Incident Wavelength Research Articles

Ultra-broadband achromaticity of metalens with low-relative phase enabled by wide-band fusion

Metalenses have a high design degree of freedom in controlling the light field and excellent performance in chromatic aberration elimination. However, in designing ultra-broadband achromatic metalenses, integrating multiple types of unit structures is necessary to compensate for phase differences caused by different incident wavelengths. Here, we propose an ultra-broadband achromatic metalens composed only of a single type of square nano-pillar. which controls the entire operating band by utilizing three wide-band fusions, and have characteristics depending on the phase coverage and relative phase. In the operational range of 2–5 μm, the achromatic metalens demonstrates a maximum focal shift of 2.1 μm. The average focal shift is 0.98 %, the average NA value is 0.35, with an average relative phase of 0.77π. The average transmittance and focus efficiency are 94.17 % and 58.7 %, respectively. This broad-spectrum fusion design strategy simplifies manufacturing complexity while maintaining high focusing efficiency and transmittance levels throughout the entire operational bandwidth. This design approach can improve image resolution and quality by minimizing chromatic aberration.

High-performance flexible and broadband photodetectors on paper substrates using FeSnS bimetallic sulfide nanosheets

Advancements in technology have made it easier to construct flexible broadband photodetectors for wearable devices, improving light harvesting and detecting capabilities. This work described a new study that used bimetallic sulfide nanosheets (FeSnS) to produce flexible and broadband photodetectors on paper substrates using hand-print method. A simple, economical, one-step hydrothermal technique was employed to synthesise FeSnS materials, which were characterised using XRD, UV–Vis Spectroscopy, FESEM, EDS, XPS, and UPS. Photodetection tests found that 2-FeSnS (Fe at 2 wt%) outperformed similar work on paper-based devices, with a responsivity of 32.4 mA/W under a 470 nm incident wavelength, high specific detectivity, and a response time of 1.16 s. Durability and flexibility testing validated the robustness of the device. The use of a simple hydrothermal synthesis and hand-print fabrication method to create high-performance, eco-friendly, and flexible photodetectors is novel, expanding their potential applications in wearable electronics, environmental monitoring, and low-cost disposable sensing platforms.

Holographic Multi-Notch Filters Recorded with Simultaneous Double-Exposure Contact Mirror-Based Method

This study presents a novel simultaneous double-exposure contact mirror-based method for fabricating holographic multi-notch filters with dual operational central wavelengths. The proposed method leverages coupled wave theory, the geometric relationships of K-vectors, and a reflection-type recording setup, incorporating additional reflecting mirrors to guide the recording beams. To validate the approach, a holographic notch filter was fabricated using photopolymer recording materials, resulting in operational wavelengths of 531.13 nm and 633.01 nm. The measured diffraction efficiencies at these wavelengths were ηs = 52.35% and ηp = 52.45% for 531.13 nm, and ηs = 67.30% and ηp = 67.40% for 633.01 nm. The component’s performance was analyzed using s- and p-polarized spectral transmission intensities at various reconstruction angles, revealing polarization-independent characteristics under normal incidence and polarization-dependent behavior under oblique incidence. The study also explored the relationships between recording parameters, such as incident angle, wavelength, emulsion expansion, and dispersion. The findings demonstrate that the first operational central wavelength is primarily influenced by the recording wavelength, while the second is primarily determined by the incident angle, covering a range from visible light to near-infrared. This method offers significant potential for cost-effective, mass-produced filters in optoelectronic applications.

Self-induced transparency of long water waves over bathymetry: the dispersive shock mechanism

The shoreline hazard posed by ocean long waves such as tsunamis and meteotsunamis critically depends on the fraction of energy transmitted across the shallow near-shore shelf. In linear setting, bathymetric inhomogeneities of length comparable to the incident wavelength act as a protective high-pass filter, reflecting long waves and allowing only shorter waves to pass through. Here, we show that, for weakly nonlinear waves, the transmitted energy flux fraction can significantly depend on the amplitude of the incoming wave. The basis of this mechanism is the formation of dispersive shock waves (DSWs), a salient feature of nonlinear evolution of long water waves, often observed in tidal bores and tsunami/meteotsunami evolution. Within the framework of the Boussinesq equations, we show that the DSWs efficiently transfer wave energy into the high wavenumber band, where reflection is negligible. This is phenomenologically similar to self-induced transparency in nonlinear optics: small amplitude long waves are reflected by the bathymetric inhomogeneity, while larger amplitude waves that develop DSWs blueshift into the transparency regime and pass through. We investigate this mechanism in a simplified setting that retains only the key processes of DSW disintegration and reflection, while the effects such as bottom dissipation and breaking are ignored. The results suggests that the phenomenon is a robust, order-one effect. In contrast, the increased transmission due to the growth of bound harmonics associated with the steepening of the wave is weak. The results of the simplified modelling are validated by simulations with the FUNWAVE-TVD Boussinesq model.

Analysis and Optimization of Light Absorption and Scattering Properties of Metal Nanocages.

Metal nanocages exhibit localized surface plasmon resonance that strongly absorbs and scatters light at specific wavelengths, making them potentially valuable for photothermal therapy and biological imaging applications. However, investigations on metal nanocages are still confined to high-cost and small-scale synthesis. The comprehensive analysis of optical properties and optimal size parameters of metal nanocages is rarely reported. This paper simulates the effects of materials (Ag, Au, and Cu), size parameters, refractive index of the surrounding medium, and orientation on the light absorption and scattering characteristics of the nanocages using the finite-element method and the size-dependent refractive-index model for metal nanoparticles. The results show that the Ag nanocages have excellent light absorption and scattering characteristics and respond significantly to the size parameters, while the refractive index and orientation of the surrounding medium have less effect on them. The Au nanocages also possess superior light absorption properties at specific incident wavelengths. This study also identified the optimized sizes of three metal nanocages at incident light wavelengths commonly used in biomedicine; it was also found that, under deep therapy conditions, Ag nanocages in particular exhibit the highest volume absorption and scattering coefficients of 0.708 nm-1 and 0.583 nm-1, respectively. These findings offer theoretical insights into preparing target nanocage particles for applications in photothermal therapy and biological imaging.

Physical modelling study on wave damping induced by an idealized floating kelp farm

A physical modelling study was carried out to investigate random wave damping promoted by an idealized floating kelp farm. The experimental conditions spanned intermediate water depths and both linear and nonlinear water waves. Unlike previous studies of wave damping promoted by vegetation, the floating kelp farm was placed close to the water surface with a ratio between vegetation height and water depth close to 0.25. The wave transmission coefficient induced by the floating kelp farm ranged between 0.56 and 0.96. This coefficient decreased for longer floating kelp farms and it was a function of the ratio between kelp farm length and incident wavelength and of the relative wave depth. Spectral analysis showed that wave damping was not frequency-dependent for wave frequencies close to the peak frequency. The wave transmission coefficients of a floating kelp farm with about 100 culture lines and with an extension of approximately 200 m were similar to those of submerged detached breakwaters with a relative crest freeboard smaller than -0.4. Furthermore, the bulk drag coefficient of near-surface idealized floating kelp farms can be modelled as a function of the Keulegan-Carpenter number. This study highlights the potential viability of nature-based solutions such as floating kelp farms for coastal protection.

Chirped grating for TE-five/TM-three reflective distribution feature

This research expounds on a novel reflective chirped grating, characterized by its differentiated functionality under various polarization modes. Under perpendicular incidence, this intricately grating produces a quintuple-channel diffraction output of the 0th, ±1st, and ±2nd orders in transverse electric (TE) polarization and a triple-channel diffraction output of the 0th and ±1st orders in transverse magnetic (TM) polarization. Both polarization modes exhibit excellent overall diffraction efficiency and uniformity. At an incident wavelength of 1550 nm, the diffraction efficiencies for the 0th, ±1st, and ±2nd orders under TE polarization are 20.16%, 19.27%, and 20.25%, respectively. Simultaneously, under TM polarization, the efficiencies for the 0th and ±1st orders are 31.79% and 31.57%, respectively. Grating parameters were meticulously derived using the finite element method (FEM) and subsequently corroborated through rigorous coupled-wave analysis (RCWA) to ensure superior grating accuracy. The study also exhaustively analyzes the manufacturing tolerances and robustness of the grating, affirming its practical applicability and effectiveness in practical applications. The dual-function grating splitter proposed in this paper enables the implementation of multiple functionalities within simple setups, suitable for applications requiring varied beam splitting. As photonic systems and fiber technology evolve, the potential applications of dual-function reflective splitters in these fields are increasingly highlighted.

Polarization-independent and high-efficiency 2D dielectric transmission grating under Littrow incidence

In this paper, a transmission two-dimensional (2D) all-dielectric grating with cuboid arrays is proposed, which has high diffraction efficiency and good polarization independence under Littrow mounting conditions at an incident wavelength of 780 nm. The optimization results indicate that when the incident wavelength is 780 nm, the diffraction efficiency of the (−1, 0) order of transverse electric (TE) and transverse magnetic (TM) polarizations can reach 98.62% and 98.23%, respectively, with the polarization-dependent loss (PDL) of 0.017 dB. To the best of our knowledge, high-efficiency polarization-independent 2D transmission grating with a simpler and more effective structure is proposed for the first time, which demonstrates significant enhancements in bandwidth and manufacturing tolerances while maintaining high diffraction efficiency. The results suggest that the grating has great potential for applications in high-precision displacement measurements such as grating interferometers.

Generation of conventional and reflective photonic nanojets and improving intensity enhancement with their superposition

Herein, we report the theoretical investigation on photonic nanojets (PNJs) of substrate-supported single-spherical dielectric microparticles. Conventional and reflective PNJs (CPNJs and RPNJs) are observed in the case of metal and dielectric substrates. The dependence of the maximum electric field intensity enhancement (ηmax) of the CPNJs and RPNJs on the nanogap between the metal substrate and dielectric microsphere, the metal substrate's refractive indices, and the incident light's wavelength is studied. More importantly, the spatial separation between the CPNJs and RPNJs is found to be strongly dependent upon the angle of incidence (θ). A significant improvement in the EFIE is observed for the grazing incidence upon the superposition of CPNJ and RPNJ. The theoretical investigation is also performed by replacing the metal substrate with a dielectric substrate, and the results obtained are reported here for comparison. Finally, this investigation is extended for the dielectric microsphere placed on a thin metal film deposited on a dielectric substrate and studied the role of θ on the characteristic parameters of the CPNJs and RPNJs.

High Efficiency Non‐Doped Organic Light Emitting Diodes Based on Pure Organic Room Temperature Phosphorescence by High‐Lying Singlet Exciton Fission

AbstractHeavy‐metal‐free pure organic room temperature phosphorescence (ORTP) holds great potential in the field of organic optoelectronic devices owing to low economic cost, simple preparation techniques, and high exciton utilization. However, it is still filled with challenges in realizing high efficiency organic light‐emitting diodes (OLEDs) and exploring the internal physical mechanism based on these ORTP molecules. Here, a high‐performance OLED induced by an unexpected interfacial spin‐mixing process between the ORTP molecule and interlayers is demonstrated, and the high efficiency electroluminescence (EL) mechanism is studied through magneto–electroluminescence (MEL) and magneto–photoluminescence (MPL) measurements. The steady‐state and transient PL properties imply that the interfacial effect is related to a high‐lying singlet fission (HLSF) process in the ORTP molecule itself. Further, the HLSF process and the corresponding energy level position are confirmed by the incident wavelength‐ and temperature‐dependent PL spectra and the magnetic‐field‐dependent transient PL. Finally, by optimizing the interfacial material adjacent to the emissive layer to utilize this interfacial spin mixing effect, a high‐efficiency non‐doped ORTP‐OLED with external quantum efficiency of 16% and CIE coordinates of (0.27, 0.49) is developed. The proposed mechanism during the EL process will give insight to produce more efficient OLEDs based on ORTP materials in the future.

Multifaceted control of focal points along an arbitrary 3D curved trajectory

Metalenses can integrate the functionalities of multiple optical components thanks to the unprecedented capability of optical metasurfaces in light control. With the rapid development of optical metasurfaces, metalenses continue to evolve. Polarization and color play a very important role in understanding optics and serve as valuable tools for gaining insights into our world. Benefiting from the design flexibility of metasurfaces, we propose and experimentally demonstrate a super metalens that can realize multifaceted control of focal points along any 3D curved trajectory. The wavelengths and polarization states of all focal points are engineered in a desirable manner. The super metalens can simultaneously realize customized 3D positioning, polarization states, and wavelengths of focal points, which are experimentally demonstrated with incident wavelengths ranging from 501 to 700 nm. We further showcase the application of the developed super metalenses in 3D optical distance measurement. The compact nature of metasurfaces and unique properties of the proposed super metalenses hold promise to dramatically miniaturize and simplify the optical architecture for applications in optical metrology, imaging, detection, and security.

Simple and eco-friendly fabrication of hempseed protein by one-step low-temperature-induced phase separation and centrifugal removal of oil

Hempseed protein is an emerging plant-derived alternative protein with unmatched nutritional and health benefits. However, the currently available industrial hempseed protein production relies on a defatting step using an organic solvent, hexane with health and environmental risks, which also damages the proteins’ structural and functional properties. In this study, we describe a successful method for the simple and eco-friendly simultaneous extraction of proteins and removal of oil based on the “hydrophilic” properties of hempseed oil. Both hempseed protein isolates (HPIs) extracted from hexane-defatted hempseed flour (HHPI) and non-defatted hempseed flour (NHHPI) exhibited great similarities in protein contents (both >90%), amino acid composition, protein subunits and functional properties (solubility, water retention and foaming). However, NHHPI significantly outperformed HHPI in keeping native structural and some processing properties. NHHPI exhibited a higher percentage of α-helix (44.29%) with lower amount of random coil (15.33%) than HHPI (α-helix 41.71%, random coil 19.07%), higher fluorescence intensity with lower incident wavelength (λmax = 326) than HHPI (incident wavelength λmax = 329). Meanwhile, NHHPI displayed higher surface hydrophobicity (807.01), fat absorption (1.35 g/g) and emulsion activity (2.36 m2/g) as compared to HHPI (743.48, 1.14 g/g, 1.78 m2/g, respectively). These findings highlight the importance of a new defatting method for HPI extraction, which may also be applicable to other oilseed proteins.

Wavelet-fusion image super-resolution model with deep learning for downscaling remotely-sensed, multi-band spectral albedo imagery

Generating granular-scale surface albedo data is extremely important for solar photovoltaic site planning and to optimise renewable energy yield of bifacial panel installations. The albedo effect brings about a significant increase in power in bifacial photovoltaic systems, compared to their mono-facial counterparts, since the spectral response of bifacial solar panels correlates with the incident solar radiation wavelength on the back of the panel, to provide additional power generation capacity. Thus, harnessing the albedo data at relatively local scales is critical towards boosting solar power generation and providing greater power density in local electricity grids. This paper develops novel modelling approaches to produce high-resolution spectral albedo imagery across the Visible and Near Infrared (VNIR) bands, using the Wavelet-Fusion super-resolution model (i.e., Wavelet-FusionSR) trained with the Learned Gamma Correction approach by applying satellite image enhancement methodology. The proposed Wavelet-FusionSR model utilises the low-resolution moderate-resolution Imaging Spectroradiometer (MODIS) as well as high-resolution multi-spectral Advanced Space-borne Thermal Emission Reflection Radiometer (ASTER) satellite images, as critical inputs and ground-truth imagery, respectively, in order to perform sensor-to-sensor deep downscaling, without employing any synthetic or low-resolution satellite imagery data pairs. To augment the proposed deep learning algorithm across the decomposed sub-images of low-resolution inputs, we integrate local and global feature representation learning to train the proposed Wavelet-FusionSR model with Cauchy loss functions. In comparison with five competing benchmark models, the proposed Wavelet-FusionSR model demonstrates performance superiority using quantitative image downscaling metrics and visual assessments of the downscaled images for the visible band of solar radiation. The proposed Wavelet-FusionSR model yielded a Mean Square Error (MSE) of 0.00017, Signal-to-noise-ratio (PSNR) of 37.80, Structural Similarity Index (SSIM) of 0.999 and combined loss, MS-SSIMLoss, based on Multi Structural Similarity and Mean Absolute Error of 2.354 for the Visible Band images, and an MSE of 0.0014, PSNR of 28.43, SSIM of 0.999 and MS-SSIMLoss of 7.426 for the NIR spectral bands, demonstrating high efficacy of the proposed Wavelet-FusionSR method. The Wavelet-FusionSR method therefore attains high-resolution spectral albedo imagery outputs.

Interactive effects of deformable wave energy converters operating in close proximity

Flexible wave energy converters (FlexWECs) have been gaining increasing research and industrial interest as their deformable nature can potentially remedy the structural issues that limit the development of rigid WECs. To maximise the usage of space and infrastructure and improve energy efficiency, FlexWECs are normally deployed in close proximity, where the wave interaction with one device can influence others, signifying the opportunity to obtain energy efficiency enhancement from the interactions. To investigate the power capture performance of a FlexWEC array, this study employed a validated three-dimensional high-fidelity computational method to simulate the wave interaction with three FlexWECs in various array arrangements including power-take off. Based on systematic simulation cases, the present work analysed the relation between the geometrical characteristics of an isolated FlexWEC's perturbed wave field and the array's overall energy capture efficiency. The constructive interaction of the array was found the strongest when the longitudinal and lateral spacings of the array were 0.6 and 1 times of incident wavelength respectively, with a 15 % enhancement of overall captured energy compared to three devices operating in isolation. Overall, this study provides insights into the fluid-structure interaction of waves with multiple deformable structures, facilitating the modelling and planning of FlexWECs.

Highly stable, low voltage, flexible photodetector in UV-visible region from self-assembled organic small molecule

The fabrication of a high-performance, low voltage operated flexible organic photodetector (OPD) based on solution self-assembled crystalline thin film of a small molecule, viz, 6,13 bis(tri-isopropylsilylethynyl) pentacene (Tips pentacene) is reported. The OPD demonstrated excellent photodetection ability under range of visible light as well as under UV light, with low illumination intensity. Under 590 nm illumination (5.6 µW/cm2), the device showcased photo to dark current ratio (Iphoto/Idark), ca. 25, photoresponsivity (P) of 89 mA/W, detectivity of 1.81×1010 jones at 1 V bias and response times of 0.04/0.2 sec. Photocurrent modulation of the OPD has been realized by varying the channel width, incident wavelength, applied bias and the illumination intensity. The OPD exhibited excellent photodetection ability under different tensile bending, with roughly 55 % decline in Iphoto/Idark value and 30 % decline in R value under bending radius of 7.5 mm. The OPD could withstand thousands of repeated bending/folding cycles, and regain its initial photoresponse characteristics, if put at rest for 2 hours. The excellent device performances with its precise tuning via various input stimuli suggests that present OPD have great potential for future low cost, low energy and wearable optoelectronics.

(Invited) Changes in Electric Double-Layer Structures Under Localized Surface Plasmon Excitation

For the visible light energy conversion, the localized surface plasmon resonance (LSPR), which is the collective oscillations of free electrons, should be promising. With the excitation of LSPR, the highly localized electric field generates in the vicinity of metal nanostructures. It is interesting that various unique photo-response properties, such as chemical reactions or molecular excitations, can be observed due to the enhancement of light-matter interaction.[1] To understand and control such mediated chemical reactions or electrochemical reactions, the precise understanding about the electrified interfaces of plasmonic nanostructures should be required.Especially in the electrochemical system, the electric double layer is formed due to the difference in electrochemical potential between the metal interface and solution. The study of the surface potential is important for the design of chemical reactions because the surface potential at the liquid-solid interface is dependent on the physical properties of the systems. The zeta potential which is the potential of the slipping surface near the Stern layer of the diffusion layer could provide such information. From this point of view, in this study, we investigated the electric double-layer structures through the examination of the zeta potential under LSPR excitation condition. To obtain the zeta potential, we have performed the streaming potential method using Au nanoisland structures under visible light illuminations to excite the LSPR. It was interesting that the zeta potential was drastically changes under the visible light illumination conditions. This zeta potential change indicates the changes in the electric double layer structures through the excitation of LSPR. Through the investigations of incident wavelength dependence or the substrate dependences, the effects for the LSPR excitations on the electric double layer structure have been revealed. The present work would provide the fundamental knowledge about the effect on the LSPR excitation at solid-liquid interfaces.[1] H. Minamimoto et al., Acc. Chem. Res., 2022, 55(6), 809.

High‐Performance Flexible PbS Nanofilm Wavelength Sensor with Detection Region Ranging from DUV to NIR

AbstractIn this study, on the fabrication of a flexible wavelength sensor is reported, which is achieved by growing a layer of lead sulfide (PbS) nanofilm on both sides of a polyethylene terephthalate substrate using the chemical bath deposition method, followed by the deposition of two parallel Au interdigital electrodes. Experimental result shows that the photocurrent ratio of the two photodetectors monotonically decreases with increasing wavelength in the range from 265 nm (UV) to 2000 nm (NIR), indicating that the incident light wavelength can be distinguished by the photocurrent ratio. Notably, the as‐constructed wavelength sensor exhibits superior performance compared to most previously reported filter‐less designs, achieving an average absolute error of 11.5 nm and an average relative error of 1.1%. It is also found that the sensor exhibits excellent mechanical flexibility and environmental stability. Furthermore, by introducing the back‐end circuit, real‐time detection of the wavelength of monochromatic light and the peak wavelength of LED light are achieved, with detection errors not exceeding 2.8% and 2.6%, respectively. It is believed that the flexible PbS nanofilm wavelength sensor prepared in this study has potential application in future portable and flexible optoelectronic devices.

Using Femtosecond Laser Pulses to Explore the Nonlinear Optical Properties of Ag/Au Alloy Nanoparticles Synthesized by Pulsed Laser Ablation in a Liquid.

Metallic nanoparticles have gained attention in technological fields, particularly photonics. The creation of silver/gold (Ag/Au) alloy NPs upon laser exposure of an assembly of these NPs was described. First, using the Nd: YAG pulsed laser ablation's second harmonic at the same average power and exposure time, Ag and Au NPs in distilled water were created individually. Next, the assembly of Ag and Au NP colloids was exposed again to the pulsed laser, and the effects were examined at different average powers and exposure times. Furthermore, Ag/Au alloy nanoparticles were synthesized with by raising the average power and exposure time. The absorption spectrum, average size, and shape of alloy NPs were obtained by using an ultraviolet-visible (UV-Vis) spectrophotometer and transmission electron microscope instrument. Ag/Au alloy NPs have been obtained in the limit of quantum dots (<10 nm). The optical band gap energies of the Ag/Au alloy colloidal solutions were assessed for different Ag/Au alloy NP concentrations and NP sizes as a function of the exposure time and average power. The experimental data showed a trend toward an increasing bandgap with decreasing nanoparticle size. The nonlinear optical characteristics of Ag/Au NPs were evaluated and measured by the Z-scan technique using high repetition rate (80 MHz), femtosecond (100 fs), and near-infrared (NIR) (750-850 nm) laser pulses. In open aperture (OA) Z-scan measurements, Ag, Au, and Ag/AuNPs present reverse saturation absorption (RSA) behavior, indicating a positive nonlinear absorption (NLA) coefficient. In the close-aperture (CA) measurements, the nonlinear refractive (NLR) indices (n2) of the Ag, Au, and Ag/Au NP samples were ascribed to the self-defocusing effect, indicating an effective negative nonlinearity for the nanoparticles. The NLA and NLR characteristics of the Ag/Au NPs colloids were found to be influenced by the incident power and excitation wavelength. The optical limiting (OL) effects of the Ag/Au alloy solution at various excitation wavelengths were studied. The OL effect of alloy NPs is greater than that of monometallic NPs. The Ag/Au bimetallic nanoparticles were found to be more suitable for optical-limiting applications.

Toward Machine-Learning-Accelerated Design of All-Dielectric Magnetophotonic Nanostructures.

All-dielectric magnetophotonic nanostructures are promising for integrated nanophotonic devices with high resolution and sensitivity, but their design requires computationally demanding electromagnetic simulations evaluated through trial and error. In this paper, we propose a machine-learning approach to accelerate the design of these nanostructures. Using a data set of 12 170 samples containing four geometric parameters of the nanostructure and the incidence wavelength, trained neural network and polynomial regression algorithms were capable of predicting the amplitude of the transverse magneto-optical Kerr effect (TMOKE) within a time frame of 10-3 s and mean square error below 4.2%. With this approach, one can readily identify nanostructures suitable for sensing at ultralow analyte concentrations in aqueous solutions. As a proof of principle, we used the machine-learning models to determine the sensitivity (S = |Δθres/Δna|) of a nanophotonic grating, which is competitive with state-of-the-art systems and exhibits a figure of merit of 672 RIU-1. Furthermore, researchers can use the predictions of TMOKE peaks generated by the algorithms to assess the suitability for experimental setups, adding a layer of utility to the machine-learning methodology.

Configurable anti-ambipolar photoresponses for optoelectronic multi-valued logic gates

Anti-ambipolar transistors (AATs) are the leading platform for the paradigm shift from binary to multi-valued logic (MVL) circuits, increasing circuit integration density and data processing capacity. However, most AATs with p–n heterojunctions present limited controllability of the transconductance peak, which is key to MVL operation. Here, we report optically configurable AAT/bi-AAT photoresponses implemented with an InSe field-effect transistor for potential MVL operations. The charge trapping and detrapping processes incorporated with manually introduced trap states form the AAT peaks. Furthermore, leveraging a symmetric device configuration, the dark current is significantly suppressed, and AAT photoresponses are highlighted. Contributed by two pathways of trap states, the AAT/bi-AAT photoresponses are switchable by incident optical wavelength. This dependence facilitates optical wavelength to be one of the logic inputs for MVL, based on which we propose circuit-free ternary logic gates in a single device that can achieve more than ∼6 and ∼19 times improved data density (1 bit per transistor) for NMAX and XNOR, compared with such circuits in a traditional binary design. This work realizes optically controlled AAT photoresponses, paving the way to exploit optical wavelength as a new degree of freedom in MVL computing, offering a route toward ultra-high-density, ultra-low-power, and optically programmable optoelectronic integrated circuits.