Two-level Quantum System Research Articles

General Non-Markovian Quantum Dynamics.

A general approach to the construction of non-Markovian quantum theory is proposed. Non-Markovian equations for quantum observables and states are suggested by using general fractional calculus. In the proposed approach, the non-locality in time is represented by operator kernels of the Sonin type. A wide class of the exactly solvable models of non-Markovian quantum dynamics is suggested. These models describe open (non-Hamiltonian) quantum systems with general form of nonlocality in time. To describe these systems, the Lindblad equations for quantum observable and states are generalized by taking into account a general form of nonlocality. The non-Markovian quantum dynamics is described by using integro-differential equations with general fractional derivatives and integrals with respect to time. The exact solutions of these equations are derived by using the operational calculus that is proposed by Yu. Luchko for general fractional differential equations. Properties of bi-positivity, complete positivity, dissipativity, and generalized dissipativity in general non-Markovian quantum dynamics are discussed. Examples of a quantum oscillator and two-level quantum system with a general form of nonlocality in time are suggested.

Experimental demonstration of optimal probabilistic enhancement of quantum coherence

We theoretically and experimentally investigate conditional enhancement of overall coherence of quantum states by probabilistic quantum operations that apply to the input state a quantum filter diagonal in the basis of incoherent states. We identify the optimal filters that for a given probability of successful filtering maximize the output coherence. We verify the performance of the studied quantum filters in a proof-of-principle experiment with linear optics, where a pair of two-level quantum systems is represented by polarization states of two photons. We comprehensively characterize the implemented two-qubit linear optical quantum filters by full quantum process tomography and we experimentally observe the optimal quantum coherence enhancement by quantum filtering.

Subharmonics and superharmonics of the weak field in a driven two-level quantum system: Vibrational resonance enhancement.

We consider a quantum two-level system in bichromatic classical time-periodic fields, the frequency of one of which far exceeds that of the other. Based on systematic separation of timescales and averaging over the fast motion a reduced quantum dynamics in the form of a nonlinear forced Mathieu equation is derived to identify the stable oscillatory resonance zones intercepted by unstable zones in the frequency-amplitude plot. We show how this forcing of the dressed two-level system may generate the subharmonics and superharmonics of the weak field in the stable region, which can be amplified by optimization of the strength of the high frequency field. We have carried out detailed numerical simulations of the driven quantum dynamics to corroborate the theoretical analysis.

On Reachable and Controllability Sets for Minimum-Time Control of an Open Two-Level Quantum System

On Reachable and Controllability Sets for Minimum-Time Control of an Open Two-Level Quantum System

Measurement of work and heat in the classical and quantum regimes

Despite the increasing interest, the research field which studies the concepts of work and heat at quantum level has suffered from two main drawbacks: first, the difficulty to properly define and measure the work, heat and internal energy variation in a quantum system and, second, the lack of experiments. Here, we report a full characterization of the dissipated heat, work and internal energy variation in a two-level quantum system interacting with an engineered environment. We use the IBMQ quantum computer to implement the driven system's dynamics in a dissipative environment. The experimental data allow us to construct quasi-probability distribution functions from which we recover the correct averages of work, heat and internal energy variation in the dissipative processes. Interestingly, by increasing the environment coupling strength, we observe a reduction of the pure quantum features of the energy exchange processes that we interpret as the emergence of the classical limit. This makes the present approach a privileged tool to study, understand and exploit quantum effects in energy exchanges.

Fermi's Golden Rule for Spontaneous Emission in Absorptive and Amplifying Media.

We demonstrate a fundamental breakdown of the photonic spontaneous emission (SE) formula derived from Fermi's golden rule, in absorptive and amplifying media, where one assumes the SE rate scales with the local photon density of states, an approach often used in more complex, semiclassical nanophotonics simulations. Using a rigorous quantization of the macroscopic Maxwell equations in the presence of arbitrary linear media, we derive a corrected Fermi's golden rule and master equation for a quantum two-level system (TLS) that yields a quantum pumping term and a modified decay rate that is net positive. We show rigorous numerical results of the temporal dynamics of the TLS for an example of two coupled microdisk resonators, forming a gain-loss medium, and demonstrate the clear failure of the commonly adopted formulas based solely on the local density of states.

Quantum Wave-Particle Duality in Free-Electron-Bound-Electron Interaction.

We present a comprehensive relativistic quantum-mechanical theory for interaction of a free electron with a bound electron in a model, where the free electron is represented as a finite-size quantum electron wave packet (QEW) and the bound electron is modeled by a quantum two-level system (TLS). The analysis reveals the wave-particle duality nature of the QEW, delineating the point-particle-like and wavelike interaction regimes and manifesting the physical reality of the wave function dimensions when interacting with matter. This QEW size dependence may be used for interrogation and coherent control of superposition states in a TLS and for enhancement of cathodoluminescence and electron energy-loss spectroscopy in electron microscopy.

Spin dynamics under the influence of elliptically rotating fields: Extracting the field topology from time-averaged quantities.

Systems that can be effectively described as a localized spin-s particle subject to time-dependent fields have attracted a great deal of interest due to, among other things, their relevance for quantum technologies. Establishing analytical relationships between the topological features of the applied fields and certain time-averaged quantities of the spin can provide important information for the theoretical understanding of these systems. Here, we address this question in the case of a localized spin-s particle subject to a static magnetic field coplanar to a coexisting elliptically rotating magnetic field. The total field periodically traces out an ellipse which encloses the origin of the coordinate system or not, depending on the values taken on by the static and the rotating components. As a result, two regimes with different topological properties characterized by the winding number of the total field emerge: the winding number is 1 if the origin lies inside the ellipse, and 0 if it lies outside. We show that the time average of the energy associated with the rotating component of the magnetic field is always proportional to the time average of the out-of-plane component of the expectation value of the spin. Moreover, the product of the signs of these two time-averaged quantities is uniquely determined by the topology of the total field and, consequently, provides a measurable indicator of this topology. We also propose an implementation of these theoretical results in a trapped-ion quantum system. Remarkably, our findings are valid in the totality of the parameter space and regardless of the initial state of the spin. In particular, when the system is prepared in a Floquet state, we demonstrate that the quasienergies, as a function of the driving amplitude at constant eccentricity, have stationary points at the topological transition boundary. The ability of the topological indicator proposed here to accurately locate the abrupt topological transition can have practical applications for the determination of unknown parameters appearing in the Hamiltonian. In addition, our predictions about the quasienergies can assist in the interpretation of conductance measurements in transport experiments with spin carriers in mesoscopic rings.

Entanglement dynamics for two-level quantum systems coupled with massive scalar fields

Entanglement is essential in quantum information science. Typically, the inevitable coupling between quantum systems and environment inhibits entanglement from being created between long-distance subsystems and being maintained for a long time. In this paper, we show that when the environment is composed of a bath of massive scalar fields, the region of the separation within which entanglement can be generated is significantly enlarged, and the decay rate of entanglement is significantly slowed down compared with those in the massless case, when the mass of the field m is smaller than but close to the transition frequency of the qubits ω. When m≥ω, the initial entanglement can be maintained for an arbitrarily long time, regardless of the environmental temperature. Therefore, in principle, it is possible to achieve long-distance entanglement generation and long-lived entanglement by manipulating the energy level spacing of the two-level systems with respect to the mass of the field.

Angle-resolved Rabi flopping in strong-field dissociation of molecules

Rabi flopping is a paradigm of two-level quantum systems in the presence of an oscillatory driving field. Different from atoms, the Rabi flopping in a molecule depends on its bond length and orientation with respect to the light polarization direction. Here we explore the Rabi flopping in the strong-field dissociation of ${\mathrm{H}}_{2}{}^{+}$ in which the two lowest electronic states are photon coupled. ${\mathrm{H}}_{2}{}^{+}$ aligned along different angles experiences different laser intensities, building the Rabi flopping with angle-dependent frequencies. During the laser-${\mathrm{H}}_{2}{}^{+}$ interaction, the electron completes different fractions of Rabi flopping for ${\mathrm{H}}_{2}{}^{+}$ aligned in different directions, leading to the angular nodes and maxima in the dissociative proton momentum distribution. Our study reveals that one-photon dissociation undergoes the alternation of absorbing and emitting one photon, instead of the one-off photon absorption. This study also provides a universal explanation for the angular distribution of the dissociative fragments in strong laser fields.

Transition probabilities for flavor eigenstates of non-Hermitian Hamiltonians in the PT-broken phase

We investigate the transition probabilities for the “flavor” eigenstates in the two-level quantum system, which is described by a non-Hermitian Hamiltonian with the parity and time-reversal (PT) symmetry. Particularly, we concentrate on the so-called PT-broken phase, where two eigenvalues of the non-Hermitian Hamiltonian turn out to be a complex-conjugate pair. In this case, we find that the transition probabilities will be unbounded in the limit of infinite time t → +∞. However, after performing a connection between a non-Hermitian system, which exhibits passive PT symmetry and global decay, and the neutral-meson system in particle physics, we observe that the diverging behavior of the transition probabilities is actually applicable to the gauge-transformed neutral-meson states, whereas the transition probabilities for physical states are exponentially suppressed by the global decay. We also present a brief review on the situation at the so-called exceptional point, where both the eigenvalues and eigenvectors of the Hamiltonian coalesce.

Dynamical formulation of low-energy scattering in one dimension

The transfer matrix M of a short-range potential may be expressed in terms of the time-evolution operator for an effective two-level quantum system with a time-dependent non-Hermitian Hamiltonian. This leads to a dynamical formulation of stationary scattering. We explore the utility of this formulation in the study of the low-energy behavior of the scattering data. In particular, for the exponentially decaying potentials, we devise a simple iterative scheme for computing terms of arbitrary order in the series expansion of M in powers of the wavenumber. The coefficients of this series are determined in terms of a pair of solutions of the zero-energy stationary Schrödinger equation. We introduce a transfer matrix for the latter equation, express it in terms of the time-evolution operator for an effective two-level quantum system, and use it to obtain a perturbative series expansion for the solutions of the zero-energy stationary Schrödinger equation. Our approach allows for identifying the zero-energy resonances for scattering potentials in both full line and half-line with zeros of the entries of the zero-energy transfer matrix of the potential or its trivial extension to the full line.

Density-matrix formalism for PT -symmetric non-Hermitian Hamiltonians with the Lindblad equation

In the presence of Lindblad decoherence, i.e. dissipative effects in an open quantum system due to interaction with an environment, we examine the transition probabilities between the eigenstates in the two-level quantum system described by non-Hermitian Hamiltonians with the Lindblad equation, for which the parity-time-reversal (PT) symmetry is conserved. First, the density matrix formalism for PT-symmetric non-Hermitian Hamiltonian systems is developed. It is shown that the Lindblad operators $L^{}_j$ are pseudo-Hermitian, namely, $\eta L^{}_j \eta^{-1} = L^\dagger_j$ with $\eta$ being a linear and positive-definite metric, and respect the PT symmetry as well. We demonstrate that the generalized density matrix $\rho^{}_{\rm G}(t) \equiv \rho(t) \eta$, instead of the normalized density matrix $\rho^{}_{\rm N}(t) \equiv \rho(t)/{\rm tr}\left[\rho(t)\right]$, should be implemented for the calculation of the transition probabilities in accordance with the linearity requirement. Second, the density matrix formalism is used to derive the transition probabilities in general cases of PT-symmetric non-Hermitian Hamiltonians. In some concrete examples, we calculate compact analytical formulas for the transition probabilities and explore their main features with numerical illustrations. We also make a comparison between our present results and our previous ones using state vectors in the absence of Lindblad decoherence.

Exponential stabilization of two-level quantum systems based on continuous noise-assisted feedback

The exponential stabilization of the eigenstates for two-level quantum systems based on continuous noise-assisted feedback control is investigated in this paper. Due to the symmetric structure of state space, quantum systems may converge to an undesired eigenstate under continuous measurement. In order to overcome the convergence obstacle, the continuous noise-assisted feedback strategy, in which the control signal is driven by an exogenous Brownian noise, is proposed to make the quantum systems converge to the target eigenstates exponentially, and the noise gain is designed as a continuously differentiable function of quantum state, which is negatively related to the distance between system state and the target eigenstate. In particular, the exponential convergence is proved based on the stability theory of stochastic differential equations. Moreover, the numerical simulations on a two-level quantum system are performed to verify the effectiveness of noise-assisted feedback control and study the influences of physical parameters and control parameters on convergence rate.

Auxiliary open quantum system for the Floquet quantum master equation.

By directly using the probability formulas of quantum trajectories, we construct an auxiliary open quantum system for a periodically driven open quantum system whose dynamics is governed by the Floquet quantum master equation. This auxiliary system can generate a quantum trajectory ensemble that is consistent with the canonical quantum trajectory ensemble. We find that, at a long time limit, though the Lindblad operators are modified, the coherent dynamics of the auxiliary system is the same as that of the original system. A periodically driven two-level quantum system is used to illustrate this construction.

Split-ring polariton condensates as macroscopic two-level quantum systems

Superposition states of circular currents of exciton-polaritons mimic the superconducting flux qubits. The phase of a polariton fluid must change by an integer number of $2\pi$, when going around the ring. If one introduces a ${\pi}$-phase delay line in the ring, the fluid is obliged to propagate a clockwise or anticlockwise circular current to reduce the total phase gained over one round-trip to zero or to build it up to $2\pi$. We show that such a $\pi$-delay line can be provided by a dark soliton pinned to a potential well created by a C-shape non-resonant pump-spot. The resulting split-ring polariton condensates exhibit pronounced coherent oscillations passing periodically through clockwise and anticlockwise current states. These oscillations may persist far beyond the coherence time of polariton condensates. The qubits based on split-ring polariton condensates are expected to possess very high figures of merit that makes them a valuable alternative to superconducting qubits. The use of the dipole-polarized polaritons allows to control coherently the state of the qubit with the external electric field. This is shown to be one of the tools for realization of single-qubit logic operations. We propose the design of an $i$SWAP gate based on a pair of coupled polariton qubits. To demonstrate the capacity of the polariton platform for quantum computations, we propose a protocol for the realization of the Deutsch's algorithm with polariton qubit networks.

Vibrational resonance in a driven two-level quantum system, linear and nonlinear response.

We consider a two-level quantum system interacting with two classical time-periodic electromagnetic fields. The frequency of one of the fields far exceeds that of the other. The effect of the high-frequency field can be averaged out of the dynamics to realize an effective transition frequency of the field-dressed two-level system. We examine the linear response, second harmonic response and Stokes and anti-Stokes Raman response of the dressed two-level system, to the weak frequency field. The vibrational resonance enhancement in each case is demonstrated for optimal strength of the high-frequency field. Our theoretical scheme is corroborated by full numerical simulation of the two-level, two-field dynamics governed by loss-free Bloch equations. We suggest that quantum optics can offer an interesting arena for the study of the vibrational resonance. This article is part of the theme issue 'Vibrational and stochastic resonance in driven nonlinear systems (part 1)'.

Experimental simulation of the parity-time symmetric dynamics using photonic qubits

The concept of parity-time (PT) symmetry originates from the framework of quantum mechanics, where if the Hamiltonian operator satisfies the commutation relation with the parity and time operators, it shows real energy spectrum. Recently, PT symmetry was introduced into various systems, such as optics, electronic circuits, acoustics, and other classical fields to further study the dynamical behaviors of the Hamiltonian and the energies. To focus on the dynamical evolution of the quantum state, here we experimentally studied the dynamical evolution of a two-level quantum system under the PT symmetric Hamiltonian using single-photon system. By enlarging the system using ancillary qubit and encoding the subsystem under the non-Hermitian Hamiltonian with post-selection, the evolution of the state can be characterized with a high fidelity. Owing to the effectively operation of the dilation method, our work provides a route for further exploiting the exotic properties of PT symmetric Hamiltonian for quantum simulation and quantum information processing.

Transfermatrix in scattering theory: a survey of basic properties and recent developments

We give a pedagogical introduction to time-independent scattering theory in one dimension focusing on the basic properties and recent applications of transfer matrices. In particular, we begin surveying some basic notions of potential scattering such as transfer matrix and its analyticity, multi-delta-function and locally periodic potentials, Jost solutions, spectral singularities and their time-reversal, and unidirectional reflectionlessness and invisibility. We then offer a simple derivation of the Lippmann-Schwinger equation and Born series, and discuss the Born approximation. Next, we outline a recently developed dynamical formulation of time-independent scattering theory in one dimension. This formulation relates the transfer matrix and therefore the solution of the scattering problem for a given potential to the solution of the time-dependent Schrodinger equation for an effective non-unitary two-level quantum system. We provide a self-contained treatment of this formulation and some of its most important applications. Specifically, we use it to devise a powerful alternative to the Born series and Born approximation, derive dynamical equations for the reflection and transmission amplitudes, discuss their application in constructing exact tunable unidirectionally invisible potentials, and use them to provide an exact solution for single-mode inverse scattering problems. The latter, which has important applications in designing optical devices with a variety of functionalities, amounts to providing an explicit construction for a finite-range complex potential whose reflection and transmission amplitudes take arbitrary prescribed values at any given wavenumber.

Long-Range Coherence and Multiple Steady States in a Lossy Qubit Array.

We show that a simple experimental setting of a locally pumped and lossy array of two-level quantum systems can stabilize states with strong long-range coherence. Indeed, by explicit analytic construction, we show there is an extensive set of steady-state density operators, from minimally to maximally entangled, despite this being an interacting open many-body problem. Such nonequilibrium steady states arise from a hidden symmetry that stabilizes Bell pairs over arbitrarily long distances, with unique experimental signatures. We demonstrate a protocol by which one can selectively prepare these states using dissipation. Our findings are accessible in present-day experiments.