Thermoelectric Generator Research Articles

Thermoelectric and electrical transport properties of mixed-conducting multicomponent oxides based on Ba(Zr,Ce)O3-δ

In this work, the chosen physicochemical properties of single-phase multicomponent oxides BaTi1/8Fe1/8Co1/8Y1/8Zr1/8Sn1/8Ce1/8Hf1/8O3-δ and BaTi1/9Fe1/9Co1/9Y1/9Zr1/9Sn1/9Ce1/9Hf1/9Bi1/9O3-δ were studied. The microstructure of the compounds strongly depended on the presence of bismuth in the structure. The electrical transport studies showed a level of electrical conductivity of ∼10-3 - 10-2 S/cm in the temperature range 673 – 1073 K. Electrical conductivity was thermally activated and the dominant conduction mechanism was the hopping of small polarons. Moreover, total electrical conductivity changes in the dry and humidified atmosphere at lower temperatures due to the presence of protonic defects in the structure. Thermoelectric measurements showed a relatively high value of the Seebeck coefficient for studied ceramics. Its values ranged between 50 and 250 μV/K depending on the sample and temperature. The Seebeck coefficient sign was positive, meaning that electron holes and/or oxygen vacancies were predominant charge carriers in oxidising atmospheres. Additionally, the Seebeck coefficient was found to be different in the humidified atmosphere which indicates an influence of protonic defects on thermoelectric transport. The obtained power factor Pf turned out to be low and dependent on the presence of protonic defects in the structure. This indicates, that the efficiency of the MOs-based operating thermoelectric generators can be controlled by changing the partial pressure of water vapor.

Preliminary study of the thermoelectric cooler and heat pipe application for the cooling system in cabin pickup car

Abstract Car cooling systems are essential equipment to make passengers comfortable, but their energy consumption is very high. Thermoelectric technology has been widely applied as a cooler in many applications, but its use as a car cooler has not been widely used. This research aims to conduct a preliminary study using thermoelectric coolers (TEC) as alternative coolers in pickup cars and to investigate the effect of thermoelectric module and heat exchanger configurations on cooling systems performance. A-TEC cooling system usually uses conventional heat sinks on the cold side and hot side of the TEC. In this study, heat pipes are used as heat exchangers on the hot side of TEC to improve its performance. The cooling system consists of 2 units installed at the rear of the pickup car cabin. Tests were varied using 2 TEC modules arranged in series and 4 TECs arranged in parallel thermal and electrical series. The results showed that using two cooling system units consisting of four TEC modules equipped with heat pipes was able to cool the temperature of the pickup car cabin at 27.4 °C and obtained the highest COP value of 1.16. It shows heat pipes can enhance TEC cooling system performance, producing lower cabin temperatures than conventional heat sinks.

Development of dynamic simulation model for 20 kWe micro heat pipe fission battery with dual power conversion system

Recent advancements in politics, technology, and economics have sparked interest in small-scale nuclear power generation. Heat-pipe micro-reactors, a type of small modular reactor (SMR), are ideal for remote and specialized applications like deep-sea and deep-space exploration. Traditionally, these reactors have used thermoelectric generators (TEGs) or Stirling engines for power conversion. However, TEGs suffer from low efficiency, and while Stirling engines have improved, they still have lower long-term stability compared to TEGs. Furthermore, comprehensive studies on system-level transients, dynamic behavior, and thermal responses are lacking. This study designs and models a dual power conversion system integrating TEGs and Free-Piston Stirling Generators (FPSGs) for micro heat pipe reactors to enhance efficiency, stability, and reliability. By integrating the two systems in parallel, the limitations of each technology are addressed, offering a robust solution for small, portable nuclear power generation. A dynamic simulation model incorporating the reactor core, heat pipes, and power conversion system enabled a comprehensive study of system transients and interactions. The core was modeled using thermal energy balance equations, and a thermal resistance approach was applied to the heat pipe. The TEG model included the Thomson and Seebeck effects, while neutronics feedback used a point kinetics model. The nonlinear analysis model was applied to simulate the FPSG. The system reached a stable operation after about 1000 s, generating 20kWe with 29.39% efficiency. It maintained stability without external control during transients within a specific range, demonstrating its feasibility. The TEG and FPSG exhibited independent yet complementary behaviors, ensuring reliable performance across scenarios.

Performance of thermoelectric generator system to generate electrical output from a low-grade waste heat temperature under linear and swirling waste heat streams

A thermoelectric generator (TEG) module converts heat directly into electrical energy. Waste heat from a process is a viable heat source for TEG modules to support the energy sustainability agenda. A module was designed to recover low-temperature waste heat from a 1 kW fuel cell stack used in a mini hydrogen vehicle. The module was constructed using a single TEG cell that receives heat directly on its surface from the waste heat stream, coupled with a heat pipe connected to a finned heat sink to effectively cool the cold junction of the TEG cell. This research presents a comparison of the module characteristics when it is operated under direct impinging jet flow and swirl flow waste heat streams at 60°C, while the cold junction of the cell is cooled under stationary vehicle conditions (natural convection cooling) and cruising conditions (forced convection cooling) at an air speed of 5 m/s. Results indicate that the swirling effect increases the maximum power point (MPP) by 60%. The introduction of swirl to the heating stream is a viable approach to significantly enhance the recovery of low-grade waste heat using TEG. However, the MPP shows a greater increase of 70 to 80% due to the forced cooling effect, indicating that cold junction cooling has a more significant influence on the MPP compared to the swirl effect.

Enhanced Thermoelectric Properties of Stable n-Type Ferrocene Derivatives-Doped Polyethylenimine/Single-Walled Carbon Nanotube Composite Films.

Preparing stable n-type flexible single-walled carbon nanotube (SWCNT)-based thermoelectric films with high thermoelectric (TE) performance is desirable for self-powering wearable electronics but remains a challenge. Here, the interface regulation and thermoelectric enhancement mechanism of ferrocene derivatives on polyethylenimine/single-walled carbon nanotube (PEI/SWCNT) composite films have been explored by doping ferrocene derivatives (f-Fc-OH) into PEI/SWCNT films. The results show that the introduction of f-Fc-OH leads to the formation of "thorn" structures on the surfaces of SWCNT bundles via hydrophilic and hydrophobic interactions, the generated energy-filtering effect improves the thermoelectric properties of the PEI/SWCNT film, and the f-Fc-OH-doped PEI/SWCNT (f-Fc-OH/PEI/SWCNT) achieves the highest room-temperature power factor of 182.22 ± 8.60 μW m-1 K-2 with a Seebeck coefficient of -64.28 ± 0.96 μV K-1 and the corresponding ZT value of 4.69 × 10-3. The Seebeck coefficient retention ratio of the f-Fc-OH/PEI/SWCNT nearly remained 68% after being exposed to air for 3672 h, while the PEI/SWCNT film changed from n-type to p-type after being exposed to air for about 432 h. In addition, the temperature-dependent thermoelectric properties show that the f-Fc-OH/PEI/SWCNT achieves a high power factor of 334.57 μW m-1 K-2 at 353 K. Finally, a flexible TE module consisting of seven pairs of p-n junctions is assembled using the optimum composite film, which produces an open-circuit voltage of 42 mV and a maximum output power of 4.32 μW at a temperature gradient of 60 K. Therefore, this work provides guidance for preparing stable n-type SWCNT-based composite films with enhanced thermoelectric properties, which have potential applications in flexible generators and wearable electronic devices.

Photothermal/magnetothermal coupled polyphenylene sulfide composite membranes for ultra-efficient and continuous seawater desalination

As the population continues to expand and industrialization gathers pace, the rate at which freshwater resources are dwindling is alarming. Solar desalination technology has shown encouraging results in generating clean water. However, solar-driven interfacial evaporation technology still faces a series of major challenges, specifically manifested in its low efficiency, poor chemical stability, and the tendency for salt crystallization to accumulate on the evaporation surface during operation. In this work, we proposed a novel magneto/photo-thermal coupled evaporator based on polyphenylene sulfide (PPS) fibrous membrane, which showed excellent high temperature and corrosion resistance. This non-contact responsive interfacial evaporator exhibited outstanding photothermal and magnetothermal conversion performance properties. Under one solar illumination, the evaporation rate of this evaporator could reach 1.52 kg m−2 h−1, corresponding to an evaporation efficiency of 91.84 %. In addition, under a magnetic field power of 2 kW m−2, the evaporator could achieve a remarkable evaporation rate of 4.2 kg m−2 h−1 under one solar illumination, with an evaporation efficiency of up to 93.77 %. Moreover, it also exhibited superb salt resistance, great mechanical properties, long-term operational stability, and outstanding dye purification property. Furthermore, by integrating the thermoelectric generator with the evaporator and utilizing the waste heat from the evaporation process to generate electricity, the efficiency of energy utilization has been improved. The interfacial evaporator opens up vast prospects for efficient and rapid clean water production, demonstrating significant potential and advantages.

Tailoring of Polypyrrole Wrapped Cotton Fiber Sponge for Simultaneous Solar Steam and Solar Thermoelectric Generation

AbstractSolar steam generation (SSG) using floatable evaporators to absorb solar energy and generate heat at the water–air interface has attracted increasing interest in achieving water purification and desalination. Using biodegradable and porous biomass materials as evaporators to fabricate high‐performance SSG devices is a promising route, but the poor efficiency and fussy and energy‐intensive manufacturing process for biomass material‐based evaporators will restrict their practical application. Here, an old commercial cotton quilt is used to prepare porous cotton fiber sponges (CFS) via a simple and scalable mechanical foaming strategy. After being decorated by the polypyrrole (PPy), the CFS@PPy sponge with a hierarchical porous structure shows broadband light absorption capacity, good hydrophilicity, and excellent photothermal capacity. The obtained sponge can be directly used as an evaporator floating on the seawater and shows a high steam‐generation efficiency of 85.07% under 1 sun irradiation. Additionally, it can be used as a photothermal material to construct a solar thermoelectric generation (STG) device and achieve an enhanced open‐circuit voltage (Vout) of 0.4 V and output current (Iout) of ≈59.6 mA under 5 sun irradiations. With the help of a boost converter, the power generation from the STG device can continuously charge the electric bulb and wristband.

On-Chip Thermoelectric Devices Based on Standard Silicon Processing.

The strong reduction of thermal conductivity with respect to bulk silicon makes nanostructured silicon one of the best materials for highly efficient direct conversion of heat into electrical power and vice-versa. The widespread technologies for the integration of silicon devices can be used to define on-chip micro thermoelectric generators (scavengers); similar structures could also be used for precise and well-localized cooling through the reverse process of heat pumping. However, the road to the fabrication of integrated thermal energy scavengers or cooler, based on silicon, is still very long. In this work, the design and the fabrication process of on-chip thermoelectric devices based on a large number of interconnected monocrystalline silicon nanobeams, very tall (>1 µm) and thin (less than 200 nanometers), arranged in large areas combs is shown. The small width of the nanobeams gives a reduced thermal conductivity, and the height perpendicular to the substrate allows the definition of a highly dense collection of nanostructures. The total cross-sectionis far broader than that of other nanostructures, a characteristic that guarantees both mechanical stability and larger deliverable power per unit area.

Potential for Electrical Energy Savings in AC Systems by Utilizing Exhaust Heat from Outdoor Unit

This study explores the potential of utilizing waste heat from air conditioning systems, one of the largest consumers of electrical energy. Currently, most of the waste heat generated by outdoor units is typically released into the environment without being utilized, leading to missed energy-saving opportunities. This study analyzes the potential for improving electrical energy efficiency in air conditioning (AC) systems by harnessing this waste heat. Two primary approaches are evaluated: the first is the use of waste heat for domestic water heating, and the second is the conversion of heat into electrical energy using thermoelectric generators (TEG). The results of this research indicate that both methods have the potential to improve overall energy efficiency significantly. However, challenges related to conversion efficiency and integration of these technologies with AC systems require further, more specific studies. These findings are expected to contribute to more efficient and environmentally friendly cooling systems by optimizing technology and overcoming barriers to wider implementation.

Effect of nanofluid cooling on electrical power of solar panel system in existence of TEG implementing magnetic force

This study investigates the efficacy of applying a Lorentz force to improve the efficiency of a photovoltaic-thermal (PVT) system featuring a finned duct, while also addressing challenges associated with dust accumulation. The magnetic field helps to prevent nanoparticle aggregation, enhancing the cooling process. The use of a finned duct combined with a nanofluid as the cooling medium efficiently dissipates excess heat from the silicon layer. Dust accumulation on the glass layer reduces transmissivity, negatively impacting system performance. The magnetic field's interaction with the nanoparticles enhances convective cooling of the upper layer, leading to an overall improvement in performance. Increased pumping power results in higher cooling rates, with improvements of approximately 3.48 % in thermal efficiency (ηth), 75.01 % in thermoelectric generator efficiency (ηTEG), and 39.37 % in photovoltaic efficiency (ηPV). An increase in the Hartmann number (Ha) improves ηth by about 1.87 %, with corresponding enhancements in electrical performance components. A higher concentration of ferrofluid further boosts performance, with the effect being roughly 1.7 times more significant in the absence of MHD compared to when Ha = 97. Dust presence decreases ηth, ηTEG, and ηPV by approximately 9.39 %, 8.55 %, and 25.77 %, respectively. Furthermore, the presence of Ha diminishes the influence of Vin on ηth by around 1.33 %.

A reconfigurable architecture for maximizing energy harvesting of thermoelectric generators in non-stationary conditions

The use of Thermoelectric Generators (TEGs) has proliferated across a multitude of applications for energy harvesting. As more modules are employed to recover greater amounts of energy, the temperature mismatch between them increases. This results in each module operating at a distinct maximum power point, thereby reducing the overall system efficiency. Furthermore, in dynamic applications such as automotive scenarios, the temperatures of the thermoelectric generators are not constant, and the maximum power point accordingly shifts. A fixed architecture is unable to cope with these fluctuating situations. Therefore, this paper introduces a reconfigurable architecture capable of harnessing maximum energy at any given moment, improving energy recovery compared to a fixed architecture. Optimization techniques, lean methodologies, and clustering approaches are employed to efficiently design the reconfigurable TEG, which enables modification of the electrical connections inside the TEG modules and the number of Maximum Power Point Tracking (MPPT) modules. A use case is presented where the reconfigurable TEG is compared with fixed, yet optimized, TEG configurations under mixed driving modes. In this specific case, the results demonstrate that the reconfigurable TEG achieves enhanced performance in dynamic environments with two MPPTs under mixed scenarios, reaching an efficiency of 96.3% and a 0.29% improvement in energy recovery.

Performance investigation of a thermoelectric generator for vehicle exhaust recovery using graded pore density foam metal

Improving the efficiency of thermoelectric generators (TEGs) used to harness residual heat from automobile exhausts is crucial for their widespread adoption. To enhance fluid heat transfer, the Kelvin tetrahedron model is employed for metal foam, and a multiphysical field model of the thermoelectric generator based on metal foam is established. The effects of inserting metal foam with uniform and gradient pore densities into the heat exchanger on the performance of the TEG are investigated. Experimental verification is conducted by constructing a test bench with dimensions identical to those of the model The findings suggest that inserting foam metal significantly enhances the output performance of the TEG, resulting in increases in both output power and efficiency as pore density rises. At Ta = 573 K and ma = 30 g/s, the output power of the TEG with inserted 20 PPI foam metal is enhanced by 140.46 %, while the efficiency experiences a remarkable increase of 197.50 % compared to a smooth pipe. Compared to the performance metrics of uniform foam metal, the positive gradient foam metal exhibits a maximum power increase of 7.89 % and a maximum efficiency increase of 34.46 %, along with an average pressure drop reduction of 27.29 %.

Advancement of germanium-based thermoelectric materials: a bibliometric and network analysis

Germanium (Ge)-based thermoelectric materials have proven to be a reliable and sustainable solution for efficient energy harvesting across a wide range of temperatures for an extended period. Numerous investigations have been published addressing the future scope of Ge as a thermoelectric material. This article offers a comprehensive bibliometric analysis of the literature related to Germanium-based thermoelectric energy harvesting (Ge-TEH) materials available on Scopus to identify how this material contributes to thermoelectric energy generation. Methodologies such as citation analysis, co-authorship, and co-occurrence analysis are employed to analyze refined data of ‘1867’ documents using 'Visualization of similarity' (VOS) viewer and Biblioshiny. The analysis shows that Ge-TEH has grown significantly worldwide, especially in the last decade. The social and intellectual networks were generated, and the most influencing countries, sources, and institutions were identified. China and the United States (USA) were found to have the highest number of publications, citations, and collaborations. The keywords analysis reveals that ‘lattice thermal conductivity,’ ‘Germanium,’ ‘Seebeck coefficient,’ ‘spark plasma sintering’, and ‘density functional theory’ are the most occurring words, indicating that the dataset features keywords related to thermoelectric materials and their properties. It also suggests a strong emphasis on fabrication methods for optimizing thermoelectric properties. The mutual relevance and categorical patterns of frequently occurring keywords were studied using a factorial analysis graph. This detailed analysis provides critical findings into the evolution and future scope of the research in Ge-TEH.

Impact of electric circuit configurations on power generation in a photovoltaic and thermoelectric generator hybrid system

Energy harvesting using a thermoelectric generator (TEG) leverages the Seebeck effect to generate electricity from temperature differences. As the demand for electrical energy rises, especially in zero-energy buildings and building conversions, there is an increasing focus on recovering untapped energy sources within buildings. This study aims to analyze the thermal characteristics of a hybrid energy harvester that integrates a TEG with phase change materials (PCM), with the objective of recovering and generating power from wasted sunlight and heat within a building envelope. Additionally, we experimentally investigated the circuit configuration of the TEG to optimize energy harvesting. The experimental results highlighted distinct power generation patterns depending on the TEG's location. To achieve maximum power output, TEGs exhibiting similar power generation patterns should be configured in series to ensure optimal performance. Implementing the maximum power circuit configuration resulted in a 70 % increase in power generation compared to a non-optimized configuration. Moreover, configuring an equal number of TEGs in series yielded a 94.4 % increase in power generation compared to a scenario where all TEGs were connected in series on a single panel.

Scalable Fabrication of Thermochromic Smart Windows for Broadening Temperature Ranges and Their Coupled Thermoelectric Power Generation

Scalable Fabrication of Thermochromic Smart Windows for Broadening Temperature Ranges and Their Coupled Thermoelectric Power Generation

Flexible Porous Ag2Se Films: From Freestanding Inorganic Films to Inorganic‐Network/Organic‐Skeleton Thermoelectric Generators

AbstractSilver selenide (Ag2Se) flexible films are promising near‐room‐temperature thermoelectric candidates for low‐grade heat harvesting. However, existing Ag2Se films are generally attached on substrates, which impedes further flexibility improvement of the films and constrains the scenarios of applications. Here a cost‐effective and scalable strategy is presented, which combines screen printing and annealing, for synthesizing freestanding Ag2Se inorganic films with different densities of pores. High‐density pores and thin thickness endow the films with high flexibility, while films with low‐density pores obtain higher power factor. Furthermore, by utilizing the porous microstructure, a composite structure consisting of a Ag2Se conductive network and an organic polydimethylsiloxane (PDMS) skeleton is fabricated, which further improves films’ stability under bending and torsion. Finally, a flexible thermoelectric generator comprising five Ag2Se/PDMS legs and encapsulated PDMS outputs a voltage of 20.2 mV and a maximum power of 810 nW (the corresponding power density is 5.4 W m−2) at a temperature difference of 30 K, verifying potential application at near room temperature. This work offers a useful paradigm for fabricating substrate‐free Ag2Se porous films with high flexibility for near‐room‐temperature thermoelectric applications.

A π−π stacked porous framework for highly efficient second near-infrared photothermal effects and photo-thermo-electric conversion

Near-infrared (NIR) photothermal compounds, which convert low-energy NIR photons into heat, have recently attracted significant attention due to their potential applications in many areas such as photothermal imaging, diagnosis and therapy, photosensors, and catalysis. Photothermal conversion efficiency (PCE), a critical parameter of NIR photothermal materials, significantly influences their practical performance. However, exploring highly efficient NIR photothermal compounds, particularly in the NIR-II domain, remains a significant challenge. Herein, we report on a highly efficient NIR-II photothermal compound based on a novel π−π stacked porous framework {[Ni4Cl2(ONDI)2(bpy)4]⋅2Cl⋅2H2O⋅xDMF⋅yH2O}n (1). This compound features a porous supramolecular framework constructed through intermolecular π−π interactions. Additionally, compound 1 exhibits broad optical absorption spanning from the ultraviolet to the NIR region, with an edge extending to 1600 nm. Under irradiation with a 1064 nm laser, compound 1 demonstrates significant NIR-II photothermal effects, achieving a remarkable PCE of 84.4 %, attributed to the formation of charge states and the abundant π−π interactions in its crystal structure. When integrated with commercial thermoelectric generators, compound 1 shows promising potential for photo-thermo-electric conversion, with a maximum open-circuit voltage of 250 mV and 350 mV under irradiation of 1 sun and 2 suns, respectively. Furthermore, the output power density of 1@TEC1-12701 reaches 0.53 W/m2 under 1 sun and 1.23 W/m2 under 2 suns.

Concentrated solar thermoelectric power generator equipped with a novel ultrathin wet porous membrane cooling technique; experimental study

One side of any thermoelectric power generator (TEG) is hot while the other side should always stay cold. The higher the temperature difference, the greater the power generation. This paper offers a particular ultrathin wet porous membrane (UWPM) as a new cooling method for a solar thermoelectric power generator. According to the graphical abstract, the membrane has a capillary-wicking feature on one side, making it possible to be soaked spontaneously and create a steady thin water film on the ceramic layer of the thermoelectric, thereby serving as an energy-free, enthalpy of vaporization-based cooling method (surface vaporization). Interestingly, water is replenished spontaneously as long as the water exists in the tank. The suggested mechanism is tested under two weather conditions: one hot, dry day (ambient air around 40 °C) and one moderate day (ambient air around 30 °C), with different air speeds between 1.5 and 4.5 m/s to simulate different wind speeds in real applications. Power, cold side surface temperature, maximum conversion efficiency, etc., are measured, evaluated, discussed, and compared with the common fin-pin heatsink/fan thermal management tool. Notably, the implementation of the UWPM demonstrates a substantial enhancement in thermoelectric generator performance. It is noted that the lowest temperature that can be obtained through vaporization can be colder than ambient air temperature, approaching the wet-bulb temperature. The UWPM keeps the cold side temperature up to 10 degrees colder than that achieved in the heatsink method. This is why the generated power by the TEG is around 2.5 times higher when utilizing the UWPM. Furthermore, unlike the fin-pin heatsink (FPH) thermal management tool, warmer weather conditions do not diminish the cooling quality of the UWPM method. Indeed, the cold side temperature on a hot, dry day is almost the same as that on a moderate day using the UWPM technique. This is because hot ambient temperature induces greater and easier vaporization, leading to a higher cooling effect.

Organic thermoelectric device utilizing charge transfer interface as the charge generation by harvesting thermal energy

We propose an organic thermoelectric device having a new power generation mechanism that extracts small-scale thermal energy, i.e., a few tens of millielectronvolts, at room temperature without a temperature gradient. We demonstrate a new operating mechanism based on an organic thermoelectric power generation architecture that uses the charge separation capabilities of organic charge transfer (CT) interfaces composed of copper (II) phthalocyanine and copper (II) 1,2,3,4,8,9,10,11,15,16,17,18,22,23,24,25-hexadecafluoro-29H,31H-phthalocyanine as the donor and acceptor, respectively. With the optimized device architecture, values of open-circuit voltage VOC of 384 mV, short-circuit current density JSC of 1.1 μA/cm2, and maximum output Pmax of 94 nW/cm2 are obtained. The temperature characteristics of the thermoelectric properties yield activation energy values of approximately 20–60 meV, confirming the low-level thermal energy’s contribution to the power generation mechanism. Furthermore, from surface potential analysis using a Kelvin probe, we confirm that charges are generated at the CT interface, and the electrons and holes are diffused to the counter-electrodes with the aid of Fermi-level alignment between adjacent layers.

Flexible Ag2Se/Ag2S nanocomposite on carbon fabric optimized via interfaced engineered energy filtering effect for a textile based wearable thermoelectric generator

Wearable devices have become increasingly attractive in wearable electronics due to their advantages of environmental friendliness and foldability. The state-of-the-art thermoelectric system depends on inorganic semiconductors that show high electron mobility but lack mechanical stability and thermoelectric performance. Here, We have proposed a solvothermal method to grow Ag2Se/Ag2S nanocomposite on carbon fabric with outstanding properties, demonstrating excellent flexibility. The crystallographic analysis was performed for all samples through XRD and confirmed the orthorhombic Ag2Se and mono-clinic Ag2S. Further, the morphological analysis revealed the enhanced growth on the carbon fabric. We investigated the thermoelectric properties of Ag2Se/Ag2S nanocomposite and achieved a high power factor of 8.1 μW/mK2 which is twice as high as the percentage of the pure Ag2Se. Additionally, thermoelectric legs were fabricated using Ag2Se/Ag2S nanocomposite in a 2-pair module. They produced an output voltage of 0.1 mV to 7.4 mV at a temperature gradient (ΔT) of 3–8 K. This work is a promising approach for obtaining high-performance wearable thermoelectric device.