Waste Carbon Fiber Research Articles

Exploring the potential of waste carbon fiber reinforced epoxy for high‐performance electromagnetic interference shielding

AbstractThe waste carbon fiber reinforced epoxy (WFRE) is difficult to recycle and high‐value reuse due to its irreversible cross‐linked structure. Currently, many recycling methods are flawed, rendering effective recycling unattainable and resulting in the waste of high‐value carbon fibers and increased environmental pollution. In this study, the production of high‐aspect‐ratio carbon fiber powder from WFRE was achieved through the application of solid‐state shear milling technology. The prepared EP/WFRE/CNT composites exhibited commendable mechanical properties and good electromagnetic interference (EMI SE) shielding efficiency, owing to the excellent dispersion and interfacial adhesion. The EMI SE value of EP/WFRE/CNT composites reached 21.9 dB, meeting the basic demand in the civil field. The flexural modulus of EP/WFRE/CNT composites reached 5914 MPa with the incorporation of 5 wt.% CNT. Moreover, the storage modulus of composite at 40°C increased from 2299 MPa for neat epoxy to 3006 MPa for composites. This research proposes a novel application of WFRE as good mechanical performance material for electromagnetic interference shielding, demonstrating the potential for commercial‐scale applications.Highlights Solid‐state shear milling can effectively peel epoxy resin. Solid‐state shear milling can preserve the high aspect ratio of carbon fiber. EP/WFRE/CNT has a flexural modulus of up to 5914.8 MPa. EP/WFRE/CNT has EMI SE that reaches 21.9 dB. CNT and carbon fiber synergistically formed conductive network.

Identification of mechanisms and experimental implementation for enhancing the interfacial force between oxygen functionalized waste carbon fibers and polyamide resin

To recycle waste carbon fibers (CFs) and utilize them as a composite material with polyamide–6 (PA–6), the oxidation of the carbon surface is crucial for enhancing its bonding with PA–6 without damaging the waste CFs. However, the most effective oxygen-containing functional group (O–group) was hitherto unknown. In this study, computational simulations demonstrated that incorporating O–groups enhanced the interfacial bonding force via hydrogen bonding between the oxygen of the O–groups and hydrogen (N–H) of PA–6. Among various O–groups, the bonding of lactone groups to PA–6 was energetically most favorable, corroborated by different oxidation treatments such as acid, heat, and plasma. As the reaction time or temperature increased, the amount of O–groups, such as lactones, increased. Regardless of the oxidation treatment type, an increase in the amount of O–groups increased the interfacial force, and this tendency was predominantly observed in lactone groups. However, excessive surface oxidation introduced defects on the surface of CFs, which reduced the interfacial force. The modification of waste CFs by identifying the proposed mechanisms lays the groundwork for synthesizing high-quality waste CF composites.

Effect of concentration on PVA solutions and its usage in recycling carbon fiber/polyamide 12 prepregs

Abstract Polyvinyl alcohol (PVA) is a biodegradable synthetic polymer with high chemical resistance and excellent mechanical and oxygen barrier properties. Besides these superior properties, it is water-soluble, which provides its wide usage. However, its solubility depends on some factors. Although the temperature is one of these factors and increasing temperature could promote solubility, there is a solubility limit according to hydrolysis degree. In this study, PVA solutions at various concentrations were obtained by mixing fully hydrolyzed PVA1500 and water. Solutions were characterized by density, surface contact angle and dynamic viscosity measurements. Then, solvent casting was used to obtain films, and physical and mechanical properties were determined. Tensile test results showed optimum values at 10–12.5 wt.% PVA concentration. Also, vacuum drying changed the mechanical behavior of films significantly at all concentrations. While ultimate tensile stress values almost doubled and modulus values increased approximately three times, elongations critically decreased. Solutions were also subjected to waste carbon fiber (CF)/polyamide 12 (PA12) prepregs for recycling purposes. Lay-up and compression molding processes were applied to produce CF/PA12 composites. It was seen that mechanical results were significantly increased with increasing PVA concentration.

Optimum moment to heal cracks in asphalt pavement by means of waste carbon fiber-enhanced electromagnetic induction heating during multiple damage-healing cycles

This study investigated the optimal timing for healing asphalt pavement cracks using waste carbon fibers (WCFs) reinforced electromagnetic induction (EMI) technology through multiple "damage-healing" cycles, focusing on mechanical and fatigue performance. Initially, an extensive research project was carried out to evaluate the rate of induction heating, surface temperature decline rate, and effective heating depth of the asphalt mixture. Subsequently, from a mechanical performance perspective, semi-circular bending (SCB) tests were employed. By setting four different load termination conditions, the extent of cracking in the specimens was quantitatively controlled, followed by multiple "damage-healing" tests to analyze the impact of healing timing on the mechanical properties and healing efficiency of the asphalt mixture. Lastly, from the perspective of fatigue performance, using the four-point bending fatigue test (4 PB), the fatigue damage extent of specimens was quantitatively controlled through the attenuation rate of stiffness modulus. Multiple "damage-healing" tests were carried out at four different healing timings to study the effect of healing timing on the fatigue performance and healing efficiency of the asphalt mixture. The results indicated that WCFs improved the heating performance of asphalt mixture, enabling 5 cm-thick specimens to be fully heated within 6 min. Both SCB and 4 PB tests yielded similar conclusions: in the process of multiple "damage-healing" cycles, earlier healing interventions were beneficial for the recovery and maintenance of the mechanical properties of asphalt mixtures and effectively extended their service life. However, the fatigue tests also revealed that overly early self-healing interventions, where cracks were insufficiently formed, did not fully exploit the potential of the healing process. Conversely, healing interventions conducted too late were extremely detrimental to the restoration of mechanical characteristics and the prolongation of the asphalt mixture's lifespan.

Investigation of Desiccation Cracking Behavior of Waste Carbon Fiber–Reinforced Clay Material

Carbon fiber is a common waste building material, but its effect on the drying and cracking properties of clay materials is unknown. In this paper, crack rate and fractal dimension are used to characterize the influence of waste carbon fiber materials on the development of soil cracking. With the rise in carbon fiber content to 0.2%, 0.4% and 0.6%, the crack rate of soil cracking decreased by 7.9%, 17.3% and 23.3%, respectively, while the fractal dimension of soil cracking decreased by 2.4%, 8.7% and 21.2%, respectively. Accordingly, the critical moisture content of the soil samples increased by 33.2%, 110% and 151%, and the time of the soil constant evaporation stage decreased by 5.1%, 13.8% and 34.5%, respectively. When carbon fiber is combined with soil, carbon fiber will increase the interface bonding strength, friction and interlocking force, effectively inhibiting the cracking of soil, and it provides a channel for water transport in the soil in the early stage.

Investigation of recycled carbon fiber-reinforced ultrafine-grain carbon-matrix composites

To broaden the usefulness of recycled carbon fibers and develop the high value-added product, the recycled carbon fiber-reinforced carbon-matrix composites were prepared using ultrafine-grain coke as a filler and coal tar pitch as a binder via a liquid mixing process. A comprehensive study and investigation of the microstructures and properties of recycled carbon fibers and composites were conducted. It was found that the recycled PAN-based carbon fiber (rPCF) outperformed the recycled rayon-based carbon fiber (rRCF) in terms of fiber integrity and pitch-coated effect in the recycling and forming processes. By relieving thermal stress, lowering stacking pores, and inhibiting the growth of shrinkage pores, the rCF can promote the sintering of the green body. The flexural strength of rPCF-reinforced carbon-matrix composite (30.70 MPa) and rRCF-reinforced carbon-matrix composite (20.75 MPa) increased by 60.6% and 8.6% than that of pristine carbon-matrix composite (19.11 MPa), respectively. The difference in mechanical properties between rPCF-reinforced carbon-matrix composite and rRCF-reinforced carbon-matrix composite is attributed to the mechanical interlock mechanism and fiber pull-out mechanism. This work provides a propagable, affordable, and environment-friendly idea for recycling waste carbon fiber and producing recycled carbon fiber reinforced composites.

Recycling waste carbon fibers for solar-driven clean water production by one-step electrochemical process

Waste carbon fibers (WCF), as a co-product of carbon-based textile material, presented a high recycling value. However, it is difficult to utilize the short carbon fibers by traditional process, recycling and using these WCF effectively has thus attracted increasing attention. Herein, we propose a novel strategy that utilizes simultaneous electrochemical exfoliation and deposition processes to convert WCF into photothermal materials. Stainless steel felt (SS) was selected as the substrate to verify this strategy. Through this strategy, the reduced graphene oxide-coated SS (rGO-SS) was obtained. The 2D solar-driven interfacial evaporator based on rGO-SS enabled stable evaporation in actual wastewater with an excellent rate of 1.44 ∼ 1.50 kg m−2 h−1 under 1 sun. Additionally, by constructing a 3D evaporation structure, rGO-SS performed a high evaporation rate of ∼16.88 kg m−2 h−1 under 1 sun. Finally, this work proposes a novel method for the waste carbon fibers and gives new insights into fabricating a novel solar-driven interfacial evaporator.

Circular economy innovation: A deep investigation on 3D printing of industrial waste polypropylene and carbon fibre composites

Transforming waste polypropylene (PP) and waste carbon fibre into upcycled composite materials for additive manufacturing represents an ideal circular economy challenge. An optimized method for material extrusion and 3D printing was developed to overcome adhesion and warpage challenges during printing. The study explored the impact of varying waste carbon fibre weight fractions (0 wt%, 2 wt%, 5 wt%, 8 wt%, 15 wt%, and 25 wt%), firstly on the properties of filament and then on printability and mechanical properties of printed specimens. Optimized extrusion parameters yielded the successful fabrication of fibre-reinforced filaments. Micro-level assessment of the polymer revealed a decrease in mechanical properties due to thermal processes during filament making and 3D printing. Microstructural analysis, along with optical and scanning electron microscopy, provided insights into inter-bead voids, debonding, fibre dispersion, fracture modes, and filament/sample quality. Differential Scanning Calorimetry indicated slight matrix degradation during filament extrusion, leading to slightly reduced melting and crystallization temperatures.

Transformation of waste carbon fiber prepreg into sustainable composites: Application in the automotive industry components

AbstractCarbon fiber (CF) prepregs are employed in the manufacture of many different aeronautical structural and non‐structural components. Following the cure of the prepregs in molds, trimming is generally used to give the final shape to the components. Considering the aircraft's vast surface area and the use of multiple prepreg layers in each component, an extensive amount of carbon fiber prepreg is discarded. The unique characteristics of carbon fibers render this CF waste highly valuable and requires its efficient recycling. Cured waste CF prepregs were milled and processed in this research to produce chopped carbon fibers for use in the novel composite development. The matrix material used in the composites was selected as recycled polypropylene sourced from old surgical masks, which highlighted the sustainability of the developed composites. To enhance the quality of the fiber‐matrix interface and improve the impact resistance of the composites an anhydride‐grafted polyethylene (Fusabond) was employed in small quantities. From mechanical characterizations, synergistic effects of the fillers were observed. Besides, compositions containing CF and Fusabond are found more impact resistant than neat matrix. In addition, the use of carbon fibers increased fracture toughness of the matrix through various mechanisms including fiber bridging, fiber pullout, and matrix plastic deformation identified by scanning electron microscopy fractography. Thermomechanical characterizations using dynamic mechanical analysis revealed that carbon fiber raises the neat matrix's glass transition temperature. The developed materials are intended to be employed in the automotive industry to produce inner fender liners, with an optimal composition determined by an optimization research.Highlights Carbon fiber (CF) derived from aerospace fresh scraps significantly improved the mechanical properties of the polymer matrix. Anhydride‐grafted polyethylene incorporation remarkably enhanced the impact resistance of the polymer. CF demonstrated a bridge effect and improved the fracture toughness of the composites. The use of recycled CF presents encouraging prospects in the automotive industry for the production of inner fender liners.

Pengaruh Perlakuan Kimia Alkalinasi dan Asetilasi terhadap Kekuatan Tarik dan Mikrostruktur Serat Abaka

Today, environmental problems, especially soil pollution due to inorganic waste or waste that does not decompose, are a major problem and need to be solved, especially in developing countries with high populations such as Indonesia. One of the causes of soil pollution problems is the use of inorganic fibers such as glass fiber and carbon fiber. The use of materials that are not environmentally friendly in the industry will cause environmental problems due to nature's inability to decompose the glass fiber material in nature. The focus of this research is to reduce environmental pollution by using natural fibers such as abaca fiber as an alternative to inorganic fibers. This is due to its properties, namely: low density, good specific strength, low price, and a high biodegradable ability so that it can reduce glass fiber or carbon fiber waste that does not decompose. To support this, abaca fiber needs to be hydrophobic so that it becomes compatible with other materials when combined together with other materials. One of the ways that can be done is by alkaline chemical treatment and acetylation using KOH and CH3COOH. Chemical treatment was carried out by dipping abaca banana fibers into a solution of alkaline compounds and acetylated compounds KOH and CH3COOH with a concentration of 5 M and 10 M for 4 hours. After chemical treatment, the abaca banana fibers were characterized for mechanical properties using ASTM D 3379 standards to determine the tensile strength of the fibers and using an optical microscope to determine the microstructure of the abaca fibers.

Bio-inspired polydopamine modification of recycled carbon fibers for improving the performance of recycled carbon fiber reinforced mortars

The hydrophobicity nature of the waste carbon fiber felt (WCF) surface results in the formation of a weak interface with the paste during the curing process of WCF concrete, which seriously affects the performance of WCF concrete and the reuse of WCF. To address this problem, this paper utilized polydopamine (PDA) for the functionalization of WCF to enhance bonding between WCF and paste. The wettability, Ca2+ complexation, and functional groups of PDA coating on WCF were analyzed by contact angle, ICP-OES, and XPS, respectively. Additionally, the effects of incorporating PDA-functionalized WCF on the flowability, compressive strength, hydration kinetics, pore structure, water absorption capillary, and SEM of mortars were tested. Experimental results showed that the PDA coating improved the wettability of WCF and enhanced the flowability of WCF mortar. What's more, the PDA coating could chelate Ca2+ and promote the formation and deposition of hydration products on the WCF surface, resulting in a denser interfacial transition zone (ITZ). Compared with ordinary WCF mortar, the compressive strength of the PDA-modified WCF mortar was increased by 18% at 28d. Furthermore, the capillary water absorption of the modified group mortar was also decreased by up to 13%, significantly enhancing the durability of mortars. This paper presents a green and simple bio-inspired method to strengthen the ITZ between WCF and paste, which is fundamentally different from the traditional modification methods, and also offers a theoretical basis and technical foundation for the sustainable utilization of WCF.

Upcycling Waste Thermosetting Polyimide Resins into High-Performance and Sustainable Low-Temperature-Resistance Adhesives.

Thermosetting polyimide (PI) has attracted extensive attention for its excellent properties, but the approaches to its end-of-life management are not sustainable, posing great threat to the ecosystem. Herein, this work proposes a mild, sustainable, and full recovery path for recycling waste carbon fiber reinforced phenylethynyl end-capped PI resin composites. In addition to recycling reaction reagent and woven carbon fiber, degraded products (DPETI) can be fully and directly used as high-performance and sustainable adhesives. DPETI exhibits strong adhesion to various surfaces, with a maximum adhesion strength of 1.84MPa. Due to the strong supramolecular polymerization behavior without solvent dependence, DPETI demonstrates higher adhesive strength of 2.22MPa in the extreme environment (-196 °C), which is maintained even after 10 cycles. This work sparks a new thinking for plastic wastes recycling that is to convert unrecyclable wastes into new and sustainable materials, which has the potential to establish new links within circular economies and influence the development of materials science.

Roles of waste carbon fibers on the efficiency of multiple induction heating healing behavior in asphalt mixture for sustainable infrastructure

This study systematically investigated the potential of waste carbon fibers (WCFs) as a sustainable solution in enhancing the multiple induction heating healing of asphalt mixture, thereby tackling two major concerns: the environmental impact of WCFs and the durability of asphalt pavement. Firstly, four groups of asphalt binder samples with different WCFs contents were prepared. The viscosity and workability of WCFs modified asphalt binder were analyzed. Next, asphalt mixture containing 2% steel fibers was prepared at the optimal WCFs content, while control groups without WCFs were prepared with 2% and 4% steel fibers content. A comprehensive study was conducted on the induction heating rate, effective heating depth and surface temperature cooling rules of the asphalt mixture. Finally, by conducting multiple "fracture-healing" tests, the influence of WCFs on the healing efficiency of asphalt mixture was analyzed. The results revealed that WCFs increased the viscosity of the virgin asphalt, but excessive WCFs content hindered the workability. The optimal WCFs content was determined to be 1% (by weight of asphalt binder). WCFs enhanced the thermal conductivity of the asphalt mixture, accelerating heating and improving vertical heat transfer while reducing surface temperature decline. During multiple "fracture -healing" processes, the inclusion of WCFs enhanced the mechanical strength of the asphalt mixture, improved its healing efficiency, and increased the number of healings. Even after five cycles, the specimen with the most damage still showed a fracture energy recovery rate (FERR) of over 30%. In conclusion, WCFs significantly enhanced the multiple induction heating healing efficiency of the asphalt mixture.

Recycling and Reutilization of Waste Carbon Fiber Reinforced Plastics: Current Status and Prospects.

The extensive use of carbon fiber-reinforced plastics (CFRP) in aerospace, civil engineering, and other fields has resulted in a significant amount of waste, leading to serious environmental issues. Finding appropriate methods for recycling CFRP waste and effectively reusing recycled carbon fibers (rCFs) has become a challenging task. This paper presents an overview of the current status of CFRP waste and provides a systematic review and analysis of recycling technologies. In addition to discussing mechanical recycling, thermal decomposition, and chemical solvent degradation methods, the organic alkali/organic solvent method for recycling resins is also elucidated. By introducing the recycling conditions and outcomes of the organic alkali/organic solvent method, the study highlights its significance as a reference for carbon fiber recycling. Furthermore, the paper reviews the current state of rCFs utilization based on its application domains, focusing on research advancements in fiber composites and cementitious composites. Based on these findings, the paper summarizes the existing research limitations and identifies specific areas that require further attention in recycling techniques and rCFs utilization. Lastly, this review provides a prospect on the future of recycling and reusing CFRP waste.

Enhanced Compatibility of Secondary Waste Carbon Fibers through Surface Activation via Nanoceramic Coating in Fiber-Reinforced Cement Mortars

The utilization of waste fibers in the production of reinforced concrete materials offers several advantages, including reducing environmental strain and socio-economic impacts associated with composite waste, as well as enhancing material performance. This study focuses on the development of cementitious mortars using secondary waste carbon fibers, which are by-products derived from the industrial conversion of recycled fibers into woven/non-woven fabrics. The research primarily addresses the challenge of achieving adequate dispersion of these recycled fibers within the matrix due to their agglomerate-like structure. To address this issue, a deagglomeration treatment employing nanoclay conditioning was developed. The functionalization with nanoclay aimed to promote a more uniform distribution of the reinforcement and enhance compatibility with the cementitious matrix. Various fiber weight percentages (ranging from 0.5 w/w% to 1 w/w% relative to the cement binder) were incorporated into the fiber-reinforced mix designs, both with and without nanoceramic treatment. The influence of the reinforcing fibers and the compatibility effects of nanoclay were investigated through a comprehensive experimental analysis that included mechanical characterization and microstructural investigation. The effectiveness of the nanoceramic conditioning was confirmed by a significant increase in flexural strength performance for the sample incorporating 0.75 w/w% of waste fibers, surpassing 76% compared to the control material and exceeding 100% compared to the fiber-reinforced mortar incorporating unconditioned carbon fibers. Furthermore, the addition of nanoclay-conditioned carbon fibers positively impacted compression strength performance (+13% as the maximum strength increment for the mortar with 0.75 w/w% of secondary waste carbon fibers) and microstructural characteristics of the samples. However, further investigation is required to address challenges related to the engineering properties of these cementitious composites, particularly with respect to impact resistance and durability properties.

High-quality electrostatic recycling of waste carbon fiber via spark-driven shock waves and Joule heating

The recycling of waste carbon fibers (CF) has emerged as a crucial research area for both environmental protection and economic sustainability. To sufficiently exert the potential and extend the application life cycle of CFs, here we propose an eco-friendly and efficient electrostatic method for rapid recycling of tightly entangled reclaimed carbon fibers (rCFs) by spark-driven disentanglement and depolymerization. Our research indicates that the spark discharge generated by fiber induction under low-voltage conditions can excite the shock waves and Joule heating effects, resulting in the separation of individual rCFs and the removal of surface organic matrix. Furthermore, the constructed electric field can synchronously and continuously orient the dispersed rCFs to form a vertical alignment in a short time with good maneuverability and directionality for reutilization. The results demonstrate that this one-step disentanglement, depolymerization, and alignment method achieves a high-quality recycling process with 100% dispersion efficiency, minimal damage, cost-effectiveness, uniform distribution, upright orientation, and high-speed embedding performance. Our findings reveal the potential of the electrostatic strategy for the high-quality recycling of rCFs, in line with the principles of the circular economy. The proposed method offers broad prospects for application in continuous in-line production and material manufacturing, and is a step towards sustainable and cost-effective CF recycling.

Impacts of Annealing Temperature and Time on the Thermoelectric Performance of Recycled Carbon Fiber (RCF)/n-Bi2Te3 Heterostructure Thermoelectric Composites

Recycling carbon fibre waste is crucial for sustainability in the composites industry. Herein, we report the fabrication of a heterostructure composite using recycled carbon fiber (RCF) and n-type bismuth telluride (n-Bi2Te3) for thermoelectric applications. In the present study, we have comprehensively investigated the effects of annealing temperature and time on the thermoelectric, structural, charge carrier transport, morphological, and thermal stability properties of annealed RCF/n-Bi2Te3 composites. The optimum annealing temperature and time were at 350 °C and 2 h, respectively, which yielded a maximum power factor of 7.83 μWK−2m−1. Annealing redistributed the bismuth and tellurium atomic percentage, decreased carrier concentration, improved carrier mobility, enhanced the crystallinity and increased the grain size of the bismuth telluride particles, subsequently improving the thermoelectric performance as well as the thermal stability of annealed RCF/n-Bi2Te3 composites. In addition, this study has explored the plausibility of a cross-plane configured Seebeck coefficient measurement utilizing recycled carbon fibre/n-type bismuth telluride heterostructure thermoelectric composite. Energy band diagram analysis indicated favorable heterojunction alignment between RCF and n-Bi2Te3, validating the viability of the thermoelectric composite in a cross-plane configuration. Our study provides a promising route for closing the recycling loop of carbon fiber waste and achieving sustainable thermoelectric materials.

Simultaneous Optimization of Carbon Fiber Allocation and Orientation by IFM-GA

This paper proposes an individual fitness method genetic algorithm (IFM-GA) for carbon fiber-reinforced plastic (CFRP). The strength of CFRP depends on the carbon fiber allocation and orientation. Waste carbon fiber is generated if this design is inappropriate. Consequently, CFRPs are less cost-effective. It is necessary to optimize the allocation and orientation as design variables to solve this problem. The problem involves combinatorial optimization. The genetic algorithm (GA) is suitable for combinatorial optimization. However, it is difficult to obtain an optimal solution using the GA owing to the large number of combinations. Hence, the IFM-GA is developed in this study. It is a GA-based method with a different fitness calculation. The GA calculates the fitness of each design, whereas the IFM-GA calculates the fitness of each design element. As a result, the IFM-GA yields a higher-stiffness design than the GA. To conclude, the IFM-GA can enable optimum fiber allocation and orientation, whereas the GA cannot.

Towards recycling of waste carbon fiber: Strength, morphology and structural features of recovered carbon fibers

Carbon fiber is one of the most widely used materials in high demand applications due to its high specific properties, however, its post-recycling properties limit its use to low performance applications. In this research, the carbon fiber recovering is examined using two methods: two-step pyrolysis and microwave-assisted thermolysis. The results indicate that the fibers recovered by pyrolysis show reduced surface and structural damage, maintaining the original mechanical properties of the fiber with losses below 5%. The fibers recovered by microwaves undergo significant surface changes that reduce their tensile strength by up to 60% and changes in their graphitic structure, increasing their degree of crystallinity by Raman index ID/IG from 1.98 to 2.86 and their amorphous degree by ID”/IG ratio from 0.411 to 1.599. Recovering fibers from microwave technique is 70% faster compared to two step pyrolysis, and provides recycled fibers with superior surface activation with the presence of polar functional groups –OH, –CO, and –CH that react with the epoxy matrix. The thermal, morphological, structural and mechanical characterizations of the recovered fibers detailed in this work provide valuable findings to evaluate their direct reuse in new composite materials.

Lightweight, flexible rCEF@PPy/MXene for ultra-efficient EMI shielding felt with Joule heating performance

Lightweight, flexible and multifunctional characteristics have attracted widespread attention in recent years for electromagnetic interference (EMI) shielding materials in the field of portable electronics. In this work, conductive polymer PPy and MXene nanosheets were anchored on the surface of the recycled carbon felts fixed with ES fibers (rCEF@PPy/MXene) to construct porous conductive networks, resulting in high conductivity, excellent EMI shielding property (60 dB) and electro-thermal conversion abilities. The rCEF@PPy/MXene shows great potential for wearable devices and heat management, together with promoting the sustainable reuse of waste carbon fiber resources.