Dielectric properties of nanocrystalline Nd-modified Pb(ZrxTi1-x)O3 thin films were studied in frequency range f = 100 Hz –20 GHz. Thin films were prepared by pulsed laser deposition on MgO(100) substrates. Inter-digital electrodes and coplanar waveguide transmission line technique were used for dielectric characterization. In the dielectric function ɛr(f, T), two interesting anomalies were found at low frequencies. Diffusive phase transition had relaxor-type behaviour, and an extra dielectric relaxation maxima were found below Curie temperature TC. At higher frequencies above 5 GHz, relative permittivity ɛr(f) response was flat up to 20 GHz, and high maximum tunability nr,max = 19% was achieved.
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