Ultrashort-pulsed Laser Beam Research Articles

Highly efficient four-wave parametric amplification in transparent bulk Kerr medium

We report on highly efficient four-wave optical parametric amplification in a water cell pumped by an elliptically shaped, ultrashort pulsed laser beam under non-collinear phase-matching configuration. Energy conversion from pump to parametric waves as high as 25 % is obtained owing to the achievement of 1-dimensional spatial-soliton regime, which guarantees high intensity over a large interaction length and ensures high beam quality.

Digital in-line holography with a sub-picosecond laser beam

The diffraction of an ultrashort pulsed laser beam by an opaque particle is studied. The case of a pulse with a Gaussian spectrum is investigated analytically by using the steepest descent method. This analytical solution allows us to calculate the intensity distribution of the diffraction field. This result enables to determine the optimal fractional orders Fourier transform to reconstruct digital in-line particle hologram.

Measuring pulse-front tilt in ultrashort pulse laser beams without ambiguity of its sign using single-shot tilted pulse-front autocorrelator

The measurement of pulse-front tilt (PFT) in ultrashort pulse laser beams, without ambiguity of its sign, has been carried out using an in-house built single-shot tilted pulse-front autocorrelator (TPFAC) based on second harmonic generation in non-linear crystal. The experiment is carried out for the beam propagation through a single prism and a pair of prisms. Expressions of PFT angle have been derived to account for beam size, beam propagation effects and for arbitrary incidence of the laser beam. The measured PFT angles were found in accordance with theoretically calculated values. The calculated sensitivity of TPFAC is found to be larger than that offered by the other techniques.

Sm(DBM)_3Phen - doped poly(methyl methacrylate) for three-dimensional multilayered optical memory

We report on the formation of submicrometer voids within Sm(DBM)3Phen-doped poly(methyl methacrylate) (PMMA) under multiphoton absorption excited by an infrared laser beam. An ultrashort-pulsed laser beam with a pulse width of 200 fs at a wavelength of 800 nm is focused into doped PMMA. The large changes in refractive index and the fluorescence associated with a void allow conventional optical microscopy and reflection-type confocal microscopy to be used as detection methods. Voids can be arranged in a three-dimensional multilayered structure for high-density optical data storage.

Use of a single-mode fiber coupler for second-harmonic-generation microscopy

We present a compact second-harmonic-generation (SHG) microscope based on a three-port single-mode fiber coupler. The fiber coupler is used to deliver a near-infrared ultrashort-pulsed laser beam as well as to collect the SHG signal in the visible wavelength range. The SHG microscope exhibits an axial resolution of 1.8 microm, which shows a slight enhancement of the optical sectioning effect compared with that for two-photon excitation at the same excitation wavelength. It is also demonstrated that SHG and two-photon fluorescence images under parallel and perpendicular laser excitation polarization can be simultaneously obtained.

Ultrafast spatiotemporal processing with thin-film micro-optics

For spatiotemporal transformation and processing of ultrashort-pulse laser beams, serious design constraints arise from dispersion and diffraction. At pulse durations in 10-fs range, temporal and spatial parameters of propagating wave packets are coupled and significant inhomogeneities appear. To enable a controlled shaping or encoding and a reliable detection or decoding with 2-D spatial resolution, specific advantages of thin-film micro-optical arrays can be exploited. Transmitting and reflecting components of extremely small conical angles are used to generate multiple nondiffracting beams and self-imaging phase patterns. With novel-type metal-dielectric microaxicons, low-dispersion reflective devices are realized. Beam propagation is simulated numerically with Rayleigh-Sommerfeld diffraction theory. For ultrafast time-space conversion, matrix processors consisting of dielectric thin-film microaxicons are tested. Transversally resolving linear and nonlinear autocorrelation techniques are applied to characterize the space-time structure of localized few-cycle wave packets shaped from Ti:sapphire laser beams at pulse durations down to 8 fs. Bessel-like X waves are generated and their propagation is studied. In combination with autocorrelation, wavefront analysis of ultrashort-pulse lasers with Bessel-Shack-Hartmann sensors operated in reflection setup is demonstrated.

Two-photon fluorescence endoscopy with a micro-optic scanning head.

A major obstacle in the race to develop two-photon fluorescence endoscopy is the use of complicated bulk optics to transmit an ultrashort-pulsed laser beam and return the emitted fluorescence signal. We describe an all-fiber two-photon fluorescence microendoscope based on a single-mode optical fiber coupler, a microprism, and a gradient-index rod lens. It is found that the new endoscope exhibits an axial resolution of 3.2 microm and is capable of imaging transverse cross sections of internal cylindrical structures as small as approximately 3.0 mm in diameter. This device demonstrates the potential for developing a real-time diagnostic tool for biomedical research without the need for surgical biopsy and may find applications in photodynamic therapy, microsurgery, and early cancer detection.

Fibre-optic two-photon scanning fluorescence microscopy.

Two geometries of a novel two-photon fluorescence microscope incorporating single-mode fibre optics for the delivery of ultrashort-pulsed illumination to a remote sample are characterized. First, a 785 nm single-mode optical fibre is implemented in a scanning microscope, which demonstrates that an improvement in axial resolution is achieved due to the non-linear response of the fibre to intense ultrashort-pulsed light. Second, a 785 nm single-mode optical fibre coupler is adapted, in which case spectral broadening and blue shifting of the ultrashort-pulsed laser beam caused by the non-linear response of the fibre to ultrashort-pulsed illumination are experimentally characterized. An investigation into the impact of temporal broadening of the ultrashort-pulsed beam on the systems is also considered. The coupling efficiency of both geometries for various illumination wavelengths is also presented. The introduction of the fibre coupler to the system has significant advantages, including an improved optical sectioning effect and a reduction in the number of bulk optical components resulting in a low-cost, compact instrument. Sets of three-dimensional images of fluorescent polymer microspheres and biological material confirm these features.

The effect of polarization on ultrashort pulsed laser ablation of thin metal films

Ultrashort pulse lasers have proven to have superior advantages over conventional continuous wave and long pulse lasers for ablation of thin metal films. Though several investigations have been carried out to understand the phenomena of ultrashort pulse laser machining, the effect of the beam polarization on ablation of thin metal films has been seldom investigated. In this article, we report our recent observations on how the shape of the machined feature and also the damage threshold of the material varies according to the polarization of the ultrashort pulse laser beam. Based on this we have explained how the polarization of the beam controls the laser cutting rate, kerf width, edge quality, and ablation depth of the ablated feature.

Compact two-photon fluorescence microscope based on a single-mode fiber coupler

We present a two-photon fluorescence microscope based on a three-port single-mode optical fiber coupler. It is found that the coupler behaves as a low-pass filter that can deliver an ultrashort-pulsed laser beam of as much as 150 mW of power in the wavelength range from 770 to 870 nm as well as collect a two-photon fluorescence signal in the visible range. As a result of using the fiber coupler, the new two-photon imaging system exhibts a number of advantages, including a compact arrangement, freedom from vibration from lasers and electronic devices, self-alignment, reduction of multiple scattering, and an enhanced optical sectioning effect. The effectiveness of the new instrument is demonstrated with a set of three-dimensional images of biological samples. This instrument may make two-photon fluorescence endoscopy possible for in vivo medical applications.

Polarization-Modulated Second Harmonic Generation in Collagen

Collagen possesses a strong second-order nonlinear susceptibility, a nonlinear optical property characterized by second harmonic generation in the presence of intense laser beams. We present a new technique involving polarization modulation of an ultra-short pulse laser beam that can simultaneously determine collagen fiber orientation and a parameter related to the second-order nonlinear susceptibility. We demonstrate the ability to discriminate among different patterns of fibrillar orientation, as exemplified by tendon, fascia, cornea, and successive lamellar rings in an intervertebral disc. Fiber orientation can be measured as a function of depth with an axial resolution of ∼10 μm. The parameter related to the second-order nonlinear susceptibility is sensitive to fiber disorganization, oblique incidence of the beam on the sample, and birefringence of the tissue. This parameter represents an aggregate measure of tissue optical properties that could potentially be used for optical imaging in vivo.

Resolution improvement in two-photon fluorescence microscopy with a single-mode fiber.

The dependence of spectral broadening of an ultrashort-pulsed laser beam on the fiber length and the illumination power is experimentally characterized in order to deliver the laser for two-photon fluorescence microscopy. It is found that not only the spectral width but also the spectral blue shift increases with the fiber length and illumination power, owing to the nonlinear response in the fiber. For an illumination power of 400 mW in a 3-m-long single-mode fiber, the spectral blue shift is as large as 15 nm. Such a spectral blue shift enhances the contribution from the short-wavelength components within the pulsed beam and leads to an improvement in resolution under two-photon excitation, whereas the efficiency of two-photon excitation is slightly reduced because of the temporal broadening of the pulsed beam. The experimental measurement of the axial response to a two-photon fluorescence polymer block confirms this feature.

Formation of voids in a doped polymethylmethacrylate polymer

We report on the formation of submicrometer voids within a doped polymethylmethacrylate (PMMA) polymer under multiphoton absorption excited by an infrared laser beam. An ultrashort pulsed laser beam of pulse width 80 fs at a repetition rate of 82 MHz and a wavelength of 800 nm is focused into a PMMA-based photorefractive polymer consisting of 2,5-dimethyl-4(p-nitrophenylazo)anisole, 2,4,7-trinitro-9-fluorenone, and N-ethylcarbazole. The large change in refractive index associated with a void allows confocal reflection microscopy to be used as a detection method. Voids can be arranged in a multilayered structure for read-only high-density optical data storage.

The temporal Fresnel diffractive field of a grating illuminated by an ultrashort pulsed-laser beam

An analytical expression is given to calculate the temporal Fresnel diffractive field of a grating illuminated by an ultrashort pulsed-laser beam. Numerical simulation shows that the temporal diffractive intensity distribution is different from that of the input pulse if the width of the input pulse is within several tens of femtoseconds. It is useful to develop a new simple reshaping method for an ultrashort pulse from our approach.

Filamentation of ultrashort pulse laser beams resulting from their propagation over long distances in air

The propagation of high-power short-pulse laser beams over considerable distances in air is studied both experimentally and via numerical simulations. Filaments are formed after 5–10 m and their propagation over distances in excess of 200 m is reported for the first time. The lateral dimensions of the filaments are found to range from about 100 μm to a few millimeters in diameter. The early values of plasma electron density have been inferred to be a few times 1016 cm−3 using longitudinal spectral interferometry. For 500 fs pulses and a wavelength of 1053 nm, the energy in the filament can be quite high initially (∼8 mJ) and is found to stabilize at about 1.5–2 mJ, after about 35 m. A simple model based on the nonlinear Schrödinger equation coupled to a multiphoton ionization law appears to describe several experimental results quite well.

Three-dimensional autofluorescence spectroscopy of rat skeletal muscle tissue under two-photon excitation

We report on three-dimensional autofluorescence spectroscopy obtained from rat skeletal muscle tissue under two-photon excitation by an ultrashort pulsed-laser beam. It is demonstrated that two types of fluorophores within the skeletal muscle tissue can be simultaneously excited with the laser beam at a wavelength of 800 nm. The two fluorophores exhibited unique fluorescence spectral peaks at wavelengths of 450 and 550 nm. These spectroscopic signals can be used to form a three-dimensional image, giving the information about the biochemical makeup of the skeletal muscle tissue.

Fresnel diffraction by circular and serrated apertures illuminated with an ultrashort pulsed-laser beam

Fresnel diffraction patterns by circular and serrated apertures under ultrashort pulsed-laser illumination are investigated in detail. A comparison of the diffraction patterns for pulsed and continuous wave illuminations reveals that an ultrashort pulsed beam of 10 fs can result in a significant effect on the distribution of the intensity. As a result a uniform intensity distribution in the transverse direction of the beam can be achieved as a result of the interference of the different frequency components within the pulsed beam. The interference fringes caused by the wavelets originating from the diffraction aperture can be further reduced when a serrated aperture is used.