with single‐mode lens fiber, reducing coupling loss and ensuring easy packaging. The method provides a new approach to span the wavelength range of coherent light with ‐based wavelength translation for supercontinuum or frequency combs into the visible regime. The result would find applications in spectroscopy, astrophysics, atomic optics, optical synthesis, etc.

Science development study for the Atacama Large Aperture Submillimeter Telescope (AtLAST): Solar and stellar observations.

Observations at (sub-)millimeter wavelengths offer a complementary perspective on our Sun and other stars, offering significant insights into both the thermal and magnetic composition of their chromospheres. Despite the fundamental progress in (sub-)millimeter observations of the Sun, some important aspects require diagnostic capabilities that are not offered by existing observatories. In particular, simultaneously observations of the radiation continuum across an extended frequency range would facilitate the mapping of different layers and thus ultimately the 3D structure of the solar atmosphere. Mapping large regions on the Sun or even the whole solar disk at a very high temporal cadence would be crucial for systematically detecting and following the temporal evolution of flares, while synoptic observations, i.e., daily maps, over periods of years would provide an unprecedented view of the solar activity cycle in this wavelength regime. As our Sun is a fundamental reference for studying the atmospheres of active main sequence stars, observing the Sun and other stars with the same instrument would unlock the enormous diagnostic potential for understanding stellar activity and its impact on exoplanets. The Atacama Large Aperture Submillimeter Telescope (AtLAST), a single-dish telescope with 50m aperture proposed to be built in the Atacama desert in Chile, would be able to provide these observational capabilities. Equipped with a large number of detector elements for probing the radiation continuum across a wide frequency range, AtLAST would address a wide range of scientific topics including the thermal structure and heating of the solar chromosphere, flares and prominences, and the solar activity cycle. In this white paper, the key science cases and their technical requirements for AtLAST are discussed.

Space–time characterization of ultrashort laser pulses: A perspective

The characterization of ultrashort laser pulses has significantly advanced beyond the standard spatial and temporal diagnostics to now include sophisticated spatio-temporal measurement techniques. In this perspective, we provide an overview of the current state of space–time characterization, discussing the theoretical foundations of ultrashort laser pulses, the various measurement techniques and their design trade-offs, and the challenges and opportunities for future development. We explore the extension of these techniques to different wavelength regimes and delve into the unique challenges posed by the characterization of polarization-structured beams. The potential for data-driven analysis to enhance the information extracted from the measurements is highlighted, along with the need for direct measurement of previously inaccessible field components, such as the longitudinal electric field in tightly focused beams. As these diagnostic tools continue to evolve, we anticipate a future where the intricate space–time structure of light can be analyzed on a routine basis, opening up new frontiers in ultrafast science and technology.

Modulation instability of magnetosonic waves in semiconducting quantum plasma considering Fermi degenerate pressure, exchange correlation potential, and Bohm potential

This study investigates the modulation instability of magnetosonic waves in a semiconducting quantum plasma system. Utilizing the quantum hydrodynamic model, we derive the nonlinear Schrödinger equation and its solution through the reductive perturbation technique. The growth rate of modulation instability for magnetosonic waves has been derived. This study incorporates various quantum corrections, including Fermi degenerate pressure, exchange-correlation potential, and Bohm potential. We study the bright soliton profiles of magnetosonic waves, and additionally, we conduct graphical analyses of the linear dispersion relation and the product of the dispersive coefficient (P) and nonlinear coefficient (Q) of the nonlinear Schrödinger equation. It has been found that magnetosonic waves exhibit modulation instability within specific parameter ranges of the semiconductor plasma and at certain wavelength regimes. Further, we present a comparative study between GaSb and InSb semiconducting plasma systems. The exchange-correlation potential and Fermi degenerate pressure have significantly impacted the modulation instability growth rate, whereas the effect of the Bohm potential is much lower.

3D laser activatable alloy-free solid/liquid biphasic conductive composites for additive manufacturable electronics

Recently, biphasic soft conductors have gained tremendous attention owing to their characteristic advantages by co-existence of solid and liquid metals. In this study, we developed the 3D printable composite that can generate alloy-free solid/liquid biphasic conductive features by 3D green-laser activation process. It comprises copper nanoparticles with localized surface plasmonic resonance in the visible wavelength regime, eutectic indium-gallium liquid metal droplets, and polyvinylpyrrolidone as a multifunctional polymeric additive. We clarify that, based on the photothermal simulation results, an instant thermal heating is triggered in the vicinity of copper nanoparticles upon green laser irradiation, which activates, comprehensively, the overall microstructural evolution reactions, including a rupture of the oxide shell surrounding the liquid metal droplets, a formation of networked copper particulate assemblies, and a combustion-free carbonization of polymeric substances. This allows us to generate double-layered biphasic conductive features in which the solid conductive compartments are in individual contact with the densified liquid metal bulks, enabling to achieve a high conductivity, excellent flexibility, self-healing capability, and solder processability without the critical problem of leakage of liquid metals.

Nuclear quantum memory for hard x-ray photon wave packets.

Optical quantum memories are key elements in modern quantum technologies to reliably store and retrieve quantum information. At present, they are conceptually limited to the optical wavelength regime. Recent advancements in x-ray quantum optics render an extension of optical quantum memory protocols to ultrashort wavelengths possible, thereby establishing quantum photonics at x-ray energies. Here, we introduce an x-ray quantum memory protocol that utilizes mechanically driven nuclear resonant 57Fe absorbers to form a comb structure in the nuclear absorption spectrum by using the Doppler effect. This room-temperature nuclear frequency comb enables us to control the waveform of x-ray photon wave packets to a high level of accuracy and fidelity using solely mechanical motions. This tunable, robust, and highly flexible system offers a versatile platform for a compact solid-state quantum memory at room temperature for hard x-rays.

Measurement of the linewidth of a home-built vacuum ultraviolet comb by frequency comb spectroscopy on NO2.

Optical frequency comb in the vacuum ultraviolet (VUV)/extreme ultraviolet (XUV) region has attracted a great deal of attention, as it provides coherent VUV/XUV radiation source with a rather narrow bandwidth, facilitating precise spectroscopic measurements in the short wavelength regime. In this study, we report on the linewidth measurement of a home-built VUV comb centered at 148 nm using direct frequency comb spectroscopy with NO2. The measurement reveals that the upper bound of our comb linewidth is less than 28 MHz. Fitting the whole trace with different repetition rates shows that the center frequency of the excitation is 2 021.25 ± 0.24 THz (∼148.32 nm). Thus, we assigned this excitation to the transition from the 6a1 orbital (ν1'=0, ν2'=0) to the 3pσu orbital (ν1'=3, ν2'=8) in NO2. Our work demonstrates that VUV combs are potentially powerful tools for precision spectroscopic measurements in the short wavelength regime.

Extrapolation of Type Ia Supernova Spectra into the Near-infrared Using Principal Component Analysis

We present a method of extrapolating the spectroscopic behavior of Type Ia supernovae (SNe Ia) in the near-infrared (NIR) wavelength regime up to 2.30 μm using optical spectroscopy. Such a process is useful for accurately estimating K-corrections and other photometric quantities of SNe Ia in the NIR. A principal component analysis is performed on data consisting of Carnegie Supernova Project I & II optical and NIR FIRE spectra to produce models capable of making these extrapolations. This method differs from previous spectral template methods by not parameterizing models strictly by photometric light-curve properties of SNe Ia, allowing for more flexibility of the resulting extrapolated NIR flux. A difference of around −3.1% to −2.7% in the total integrated NIR flux between these extrapolations and the observations is seen here for most test cases including Branch core-normal and shallow-silicon subtypes. However, larger deviations from the observation are found for other tests, likely due to the limited high-velocity and broad-line SNe Ia in the training sample. Maximum-light principal components are shown to allow for spectroscopic predictions of the color-stretch light-curve parameter, s BV, within approximately ±0.1 units of the value measured with photometry. We also show these results compare well with NIR templates, although in most cases the templates are marginally more fitting to observations, illustrating a need for more concurrent optical+NIR spectroscopic observations to truly understand the diversity of SNe Ia in the NIR.

Spectroflat: A generic spectrum and flat-field calibration library for spectro-polarimetric data

Flat-fielding spectro-polarimetric data with one spatial and one spectral dimension is inherently difficult as the imprint of the spectral lines needs to be separated from other wavelength-dependent instrumental effect (e.g., fringes or prefilter profiles) and wavelength-independent effects (e.g., dust and sensor response). Current approaches for spectrometers are often based on moving the grating or they depend on optical models and/or on lab calibration data. They are also limited to small spectral regions and are instrument-specific. Approaches that would be suitable for polarimeters have not been reported yet. We present an approach that allows for flat-field calibration data to be to obtained for diffraction-grating-based, long-slit spectrographs combined with temporally modulated polarimetry from high-resolution solar telescopes. This approach is based on nominal flat-fielding procedures performed during the instrument's science operations. We performed a precise and field-dependent correction of the spectrographic distortion effect (resulting in curved spectral lines, typically denoted as a "smile" effect) to ensure the orthogonality of the spectral and spatial dimensions. We identified distortions by tracking the position of multiple spectral lines within the full spectral field of view. From the raw modulated flats, we then removed the solar line imprints and derived separate flat-fields for sensor and slit dust features. Optionally, wavelength calibration and continuum correction can be included in this process. We have created generic Python libraries that can be plugged into existing Python-based data reduction pipelines or used as a standalone calibration tool. We show that for spectrographs covering many spectral lines, a correction of the smile distortion based on optical models alone is not sufficient. Our results demonstrate a suppression of fringes, sensor artifacts, and fixed-pattern imprints in demodulated data by one order of magnitude. For intensity images, the photon noise level can be closely attained after calibration. Our correction works across the full spectral range. The algorithm was tested for different wavelength regimes with emission (EUV range) or absorption (near-UV, VIS, IR range) spectra, on data acquired with ground-based (SST/TRIPPLE-SP, GREGOR/GRIS), balloon-borne (SUNRISE-III/SUSI), and space-based (SolO/SPICE) instruments. The data calibrated with our method offer robust and precise inversion results. We have extended existing spectroscopic flat-field techniques to modern instruments with large imaging sensors covering many spectral lines simultaneously, and with polarimetric capabilities, where methods described so far are not adequate. We believe that our method is applicable as a standard calibration approach for most modern high resolution large-FOV, long-slit spectrographs -- both with and without polarimetric capabilities.

High-power and high-speed all-optical all-fiber wavelength-swept source at 2 μm based on a femtosecond laser and time stretch technique

We present an all-fiber all-optical high-speed wavelength-swept laser source at 2 μm with a 3-dB bandwidth of 33 nm and repetition rate of 18.4 MHz, by using optical time-stretch technology, which to our knowledge is the first report of a 2 μm wavelength-swept source without any bulk, free-space optical elements. The light source is built upon a nonlinear polarization rotation mode-locked femtosecond oscillator. A chirped fiber Bragg grating (CFBG) is employed to realize the all-optical wavelength sweeping. In comparison with the commonly used dispersive fibers, the CFBG possesses outstanding power efficiency and temporal stability, especially for wavelength sweeping in the 2.0 μm wavelength regime. A two-stage fiber amplifier system is utilized to boost the output power up to 1.01 W. This all-fiberized mode-locked swept source with high speed and high stability shows great potential as a valuable source for various spectroscopy applications and swept source optical coherence tomography, particularly for highly scattering medium with low water content.

Coherent light-emitting metasurfaces based on bound states in the continuum

Abstract An emergent need exists for solid state tunable coherent light emitters in the mid-infrared range for spectroscopy, sensing, and communication applications where current light sources are dominated by spontaneous emitters. This paper demonstrates a distinct class of coherent thermal emitters operating in the mid-infrared wavelength regime. The structure of the light source consists of a dielectric metasurface fabricated on a phononic substrate. In this study, we present the first implementation of off-Γ Friedrich–Wintgen bound states in the continuum at mid-infrared wavelengths suitable for developing the next generation of coherent light emitters. Numerical analysis of the emissivity spectrum reveals the interference of resonances leading to avoided crossings and the formation of Friedrich–Wintgen bound states in the radiation spectrum. Additionally, significant localized field enhancements are observed within the metasurface at operating wavelengths. The emissivity spectra measured by reflectivity and emission experiments exhibit temporally coherent emission peaks in the vicinity of the bound state in the continuum, the first such demonstration in the mid-infrared region for wavelengths longer than 7 µm. These results represent a new approach for significant advancement in realizing mid-infrared coherent light emitters with promising implications for future technologies.