Vehicle-to-grid (V2G) control of electric vehicles (EVs) has the potential to provide frequency regulation for power system operation. The authors study the frequency droop control with EVs’ participation. The challenge is to simultaneously suppress frequency fluctuation and satisfy transportation usages of EV owners. A V2G control consisting of frequency droop control and scheduled charging is developed to overcome this challenge. Frequency droop control can suppress frequency fluctuation by responding to frequency deviation signal, while scheduled charging can achieve the charging demands of EV owners. Although uncertain regulation may result in deviation of the battery energy levels from the expected, the scheduled charging made based on the departure time, the real-time, the real-time battery energy levels, and the expected battery energy levels can compensate this change in real time. The proposed V2G control can ensure different types of charging demands such as holding battery energy levels and elevating battery energy levels, unlike existing methods in which different V2G control strategies have to be developed. Simulations on a two-area interconnected power grid using real power grid data in China validate the effectiveness of the proposed V2G control in suppressing frequency fluctuation and achieving the charging demands of EV owners.