Ultrafast Research Articles

Laser frequency stabilization for continuous-wave laser enhanced direct frequency comb spectroscopy system

We present the observation of high-precision direct frequency comb spectroscopy excited by an optical frequency comb and a diode laser when each of them drives one step of the two-photon transition in a rubidium vapor system. We demonstrate a stable and low noise system by directly locking the frequency of the continuous-wave laser to the rubidium two-photon transition. The frequency stability of a diode laser via the two-photon transition locking technique is 8 × 10−11 for a 1 s gate time and 3 × 10−12 for 1000 s. It proves to be a potential technique for locking the diode laser with high stability. We chose a suitable optical frequency comb pulse and the frequency of the diode laser to fulfill the double-resonance condition. These techniques eliminate spectrum line overlap and would benefit spectroscopy measurements.

Single-Step Fabrication of Highly Tunable Blazed Gratings Using Triangular-Shaped Femtosecond Laser Pulses

Blazed gratings are periodic surface structures of great interest for applications such as friction control, light trapping, and spectrometry. While different laser processing methods have been explored to produce these elements, they have not yet surpassed conventional surface manufacturing techniques, often based on lithography processes or mechanical ruling. This work introduces a new approach based on the combination of ultrashort pulses and triangular beam shaping, which enables the generation of asymmetrical grooves in a single step. The main advantage of this strategy is that by simply changing the laser processing direction we can induce a significant modification in the ratio of asymmetry between the sidewall angles of the machined channels. The paper includes a comprehensive study, which has been supported by statistical tools, of the effect of this and other experimental parameters on the morphology of grooves machined on stainless steel. As a result, we achieved a wide range of geometries, with asymmetry ratios spanning from 1 to 5 and channel depths between 3 and 15 µm. Furthermore, we demonstrate the validity of the approach through the successful manufacture of blazed gratings of various slopes. The results reflect the versatility and cost-efficiency of the proposed fabrication strategy, and thus its potential to streamline the production of sawtooth gratings and other devices that are based on asymmetrical features.

Direct observation of entangled electronic-nuclear wave packets

We present momentum resolved covariance measurements of entangled electronic-nuclear wave packets created and probed with octave spanning phaselocked ultrafast pulses. We launch vibrational wave packets on multiple electronic states via multiphoton absorption, and probe these wave packets via strong field double ionization using a second phaselocked pulse. Momentum resolved covariance mapping of the fragment ions highlights the nuclear motion, while measurements of the yield as a function of the relative phase between pump and probe pulses highlight the electronic coherence. The combined measurements allow us to directly visualize the entanglement between the electronic and nuclear degrees of freedom and follow the evolution of the complete wavefunction. Published by the American Physical Society 2024

Fractional Fokas-Lenells equation: analyzing travelling waves via advanced analytical method

In this paper, we consider the fractional Fokas-Lenells equation, which allows us to analyze how a nonlinear optic pulse spreads in time as single-mode fiber produces higher-order nonlinear effects. We have computed perfectly accurate travelling wave solutions for the Fokas-Lenells equation using the Riccati-Bernoulli sub-Ode approach. For the corresponding equation, we have established three distinct classes of perfectly accurate travelling wave solutions with different free parameters; hyperbolic, trigonometric, and rational. A sophisticated Backlund transformation is implemented to the equation to change it to ordinary differential equation domain, leading to many extra exact solutions.

Wideband spectrum compressive sensing utilizing photonic multi-coset sampling with dual low-rate optical pulses

Wideband spectrum compressive sensing utilizing photonic multi-coset sampling with dual low-rate optical pulses

Multiscale Texture Features to Enhance Lubricant Film Thickness for Prosthetic Hip Implant Bearing Surfaces

The longevity of prosthetic hip implants is significantly influenced by wear. Surface textures of various length scales can reduce the friction coefficient and wear of lubricated bearing surfaces. The optimization of multiscale texture parameters, aimed at maximizing lubricant film thickness, was achieved through hydrodynamic lubrication simulations that solve the Reynolds equation with a mass-conserving cavitation model under various operating conditions. The outcomes indicate that adding “interstitial” texture features to a pattern of microscale texture features can further increase the lubricant film thickness. Additionally, the lubricant film thickness increases as the interstitial texture feature aspect ratio and texture density decrease. Pin-on-disc experiments align with simulation findings, demonstrating that multiscale texturing with ultra-fast laser ablation on Ti6Al4V discs significantly improves wettability and reduces the friction coefficient of ultra-high molecular weight polyethylene pins when compared to untextured and microscale textured surfaces. The multiscale surface texturing also changes the evident wear mechanisms on the pins, reducing the incidence of abrasive scratches and adhesive wear compared to both untextured and just microscale textured surfaces.

Cardiovascular magnetic resonance 3D LGE imaging for atrial fibrillation ablation

Abstract Objective To assess feasibility and reliability of cardiac magnetic resonance (CMR) imaging in visualizing left atrial (LA) structural changes that patients with paroxysmal atrial fibrillation (PAF) undergo acutely and long-term post ablation. Two different ablation methods i.e pulsed filed ablation (PFA) and cryoablation were studied. Background Pulmonary vein (PV) isolation has become the cornerstone technique for catheter ablation in patients with drug-refractory atrial fibrillation (AF). At present, almost all ablation technologies are mediated by a thermal effect. Recently, pulsed field ablation (PFA) has been introduced as a new energy source. PFA is a non-thermal ablative modality in which high voltage ultra-short pulses are applied to target tissue, while preserving the extracellular matrix architecture, nerves, and microvascular structures. Few data exist showing different structural LA changes between the two methods using Three-Dimensional (3D) Late Gadolinium Enhancement (LGE) Imaging. Methods CMR imaging was performed pre-ablation, acutely (<24 h), and 3 months post-ablation in 10 patients with paroxysmal atrial fibrillation (AF) undergoing pulmonary vein (PV) isolation with PFA (n = 5) or cryoablation (n = 5). 3D LGE and T2-weighted images were analysed. We obtained two data sets of 3D whole heart LGE imaging with high resolution, 20minutes post gadolinium injection. Patients underwent two acquisitions: the conventional respiratory navigated, electrocardiographically-gated 3D fast gradient echo (1.3slice thickness, 256x256 matrix acquisition) and the image-navigated isotropic high resolution 3D LGE with Dixon water-fat separation. 3D LGE data were analysed using a dedicated (ADAS LA) software in order to produce a 3D-LA model visualization of LGE areas. Results In the acute stage, LGE volume was 50% larger after PFA vs. cryoablation (P < 0.001), and oedema on T2 imaging was significantly smaller (visual estimation) on PFA cases. LGE rings surrounding PV ostia were more homogeneous after PFA, with no sign of microvascular damage or intramural hemorrhage as compared to cryoablation cases. In the chronic stage, the majority of acute LGE had disappeared after PFA, whereas most LGE persisted after cryo-ablation. The two 3D LGE sequences used for analysis showed complete agreement in the visualization of atrial scar with superior image quality of the novel sequence. The mean acquisition time for 3D LGE imaging was 11±4minutes for the conventional fast gradient echo sequence, and 5±2minutes for the novel 3D self-image navigated LGE sequence. Conclusions CMR imaging may help in visualization and understanding of LA structural remodeling post different ablation techniques.

Ultrafast all-optical toggle writing of magnetic bits without relying on heat

Ultrafast excitation of matter can violate Curie’s principle that the symmetry of the cause must be found in the symmetry of the effect. For instance, heating alone cannot result in a deterministic reversal of magnetization. However, if the heating is ultrafast, it facilitates toggle switching of magnetization between stable bit-states without any magnetic field. Here we show that the regime of ultrafast toggle switching can be also realized via a mechanism without relying on heat. Ultrafast laser excitation of iron-garnet with linearly polarized light modifies magnetic anisotropy and thus causes toggling magnetization between two stable bit states. This new regime of ‘cold’ toggle switching can be observed in ferrimagnets without a compensation point and over an exceptionally broad temperature range. The control of magnetic anisotropy required for the toggle switching exhibits reduced dissipation compared to laser-induced-heating mechanism, however the dissipation and the switching-time are shown to be competing parameters.

GHz-rate 57-fs acousto-optic mode-locking fiber laser based on cascaded all-fiber pulse compression

We demonstrate a compact ultrafast fiber laser system that can deliver 1.87 GHz pulse train at 1550 nm with a pulse energy of 52 pJ and an ultrashort pulse duration of 57 fs. While an acousto-optic mode-locking fiber laser was used as the seed light source at GHz rate, a stage of Er-doped fiber amplifier boosted the laser power to ∼320 mW, giving a pulse energy of ∼170 pJ. Then, a pulse compression setup was constructed, providing a high compression ratio of ∼10 with a total efficiency of ∼32%. In the cascaded compression configuration, multiple fiber samples with alternately normal and anomalous dispersion were fused together, providing efficient nonlinear spectral broadening while suppressing excessive pulse broadening over propagation. This GHz-rate ultrafast fiber laser, with compact configuration, broad optical spectrum, and high time-resolving ability could be used as the seed light source for constructing high-rate, high-power ultrafast laser systems and may find a few applications in optical measurements and microwave photonics.

Few-cycle pulse retrieval using amplitude swing technique

Ultrashort pulses have garnered significant attention across various scientific disciplines and applications. In this paper, we demonstrate that the recently introduced amplitude swing technique is a robust method for characterizing pulses in the few-cycle temporal domain by analyzing compressed and chirped pulses from a Ti:Sapphire laser oscillator. The duration of the measured pulse for the case of best compression was 5.98 fs (Fourier limit 5.50 fs) corresponding to 2.2 cycles, while the chirped pulses were up to 15 times temporally stretched. The results obtained have been validated using the d-scan technique, showing excellent agreement in all situations. Therefore, the capability of the amplitude swing technique to measure ultra-broadband pulses in the few-cycle regime is demonstrated, as well as very far from optimum compression, while only being limited by the transparency and birefringence of its elements.

Capturing electron-driven chiral dynamics in UV-excited molecules.

Chiral molecules, used in applications such as enantioselective photocatalysis1, circularly polarized light detection2 and emission3 and molecular switches4,5, exist in two geometrical configurations that are non-superimposable mirror images of each other. These so-called (R) and (S) enantiomers exhibit different physical and chemical properties when interacting with other chiral entities. Attosecond technology might enable influence over such interactions, given that it can probe and even direct electron motion within molecules on the intrinsic electronic timescale6 and thereby control reactivity7-9. Electron currents in photoexcited chiral molecules have indeed been predicted to enable enantiosensitive molecular orientation10, but electron-driven chiral dynamics in neutral molecules have not yet been demonstrated owing to the lack of ultrashort, non-ionizing and perturbative light pulses. Here we use time-resolved photoelectron circular dichroism (TR-PECD)11-15 with an unprecedented temporal resolution of 2.9 fs to map the coherent electronic motion initiated by ultraviolet (UV) excitation of neutral chiral molecules. We find that electronic beatings between Rydberg states lead to periodic modulations of the chiroptical response on the few-femtosecond timescale, showing a sign inversion in less than 10 fs. Calculations validate this and also confirm that the combination of the photoinduced chiral current with a circularly polarized probe pulse realizes an enantioselective filter of molecular orientations following photoionization. We anticipate that our approach will enable further investigations of ultrafast electron dynamics in chiral systems and reveal a route towards enantiosensitive charge-directed reactivity.

Observation of mammalian living cells with femtosecond single pulse illumination generated by a soft X-ray free electron laser

Soft X-ray transmission microscopy is a powerful tool for visualizing cellular structures due to the natural contrast between organic material and water, but radiation damage has hindered its application to living cells. We have developed a soft X-ray microscope using femtosecond pulse illumination generated by a soft X-ray free electron laser, with which structural change of cells caused by radiation damage is negligible. Employing Wolter mirrors for illumination and objective optics allowed us to perform soft X-ray imaging with a large field of view, enabling observation of mammalian cells. We successfully captured images of living cells in a culture medium visualizing their carbon distribution. The broad wavelength-tunability of soft X-ray free electron lasers, in conjunction with the achromaticity of Wolter mirrors, enabled wavelength resolved cellular imaging.

Nonlinear Optics: feature issue introduction

This joint issue of Optics Express and Optical Materials Express showcases 29 articles that report the latest advancements in nonlinear optics. These articles include contributions from authors who participated in the Optica Nonlinear Optics Topical Meeting, which took place in Honolulu, Hawaii, from July 10th to July 14th, 2023. The conference was organized by Optica (formerly known as OSA). As an introduction, the editors provide a summary of these articles, which cover a broad range of topics in nonlinear optics, spanning from fundamental nonlinear optical concepts to novel nonlinear effects, and from innovative nonlinear materials to topics such as ultrafast optics, machine learning empowered nonlinear optics, and unconventional applications. This diverse array of contributions reflects the dynamic and interdisciplinary nature of contemporary research in the field of nonlinear optics while showcasing some of the most recent developments.

Nonlinear Optics: feature issue introduction

This joint issue of Optics Express and Optical Materials Express showcases 29 articles that report the latest advancements in nonlinear optics. These articles include contributions from authors who participated in the Optica Nonlinear Optics Topical Meeting, which took place in Honolulu, Hawaii, from July 10th to July 14th, 2023. The conference was organized by Optica (formerly known as OSA). As an introduction, the editors provide a summary of these articles, which cover a broad range of topics in nonlinear optics, spanning from fundamental nonlinear optical concepts to novel nonlinear effects, and from innovative nonlinear materials to topics such as ultrafast optics, machine learning empowered nonlinear optics, and unconventional applications. This diverse array of contributions reflects the dynamic and interdisciplinary nature of contemporary research in the field of nonlinear optics while showcasing some of the most recent developments.

High-precision spatiotemporal three-dimensional ultrashort pulse synchronization with optical Kerr effect

In studying the interaction of multiple ultrashort pulses with matter, high requirements are put forward for spatiotemporal synchronization accuracy. Limited by the response time and bandwidth of existing devices, the synchronization of multiple ultrashort pulses still faces significant difficulties. By observing the transient phenomena of the optical Kerr effect, high-precision, three-dimensional (x, y, t) synchronization of ultrashort pulses at different angles was achieved. In the optical Kerr effect, the polarization state of the signal pulse changes only when it coincides with the pump pulse, at which point the signal pulse passes through the analyzer. The changes in the intensity and phase of the signal pulse is positively correlated with the degree of spatiotemporal coincidence. In this study, 10-ps pulses were used in the experiments. By observing the intensity and phase distribution of the signal pulses, a time synchronization accuracy between two pulses of less than 1 ps and spatial synchronization accuracy of ±125 µm and ±3 µm in the x and y directions, respectively, were achieved. Moreover, the synchronization of two pulses at an angle of 90 ° was measured, further proving that the method can achieve the spatiotemporal synchronization of pulses with large angles. Therefore, this method has important application prospects in the study of multi-beam interactions with matter and other ultrafast physical phenomena.

Time distribution of stimulated transition probabilities

In recent years, an increasing number of experimental results have been published for a wide variety of systems in which high-precision, ultra-fast, and ultra-short laser pulses techniques have been used to study time-resolved dynamical processes. In the absence of a theoretical prediction of the time distribution of the transition probabilities, the lifetimes τ are generally extracted by fitting the decay time with an exponential, bi-exponential or three-exponential function. In fitting the data, the short-time behavior is generally neglected. The purpose of this study is to show that an explicit formula for the time distribution of the transition probability can be determined rigorously using time-dependent perturbation theory. A formula that perfectly fits an important subset of the experimental results from t = 0 to t=∞ . We show that by following a route different from the usual procedure for deriving transition amplitudes and Einstein coefficients in time-dependent perturbation theory, one ends up with a time-dependent factor, that is, a temporal distribution function of the transition probabilities, and for the Einstein coefficients. The time distribution reported here looks in the time domain similar to the Planck distribution in the frequency domain. In fact, the behavior of the time distribution, with a maximum at 2τln⁡2 , and with τ playing the role of temperature, resembles the behavior of the Planck frequency distribution. We present several examples to demonstrate that the theoretical formula allows for easier fitting of the experimental results reported in the literature. We also show that the time distribution explains the difference in resonance heights between the experimental and theoretical blue laser spectra.

Design of an ultrafast plasmonic nanolaser for high-intensity broadband emission operating at room temperature

We propose a plasmonic nanolaser based on a metal–insulator–semiconductor–insulator–metal (MISIM) structure, which effectively confines light on a subwavelength scale (∼λ/14). As the pump power increases, the proposed plasmonic nanolaser exhibits broadband output characteristics of 20 nm, and the maximum output power can reach 20 µW. Furthermore, the carrier lifetime at the upper energy level in our proposed structure is measured to be about 400 fs using a double pump-probe excitation. The ultrafast characteristic is attributed to the inherent Purcell effect of plasmonic systems. Our work paves the way toward deep-subwavelength mode confinement and ultrafast femtosecond plasmonic lasers in spaser-based interconnected, eigenmode engineering of plasmonic nanolasers, nano-LEDs, and spontaneous emission control.

Antiferromagnetic magnonic charge current generation via ultrafast optical excitation

Néel spin-orbit torque allows a charge current pulse to efficiently manipulate the Néel vector in antiferromagnets, which offers a unique opportunity for ultrahigh density information storage with high speed. However, the reciprocal process of Néel spin-orbit torque, the generation of ultrafast charge current in antiferromagnets has not been demonstrated. Here, we show the experimental observation of charge current generation in antiferromagnetic metallic Mn2Au thin films using ultrafast optical excitation. The ultrafast laser pulse excites antiferromagnetic magnons, resulting in instantaneous non-equilibrium spin polarization at the antiferromagnetic spin sublattices with broken spatial symmetry. Then the charge current is generated directly via spin-orbit fields at the two sublattices, which is termed as the reciprocal phenomenon of Néel spin-orbit torque, and the associated THz emission can be detected at room temperature. Besides the fundamental significance on the Onsager reciprocity, the observed magnonic charge current generation in antiferromagnet would advance the development of antiferromagnetic THz emitter.

Laboratory Demonstration of Grating Embedded Mirrors for Single-Shot Heliostat Optical Metrology

Abstract Concentrated solar power (CSP) plants need to monitor the surface slope error of thousands of heliostats with sub-milliradian accuracy. Large numbers of heliostats installed in harsh environments mean that measurement speed and durability are key design considerations for metrology systems. We present a compact, accurate, and high-speed heliostat slope error metrology system that is robust to the harsh environmental conditions at CSP plants. The system is composed of (1) grating embedded mirrors (GEMs), which have multiple different phase diffraction gratings written within a glass mirror substrate, and (2) a compact optical system, the diffractive auto-stigmatic Hartmann camera (DASHCam). Using focused ultrafast laser pulses, we write phase gratings within second-surface float glass mirror without damaging the reflective coating on the backside. The gratings direct a small fraction of incident light to non-specular directions, which the DASHCam senses from a virtual center of curvature to measure the mirror slopes at each grating patch. In a CSP plant, each heliostat mirror would be a GEM, and the DASHCam would rapidly measure slope and canting errors during heliostat manufacturing, installation, or operation. We fabricated 0.1 meter-diameter GEMs with 24 grating patches, built a prototype DASHCam system, and tested the system repeatability and accuracy by comparing against a Fizeau interferometer. Our results show, in a laboratory environment, 24μrad root mean square (RMS) measurement repeatability and 47μrad RMS accuracy, with single-shot image capture. The combination of GEMs and DASHCam is a promising metrology approach that could lead to improved optical accuracy of heliostats throughout their life cycle. This work serves as a proof of principle for this system.

CPA-ready femtosecond pulses at 1 MHz from a custom recycled output Mamyshev oscillator

CPA-ready femtosecond pulses at 1 MHz from a custom recycled output Mamyshev oscillator