Type Of Light-matter Interaction Research Articles

Plasmonic phenomena in molecular junctions: principles and applications.

Molecular junctions are building blocks for constructing future nanoelectronic devices that enable the investigation of a broad range of electronic transport properties within nanoscale regions. Crossing both the nanoscopic and mesoscopic length scales, plasmonics lies at the intersection of the macroscopic photonics and nanoelectronics, owing to their capability of confining light to dimensions far below the diffraction limit. Research activities on plasmonic phenomena in molecular electronics started around 2010, and feedback between plasmons and molecular junctions has increased over the past years. These efforts can provide new insights into the near-field interaction and the corresponding tunability in properties, as well as resultant plasmon-based molecular devices. This Review presents the latest advancements of plasmonic resonances in molecular junctions and details the progress in plasmon excitation and plasmon coupling. We also highlight emerging experimental approaches to unravel the mechanisms behind the various types of light-matter interactions at molecular length scales, where quantum effects come into play. Finally, we discuss the potential of these plasmonic-electronic hybrid systems across various future applications, including sensing, photocatalysis, molecular trapping and active control of molecular switches.

Effect of femtosecond laser pulse repetition rate on nonlinear optical properties of organic liquids

The effect of the repetition rate of femtosecond laser pulses on the two-photon absorption and nonlinear refraction of pure organic liquids is presented using the conventional Z-scan technique. Such a study provides a way to determine the nature of light-matter interaction, explicitly enabling the identification of the linear versus nonlinear regimes. Based on the type of light-matter interaction, we have identified the thermal load dissipation time for the organic liquids. Our experimental results are in good agreement with the theoretically calculated decay time for the dissipation of thermal load.

Self-assembly of predesigned optical materials in nematic codispersions of plasmonic nanorods.

Optical metamaterials and other nanostructured metal-dielectric composites hold great potential for designing and practically realizing novel types of light-matter interactions. Here we develop an approach to fabricate composites with tunable pre-engineered properties via self-assembly of anisotropic nanoparticles codispersed in a nematic liquid crystal host. Orientations of plasmonic nanorods of varying aspect ratios are controlled to align parallel or perpendicular to the nematic director and retain this relative orientation during a facile electric switching. The ensuing dynamic reconfigurability of the surface plasmon resonances of a composite enables a previously inaccessible means of controlling light and may enable tunable plasmonic filters and polarizers.

Quantum information at the interface of light with atomic ensembles and micromechanical oscillators

This article reviews recent research towards a universal light-matter interface. Such an interface is an important prerequisite for long distance quantum communication, entanglement assisted sensing and measurement, as well as for scalable photonic quantum computation. We review the developments in light-matter interfaces based on room temperature atomic vapors interacting with propagating pulses via the Faraday effect. This interaction has long been used as a tool for quantum nondemolition detections of atomic spins via light. It was discovered recently that this type of light-matter interaction can actually be tuned to realize more general dynamics, enabling better performance of the light-matter interface as well as rendering tasks possible, which were before thought to be impractical. This includes the realization of improved entanglement assisted and backaction evading magnetometry approaching the Quantum Cramer-Rao limit, quantum memory for squeezed states of light and the dissipative generation of entanglement. A separate, but related, experiment on entanglement assisted cold atom clock showing the Heisenberg scaling of precision is described. We also review a possible interface between collective atomic spins with nano- or micromechanical oscillators, providing a link between atomic and solid state physics approaches towards quantum information processing.

Nonlinear optics in spheres: from second harmonic scattering to quasi‐phase matched generation in whispering gallery modes

AbstractOver the last fifteen years, a series of theoretical and experimental investigations have demonstrated the usefulness of circular geometries to tailor second‐order nonlinear optical effects. However, until recently, such effects have remained rather weak, calling for their enhancement. In parallel, developments in the field of high quality factor spherical or ring resonators have shown that many different types of light‐matter interactions can be dramatically amplified when light is coupled in the whispering gallery modes of such resonators. In high‐quality spherical micro‐resonators, close to one million interactions can occur between a nonlinear molecule and a circulating light pulse. Recent research on nonlinear optics in spherical geometry is reviewed, from micrometer‐size spheres to whispering gallery mode resonators.