Terahertz Quantum Cascade Lasers Research Articles

Monolithic top emitting room temperature THz DFG QCL with index grating for wavelength selection

We present a high performance top emitting room temperature monolithic terahertz (THz) quantum cascade laser based on difference frequency generation (DFG) and a buried modulated distributed feedback grating. Using a semi-insulating InP:Fe substrate combined with an index-coupled grating could minimize the internal losses for the THz mode. The laser consists of two separate transversely superimposed gratings. The first grating provides selective feedback for the mid-infrared pump modes and is realized in an index-coupled DFG grating designed for single-mode operation for two distinct MIR wavelengths. The second metallic grating for THz extraction is carefully aligned to the spatial distribution of the MIR modes. The resulting device lases pulses up to 150 °C in the single mode. The maximum THz output power at RT is 100 μW measured at 3.37 THz. A THz wavelength tuning of around 0.065 nm/K was achieved through thermal tuning of the MIR pump lasers.

Terahertz Quantum-Cascade Lasers: From Design to Applications

Terahertz Quantum-Cascade Lasers: From Design to Applications

High brightness terahertz quantum cascade laser with near-diffraction-limited Gaussian beam

High-power terahertz (THz) quantum cascade laser, as an emerging THz solid-state radiation source, is attracting attention for numerous applications including medicine, sensing, and communication. However, due to the sub-wavelength confinement of the waveguide structure, direct beam brightness upscaling with device area remains elusive due to several mode competition and external optical lens is normally used to enhance the THz beam brightness. Here, we propose a metallic THz photonic crystal resonator with a phase-engineered design for single mode surface emission over a broad area. The quantum cascade surface-emitting laser is capable of delivering an output peak power over 185 mW with a narrow beam divergence of 4.4° × 4.4° at 3.88 THz. A high beam brightness of 1.6 × 107 W sr−1m−2 with near-diffraction-limited M2 factors of 1.4 in both vertical and lateral directions is achieved from a large device area of 1.6 × 1.6 mm2 without using any optical lenses. The adjustable phase shift between the lattices enables a stable and high-intensity surface emission over a broad device area, which makes it an ideal light extractor for large-scale THz emitters. Our research paves the way to high brightness solid-state THz lasers and facilitates new applications in standoff THz imaging, detection, and diagnosis.

Exploring the effects of molecular beam epitaxy growth characteristics on the temperature performance of state-of-the-art terahertz quantum cascade lasers

This study conducts a comparative analysis, using non-equilibrium Green’s functions (NEGF), of two state-of-the-art two-well (TW) Terahertz Quantum Cascade Lasers (THz QCLs) supporting clean 3-level systems. The devices have nearly identical parameters and the NEGF calculations with an abrupt-interface roughness height of 0.12 nm predict a maximum operating temperature (Tmax) of ~ 250 K for both devices. However, experimentally, one device reaches a Tmax of ~ 250 K and the other a Tmax of only ~ 134 K. Both devices were fabricated and measured under identical conditions in the same laboratory, with high quality processes as verified by reference devices. The main difference between the two devices is that they were grown in different MBE reactors. Our NEGF-based analysis considered all parameters related to MBE growth, including the maximum estimated variation in aluminum content, growth rate, doping density, background doping, and abrupt-interface roughness height. From our NEGF calculations it is evident that the sole parameter to which a drastic drop in Tmax could be attributed is the abrupt-interface roughness height. We can also learn from the simulations that both devices exhibit high-quality interfaces, with one having an abrupt-interface roughness height of approximately an atomic layer and the other approximately a monolayer. However, these small differences in interface sharpness are the cause of the large performance discrepancy. This underscores the sensitivity of device performance to interface roughness and emphasizes its strategic role in achieving higher operating temperatures for THz QCLs. We suggest Atom Probe Tomography (APT) as a path to analyze and measure the (graded)-interfaces roughness (IFR) parameters for THz QCLs, and subsequently as a design tool for higher performance THz QCLs, as was done for mid-IR QCLs. Our study not only addresses challenges faced by other groups in reproducing the record Tmax of ~ 250 K and ~ 261 K but also proposes a systematic pathway for further improving the temperature performance of THz QCLs beyond the state-of-the-art.

Design of photonic topological corner states for electrically pumped terahertz quantum cascade laser

Photonic topological corner states (PTCS) represent discrete zero modes whose frequencies stay in the topological bandgap and wavefunctions exhibit strong spatial localization, which is highly desirable for efficient surface-emitting lasers. While being extensively investigated in optically pumped lasers, the electrically pumped PTCS lasers are merely reported due to the lack of suitable configurations. In this paper, we propose a photonic cavity design based on the PTCSs that can be applied for electrically pumped terahertz quantum cascade lasers (QCLs). The cavity is constructed by following the canonical trivial-nontrivial domain, where the nontrivial domain with expanded and merged four QCL rods is surrounded by the trivial domain with shrunk and merged four QCL rods. Both domains follow the 2D Su–Schrieffer–Heeger (SSH) model. To further construct a fabrication-favorable 3D device, the designed QCL rod array is connected by 2D veins, which functionalize simultaneously as the intermedium for enhanced inter-/intra-cell coupling and the conductive connection to the device. The 3D numerical calculation is finally investigated.

Phase-locked single-mode terahertz quantum cascade lasers array

We demonstrated a scheme of phase-locked terahertz quantum cascade lasers (THz QCLs) array, with a single-mode pulse power of 108 mW at 13 K. The device utilizes a Talbot cavity to achieve phase locking among five ridge lasers with first-order buried distributed feedback (DFB) grating, resulting in nearly five times amplification of the single-mode power. Due to the optimum length of Talbot cavity depends on wavelength, the combination of Talbot cavity with the DFB grating leads to better power amplification than the combination with multimode Fabry−Perot (F−P) cavities. The Talbot cavity facet reflects light back to the ridge array direction and achieves self-imaging in the array, enabling phase-locked operation of ridges. We set the spacing between adjacent elements to be 220 μm, much larger than the free-space wavelength, ensuring the operation of the fundamental supermode throughout the laser's dynamic range and obtaining a high-brightness far-field distribution. This scheme provides a new approach for enhancing the single-mode power of THz QCLs.

Performance of a High-Speed Pyroelectric Receiver as Cryogen-Free Detector for Terahertz Absorption Spectroscopy Measurements

The application of terahertz (THz) radiation in scientific research as well as in applied and commercial technology has expanded rapidly in recent years. One example is the progress in high-resolution THz spectroscopy based on quantum cascade lasers, which has enabled new observations in astronomy, atmospheric research, and plasma diagnostics. However, the lack of easy-to-use and miniaturised detectors has hampered the development of compact THz spectroscopy systems out of the laboratory environment. In this paper, we introduce a new high-speed pyroelectric receiver as a cryogen-free detector for THz absorption spectroscopy. Its performance is characterised by absorption spectroscopy measurements on a reference gas cell (RGC) with ammonia using a tunable THz quantum cascade laser at approximately 4.75 THz as the light source. It is shown that the receiver can record spectra up to 281 Hz without any artefacts to the observed spectral absorption profile, and the results reproduce the known pressure of ammonia in the RGC. This demonstrates that the pyroelectric receiver can be reliably used as an alternative to helium-cooled bolometers for absorption spectroscopy measurements in the THz range, with its main advantages being the high bandwidth, compactness, relatively low cost, and room-temperature operation. Its simplicity and high sensitivity make this receiver a key component for compact THz spectroscopy systems.

Influence of adhesion layers on optical losses in THz quantum cascade lasers

For a GaAs/AlGaAs terahertz (THz) quantum cascade laser (QCL) with a double metal waveguide (DMWG) based on Au and Cu metal plates and Ti and Ta adhesion layers, the dumping parameters and THz mode loss spectra were calculated. It has been shown that to minimize losses in high-temperature DMWG QCL designs, it is advisable to use Ti less than 5 nm thick or Ta less than 10 nm thick as adhesion layers for Au. The use of the proposed waveguide with a thickness of 20 µm will lead to the creation of a room temperature THz QCL.

High continuous-wave power surface emitting terahertz lasers integrated with multimode interferometer

Distributed feedback (DFB) surface emitting semiconductor laser realizes power extraction by periodic photonic heterostructure. A direct method to increase the output power is scaling up the area of active region, however, the length of the device is restricted by the coupling strength of the DFB grating. Herein we develop a high-power single-mode surface emitting scheme by monolithically integrating second-order DFB terahertz quantum cascade laser and a multimode interferometer, which can significantly enhance the optical power by increasing photon density and altering field distribution in the grating region. Application of this concept leads to high continuous-wave (CW) surface emitting power of 55 mW, with single-lobed far-field pattern and single-mode operation at about 3.9 THz, which is among the best reported results. Such an integrated scheme can be combined with any one-dimensional photonic heterostructure, which has great potential in further improving the pulsed and CW output power of single-mode semiconductor lasers.

Growth of InGaSb/AlInGaSb quantum cascade laser structures on GaSb substrates by molecular beam epitaxy

An InGaSb/AlInGaSb terahertz quantum cascade laser (THz-QCL) structure was grown by molecular beam epitaxy (MBE) on a GaSb substrate with introducing an InGaSb composition graded buffer layer. It was found that the occurrence of inverted pyramid-shaped defects with a size of several micrometers is related to oxygen. The lattice matching condition between InGaSb and AlInGaSb was investigated. We grew a 3 μm-thick In0.19Ga0.81Sb/Al0.19In0.16Ga0.65Sb THz-QCL active region with a threading dislocation density of ∼ 1 × 107 cm−2. The threading dislocation density remained nearly unchanged after a several-micrometer-thick QCL region. The density of defects of several micrometers in size was ∼ 6 × 103 cm−2.

Combined resonant tunneling and rate equation modeling of terahertz quantum cascade lasers

Terahertz (THz) quantum cascade lasers (QCLs) are technologically important laser sources for the THz range but are complex to model. An efficient extended rate equation model is developed here by incorporating the resonant tunneling mechanism from the density matrix formalism, which permits to simulate THz QCLs with thick carrier injection barriers within the semi-classical formalism. A self-consistent solution is obtained by iteratively solving the Schrödinger–Poisson equation with this transport model. Carrier–light coupling is also included to simulate the current behavior arising from stimulated emission. As a quasi-ab initio model, intermediate parameters, such as pure dephasing time and optical linewidth, are dynamically calculated in the convergence process, and the only fitting parameters are the interface roughness correlation length and height. Good agreement has been achieved by comparing the simulation results of various designs with experiments, and other models such as density matrix Monte Carlo and non-equilibrium Green's function method that, unlike here, require important computational resources. The accuracy, compatibility, and computational efficiency of our model enable many application scenarios, such as design optimization and quantitative insights into THz QCLs. Finally, the source code of the model is also provided in the supplementary material of this article for readers to repeat the results presented here, investigate, and optimize new designs.

Sculpting harmonic comb states in terahertz quantum cascade lasers by controlled engineering

Optical frequency combs (OFCs), which establish a rigid phase-coherent link between the microwave and optical domains of the electromagnetic spectrum, are emerging as key high-precision tools for the development of quantum technology platforms. These include potential applications for communication, computation, information, sensing, and metrology and can extend from the near-infrared with micro-resonator combs, up to the technologically attractive terahertz (THz) frequency range, with powerful and miniaturized quantum cascade laser (QCL) FCs. The recently discovered ability of the QCLs to produce a harmonic frequency comb (HFC)—a FC with large intermodal spacings—has attracted new interest in these devices for both applications and fundamental physics, particularly for the generation of THz tones of high spectral purity for high data rate wireless communication networks, for radio frequency arbitrary waveform synthesis, and for the development of quantum key distributions. The controlled generation of harmonic states of a specific order remains, however, elusive in THz QCLs. Here, and by design, we devise a strategy to obtain broadband HFC emission of a pre-defined order in a QCL. By patterning n regularly spaced defects on the top surface of a double-metal Fabry–Perot QCL, we demonstrate harmonic comb emission with modes spaced by an (n+1) free spectral range and with an optical power/mode of ∼270µW.

Analyzing the effect of doping concentration in split-well resonant-phonon terahertz quantum cascade lasers.

The effect of doping concentration on the temperature performance of the novel split-well resonant-phonon (SWRP) terahertz quantum-cascade laser (THz QCL) scheme supporting a clean 4-level system design was analyzed using non-equilibrium Green's functions (NEGF) calculations. Experimental research showed that increasing the doping concentration in these designs led to better results compared to the split-well direct-phonon (SWDP) design, which has a larger overlap between its active laser states and the doping profile. However, further improvement in the temperature performance was expected, which led us to assume there was an increased gain and line broadening when increasing the doping concentration despite the reduced overlap between the doped region and the active laser states. Through simulations based on NEGF calculations we were able to study the contribution of the different scattering mechanisms on the performance of these devices. We concluded that the main mechanism affecting the lasers' temperature performance is electron-electron (e-e) scattering, which largely contributes to gain and line broadening. Interestingly, this scattering mechanism is independent of the doping location, making efforts to reduce overlap between the doped region and the active laser states less effective. Optimization of the e-e scattering thus could be reached only by fine tuning of the doping density in the devices. By uncovering the subtle relationship between doping density and e-e scattering strength, our study not only provides a comprehensive understanding of the underlying physics but also offers a strategic pathway for overcoming current limitations. This work is significant not only for its implications on specific devices but also for its potential to drive advancements in the entire THz QCL field, demonstrating the crucial role of e-e scattering in limiting temperature performance and providing essential knowledge for pushing THz QCLs to new temperature heights.

Terahertz in vivo imaging of human skin: Toward detection of abnormal skin pathologies.

Terahertz (THz) imaging has long held promise for skin cancer detection but has been hampered by the lack of practical technological implementation. In this article, we introduce a technique for discriminating several skin pathologies using a coherent THz confocal system based on a THz quantum cascade laser. High resolution in vivo THz images (with diffraction limited to the order of 100 μm) of several different lesion types were acquired and compared against one another using the amplitude and phase values. Our system successfully separated pathologies using a combination of phase and amplitude information and their respective surface textures. The large scan field (50 × 40 mm) of the system allows macroscopic visualization of several skin lesions in a single frame. Utilizing THz imaging for dermatological assessment of skin lesions offers substantial additional diagnostic value for clinicians. THz images contain information complementary to the information contained in the conventional digital images.

THz quantum well photodetector based on LO-phonon scattering-assisted extraction

We present a design for a quantum photodetector operating in the terahertz range, at 3.45 THz (15 meV, 87 μm). Our device relies on biased GaAs/AlGaAs heterostructure, designed to exploit LO phonon scattering as an extraction mechanism. In our design, the external potential due to the applied bias forms an extraction miniband and allows accommodating an LO phonon transition (36 meV) and use it as an extraction mechanism, even though its energy exceeds the detector's absorbing transition at 15 meV. Spectral-resolved measurements performed on arrays of patch antenna microcavities reveal a peak photocurrent at the designed photon energy with a responsivity of 80 mA/W at 20 K. The maximum operating temperature of the photodetector is found to be 40 K. Detector characterizations were performed both with a black-body source as well as with a terahertz quantum cascade laser emitting at 3.5 THz.

Theoretical model of passive mode-locking in terahertz quantum cascade lasers with distributed saturable absorbers

Abstract In research and engineering, short laser pulses are fundamental for metrology and communication. The generation of pulses by passive mode-locking is especially desirable due to the compact setup dimensions, without the need for active modulation requiring dedicated external circuitry. However, well-established models do not cover regular self-pulsing in gain media that recover faster than the cavity round trip time. For quantum cascade lasers (QCLs), this marked a significant limitation in their operation, as they exhibit picosecond gain dynamics associated with intersubband transitions. We present a model that gives detailed insights into the pulse dynamics of the first passively mode-locked QCL that was recently demonstrated. The presence of an incoherent saturable absorber, exemplarily realized by multilayer graphene distributed along the cavity, drives the laser into a pulsed state by exhibiting a similarly fast recovery time as the gain medium. This previously unstudied state of laser operation reveals a remarkable response of the gain medium on unevenly distributed intracavity intensity. We show that in presence of strong spatial hole burning in the laser gain medium, the pulse stabilizes itself by suppressing counter-propagating light and getting shortened again at the cavity facets. Finally, we study the robustness of passive mode-locking with respect to the saturable absorber properties and identify strategies for generating even shorter pulses. The obtained results may also have implications for other nanostructured mode-locked laser sources, for example, based on quantum dots.

Terahertz quantum cascade laser frequency combs with engineered operation frequency around 4.0 THz

Freely engineering the operation frequency of frequency comb sources is crucial for various applications, e.g., high-precision spectroscopy, ranging, communications, and so on. Here, by employing band structure simulations, group velocity dispersion (GVD) analysis, and experimental verifications, we demonstrate that the operation frequency of terahertz (THz) quantum cascade laser frequency combs can be engineered from 4.2 to 4.0 THz. First of all, from the viewpoint of the band structure engineering, we shift the frequency corresponding to the optical transitions in the active region from 4.2 to 4.0 THz by slightly altering the thicknesses of quantum wells. Meanwhile, a GVD analysis is applied to evaluate the potential comb performance. Finally, experimental characterizations, e.g., emission spectra, inter-mode beatnote, dual-comb operation, are performed to validate the exceptional comb operation at 4.0 THz. The advancement in simulations and experimental results present a comprehensive method to customize the desired THz radiative frequency for comb generation, which facilitates the practical development of broadband, high-precision THz comb sources.

Continuous-wave GaAs/AlGaAs quantum cascade laser at 5.7 THz.

Design strategies for improving terahertz (THz) quantum cascade lasers (QCLs) in the 5-6 THz range are investigated numerically and experimentally, with the goal of overcoming the degradation in performance that occurs as the laser frequency approaches the Reststrahlen band. Two designs aimed at 5.4 THz were selected: one optimized for lower power dissipation and one optimized for better temperature performance. The active regions exhibited broadband gain, with the strongest modes lasing in the 5.3-5.6 THz range, but with other various modes observed ranging from 4.76 to 6.03 THz. Pulsed and continuous-wave (cw) operation is observed up to temperatures of 117 K and 68 K, respectively. In cw mode, the ridge laser has modes up to 5.71 THz - the highest reported frequency for a THz QCL in cw mode. The waveguide loss associated with the doped contact layers and metallization is identified as a critical limitation to performance above 5 THz.

Extraction of the electron excess temperature in terahertz quantum cascade lasers from laser characteristics

Abstract We propose a method to extract the upper laser level’s (ULL’s) excess electronic temperature from the analysis of the maximum light output power (P max) and current dynamic range ΔJ d = (J max − J th) of terahertz quantum cascade lasers (THz QCLs). We validated this method, both through simulation and experiment, by applying it on THz QCLs supporting a clean three-level system. Detailed knowledge of electronic excess temperatures is of utmost importance in order to achieve high temperature performance of THz QCLs. Our method is simple and can be easily implemented, meaning an extraction of the excess electron temperature can be achieved without intensive experimental effort. This knowledge should pave the way toward improvement of the temperature performance of THz QCLs beyond the state-of-the-art.

Stabilized Terahertz Quantum Cascade Laser Dual-Comb Sources with a Hybrid Locking

Stabilized Terahertz Quantum Cascade Laser Dual-Comb Sources with a Hybrid Locking