When topology meets chirality, it is of great interest to search for possible topological properties in chiral crystals, thereby achieving the effect of making $1+1$ greater than 2. Here, we accomplish a complete list of topological charge-2 (C-2) Dirac fermions based on 65 S\"ohncke space groups. Such emergent fermions occurring in chiral crystals enjoy a higher topological charge number and exhibit more unique characteristics compared to C-0 cases, including multiple Fermi arcs extending to most of the Brillouin zone. For material realization, we propose that an ultralightweight chiral crystal ${\mathrm{N}}_{4}\mathrm{Cl}$ is a high-quality C-2 Dirac semimetal, where the seductive nodal points reside at the Fermi level and exhibit a large linear energy range to overcome the interruption of irrelevant bands. More interestingly, the doubly degenerate Landau levels are described by a Kramers-like degeneracy in such a C-2 Dirac fermion, featuring a doubly degenerate zero mode. Furthermore, the topological phase transitions from Dirac to Weyl states of ${\mathrm{N}}_{4}\mathrm{Cl}$ can be manipulated by applying shear strains. These fascinating findings will certainly evoke continued exploration of unconventional Dirac semimetals, in turn leading to extensive application prospects and uncommon insights.
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