Terahertz Quantum Cascade Lasers Research Articles

Performance of a High-Speed Pyroelectric Receiver as Cryogen-Free Detector for Terahertz Absorption Spectroscopy Measurements

The application of terahertz (THz) radiation in scientific research as well as in applied and commercial technology has expanded rapidly in recent years. One example is the progress in high-resolution THz spectroscopy based on quantum cascade lasers, which has enabled new observations in astronomy, atmospheric research, and plasma diagnostics. However, the lack of easy-to-use and miniaturised detectors has hampered the development of compact THz spectroscopy systems out of the laboratory environment. In this paper, we introduce a new high-speed pyroelectric receiver as a cryogen-free detector for THz absorption spectroscopy. Its performance is characterised by absorption spectroscopy measurements on a reference gas cell (RGC) with ammonia using a tunable THz quantum cascade laser at approximately 4.75 THz as the light source. It is shown that the receiver can record spectra up to 281 Hz without any artefacts to the observed spectral absorption profile, and the results reproduce the known pressure of ammonia in the RGC. This demonstrates that the pyroelectric receiver can be reliably used as an alternative to helium-cooled bolometers for absorption spectroscopy measurements in the THz range, with its main advantages being the high bandwidth, compactness, relatively low cost, and room-temperature operation. Its simplicity and high sensitivity make this receiver a key component for compact THz spectroscopy systems.

Influence of adhesion layers on optical losses in THz quantum cascade lasers

For a GaAs/AlGaAs terahertz (THz) quantum cascade laser (QCL) with a double metal waveguide (DMWG) based on Au and Cu metal plates and Ti and Ta adhesion layers, the dumping parameters and THz mode loss spectra were calculated. It has been shown that to minimize losses in high-temperature DMWG QCL designs, it is advisable to use Ti less than 5 nm thick or Ta less than 10 nm thick as adhesion layers for Au. The use of the proposed waveguide with a thickness of 20 µm will lead to the creation of a room temperature THz QCL.

High continuous-wave power surface emitting terahertz lasers integrated with multimode interferometer

Distributed feedback (DFB) surface emitting semiconductor laser realizes power extraction by periodic photonic heterostructure. A direct method to increase the output power is scaling up the area of active region, however, the length of the device is restricted by the coupling strength of the DFB grating. Herein we develop a high-power single-mode surface emitting scheme by monolithically integrating second-order DFB terahertz quantum cascade laser and a multimode interferometer, which can significantly enhance the optical power by increasing photon density and altering field distribution in the grating region. Application of this concept leads to high continuous-wave (CW) surface emitting power of 55 mW, with single-lobed far-field pattern and single-mode operation at about 3.9 THz, which is among the best reported results. Such an integrated scheme can be combined with any one-dimensional photonic heterostructure, which has great potential in further improving the pulsed and CW output power of single-mode semiconductor lasers.

Growth of InGaSb/AlInGaSb quantum cascade laser structures on GaSb substrates by molecular beam epitaxy

An InGaSb/AlInGaSb terahertz quantum cascade laser (THz-QCL) structure was grown by molecular beam epitaxy (MBE) on a GaSb substrate with introducing an InGaSb composition graded buffer layer. It was found that the occurrence of inverted pyramid-shaped defects with a size of several micrometers is related to oxygen. The lattice matching condition between InGaSb and AlInGaSb was investigated. We grew a 3 μm-thick In0.19Ga0.81Sb/Al0.19In0.16Ga0.65Sb THz-QCL active region with a threading dislocation density of ∼ 1 × 107 cm−2. The threading dislocation density remained nearly unchanged after a several-micrometer-thick QCL region. The density of defects of several micrometers in size was ∼ 6 × 103 cm−2.

Combined resonant tunneling and rate equation modeling of terahertz quantum cascade lasers

Terahertz (THz) quantum cascade lasers (QCLs) are technologically important laser sources for the THz range but are complex to model. An efficient extended rate equation model is developed here by incorporating the resonant tunneling mechanism from the density matrix formalism, which permits to simulate THz QCLs with thick carrier injection barriers within the semi-classical formalism. A self-consistent solution is obtained by iteratively solving the Schrödinger–Poisson equation with this transport model. Carrier–light coupling is also included to simulate the current behavior arising from stimulated emission. As a quasi-ab initio model, intermediate parameters, such as pure dephasing time and optical linewidth, are dynamically calculated in the convergence process, and the only fitting parameters are the interface roughness correlation length and height. Good agreement has been achieved by comparing the simulation results of various designs with experiments, and other models such as density matrix Monte Carlo and non-equilibrium Green's function method that, unlike here, require important computational resources. The accuracy, compatibility, and computational efficiency of our model enable many application scenarios, such as design optimization and quantitative insights into THz QCLs. Finally, the source code of the model is also provided in the supplementary material of this article for readers to repeat the results presented here, investigate, and optimize new designs.

Sculpting harmonic comb states in terahertz quantum cascade lasers by controlled engineering

Optical frequency combs (OFCs), which establish a rigid phase-coherent link between the microwave and optical domains of the electromagnetic spectrum, are emerging as key high-precision tools for the development of quantum technology platforms. These include potential applications for communication, computation, information, sensing, and metrology and can extend from the near-infrared with micro-resonator combs, up to the technologically attractive terahertz (THz) frequency range, with powerful and miniaturized quantum cascade laser (QCL) FCs. The recently discovered ability of the QCLs to produce a harmonic frequency comb (HFC)—a FC with large intermodal spacings—has attracted new interest in these devices for both applications and fundamental physics, particularly for the generation of THz tones of high spectral purity for high data rate wireless communication networks, for radio frequency arbitrary waveform synthesis, and for the development of quantum key distributions. The controlled generation of harmonic states of a specific order remains, however, elusive in THz QCLs. Here, and by design, we devise a strategy to obtain broadband HFC emission of a pre-defined order in a QCL. By patterning n regularly spaced defects on the top surface of a double-metal Fabry–Perot QCL, we demonstrate harmonic comb emission with modes spaced by an (n+1) free spectral range and with an optical power/mode of ∼270µW.

Analyzing the effect of doping concentration in split-well resonant-phonon terahertz quantum cascade lasers.

The effect of doping concentration on the temperature performance of the novel split-well resonant-phonon (SWRP) terahertz quantum-cascade laser (THz QCL) scheme supporting a clean 4-level system design was analyzed using non-equilibrium Green's functions (NEGF) calculations. Experimental research showed that increasing the doping concentration in these designs led to better results compared to the split-well direct-phonon (SWDP) design, which has a larger overlap between its active laser states and the doping profile. However, further improvement in the temperature performance was expected, which led us to assume there was an increased gain and line broadening when increasing the doping concentration despite the reduced overlap between the doped region and the active laser states. Through simulations based on NEGF calculations we were able to study the contribution of the different scattering mechanisms on the performance of these devices. We concluded that the main mechanism affecting the lasers' temperature performance is electron-electron (e-e) scattering, which largely contributes to gain and line broadening. Interestingly, this scattering mechanism is independent of the doping location, making efforts to reduce overlap between the doped region and the active laser states less effective. Optimization of the e-e scattering thus could be reached only by fine tuning of the doping density in the devices. By uncovering the subtle relationship between doping density and e-e scattering strength, our study not only provides a comprehensive understanding of the underlying physics but also offers a strategic pathway for overcoming current limitations. This work is significant not only for its implications on specific devices but also for its potential to drive advancements in the entire THz QCL field, demonstrating the crucial role of e-e scattering in limiting temperature performance and providing essential knowledge for pushing THz QCLs to new temperature heights.

Terahertz in vivo imaging of human skin: Toward detection of abnormal skin pathologies.

Terahertz (THz) imaging has long held promise for skin cancer detection but has been hampered by the lack of practical technological implementation. In this article, we introduce a technique for discriminating several skin pathologies using a coherent THz confocal system based on a THz quantum cascade laser. High resolution in vivo THz images (with diffraction limited to the order of 100 μm) of several different lesion types were acquired and compared against one another using the amplitude and phase values. Our system successfully separated pathologies using a combination of phase and amplitude information and their respective surface textures. The large scan field (50 × 40 mm) of the system allows macroscopic visualization of several skin lesions in a single frame. Utilizing THz imaging for dermatological assessment of skin lesions offers substantial additional diagnostic value for clinicians. THz images contain information complementary to the information contained in the conventional digital images.

THz quantum well photodetector based on LO-phonon scattering-assisted extraction

We present a design for a quantum photodetector operating in the terahertz range, at 3.45 THz (15 meV, 87 μm). Our device relies on biased GaAs/AlGaAs heterostructure, designed to exploit LO phonon scattering as an extraction mechanism. In our design, the external potential due to the applied bias forms an extraction miniband and allows accommodating an LO phonon transition (36 meV) and use it as an extraction mechanism, even though its energy exceeds the detector's absorbing transition at 15 meV. Spectral-resolved measurements performed on arrays of patch antenna microcavities reveal a peak photocurrent at the designed photon energy with a responsivity of 80 mA/W at 20 K. The maximum operating temperature of the photodetector is found to be 40 K. Detector characterizations were performed both with a black-body source as well as with a terahertz quantum cascade laser emitting at 3.5 THz.

Theoretical model of passive mode-locking in terahertz quantum cascade lasers with distributed saturable absorbers

Abstract In research and engineering, short laser pulses are fundamental for metrology and communication. The generation of pulses by passive mode-locking is especially desirable due to the compact setup dimensions, without the need for active modulation requiring dedicated external circuitry. However, well-established models do not cover regular self-pulsing in gain media that recover faster than the cavity round trip time. For quantum cascade lasers (QCLs), this marked a significant limitation in their operation, as they exhibit picosecond gain dynamics associated with intersubband transitions. We present a model that gives detailed insights into the pulse dynamics of the first passively mode-locked QCL that was recently demonstrated. The presence of an incoherent saturable absorber, exemplarily realized by multilayer graphene distributed along the cavity, drives the laser into a pulsed state by exhibiting a similarly fast recovery time as the gain medium. This previously unstudied state of laser operation reveals a remarkable response of the gain medium on unevenly distributed intracavity intensity. We show that in presence of strong spatial hole burning in the laser gain medium, the pulse stabilizes itself by suppressing counter-propagating light and getting shortened again at the cavity facets. Finally, we study the robustness of passive mode-locking with respect to the saturable absorber properties and identify strategies for generating even shorter pulses. The obtained results may also have implications for other nanostructured mode-locked laser sources, for example, based on quantum dots.

Terahertz quantum cascade laser frequency combs with engineered operation frequency around 4.0 THz

Freely engineering the operation frequency of frequency comb sources is crucial for various applications, e.g., high-precision spectroscopy, ranging, communications, and so on. Here, by employing band structure simulations, group velocity dispersion (GVD) analysis, and experimental verifications, we demonstrate that the operation frequency of terahertz (THz) quantum cascade laser frequency combs can be engineered from 4.2 to 4.0 THz. First of all, from the viewpoint of the band structure engineering, we shift the frequency corresponding to the optical transitions in the active region from 4.2 to 4.0 THz by slightly altering the thicknesses of quantum wells. Meanwhile, a GVD analysis is applied to evaluate the potential comb performance. Finally, experimental characterizations, e.g., emission spectra, inter-mode beatnote, dual-comb operation, are performed to validate the exceptional comb operation at 4.0 THz. The advancement in simulations and experimental results present a comprehensive method to customize the desired THz radiative frequency for comb generation, which facilitates the practical development of broadband, high-precision THz comb sources.

Continuous-wave GaAs/AlGaAs quantum cascade laser at 5.7 THz.

Design strategies for improving terahertz (THz) quantum cascade lasers (QCLs) in the 5-6 THz range are investigated numerically and experimentally, with the goal of overcoming the degradation in performance that occurs as the laser frequency approaches the Reststrahlen band. Two designs aimed at 5.4 THz were selected: one optimized for lower power dissipation and one optimized for better temperature performance. The active regions exhibited broadband gain, with the strongest modes lasing in the 5.3-5.6 THz range, but with other various modes observed ranging from 4.76 to 6.03 THz. Pulsed and continuous-wave (cw) operation is observed up to temperatures of 117 K and 68 K, respectively. In cw mode, the ridge laser has modes up to 5.71 THz - the highest reported frequency for a THz QCL in cw mode. The waveguide loss associated with the doped contact layers and metallization is identified as a critical limitation to performance above 5 THz.

Extraction of the electron excess temperature in terahertz quantum cascade lasers from laser characteristics

Abstract We propose a method to extract the upper laser level’s (ULL’s) excess electronic temperature from the analysis of the maximum light output power (P max) and current dynamic range ΔJ d = (J max − J th) of terahertz quantum cascade lasers (THz QCLs). We validated this method, both through simulation and experiment, by applying it on THz QCLs supporting a clean three-level system. Detailed knowledge of electronic excess temperatures is of utmost importance in order to achieve high temperature performance of THz QCLs. Our method is simple and can be easily implemented, meaning an extraction of the excess electron temperature can be achieved without intensive experimental effort. This knowledge should pave the way toward improvement of the temperature performance of THz QCLs beyond the state-of-the-art.

Stabilized Terahertz Quantum Cascade Laser Dual-Comb Sources with a Hybrid Locking

Stabilized Terahertz Quantum Cascade Laser Dual-Comb Sources with a Hybrid Locking

Frequency combs in optically injected terahertz ring quantum cascade lasers

Quantum cascade lasers (QCLs) have emerged as promising candidates for generating chip-scale frequency combs in mid-infrared and terahertz wavelengths. In this work, we demonstrate frequency comb formation in ring terahertz QCLs using the injection of light from a distributed feedback (DFB) laser. The DFB design frequency is chosen to match the modes of the ring cavity (near 3.3 THz), and light from the DFB is injected into the ring QCL via a bus waveguide. By controlling the power and frequency of the optical injection, we show that combs can be selectively formed and controlled in the ring cavity. Numerical modeling suggests that this comb is primarily frequency-modulated in character, with the injection serving to trigger comb formation. We also show that the ring can be used as a filter to control the output of the DFB QCL, potentially being of interest in terahertz photonic integrated circuits. Our work demonstrates that waveguide couplers are a compelling approach for injecting and extracting radiation from ring terahertz combs and offer exciting possibilities for the generation of new comb states in terahertz, such as frequency-modulated waves, solitons, and more.

Frequency combs induced by optical feedback and harmonic order tunability in quantum cascade lasers

This study investigates the interaction between frequency combs and optical feedback effects in Quantum Cascade Lasers (QCLs). The theoretical analysis reveals new phenomena arising from the interplay between comb generation and feedback. By considering the bias current corresponding to free-running single mode emission, the introduction of optical feedback can trigger the generation of frequency combs, including both fundamental and harmonic combs. This presents opportunities to extend the comb region and generate harmonic frequency combs with different orders through optimization of external cavity parameters, such as losses and length. Furthermore, this study demonstrates that optical feedback can selectively tune the harmonic order of a pre-existing free-running comb by adjusting the external cavity length, particularly for feedback ratios around 1%, which are readily achievable in experimental setups. Under strong feedback conditions (Acket parameter C > 4.6), mixed states emerge, displaying the features of both laser and external cavity dynamics. While this study is predominantly centered on terahertz QCLs, we have also confirmed that the described phenomena occur when utilizing mid-infrared QCL parameters. This work establishes a connection between comb technology and the utilization of optical feedback, providing new avenues for exploration and advancement in the field. In fact, the novel reported phenomena open a pathway toward new methodologies across various domains, such as the design of tunable comb sources, hyperspectral imaging, multi-mode coherent sensing, and multi-channel communication.

Frequency‐Modulated Combs via Field‐Enhancing Tapered Waveguides

AbstractFrequency‐modulated (FM) combs feature flat intensity spectra with a linear frequency chirp, useful for metrology and sensing applications. Generating FM combs in semiconductor lasers generally requires a fast saturable gain, usually limited by the intrinsic gain medium properties. Here, it is shown how a spatial modulation of the laser gain medium can enhance the gain saturation dynamics and nonlinearities to generate self‐starting FM combs. This is demonstrated with tapered planarized terahertz (THz) quantum cascade lasers (QCLs). While simple ridge THz QCLs typically generate combs presenting a mixture of amplitude and frequency modulation, the on‐chip field enhancement resulting from extreme spatial confinement leads to an ultrafast saturable gain regime, generating a pure FM comb with a flatter intensity spectrum and a clear linear frequency chirp. The observed linear frequency chirp is reproduced using a spatially inhomogeneous mean‐field theory model, which confirms the crucial role of field enhancement. In addition, the modified spatial temperature distribution within the waveguide results in an improved high‐temperature comb operation, up to a heat sink temperature of 115 K, with comb bandwidths of 600 GHz at 90 K. The spatial inhomogeneity leads as well to very intense radio frequency (RF) beatnotes up to ‐30 dBm and facilitates dynamic switching between various harmonic states in the same device.

Enhanced Delivery and Detection of Terahertz Frequency Radiation from a Quantum Cascade Laser Within Dilution Refrigerator

We report on significant enhancements to the integration of terahertz (THz) quantum cascade lasers (QCL) and THz detection with a two-dimensional electron gas (2DEG) within a dilution refrigerator obtained by the inclusion of a multi-mesh 6 THz low-pass filter to block IR radiation, a Winston cone to focus light output, and gating the 2DEG for optimised sensitivity. We show that these improvements allow us to obtain a > 2.5 times reduced sample electron temperature (160 mK compared with 430 mK previously), during cyclotron resonance (CR) measurements of a 2DEG under QCL illumination. This opens up a route to performing sub-100 mK experiments using excitation by THz QCLs.

Dynamic performance of terahertz quantum cascade laser with double optical feedbacks: Role of the external cavity

The dynamic performance of a terahertz (THz) quantum cascade laser (QCL) with double optical feedbacks (DOFs) is carefully studied within the framework of single-mode rate equations. The results have shown that the system displays three types of nonlinear dynamic phenomena under the control of different feedback strengths, which are envelope oscillations, spiking oscillations, and high-frequency small-amplitude oscillations, respectively. The fundamental frequency of oscillation is related to the ratio of the round-trip times from two external cavities and the ratio of their feedback strengths. By solving the steady-state equations, we find that the high-frequency, small-amplitude oscillations arise because a pair of modes appear at almost the same point. The output performance of THz QCL system is also studied with square wave signal modulation. The results show that the fundamental frequency of oscillation at the output is only related to the frequency of the square wave signal. And low frequency fluctuations (LFFs) dynamics can be excited by combination of DOFs and adjusting the duty cycle of the square wave signal. This work provides a novel insight into high data-bit THz communication based on QCLs.

Wireless Signal Transmission at the 2 and 3 THz-Band Enabled by Photonics-Based Transmitter and Hot Electron Bolometer Mixer

We have demonstrated terahertz (THz) wireless transmission of quadrature phase-shift keying (QPSK) signals at 2 and 3 THz-bands. Despite higher atmospheric attenuation at frequencies above 1 THz, it might be applicable for short-range wireless communications. The proposed system is composed of a photonics-based transmitter using an optical comb source and a heterodyne receiver system using a hot electron bolometer mixer (HEBM). In the transmitter, THz signals are generated by photomixing of optical carriers extracted from broadband optical combs. The receiver system consists of a quasi-optical HEBM and a phase-locked THz quantum cascade laser (THz-QCL) as a local oscillator (LO). Although the emission power of the photonics-based transmitter was on the order of tens of nW, it could be received with sufficient SNRs due to high sensitivity of the HEBM. Demonstrations of signal transmission were carried out with 2 and 3 THz-band. Optical carriers were modulated with basic LTE FDD R9 uplink signals with full filled QPSK, and converted to THz signals, transmitting to the receiver system. The THz signals were successfully demodulated, in which error vector magnitude (EVM) values of the demodulated signal was about 22% and 30% for 2 and 3 THz-band, respectively.