Ultracold Atoms In Optical Lattices Research Articles

Emulating Molecular Orbitals and Electronic Dynamics with Ultracold Atoms

In recent years, ultracold atoms in optical lattices have proven their great value as quantum simulators for studying strongly correlated phases and complex phenomena in solid-state systems. Here we reveal their potential as quantum simulators for molecular physics and propose a technique to image the three-dimensional molecular orbitals with high resolution. The outstanding tunability of ultracold atoms in terms of potential and interaction offer fully adjustable model systems for gaining deep insight into the electronic structure of molecules. We study the orbitals of an artificial benzene molecule and discuss the effect of tunable interactions in its conjugated pi electron system with special regard to localization and spin order. The dynamical time scales of ultracold atom simulators are on the order of milliseconds, which allows for the time-resolved monitoring of a broad range of dynamical processes. As an example, we compute the hole dynamics in the conjugated pi system of the artificial benzene molecule.

Dynamical instabilities and transient short-range order in the fermionic Hubbard model

We study the dynamics of magnetic correlations in the half-filled fermionic Hubbard model following a fast ramp of the repulsive interaction. We use Schwinger-Keldysh self-consistent second-order perturbation theory to investigate the evolution of single-particle Green's functions and solve the non-equilibrium Bethe-Salpeter equation to study the dynamics of magnetic correlations. This approach gives us new insights into the interplay between single-particle relaxation dynamics and the growth of antiferromagnetic correlations. Depending on the ramping time and the final value of the interaction, we find different dynamical behavior which we illustrate using a dynamical phase diagram. Of particular interest is the emergence of a transient short-range ordered regime characterized by the strong initial growth of antiferromagnetic correlations followed by a decay of correlations upon thermalization. The discussed phenomena can be probed in experiments with ultracold atoms in optical lattices.

Local origin of the pseudogap in the attractive Hubbard model

We provide a fresh perspective on the pseudogap physics for attractive fermions as described by the three-dimensional Hubbard model. The pseudogap in the single-particle spectral function, which occurs for temperatures above the critical temperature ${T}_{c}$ of the superfluid transition, is often interpreted in terms of preformed uncondensed pairs. Here we show that the occurrence of pseudogap physics can be consistently understood as due to local excitations which lead to a splitting of the quasiparticle peak for sufficiently large interaction. This effect becomes prominent at intermediate and high temperatures when the quantum-mechanical hopping is incoherent. We demonstrate the absence of the conjectured pairing temperature below which pseudogap physics is expected to occur. Our results are based on approximating the physics of the three-dimensional Hubbard model by dynamical mean-field theory calculations and a momentum independent self-energy. Our predictions can be tested with ultracold atoms in optical lattices with currently available temperatures and spectroscopic techniques.

Spontaneous magnetization and anomalous Hall effect in an emergent Dice lattice.

Ultracold atoms in optical lattices serve as a tool to model different physical phenomena appearing originally in condensed matter. To study magnetic phenomena one needs to engineer synthetic fields as atoms are neutral. Appropriately shaped optical potentials force atoms to mimic charged particles moving in a given field. We present the realization of artificial gauge fields for the observation of anomalous Hall effect. Two species of attractively interacting ultracold fermions are considered to be trapped in a shaken two dimensional triangular lattice. A combination of interaction induced tunneling and shaking can result in an emergent Dice lattice. In such a lattice the staggered synthetic magnetic flux appears and it can be controlled with external parameters. The obtained synthetic fields are non-Abelian. Depending on the tuning of the staggered flux we can obtain either anomalous Hall effect or its quantized version. Our results are reminiscent of Anomalous Hall conductivity in spin-orbit coupled ferromagnets.

Non-standard Hubbard models in optical lattices: a review

Originally, the Hubbard model was derived for describing the behavior of strongly correlated electrons in solids. However, for over a decade now, variations of it have also routinely been implemented with ultracold atoms in optical lattices, allowing their study in a clean, essentially defect-free environment. Here, we review some of the vast literature on this subject, with a focus on more recent non-standard forms of the Hubbard model. After giving an introduction to standard (fermionic and bosonic) Hubbard models, we discuss briefly common models for mixtures, as well as the so-called extended Bose–Hubbard models, that include interactions between neighboring sites, next-neighbor sites, and so on. The main part of the review discusses the importance of additional terms appearing when refining the tight-binding approximation for the original physical Hamiltonian. Even when restricting the models to the lowest Bloch band is justified, the standard approach neglects the density-induced tunneling (which has the same origin as the usual on-site interaction). The importance of these contributions is discussed for both contact and dipolar interactions. For sufficiently strong interactions, the effects related to higher Bloch bands also become important even for deep optical lattices. Different approaches that aim at incorporating these effects, mainly via dressing the basis, Wannier functions with interactions, leading to effective, density-dependent Hubbard-type models, are reviewed. We discuss also examples of Hubbard-like models that explicitly involve higher p orbitals, as well as models that dynamically couple spin and orbital degrees of freedom. Finally, we review mean-field nonlinear Schrödinger models of the Salerno type that share with the non-standard Hubbard models nonlinear coupling between the adjacent sites. In that part, discrete solitons are the main subject of consideration. We conclude by listing some open problems, to be addressed in the future.

Quantum gas microscopy with spin, atom-number, and multilayer readout

Atom- and site-resolved experiments with ultracold atoms in optical lattices provide a powerful platform for the simulation of strongly correlated materials. In this letter, we present a toolbox for the preparation, control and site-resolved detection of a tunnel-coupled bilayer degenerate quantum gas. Using a collisional blockade, we engineer occupation-dependent inter-plane transport which enables us to circumvent light-assisted pair loss during imaging and count n=0 to n=3 atoms per site. We obtain the first number- and site-resolved images of the Mott insulator "wedding cake" structure and observe the emergence of antiferromagnetic ordering across a magnetic quantum phase transition. We are further able to employ the bilayer system for spin-resolved readout of a mixture of two hyperfine states. This work opens the door to direct detection of entanglement and Kosterlitz-Thouless-type phase dynamics, as well as studies of coupled planar quantum materials.

Artificial gauge field induced cyclotron dynamics of ultra-cold atoms in optical lattices

We theoretically study the cyclotron dynamics of ultra-cold atoms in optical lattices exposed to an artificial magnetic field. The cyclotron orbit and its stability are discussed both analytically and numerically. We find that the cyclotron dynamics of atoms in optical lattices can be manipulated by adjusting the strength of the magnetic field. Atoms can be coherently localized in its initial position, or can be trapped in a priori prescribed orbit doing coherent cyclotron motion, or can be decoherently diffused with time. The stability of the orbit and the coherence of the system present asymmetric characters. Our results provide a direct theoretical evidence for the cyclotron dynamics of neutral atoms in the artificial magnetic field.

Observation of antiferromagnetic correlations in the Hubbard model with ultracold atoms.

Ultracold atoms in optical lattices have great potential to contribute to a better understanding of some of the most important issues in many-body physics, such as high-temperature superconductivity. The Hubbard model--a simplified representation of fermions moving on a periodic lattice--is thought to describe the essential details of copper oxide superconductivity. This model describes many of the features shared by the copper oxides, including an interaction-driven Mott insulating state and an antiferromagnetic (AFM) state. Optical lattices filled with a two-spin-component Fermi gas of ultracold atoms can faithfully realize the Hubbard model with readily tunable parameters, and thus provide a platform for the systematic exploration of its phase diagram. Realization of strongly correlated phases, however, has been hindered by the need to cool the atoms to temperatures as low as the magnetic exchange energy, and also by the lack of reliable thermometry. Here we demonstrate spin-sensitive Bragg scattering of light to measure AFM spin correlations in a realization of the three-dimensional Hubbard model at temperatures down to 1.4 times that of the AFM phase transition. This temperature regime is beyond the range of validity of a simple high-temperature series expansion, which brings our experiment close to the limit of the capabilities of current numerical techniques, particularly at metallic densities. We reach these low temperatures using a compensated optical lattice technique, in which the confinement of each lattice beam is compensated by a blue-detuned laser beam. The temperature of the atoms in the lattice is deduced by comparing the light scattering to determinant quantum Monte Carlo simulations and numerical linked-cluster expansion calculations. Further refinement of the compensated lattice may produce even lower temperatures which, along with light scattering thermometry, would open avenues for producing and characterizing other novel quantum states of matter, such as the pseudogap regime and correlated metallic states of the two-dimensional Hubbard model.

Controlling the Directed Quantum Transport of Ultracold Atoms in an Optical Lattice with a Periodic Driving Field

We propose a new method to control the directed quantum transport of ultracold atoms in a one-dimensional optical lattice. In this proposal, the effective tunneling between the neighboring sites can be adjusted via coherent destruction of tunneling by tuning the phase of the external field, instead of using the driving field intensity or the frequency, thus the directed quantum transport of ultracold atoms can be coherently controlled in a much easier manner. Our proposal overcomes the major drawback of the method used by Creffield et al. [Phys. Rev. Lett. 99 (2007) 110501], and can be implemented, in principle, in any one-dimensional optical lattice. Some potential applications of the scheme are also discussed.

Quantized electromagnetic response of three-dimensional chiral topological insulators

Protected by the chiral symmetry, three dimensional chiral topological insulators are characterized by an integer-valued topological invariant. How this invariant could emerge in physical observables is an important question. Here we show that the magneto-electric polarization can identify the integer-valued invariant if we gap the system without coating a quantum Hall layer on the surface. The quantized response is demonstrated to be robust against weak perturbations. We also study the topological properties by adiabatically coupling two nontrivial phases, and find that gapless states appear and are localized at the boundary region. Finally, an experimental scheme is proposed to realize the Hamiltonian and measure the quantized response with ultracold atoms in optical lattices.

18pCS-3 光格子中冷却原子気体に現れるヒッグスモード

18pCS-3 光格子中冷却原子気体に現れるヒッグスモード

Controlling coherence via tuning of the population imbalance in a bipartite optical lattice.

The control of transport properties is a key tool at the basis of many technologically relevant effects in condensed matter. The clean and precisely controlled environment of ultracold atoms in optical lattices allows one to prepare simplified but instructive models, which can help to better understand the underlying physical mechanisms. Here we show that by tuning a structural deformation of the unit cell in a bipartite optical lattice, one can induce a phase transition from a superfluid into various Mott insulating phases forming a shell structure in the superimposed harmonic trap. The Mott shells are identified via characteristic features in the visibility of Bragg maxima in momentum spectra. The experimental findings are explained by Gutzwiller mean-field and quantum Monte Carlo calculations. Our system bears similarities with the loss of coherence in cuprate superconductors, known to be associated with the doping-induced buckling of the oxygen octahedra surrounding the copper sites.

Damping of Bloch oscillations: Variational solutions of the Boltzmann equation beyond linear response

Variational solutions of the Boltzmann equation usually rely on the concept of linear response. We extend the variational approach for tight-binding models at high entropies to a regime far beyond linear response. We analyze both weakly interacting fermions and incoherent bosons on a lattice. We consider a case where the particles are driven by a constant force, leading to the well-known Bloch oscillations, and we consider interactions that are weak enough not to overdamp these oscillations. This regime is computationally demanding and relevant for ultracold atoms in optical lattices. We derive a simple theory in terms of coupled dynamic equations for the particle density, energy density, current, and heat current, allowing for analytic solutions. As an application, we identify damping coefficients for Bloch oscillations in the Hubbard model at weak interactions and compute them for a one-dimensional toy model. We also approximately solve the long-time dynamics of a weakly interacting, strongly Bloch-oscillating cloud of fermionic particles in a tilted lattice, leading to a subdiffusive scaling exponent.

Negative refraction of excitations in the Bose-Hubbard model

Ultracold atoms in optical lattices provide a unique opportunity to study Bose-Hubbard physics. In this work we show that by considering a spatially varying on-site interaction it is possible to manipulate the motion of excitations above the Mott phase in a Bose-Hubbard system. Specifically, we show that it is possible to ``engineer'' regimes where excitations will negatively refract, facilitating the construction of a flat lens.

Chiral magnetism and spontaneous spin Hall effect of interacting Bose superfluids.

Recent experiments on ultracold atoms in optical lattices have synthesized a variety of tunable bands with degenerate double-well structures in momentum space. Such degeneracies in the single-particle spectrum strongly enhance quantum fluctuations, and often lead to exotic many-body ground states. Here we consider weakly interacting spinor Bose gases in such bands, and discover a universal quantum 'order by disorder' phenomenon which selects a novel superfluid with chiral spin order displaying remarkable properties such as spontaneous spin Hall effect and momentum space antiferromagnetism. For bosons in the excited Dirac band of a hexagonal lattice, such a state supports staggered spin loop currents in real space. We show that Bloch oscillations provide a powerful dynamical route to quantum state preparation of such a chiral spin superfluid. Our predictions can be readily tested in spin-resolved time-of-flight experiments.

Optimal quench for distance-independent entanglement and maximal block entropy

We optimize a quantum walk of multiple fermions following a quench in a spin chain to generate near-ideal resources for quantum networking. We first prove a useful theorem mapping the correlations evolved from specific quenches to the apparently unrelated problem of quantum state transfer between distinct spins. This mapping is then exploited to optimize the dynamics and produce large amounts of entanglement distributed in very special ways. Two applications are considered: the simultaneous generation of many Bell states between pairs of distant spins (maximal block entropy) and high entanglement between the ends of an arbitrarily long chain (distance-independent entanglement). Thanks to the generality of the result, we study its implementation in different experimental setups using present technology: nuclear magnetic resonance, ion traps, and ultracold atoms in optical lattices.

Ultrafast dynamics of finite Hubbard clusters: A stochastic mean-field approach

Finite lattice models are a prototype for strongly correlated quantum systems and capture essential properties of condensed matter systems. With the dramatic progress in ultracold atoms in optical lattices, finite fermionic Hubbard systems have become directly accessible in experiments, including their ultrafast dynamics far from equilibrium. Here, we present a theoretical approach that is able to treat these dynamics in any dimension and fully includes inhomogeneity effects. The method consists in stochastic sampling of mean-field trajectories and is found to be more accurate and efficient than current nonequilibrium Green functions approaches. This is demonstrated for Hubbard clusters with up to 512 particles in one, two and three dimensions.

Proposal for a quantum magnetic RC circuit.

We propose a setup that is the spin analog of the charge-based quantum RC circuit. We define and compute the spin capacitance and the spin resistance of the circuit for both ferromagnetic and antiferromagnetic systems. We find that the antiferromagnetic setup has universal properties, but the ferromagnetic setup does not. We discuss how to use the proposed setup as a quantum source of spin excitations, and put forward two possible experimental realizations, using either ultracold atoms in optical lattices or artificially engineered atomic-spin chains.

Enhancing light-atom interactions via atomic bunching

There is a broad interest in enhancing the strength of light-atom interactions to the point where injecting a single photon induces a nonlinear material response. Here we show theoretically that sub-Doppler-cooled two-level atoms that are spatially organized by weak optical fields give rise to a nonlinear material response that is greatly enhanced beyond that attainable in a homogeneous gas. Specifically, in the regime where the intensity of the applied optical fields is much less than the off-resonance saturation intensity, we show that the third-order nonlinear susceptibility scales inversely with atomic temperature and, due to this scaling, can be two orders of magnitude larger than that of a homogeneous gas for typical experimental parameters. As a result, we predict that spatially bunched two-level atoms can exhibit single-photon nonlinearities. Our model is valid for all regimes of atomic bunching and simultaneously accounts for the backaction of the atoms on the optical fields. Our results agree with previous theoretical and experimental results for light-atom interactions that have considered only limited regimes of atomic bunching. For lattice beams tuned to the low-frequency side of the atomic transition, we find that the nonlinearity transitions from a self-focusing type to a self-defocusing type at a critical intensity. We also show that higher than third-order nonlinear optical susceptibilities are significant in the regime where the dipole potential energy is on the order of the atomic thermal energy. We therefore find that it is crucial to retain high-order nonlinearities to accurately predict interactions of laser fields with spatially organized ultracold atoms. The model presented here is a foundation for modeling low-light-level nonlinear optical processes for ultracold atoms in optical lattices.

Optical-lattice implementation scheme of a bosonic topological model with fermionic atoms

We present a scheme to implement a Fermi-Hubbard-like model in ultracold atoms in optical lattices and analyze the topological features of its ground state. In particular, we show that the ground state for appropriate parameters has a large overlap with a lattice version of the bosonic Laughlin state at filling factor one-half. The scheme utilizes laser assisted and normal tunneling in a checkerboard optical lattice. The requirements on temperature, interactions, and hopping strengths are similar to those needed to observe the N\'eel antiferromagnetic ordering in the standard Fermi-Hubbard model in the Mott insulating regime.