Tomonaga-Luttinger Liquid Theory Research Articles

Exact results of dynamical structure factor of Lieb–Liniger model

The dynamical structure factor (DSF) represents a measure of dynamical density–density correlations in a quantum many-body system. Due to the complexity of many-body correlations and quantum fluctuations in a system of an infinitely large Hilbert space, such kind of dynamical correlations often impose a big theoretical challenge. For one-dimensional (1D) quantum many-body systems, qualitative predictions of dynamical response functions are usually carried out by using the Tomonaga–Luttinger liquid (TLL) theory. In this scenario, a precise evaluation of the DSF for a 1D quantum system with arbitrary interaction strength remains a formidable task. In this paper, we use the form factor approach based on algebraic Bethe ansatz theory to calculate precisely the DSF of Lieb–Liniger model with an arbitrary interaction strength at a large scale of particle number. We find that the DSF for a system as large as 2000 particles enables us to depict precisely its line-shape from which the power-law singularity with corresponding exponents in the vicinities of spectral thresholds naturally emerge. It should be noted that, the advantage of our algorithm promises an access to the threshold behavior of dynamical correlation functions, further confirming the validity of nonlinear TLL theory besides Kitanine et al (2012 J. Stat. Mech. P09001). Finally we discuss a comparison of results with the results from the ABACUS method by J-S Caux (2009 J. Math. Phys. 50 095214) as well as from the strongly coupling expansion by Brand and Cherny (2005 Phys. Rev. A 72 033619).

Unambiguous Experimental Verification of Linear-in-Temperature Spinon Thermal Conductivity in an Antiferromagnetic Heisenberg Chain.

The everlasting interest in spin chains is mostly rooted in the fact that they generally allow for comparisons between theory and experiment with remarkable accuracy, especially for exactly solvable models. A notable example is the spin-1/2 antiferromagnetic Heisenberg chain (AFHC), which can be well described by the Tomonaga-Luttinger liquid theory and exhibits fractionalized spinon excitations with distinct thermodynamic and spectroscopic experimental signatures consistent with theoretical predictions. A missing piece, however, is the lack of a comprehensive understanding of the spinon heat transport in AFHC systems, due to difficulties in its experimental evaluation against the backdrop of other heat carriers and complex scattering processes. Here we address this situation by performing ultralow-temperature thermal conductivity measurements on a nearly ideal spin-1/2 AFHC system copper benzoate Cu(C_{6}H_{5}COO)_{2}·3H_{2}O, whose field-dependent spin excitation gap enables a reliable extraction of the spinon thermal conductivity κ_{s} at zero field. κ_{s} was found to exhibit a linear temperature dependence κ_{s}∼T at low temperatures, with κ_{s}/T as large as 1.70 mW cm^{-1} K^{-2}, followed by a precipitate decline below ∼0.3 K. The observed κ_{s}∼T clarifies the discrepancies between various spin chain systems and serves as a benchmark for one-dimensional spinon heat transport in the low-temperature limit. The abrupt loss of κ_{s} with no corresponding anomaly in the specific heat is discussed in the context of many-body localization.

Evolution of one-dimensional electronic dynamics in Nb2n+1SinTe4n+2

The electronic dynamics in ${\mathrm{Nb}}_{2n+1}{\mathrm{Si}}_{n}{\mathrm{Te}}_{4n+2}$ with varying component $n$ are systematically investigated by low-temperature scanning tunneling microscopy/spectroscopy (STM/STS). Our quasiparticle interferences reveal a nondecay standing wave at the Fermi level, proving the one-dimensional (1D) nature of the charge carriers (holes) in the materials. The energy and component dependence of phase relaxation length ${l}_{\ensuremath{\phi}}$ and lifetime $\phantom{\rule{4pt}{0ex}}\ensuremath{\tau}$ of 1D holes are unveiled and found to be consistent with the Tomonaga-Luttinger liquid theory. Our work demonstrates ${\mathrm{Nb}}_{2n+1}{\mathrm{Si}}_{n}{\mathrm{Te}}_{4n+2}$ as a platform to manipulate 1D physics and offers an alternative perspective for studying electronic dynamics of non-Fermi liquids through STM experiments.

Sub- to super-Poissonian crossover of current noise in helical edge states coupled to a spin impurity in a magnetic field

Edge states of two-dimensional topological insulators are helical and single-particle backscattering is prohibited by time-reversal symmetry. In this paper, we show that an isotropic exchange coupling of helical edge states (HES) to a spin 1/2 impurity subjected to a magnetic field results in characteristic backscattering current noise (BCN) as a function of bias voltage and tilt angle between the direction of the magnetic field and the quantization axis of the HES. In particular, we find transitions from sub-Poissonian (antibunching) to super-Poissonian (bunching) behavior as a direct consequence of the helicity of the edge state electrons. We use the method of full counting statistics within a master equation approach treating the exchange coupling between the spin-1/2 impurity and the HES perturbatively. We express the BCN via coincidence correlation functions of scattering processes between the HES, which gives a precise interpretation of the Fano factor in terms of bunching and antibunching behavior of electron jump events. We also investigate the effect of electron-electron interactions in the HES in terms of the Tomonaga-Luttinger liquid theory.

Spin-charge separation in a one-dimensional Fermi gas with tunable interactions.

Ultracold atoms confined to periodic potentials have proven to be a powerful tool for quantum simulation of complex many-body systems. We confine fermions to one dimension to realize the Tomonaga-Luttinger liquid model, which describes the highly collective nature of their low-energy excitations. We use Bragg spectroscopy to directly excite either the spin or charge waves for various strengths of repulsive interaction. We observe that the velocity of the spin and charge excitations shift in opposite directions with increasing interaction, a hallmark of spin-charge separation. The excitation spectra are in quantitative agreement with the exact solution of the Yang-Gaudin model and the Tomonaga-Luttinger liquid theory. Furthermore, we identify effects of nonlinear corrections to this theory that arise from band curvature and back-scattering.

Imaging gate-tunable Tomonaga-Luttinger liquids in 1H-MoSe2 mirror twin boundaries.

One-dimensional electron systems exhibit fundamentally different properties than higher-dimensional systems. For example, electron-electron interactions in one-dimensional electron systems have been predicted to induce Tomonaga-Luttinger liquid behaviour. Naturally occurring grain boundaries in single-layer transition metal dichalcogenides exhibit one-dimensional conducting channels that have been proposed to host Tomonaga-Luttinger liquids, but charge density wave physics has also been suggested to explain their behaviour. Clear identification of the electronic ground state of this system has been hampered by an inability to electrostatically gate such boundaries and tune their charge carrier concentration. Here we present a scanning tunnelling microscopy and spectroscopy study of gate-tunable mirror twin boundaries in single-layer 1H-MoSe2 devices. Gating enables scanning tunnelling microscopy and spectroscopy for different mirror twin boundary electron densities, thus allowing precise characterization of electron-electron interaction effects. Visualization of the resulting mirror twin boundary electronic structure allows unambiguous identification of collective density wave excitations having two velocities, in quantitative agreement with the spin-charge separation predicted by finite-length Tomonaga-Luttinger liquid theory.

Unconventional quantum phase transitions in a one-dimensional Lieb-Schultz-Mattis system

We study quantum phases and phase transitions in a one-dimensional interacting fermion system with a Lieb-Schultz-Mattis (LSM) type anomaly. Specifically, the inversion symmetry enforces any symmetry-preserving gapped ground state of the system to be a Kitaev chain, following a Lieb-Schultz-Mattis type theorem that we prove. Alternatively, via the Jordan-Wigner transformation, this system describes a spin system whose gapped ground states must break either the inversion or the Ising symmetry associated with fermion parity. We obtain a phase diagram using analytical methods and variational matrix product state simulations, and study the critical behaviors of the quantum phase transitions therein using entanglement entropy, energy variance and finite size scaling of order parameters. In particular, we observe continuous phase transitions between different ordered phases that are beyond the Ginzburg-Landau-Wilson paradigm, in analogy to the deconfined quantum critical points in two spatial dimensions. We show this type of 1D deconfined quantum critical point is described by the Tomonaga-Luttinger liquid theory, and extract the Luttinger parameter and critical exponents. We also identify a gapless phase between two ordered phases, which cannot be described by a U(1) Luttinger liquid.

One-dimensional repulsive Hubbard model with mass imbalance: Orders and filling anomaly

We investigate the phase diagram of the one-dimensional repulsive Hubbard model with mass imbalance. Using DMRG, we show that this model has a "triplet" paired phase (dubbed $\pi \mathrm{SG}$) at generic fillings, consistent with previous theoretical analysis. We study the topological aspect of $\pi \mathrm{SG}$ phase, determining long-range string orders and the filling anomaly which refers to the relation among the single particle gap, inversion symmetry, and filling imbalance for open chains. We also find, using DMRG, that at $1/3$ filling, commensurate effects lead to two additional phases: a crystal phase and a trion phase; we construct a description of these phases using Tomonaga-Luttinger liquid theory.

Quench dynamics and relaxation of a spin coupled to interacting leads

We study a quantum quench in which a magnetic impurity is suddenly coupled to Hubbard chains, whose low-energy physics is described by Tomonaga-Luttinger liquid theory. Using the time-dependent density-matrix renormalization-group (tDMRG) technique, we analyze the propagation of charge, spin, and entanglement in the chains after the quench and relate the light-cone velocities to the dispersion of holons and spinons. We find that the local magnetization at the impurity site decays faster if we increase the interaction in the chains, even though the spin velocity decreases. We derive an analytical expression for the relaxation of the impurity magnetization which is in good agreement with the tDMRG results at intermediate timescales, providing valuable insight into the time evolution of the Kondo screening cloud in interacting systems.

Emergence and Disruption of Spin-Charge Separation in One-Dimensional Repulsive Fermions.

At low temperature, collective excitations of one-dimensional (1D) interacting fermions exhibit spin-charge separation, a unique feature predicted by the Tomonaga-Luttinger liquid (TLL) theory, but a rigorous understanding remains challenging. Using the thermodynamic Bethe ansatz (TBA) formalism, we analytically derive universal properties of a 1D repulsive spin-1/2 Fermi gas with arbitrary interaction strength. We show how spin-charge separation emerges from the exact TBA formalism, and how it is disrupted by the interplay between the two degrees of freedom that brings us beyond the TLL paradigm. Based on the exact low-lying excitation spectra, we further evaluate the spin and charge dynamical structure factors (DSFs). The peaks of the DSFs exhibit distinguishable propagating velocities of spin and charge as functions of interaction strength, which can be observed by Bragg spectroscopy with ultracold atoms.

Helicity modulus of the quasi-one-dimensional XY model: Protection by an energy barrier

The helicity modulus of the quasi-one-dimensional classical $\mathrm{XY}$ model is examined in connection with liquid He confined in nanopores. The helicity modulus ${\mathrm{\ensuremath{\Upsilon}}}_{\mathrm{p}}$ is suppressed with phase slippage, and its suppression is found to be well described with the scaling form obtained from the Tomonaga-Luttinger liquid theory in the one-dimensional limit. For phase slippage to occur, the system has to overcome an energy barrier, and the helicity modulus ${\mathrm{\ensuremath{\Upsilon}}}_{\mathrm{p}}$ suppressed by phase slippage is not necessarily observed in experiments. The energy barrier for phase slippage is explicitly calculated. Using the result, the helicity modulus ${\mathrm{\ensuremath{\Upsilon}}}_{\mathrm{s}}$ protected by the energy barrier is found to survive up to a higher temperature than ${\mathrm{\ensuremath{\Upsilon}}}_{\mathrm{p}}$. The relation of the present results to experiments on liquid He in nanopores is also discussed.

Measurement-induced quantum criticality under continuous monitoring

We investigate entanglement phase transitions from volume-law to area-law entanglement in a quantum many-body state under continuous position measurement on the basis of the quantum trajectory approach. We find the signatures of the transitions as peak structures in the mutual information as a function of measurement strength, as previously reported for random unitary circuits with projective measurements. At the transition points, the entanglement entropy scales logarithmically and various physical quantities scale algebraically, implying emergent conformal criticality, for both integrable and nonintegrable one-dimensional interacting Hamiltonians; however, such transitions have been argued to be absent in noninteracting regimes in some previous studies. With the aid of $U(1)$ symmetry in our model, the measurement-induced criticality exhibits a spectral signature resembling a Tomonaga-Luttinger liquid theory from symmetry-resolved entanglement. These intriguing critical phenomena are unique to steady-state regimes of the conditional dynamics at the single-trajectory level, and are absent in the unconditional dynamics obeying the Lindblad master equation, in which the system ends up with the featureless, infinite-temperature mixed state. We also propose a possible experimental setup to test the predicted entanglement transition based on the subsystem particle-number fluctuations. This quantity should readily be measured by the current techniques of quantum gas microscopy and is in practice easier to obtain than the entanglement entropy itself.

Friedel oscillations of one-dimensional correlated fermions from perturbation theory and density functional theory

We study the asymptotic decay of the Friedel density oscillations induced by an open boundary in a one-dimensional chain of lattice fermions with a short-range two-particle interaction. From Tomonaga-Luttinger liquid theory it is known that the decay follows a power law, with an interaction dependent exponent, which, for repulsive interactions, is larger than the noninteracting value $-1$. We first investigate if this behavior can be captured by many-body perturbation theory for either the Green function or the self-energy in lowest order in the two-particle interaction. The analytic results of the former show a logarithmic divergence indicative of the power law. One might hope that the resummation of higher order terms inherent to the Dyson equation then leads to a power law in the perturbation theory for the self-energy. However, the numerical results do not support this. Next we use density functional theory within the local-density approximation and an exchange-correlation functional derived from the exact Bethe ansatz solution of the translational invariant model. While the numerical results are consistent with power-law scaling if systems of $10^4$ or more lattice sites are considered, the extracted exponent is very close to the noninteracting value even for sizeable interactions.

Emergent mode and bound states in single-component one-dimensional lattice fermionic systems

We study the formation of bound states in a one-dimensional, single-component Fermi chain with attractive interactions. The phase diagram, computed from DMRG (density matrix renormalization group), shows not only a superfluid of paired fermions (pair phase) and a liquid of fermion triplets (trion phase), but also a phase with two gapless modes. We show that the latter phase is described by a 2-component Tomonaga-Luttinger liquid (TLL) theory, consisting of one charged and one neutral mode. We argue based on our numerical data, that the single, pair, and trion phases are descendants of the 2-component TLL theory. We speculate on the nature of the phase transitions amongst these phases.

Tomonaga-Luttinger Liquid Spin Dynamics in the Quasi-One-Dimensional Ising-Like Antiferromagnet BaCo_{2}V_{2}O_{8}.

Combining inelastic neutron scattering and numerical simulations, we study the quasi-one-dimensional Ising anisotropic quantum antiferromagnet BaCo_{2}V_{2}O_{8} in a longitudinal magnetic field. This material shows a quantum phase transition from a Néel ordered phase at zero field to a longitudinal incommensurate spin density wave at a critical magnetic field of 3.8T. Concomitantly, the excitation gap almost closes and a fundamental reconfiguration of the spin dynamics occurs. These experimental results are well described by the universal Tomonaga-Luttinger liquid theory developed for interacting spinless fermions in one dimension. We especially observe the rise of mainly longitudinal excitations, a hallmark of the unconventional low-field regime in Ising-like quantum antiferromagnetic chains.

Low-dimensional correlations under thermal fluctuations

We study the correlation functions of quantum spin $1/2$ ladders at finite temperature, under a magnetic field, in the gapless phase at various relevant temperatures $T\neq 0$, momentum $q$ and frequencies $\omega$. We compute those quantities using the time dependent density matrix renormalization group (T-DMRG) in some optimal numerical scheme. We compare these correlations with the ones of dimerized quantum spin chains and simple spin chains, that we compute by a similar technique. We analyze the intermediate energy modes and show that the effect of temperature lead to the formation of an essentially dispersive mode corresponding to the propagation of a triplet mode in an incoherent background, with a dispersion quite different from the one occurring at very low temperatures. We compare the low energy part of the spectrum with the predictions of the Tomonaga-Luttinger liquid field theory at finite temperature. We shows that the field theory describes in a remarkably robust way the low energy correlations for frequencies or temperatures up to the natural cutoff (the effective dispersion) of the system. We discuss how our results could be tested in e.g. neutron scattering experiments.

Tomonaga-Luttinger Liquid in a Box: Electrons Confined within MoS2 Mirror-Twin Boundaries

Scanning tunneling microscope observations reveal for the first time the discrete energy spectrum of a truly 1D conductor, providing a crucial tool for testing the limits of the Tomonaga-Luttinger liquid theory that describes interacting electrons.

Terahertz Spectroscopy of Individual Carbon Nanotube Quantum Dots.

We have investigated the electronic structures of metallic carbon nanotube quantum dots (CNT QDs) by terahertz-induced photocurrent spectroscopy. Sharp peaks due to intersublevel transitions in the CNT QDs are observed at the sublevel energy spacings expected from the linear band dispersion. The line width of the photocurrent peak is as narrow as 0.3 meV and is governed by the tunnel coupling with the electrodes, indicating that the scattering time of electrons in the present CNTs is comparable to or longer than 10 ps. The observation of a sharp absorption peak at the bare quantization energy was not consistent with the Tomonaga-Luttinger liquid theory.

Thermal and quantum lattice fluctuations in Peierls chains

The thermodynamic and spectral properties of electrons coupled to quantum phonons are studied within the spinless Holstein model. Using quantum Monte Carlo simulations, we obtain accurate results for the specific heat and the compressibility, covering the entire range of electron-phonon couplings and phonon frequencies. To this end, we derive an efficient estimator for the specific heat using the properties of the perturbation expansion. This allows us to quantitatively test the predictions of Tomonaga-Luttinger liquid theory as well as the widely used adiabatic approximation for low phonon frequencies. A comparison with the spectral functions of electrons and phonons reveals that the formation of polaron excitations as well as the renormalization of the phonon mode across the Peierls transition have a pronounced effect on the specific heat in the adiabatic regime.

Dynamical structure factors in the nematic phase of frustrated ferromagnetic spin chains

Frustrated spin systems can show phases with spontaneous breaking of spin-rotational symmetry without the formation of local magnetic order. We study the dynamic response of the spin-nematic phase of one-dimensional spin-1/2 systems, characterized by slow large-distance decay of quadrupolar correlations, by numerically computing one-spin and two-spin dynamical structure factors at zero temperature using time-dependent density matrix renormalization group methods. We interpret the results in terms of an effective theory of gapped magnon excitations interacting with a quasi-condensate of bound magnon pairs. This employs an extension of the well-known Tomonaga-Luttinger liquid theory which includes the magnon states as a mobile impurity. A good qualitative understanding of the characteristic thresholds and their intensity in the structure factors is obtained this way. Our results are useful in the interpretation of inelastic neutron scattering and resonant inelastic x-ray scattering experiments.