Two-photon Events Research Articles

Electrical trace analysis of superconducting nanowire photon-number-resolving detectors

We apply principal component analysis (PCA) to a set of electrical output signals from a commercially available superconducting nanowire single-photon detector (SNSPD) to investigate their photon-number-resolving capability. We find that the rising edge as well as the amplitude of the electrical signal have the most dependence on photon number. Accurately measuring the rising edge while simultaneously measuring the voltage of the pulse amplitude maximizes the photon-number resolution of SNSPDs. Using an optimal basis of principal components, we show unambiguous discrimination between one- and two-photon events, as well as partial resolution up to five photons. This expands the use case of SNSPDs to photon-counting experiments, without the need of detector multiplexing architectures. Published by the American Physical Society 2024

Machine learning assisted reconstruction of positron-on-target annihilation events in the PADME experiment

Abstract The PADME Experiment at the Laboratori Nationali di Frascati, INFN is used in the search for a Dark photon, produced with an ordinary photon in electron-positron annihilation events. The energy of the photons, emitted in the annihilation is measured using a segmented electromagnetic calorimeter. Machine learning methods consisting of various convolutional neural networks are used for the reconstruction of close-in-time signals with high resolution. These algorithms were used on two-photon annihilation events e + e − → γγ to calibrate the photon energy values. In order to calibrate the neural network output from signal amplitude to energy, the machine learning based results were compared to the conventional methods used for reconstructing the signals. The use of machine learning models for reconstructing real data and the process of calibrating the machine learning method output are presented and discussed.

Search for Resonances in the Mass Spectrum of Two-Photon Events Produced in π+A-Interactions in the Hyperon-M Experiment at the U-70 Accelerator Complex

Studies at the Nuclotron in JINR indicate the presence of a previously unknown resonance-like structure in the two-photon mass spectrum in the region of 300–400 MeV/c2, observed in nucleus–nucleus interactions. The goal of this work is to search for such structures in the two-photon mass spectrum in meson–nuclear interactions at a momentum of 7 GeV/cat the Hyperon-M experiment of the U-70 accelerator complex. An upper limit has been established on the ratio of the cross section for the formation of unknown resonance structures to the cross section for the production ofη-mesonρ(R→2γ/η→2γ)3.2×10−3at the 95% confidence level.

Search for Resonances in the Mass Spectrum of Two-Photon Events Produced in π+A-Interactions in the Hyperon-M Experiment at the U-70 Accelerator Complex

Search for Resonances in the Mass Spectrum of Two-Photon Events Produced in π+A-Interactions in the Hyperon-M Experiment at the U-70 Accelerator Complex

Моделирование двухфотонных событий в сверхпроводящей полоске для различной длины тепловой связи

The results of the study of the evolution of two hot spots formed by the simultaneous absorption of two photons are presented. The lifetime of normal domains and the maximum resistance of the superconducting strip were estimated depending on the distance between the absorbed photons. The minimum distance between the edges of the temperature distribution of hot spots, leading to the loss of thermal coupling, is 28 nm, which is consistent with experimental data. The possibility of distinguishing two-photon events for different reading schemes was evaluated.

Adversarial autoencoder ensemble for fast and probabilistic reconstructions of few-shot photon correlation functions for solid-state quantum emitters

Second-order photon correlation measurements [${g}^{(2)}(\ensuremath{\tau})$ functions] are widely used to classify single-photon emission purity in quantum emitters or to measure the multiexciton quantum yield of emitters that can simultaneously host multiple excitations -- such as quantum dots -- by evaluating the value of ${g}^{(2)}(\ensuremath{\tau}=0)$. Accumulating enough photons to accurately calculate this value is time consuming and could be accelerated by fitting of few-shot photon correlations. Here, we develop an uncertainty-aware, deep adversarial autoencoder ensemble (AAE) that reconstructs noise-free ${g}^{(2)}(\ensuremath{\tau})$ functions from noise-dominated, few-shot inputs. The model is trained with simulated ${g}^{(2)}(\ensuremath{\tau})$ functions that are facilely generated by Poisson sampling time bins. The AAE reconstructions are performed orders-of-magnitude faster, with reconstruction errors and estimates of ${g}^{(2)}(\ensuremath{\tau}=0)$ that are lower in variance and similar in accuracy compared to Maximum likelihood estimation and Levenberg-Marquardt least-squares fitting approaches, for simulated and experimentally measured few-shot ${g}^{(2)}(\ensuremath{\tau})$ functions (\ensuremath{\sim}100 two-photon events) of InP/ZnS/ZnSe and CdS/CdSe/CdS quantum dots. The deep-ensemble model comprises eight individual autoencoders, allowing for probabilistic reconstructions of noise-free ${g}^{(2)}(\ensuremath{\tau})$ functions, and we show that the predicted variance scales inversely with number of shots, with comparable uncertainties to computationally intensive Markov chain Monte Carlo sampling. This work demonstrates the advantage of machine learning models to perform uncertainty-aware, fast, and accurate reconstructions of simple Poisson-distributed photon correlation functions, allowing for on-the-fly reconstructions and accelerated materials characterization of solid-state quantum emitters.

Single-Photon Scattering Can Account for the Discrepancies among Entangled Two-Photon Measurement Techniques.

Entangled photon pairs are predicted to linearize and increase the efficiency of two-photon absorption, allowing continuous wave laser diodes to drive ultrafast time-resolved spectroscopy and nonlinear processes. Despite a range of theoretical studies and experimental measurements, inconsistencies in the value of the entanglement-enhanced interaction cross section persist. A spectrometer that can temporally and spectrally characterize the entangled photon state before, during, and after any potential two-photon excitation event is constructed. For the molecule rhodamine 6G, which has a virtual state pathway, any entangled two-photon interaction is found to be equal to or weaker than classical, single-photon scattering events. This result can account for the discrepancies among the wide variety of entangled two-photon absorption cross sections reported from different measurement techniques. The reported instrumentation can unambiguously separate classical and entangled effects and therefore is important for the growing field of nonlinear and multiphoton entangled spectroscopy.

Quantum imaging with a photon counting camera

Classical light sources emit a randomly-timed stream of individual photons, the spatial distribution of which can be detected with a camera to form an image. Quantum light sources, based on parametric down conversion, emit photons as correlated photon-pairs. The spatial correlations between the photons enables imaging systems where the preferential selection of photon-pairs allows for enhancements in the noise performance over what is possible using classical light sources. However, until now the technical challenge of measuring, and correlating both photons has led to system complexity. Here we show that a camera capable of resolving the number of individual photons in each pixel of the detector array can be used to record an image formed from these photon-pair events and hence achieve a greater contrast than possible using a classical light source. We achieve an enhancement in the ratio of two-photon events compared to one-photon events using spatially correlated SPDC light compared to uncorrelated illumination by a LED. These results indicate the potential advantages of using photon counting cameras in quantum imaging schemes and these advantages will further increase as the technology is developed. Operating in photon sparse regimes such systems have potential applications in low-light microscopy and covert imaging.

Sensitization of Nd3+ Luminescence by Simultaneous Two-Photon Excitation through a Coordinating Polymethinic Antenna.

We have designed and synthesized two new cyaninic Nd3+ complexes where the lanthanide emission can be induced from simultaneous two-photon absorption followed by energy migration. These complexes correspond to a molecular design that uses an antenna ligand formed by the functionalization of a heptamethine dye with 5-ol-phenanthroline or 4-phenyl-terpyridine derivatives. These complexes employ the important nonlinear optical properties of symmetric polymethines to sensitize the lanthanide ion. We verified that simultaneous biphotonic excitation indirectly induces the 4F3/2 → 4I11/2 Nd3+ emission using femtosecond laser pulses tuned below the first electronic transition of the antenna. The simultaneous two-photon excitation events initially form the nonlinear-active second excited singlet of the polymethine antenna, which rapidly evolves into its first excited singlet. This state in turn induces the formation of the emissive Nd3+ states through energy transfer. The role of the first excited singlet of the antenna as the donor state in this process was verified through time resolution of the antenna's fluorescence. These measurements also provided the rates for antenna-lanthanide energy transfer, which indicate that the phenanthroline-type ligand is approximately five times more efficient for energy transfer than the phenyl-terpyridine derivative due to their relative donor-acceptor distances. The simultaneous two-photon excitation of this polymethine antenna allows for high spatial localization of the Nd3+excitation events.

Efficient quantum secure direct communication with complete Bell‐state measurement

Quantum secure direct communication (QSDC) is a powerful technique of transmitting confidential information directly and securely based on the pre-established secure quantum channel and block transmission. Here we propose an efficient QSDC protocol using the complete Bell-state measurement (CBSM) resorting to linear optical elements and temporal-polarization hyperentanglement. In this protocol, the polarized entangled photons are utilized as the information carrier, and all the detection events of CBSM can be identified with common single-photon detectors instead of photon number resolving detectors due to the introduction of temporal degree of freedom (DOF). Moreover, since all the two-photon detection events in CBSM are effective and can be preserved with the efficiency of 100% rather than 50% in the previous QSDC, the quantum efficiency of QSDC can be doubled by encoding more messages on entangled photon pairs.

Boronate carbon nanoparticles featuring efficient FRET for activatable two-photon fluorescence imaging of sialic acid surface-abundant tumor cells.

Two-photon carbon-based nanoprobes hold great potential for biomedical applications as a result of their advantages of low fluorescence background, deep tissue imaging penetration and enhanced spatial resolution. However, the development of an activatable two-photon fluorescence carbon-based nanoprobe that simultaneously has the ability to target desired organs or cells is highly desired but remained a largely unsolved challenge. Herein, we developed boronate affinity BCNP@MnO2 nanocomposites, constructed by one step in situ growth of MnO2 nanosheets on the surface of aminophenylboronic acid-functionalized CNPs (BCNPs) via a redox reaction, which can feature efficient fluorescence energy transfer quenching to the BCNPs, allowing for tumor-specific affinity recognition and two-photon fluorescence activation imaging. By utilizing the inherent two-photon optical properties and sialic acid (SA) specific targeting ability of the BCNPs, good biocompatibility of the nanocomposites as well as highly sensitive and selective responses of MnO2 nanosheets towards GSH, the developed nanocomposites have demonstrated specific two-photon fluorescence activation imaging in target cancer cells and nude mouse tissues. Therefore, our proposed novel strategy could be used for monitoring GSH-triggered two-photon fluorescence activation events in SA-overexpressed cancer cells and has promising applications in both biological exploration and clinical diagnosis.

Pulse shape discrimination of photons and neutrons in the energy range of 0.1 – 2 GeV with the KOTO un-doped CsI calorimeter

A pulse shape difference between photons and neutrons was observed in the output signals of scintillation light from the un-doped CsI calorimeter of the KOTO experiment for the KL→π0νν̄ decay. We developed a discrimination method to reject neutrons and to accept photons in the deposited energy range from 0.1 to 2 GeV. The method rejects 67% of neutron-induced single hadronic clusters and 86% of neutron-induced two-cluster events while keeping more than 90% of photon-induced single electromagnetic clusters and two-photon events.

PASSAT: particle accelerator helioScopes for Slim Axion-like-particle deTection

We propose a novel method to search for axion-like particles (ALPs) at particle accelerator experiments. ALPs produced at the target via the Primakoff effect subsequently enter a region with a magnetic field, where they are converted to photons that are then detected. Dubbed Particle Accelerator helioScopes for Slim Axion-like-particle deTection (PASSAT), our proposal uses the principle of the axion helioscope but replaces ALPs produced in the Sun with those produced in a target material. Since we rely on ALP-photon conversions, our proposal probes light (slim) ALPs that are otherwise inaccessible to laboratory-based experiments which rely on ALP decay, and complements astrophysical probes that are more model-dependent. As a first application, we reinterpret existing data from the NOMAD experiment in light of PASSAT, and constrain the parameter space for ALPs lighter than sim 100~mathrm{eV} and ALP-photon coupling larger than sim 10^{-4}~mathrm{GeV}^{-1}. As benchmarks of feasible low-cost experiments improving over the NOMAD limits, we study the possibility of re-using the magnets of the CAST and the proposed BabyIAXO experiments and placing them at the proposed BDF facility at CERN, together with some new detectors. We find that these realizations of PASSAT allow for a direct probe of the parameter space for ALPs lighter than sim 100~mathrm{eV} and ALP-photon coupling larger than sim 4times 10^{-6}~mathrm{GeV}^{-1}, which are regions that have not been probed yet by experiments with laboratory-produced ALPs. In contrast to other proposals aiming at detecting single or two-photon only events in hadronic beam dump environments, that rely heavily on Monte Carlo simulations, the background in our proposal can be directly measured in-situ, its suppression optimized, and the irreducible background statistically subtracted. Sensitivity evaluations with other beams will be the subject of a future paper. The measurements suggested in this paper represent an additional physics case for the BDF at CERN beyond those already proposed.

Quantum Pyragas control: Selective control of individual photon probabilities

Pyragas control allows to stabilize unstable states in applied nonlinear science. We propose to apply a quantum version of the Pyragas protocol to control individual photon-probabilities in an otherwise only globally accessible photon-probability distribution of a quantum light emitter. The versatility of quantum Pyragas control is demonstrated for the case of a two-level emitter in a pulsed laser-driven half cavity. We show that one- and two-photon events respond in a qualitatively different way to the half-cavity induced feedback signal. One-photon events are either enhanced or suppressed, depending on the choice of parameters. In contrast, two-photon events undergo exclusively an enhancement up to $50\%$ for the chosen pulse areas. We hereby propose an implementation of quantum Pyragas control via a time-delayed feedback setup.

A scalable multi-photon coincidence detector based on superconducting nanowires.

Coincidence detection of single photons is crucial in numerous quantum technologies and usually requires multiple time-resolved single-photon detectors. However, the electronic readout becomes a major challenge when the measurement basis scales to large numbers of spatial modes. Here, we address this problem by introducing a two-terminal coincidence detector that enables scalable readout of an array of detector segments based on superconducting nanowire microstrip transmission line. Exploiting timing logic, we demonstrate a sixteen-element detector that resolves all 136 possible single-photon and two-photon coincidence events. We further explore the pulse shapes of the detector output and resolve up to four-photon events in a four-element device, giving the detector photon-number-resolving capability. This new detector architecture and operating scheme will be particularly useful for multi-photon coincidence detection in large-scale photonic integrated circuits.

Frequency-resolved Monte Carlo

We adapt the Quantum Monte Carlo method to the cascaded formalism of quantum optics, allowing us to simulate the emission of photons of known energy. Statistical processing of the photon clicks thus collected agrees with the theory of frequency-resolved photon correlations, extending the range of applications based on correlations of photons of prescribed energy, in particular those of a photon-counting character. We apply the technique to autocorrelations of photon streams from a two-level system under coherent and incoherent pumping, including the Mollow triplet regime where we demonstrate the direct manifestation of leapfrog processes in producing an increased rate of two-photon emission events.

Fast recognition of single quantum dots from high multi-exciton emission and clustering effects.

Recognition of single quantum dots (QDs) from high multi-exciton emission and clustering effects is challenging using the conventional second-order correlation function method. Here we demonstrate a method for fast recognizing single QDs based on the probabilities of detecting single- and two-photon events. The time-tagged, time-resolved and time-correlated single-photon counting technique is applied to effectively remove multi-exciton emission and low-counting background. By this way, single QDs can be fastly recognized by the spatial coincidence-counting model. In addition, the fast recognition of single QDs by using the collected photons during the confocal scanning imaging process has been achieved synchronously.

Pulsed Rabi oscillations in quantum two-level systems: beyond the area theorem

The area theorem states that when a short optical pulse drives a quantum two-level system, it undergoes Rabi oscillations in the probability of scattering a single photon. In this work, we investigate the breakdown of the area theorem as both the pulse length becomes non-negligible and for certain pulse areas. Using simple quantum trajectories, we provide an analytic approximation to the photon emission dynamics of a two-level system. Our model provides an intuitive way to understand re-excitation, which elucidates the mechanism behind the two-photon emission events that can spoil single-photon emission. We experimentally measure the emission statistics from a semiconductor quantum dot, acting as a two-level system, and show good agreement with our simple model for short pulses. Additionally, the model clearly explains our recent results (Fischer and Hanschke 2017 et al Nat. Phys.) showing dominant two-photon emission from a two-level system for pulses with interaction areas equal to an even multiple of π.

Calibration of the KEDR detector Tagging System with two-photon lepton pair production

The tagging system of the KEDR detector for the two-photon studies is briefly described. The procedure of the energy calibration of the system is considered. Two-photon events e+e− → e+e− +μ+μ− selected with the central detector were employed to check the energy calibration and to measure the tagging efficiencies. The results obtained demonstrate that the achieved accuracy of the energy calibration is about 1%. To improve the accuracy to the level of 0.3% the upgrade of the calibration system is ongoing. The tagging efficiencies obtained with the simulation agree with the measured one within the error of the measurement.

Development of two-photon event generators for the KEDR experiment

The KEDR experiment, which started in 2002, is dedicated to a study of c- and b-quarks and the two-photon physics at the e+e− collider VEPP-4M in the Budker INP. To analyze the 2γ data and estimate contribution of two-photon background events in the 1 data samples, the event generators e+e− → e+e− + hadrons, e+e− → e+e− + π+π−, and e+e− → e+e− + PS (PS – pseudoscalar meson) have been developed.