Terahertz Quantum Cascade Lasers Research Articles

Early detection of gastric cancer via high-resolution terahertz imaging system.

Terahertz (THz) wave has demonstrated a good prospect in recent years, but the resolution is still one of the problems that restrict the application of THz technology in medical imaging. Paraffin-embedded samples are mostly used in THz medical imaging studies, which are thicker and significantly different from the current gold standard slice pathological examination in sample preparation. In addition, THz absorption in different layers of normal and cancerous tissues also remains to be further explored. In this study, we constructed a high-resolution THz imaging system to scan non-tumorous adjacent tissue slices and gastric cancer (GC) tissue slices. In this system, a THz quantum cascade laser emitted a pulsed 3THz signal and the transmitted THz wave was received by a THz detector implemented in a 65nm CMOS process. The slice thickness was only 20μm, which was close to that of the medical pathology examination. We successfully found THz transmittance differences between different layers of normal gastric tissues based on THz images, and the resolution could reach 60μm for the first time. The results indicated that submucosa had a lower THz transmittance than that of mucosa and muscular layer in non-tumorous adjacent tissue. However, in GC tissue, THz transmittance of mucosa and submucosa was similar, caused by the decreased transmittance of mucosa, where the cancer occurs. Therefore, we suppose that the similar terahertz transmittance between gastric mucosa and submucosa may indicate the appearance of cancerization. The images obtained from our THz imaging system were clearer than those observed with naked eyes, and can be directly compared with microscopic images. This is the first application of THz imaging technology to identify non-tumorous adjacent tissue and GC tissue based on the difference in THz wave absorption between different layers in the tissue. Our present work not only demonstrated the potential of THz imaging to promote early diagnosis of GC, but also suggested a new direction for the identification of normal and cancerous tissues by analyzing differences in THz transmittance between different layers of tissue.

Continuous-wave terahertz quantum cascade laser based on a hybrid bound to bound quantum design

We report a low threshold power density and high power output terahertz quantum cascade laser emitting at ∼3.9 THz operating in continuous-wave mode. The high output power and wall-plug efficiency are achieved based on a hybrid bound-to-bound quantum active design. A record output power of 312 mW and a low threshold power density of 0.8 kW/mm3 (threshold current density of 109 A/cm2) in continuous-wave mode at 20 K is demonstrated for a 300-μm-wide and 2-mm-long single-ridge device. The highest wall-plug efficiency is 1.38% and the slope efficiency is 684 mW/A with an internal quantum efficiency of ∼120 photons per injected electron. The demonstration of this low-threshold and high-power THz laser will promote THz-based remote sensing and standoff detection for pharmaceutical and health industry applications.

Tuning of the Spectral Characteristics of Terahertz Quantum-Cascade Lasers

Terahertz quantum-cascade lasers (THz QCLs) are promising radiation sources for high-resolution gas spectroscopy. A wide operating-frequency band (from 1.2 to 5.4 THz), a narrow generation line (up to 10 kHz), the ability to operate on several radiative transitions (two-color lasers, generation of frequency combs) and other unique characteristics of THz QCLs make it possible to create gas spectrometers of a new generation for biomedical and environmental applications. In this paper, we consider the possibility of controlling the spectral characteristics of THz QCLs by changing the operating temperature and injection-current pulse parameters: amplitude, duration, and repetition rate. The energy transfer between longitudinal Fabry–Perot modes in THz QCLs is studied for the first time with a change in the duty cycle of the injection-current pulse cycle.

Multimode dynamics of terahertz quantum cascade lasers: Spontaneous and actively induced generation of dense and harmonic coherent regimes

We present an extended study concerning the dynamics of dense and harmonic coherent regimes in quantum cascade lasers (QCLs) in a Fabry--Perot (FP) configuration emitting in the terahertz (THz) spectral region. Firstly, we study the device in free running operation, reproducing the main features of the self-generated of optical frequency combs (OFCs) and harmonic frequency combs (HFCs) in this spectral range, commenting on the points of difference from the mid-infrared region, and finding excellent agreement with the most recent experimental evidences. Then, we analyze the THz-QCL dynamics under radiofrequency (RF) injection, with a focus on the effect of the modulation of the current on the degree of locking of the system, and we perform a systematic investigation aimed to provide a procedure for the generation of train of pulses with short duration and high contrast. Furthermore, we extend our study to the generation of sequences of pulses with repetition frequency which is a multiple of the free-spectral range (FSR) of the laser cavity, reproducing harmonic mode-locking (HML) of the laser, a method which has been recently demontrated in experiments with THz-QCLs, and the results of which are particulary promising for a large stream of applications, ranging from optical communication to imaging.

Self-Pulsations in Terahertz Quantum Cascade Lasers under Strong Optical Feedback: The Effect of Multiple Reflections in the External Cavity.

We have recently reported the self-pulsation phenomenon under strong optical feedback in terahertz (THz) quantum cascade lasers (QCLs). One important issue, however, we left open: the effect of multiple round trips in the external cavity on the laser response to feedback. Our current analysis also casts additional light on the phenomenon of self-pulsations. Using only one external cavity round trip (ECRT) in the model has been the common approach following the seminal paper by Lang-Kobayashi in 1980. However, the conditions under which the Lang-Kobayashi model, in its original single-ECRT formulation, is applicable has been rarely explored. In this work, we investigate the self-pulsation phenomenon under multiple ECRTs. We found that the self-pulsation waveform changes when considering more than one ECRT. This we attribute to the combined effect of the extended external cavity length and the frequency modulation of the pulsation frequency by the optical feedback. Our findings add to the understanding of the optical feedback dynamics under multiple ECRTs and provide a pathway for selecting the appropriate numerical model to study the optical feedback dynamics in THz QCLs and semiconductor lasers in general.

Continuous-wave single-mode quantum cascade laser at 5.1 THz based on graded sampled grating design

We report on the terahertz (THz) quantum cascade lasers in continuous-wave (CW) operation with an emitting frequency above 5 THz. Excellent performance with a smaller leakage current and higher population inversion efficiency is obtained by one-well bridged bound-to-continuum hybrid quantum design at 5 THz. By designing and fabricating a graded metallic sampled distributed feedback grating in the waveguide, the first single-mode THz quantum cascade laser at 5.13 THz in CW operation mode is achieved. The maximum single-mode optical power of ∼ 48 mW is achieved at 15 K with a side-mode suppression ratio above 24 dB. This will draw great interest in the spectroscopy applications above the 5 THz range for THz quantum cascade lasers.

Directed delivery of terahertz frequency radiation from quantum cascade lasers within a dry 3He dilution refrigerator.

We present a scheme for the full integration of terahertz (THz) frequency quantum cascade lasers (QCLs) within a dilution refrigerator in order to provide a directed delivery of THz power into the sample space. We describe a successful operation of a 2.68THz QCL located on the pulse tube cooler stage of the refrigerator, with its output coupled onto a two-dimensional electron gas (2DEG) located on a milli-kelvin sample stage via hollow metal waveguides and Hysol thermal isolators, achieving a total loss from QCL to the sample of ∼-9 dB. The thermal isolators limit heat leaks to the sample space, with a base temperature of ∼210 mK being achieved. We observe cyclotron resonance (CR) induced in the 2DEG by the QCL and explore the heating impact of the QCL on all stages of the refrigerator. The CR effect induced by the THz QCL is observable at electron temperatures as low as ∼430 mK. The results show a viable route for the exploitation of THz QCLs within the environment of a dilution refrigerator and for the THz power delivery in very low-temperature (<0.5K) condensed matter experiments.

Increasing the output power of a heavily doped terahertz quantum cascade laser by avoiding the subband misalignment

A significant enhancement in the output power of a GaAs-based terahertz quantum cascade laser (THz QCL) was achieved by implementing a relatively high impurity doping concentration. The QC structure was precisely designed using the nonequilibrium green function method by considering the band bending effect caused by a higher doping concentration. This enabled us to avoid the subband misalignment induced by the strong band bending effect, to provide efficient carrier transport even at high doping concentrations, and to improve the output power. The maximum output power of a GaAs/Al0.16Ga0.84As 3.5 THz-band QCL at 10 K was enhanced from 390 to 600 mW by increasing the doping concentration at the depopulation layers from 6 × 1016 to 1.2 × 1017 cm−3. The average power of 21 mW was achieved by implementing the appropriate pulse drive conditions.

Analysis of High-Performing Terahertz Quantum Cascade Lasers

Detailed simulations for Terahertz quantum cascade lasers based on two-well designs are presented. We reproduce the maximal operation temperatures observed and attribute the degradation with temperature to the occupation of parasitic levels and thermal backfilling. Furthermore, we demonstrate that the current injection can be conveniently studied by using EZ states, which combine energy selectivity and spatial localisation. Improving the injection allows to achieve higher maximal operation temperatures around 265 Kelvin.

Nonrelevant quantum levels effecting on the current in 2-well terahertz quantum cascade lasers

Recent renewed operating temperatures in terahertz quantum cascade lasers emphasize on narrowing the periodic length in a 2-well resonant-phonon design for a clean quantum level structure, in which the depopulation energy is significantly higher than one longitudinal phonon. In this study, various depopulation energies (small and large) are engineered in a 2-well design; the effect of the high-lying nonrelevant levels on the currents are systematically studied by using the non-equilibrium Green’s function method. The engineering of the depopulation energy is unable to avoid the formation of leakage channels, which are activated within at least three neighboring periods via sequential close tunneling. However, a large depopulation energy relaxes the thermal backfilling process; as a result, the net leakages at high temperatures can be significantly suppressed. In addition, pre-alignment remains a critical issue in the design when using a large depopulation energy, which requires improved engineering for the barriers to obtain better laser dynamics.

New Designs of Laser Transitions in Terahertz Quantum–Cascade Lasers

New Designs of Laser Transitions in Terahertz Quantum–Cascade Lasers

Phase-locked terahertz quantum cascade laser array integrated with a Talbot cavity.

Increasing the power of a quantum cascade laser by widening laser ridges will lead to the degradation of the beam quality because of the operation of high-order transverse modes. We report on a phase-locked array scheme of terahertz quantum cascade laser (THz QCL) utilizing Talbot effect. By adjusting the absorbing boundary width of each ridge in the array, stable operation of the fundamental supermode is realized. A five-element array shows 4 times power amplification than that of a single ridge device. Due to the large power amplification efficiency, stable mode selection, and simple fabricating process, the phase-locked array scheme is very promising to further improve the performance of THz QCL.

Terahertz quantum cascade laser frequency combs with optical feedback.

Optical feedback exists in most laser configurations and strongly affects laser performances depending on the feedback strength, length, and phase. In this paper, we investigate the frequency comb behaviour of a semiconductor quantum cascade laser emitting around 4.2 THz with external optical feedback. A periodic evolution of the laser inter-mode beatnote from single-line to multiple-line structures is experimentally observed with a minor change of optical feedback length (phase) on the wavelength scale. The comb stability of the laser with feedback is also measured and compared with the same laser without feedback. Furthermore, our simulations reveal that the dynamical oscillations invoked by optical feedback are responsible for the measured multiple-line beatnotes. It is found that the characteristic feedback period is determined by the half wavelength of the laser, while the comb operation is maintained at most feedback length positions. Therefore, terahertz quantum cascade laser combs are robust against the minor position vibration of the feedback mirror in practice, owing to the much smaller feedback phase change than that of common near-infrared laser diodes.

Nonrelevant quantum levels limited laser dynamic in narrow-period terahertz quantum cascade lasers

The fundamental challenges faced by terahertz quantum cascade lasers are the operations below room temperature, and the recent improved operating temperatures are actually based on the narrow-period designs (2-well resonant-phonon scheme). In this study, we address the critical effect of nonrelevant high-confined quantum levels on the laser threshold current in such designs, i.e. at high temperatures, the resonant-tunneling channels passing through neighboring periods via those levels can dominantly increase the laser threshold current. As a result, the laser dynamics significantly shrink to zero even at 270 K. The channels cannot be easily eliminated as they are derived from the specific configuration of a two-quantum-well periodic structure, in which the width of the period is narrow, and the nonrelevant levels from the lower-well are confined down in energy. It is reasonable to suppress the current flowing across those levels by narrowing the lower-well further, but an appropriate balance of its thickness is essential.

All in One‐Chip, Electrolyte‐Gated Graphene Amplitude Modulator, Saturable Absorber Mirror and Metrological Frequency‐Tuner in the 2–5 THz Range

AbstractLayered 2D materials display unique optical and electrical properties that can enable manipulation, propagation, and detection of electromagnetic waves over a broad spectral range, with a high level of control, offering the potential to activate different functionalities, by optical or electrical means, in a single chip. Here, a compact optoelectronic device behaving as an amplitude modulator, saturable absorber mirror (SA mirror), and frequency‐tuner is conceived at terahertz (THz) frequencies. It comprises a gate‐tunable single layer graphene (SLG), embedded in a quarter‐wave cavity, operating in the 1–5 THz range. The use of electrolyte ionic liquid gate ensures 40% optical amplitude modulation depth. Z‐scan self‐mixing interferometry reveals 60% reflectivity modulation, with ≈4.5 W cm−2 saturation intensity. By integrating the modulator/SA mirror with a heterogeneous THz quantum cascade laser frequency comb, in an external cavity configuration, fine‐tuning of the intermode beatnote frequency is also demonstrated. This opens intriguing perspectives for short pulse generation, phase‐locking, frequency tuning/chirping, phase modulation, and metrological referencing, inter alia.

Resonant two-photon terahertz quantum cascade laser.

Lasers that can emit two photons from a single electron relaxation between two states of the same parity have been discussed since the early days of the laser era. However, such lasers have seen only limited success, mainly due to a lack of suitable gain medium. We propose that terahertz (THz) frequency quantum cascade lasers (QCLs) are an ideal semiconductor structure to realize such two-photon emissions. In this work, we present a THz QCL heterostructure designed to emit two resonant photons from each electronic relaxation between two same-parity states in the active region. We present coupled Maxwell-Bloch equations that describe the dynamics of such a two-photon laser and find analytical solutions for the steady-state light intensity, the steady-state energy-resolved carrier densities, and the total threshold carrier density. Due to the two-photon emission from each excited state relaxation and an increased photon-driven carrier transport rate, our simulations predict a significant enhancement of light intensity in our designed resonant two-photon THz QCL when compared to an exemplar conventional THz QCL structure.

Long-term stability of GaAs/AlAs terahertz quantum-cascade lasers

We have investigated high-performance GaAs/AlAs terahertz (THz) quantum-cascade lasers (QCLs) with respect to the long-term stability of their operating parameters. The output power of lasers that contain an additional, thick AlAs refractive-index contrast layer underneath the cascade structure decreases after three months by about 35%. The deterioration of these lasers is attributed to the oxidation processes in this contrast layer starting from the facets. However, GaAs/AlAs THz QCLs with an Al0.9Ga0.1As refractive-index contrast layer exhibit long-term stability of the operating parameters over many years even when they are exposed to atmospheric conditions. Therefore, these lasers are promising high-power radiation sources in the terahertz spectral region for commercial applications.

Extraction-Dominated Temperature Degradation of Population Inversion in Terahertz Quantum Cascade Lasers.

Degraded population inversion (PI) at elevated temperature, regarded as an important temperature degradation factor in terahertz quantum cascade lasers (THz QCL), has hindered the widespread use of these devices. Herein, the mechanism of the temperature degradation of PI is investigated microscopically. It is demonstrated that the limited extraction efficiency of the extraction system dominates the decrease of PI at elevated temperatures. To be specific, the increased temperature brings about intense thermally activated longitudinal optical phonon scattering, leading to large amounts of electrons scattering to lower level state. In this case, the resonant-phonon extraction system is incapable of depleting all the electrons from lower level states. So even though the resonant-tunneling injection seems efficient enough to compensate the electron runoff at the upper state, the electron density at lower level state increases and the overall PI turns out lower. In addition, it is found that strong electron-ionized donor separation at high temperature can induce level misalignment, which can stagger the optimal conditions of injection and extraction. Also, the extraction efficiency gets lower as the extraction system requires accurate coupling between several energy levels.

A Study on the Photoelectric Properties of Dual Ridge Terahertz Quantum Cascade Lasers at 3.1 THz.

High-power, incoherent THz array sources are widely desired in some applications due to their low energy, unique terahertz fingerprint, and image. In this work, a dual ridge terahertz quantum cascade laser lasing at 3.1 THz is presented, and the device’s performance is analyzed in detail. The maximum output power can reach 512 mW when the two ridges work simultaneously in continuous-wave mode, with a threshold current density of 281 A/cm2 at 15 K. While the peak power is approximately 704 mW in pulse-wave mode at 15 K, the lasing still could be observed approximately 7 mW at 125 K. The far-field pattern of the dual ridge THz QCL is detected by a THz camera; two light spots typically show a single-lobe Gaussian distribution. The experimental results provide a reference for realizing high-power THz quantum cascade lasers, and they will provide some guidance for the structural design of multiple ridges or laser arrays.

Broadband Terahertz Quantum Cascade Laser Dual‐Comb Sources under Off‐Resonant Microwave Injection

Broadband dual‐comb spectroscopy has attracted increasing interests due to its unique advantages in high spectral resolution, fast detection, and so on. Although the dual‐comb technique is relatively mature in the infrared wavelengths, it is, currently, not commercially capable of practical applications in the terahertz regime due to the lack of high‐performance broadband terahertz dual‐comb sources. In the terahertz frequency range, the electrically pumped quantum cascade laser (QCL) is a suitable candidate for the dual‐comb operation. Although the resonant microwave injection locking is widely used to broaden the emission spectra of terahertz QCLs, it is challenging to be employed to obtain broadband dual‐comb sources that can fully exploit the laser gain bandwidth due to the large phase noise induced by the resonant injection and nonideal microwave circuits. Herein, an off‐resonant microwave injection to significantly broaden the dual‐comb bandwidth of a terahertz QCL dual‐comb source is used. The measured optical dual‐comb bandwidth is broadened from 147 GHz in free running to 450 GHz under the off‐resonant injection. By performing a numerical analysis based on a rate equation model, the broadband dual‐comb operation under the off‐resonant microwave injection can result from a wider lasing bandwidth and a higher degree of phase matching.