We report a performance comparison of Zr, Bi, Ti, and Ga as metal contacts on solution-grown CsPbBr <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> single-crystal gamma-ray detectors. The same CsPbBr <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> single crystal was repeatedly deposited with different metal contacts for the evaluation of gamma spectral performance to eliminate crystal-to-crystal variation. Leakage current as low as 2-3 nA at -200 V with detector thickness 2-3 mm was consistently achieved with Zr, Bi, Ti, and Ga as Schottky contact metal, which is comparable to the leakage current level of a commercial cadmium zinc telluride (CZT) detector. Gamma energy spectra with a prominent photopeak at 662 keV were consistently acquired with all studied metal contacts. The best resolution at 662 keV is 11% with a peak-to-Compton valley ratio of 2, indicating an improved spectrum shape than previous results. Through Americium-241 ( <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">241</sup> Am) alpha spectra acquisition, the hole mobility of the CsPbBr <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> single crystal is evaluated to be 1.78 cm <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">2</sup> V <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">-1</sup> s <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">-1</sup> . We also discussed issues related with the CsPbBr <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> gamma detector architecture and interface layers, commonly encountered during CsPbBr <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> gamma detector fabrication, that is, impact of electron/hole transport layer and surface oxide layer on gamma detector spectral performance, comparison of different metal-perovskite-metal structures. The persistent CsPbBr <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> gamma spectral performance marks the good reproducibility of CsPbBr <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> gamma detectors, further enabling CsPbBr <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> detector field applications.
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