Temporal Emission Characteristics Research Articles

Study of temporal and spectral characteristics of the X-ray emission from solar flares

Temporal and spectral characteristics of X-ray emission from 60 flares of intensity ≥C class observed by the Solar X-ray Spectrometer (SOXS) during 2003–2011 are presented. We analyze the X-ray emission observed in four and three energy bands by the Si and Cadmium-Zinc-Telluride (CZT) detectors, respectively. The number of peaks in the intensity profile of the flares varies between 1 and 3. We find moderate correlation (R ≃ 0.2) between the rise time and the peak flux of the first peak of the flare irrespective of energy band, which is indicative of its energy-independent nature. Moreover, the magnetic field complexity of the flaring region is found to be highly anti-correlated (R = 0.61) with the rise time of the flares while positively correlated (R = 0.28) with the peak flux of the flare. The time delay between the peak of the X-ray emission in a given energy band and that in 25–30 keV decreases with increasing energy, suggesting conduction cooling is dominant in the lower energies. Analysis of 340 spectra from 14 flares reveals that the peak of differential emission measure (DEM) evolution is delayed by 60–360 s relative to that of the temperature, and this time delay is inversely proportional to the peak flux of the flare. We conclude that temporal and intensity characteristics of flares are dependent on energy as well as the magnetic field configuration of the active region.

Emissions and low-carbon development in Guangdong-Hong Kong-Macao Greater Bay Area cities and their surroundings

Cities are the major contributors to energy consumption and CO2 emissions, as well as being leading innovators and implementers of policy measures in climate change mitigation. Guangdong-Hong Kong-Macao Greater Bay Area (GBA) is an agglomeration of cities put forward by China to strengthen international cooperation among “Belt and Road” countries and promote low-carbon, inclusive, coordinated and sustainable development. Few studies have discussed the emission characteristics of GBA cities. This study, for the first time, compiles emission inventories of 11 GBA cities and their surroundings based on IPCC territorial emission accounting approach, which are consistent and comparable with the national and provincial inventories. Results show that (a) total emissions increased from 426 Mt in 2000 to 610 Mt in 2016, while emissions of GBA cities increased rapidly by 6.9% over 2000–2011 and peaked in 2014 (334 Mt); (b) raw coal and diesel oil are the top two emitters by energy type, while energy production sector and tertiary industry are the top two largest sectors; (c) GBA cities take the lead in low-carbon development, emitted 4% of total national emissions and contributed 13% of national GDP with less than a third of national emission intensities and less than three-quarters of national per capita emissions; (d) Macao, Shenzhen and Hong Kong have the top three lowest emission intensity in the country; (e) most of GBA cities are experiencing the shift from an industrial economy to a service economy, while Hong Kong, Shenzhen, Foshan and Huizhou reached their peak emissions and Guangzhou, Dongguan and Jiangmen remained decreasing emission tendencies; (g) for those coal-dominate or energy-production cities (i.e. Zhuhai, Zhongshan, Zhaoqing, Maoming, Yangjiang, Shanwei, Shaoguan and Zhanjiang) in mid-term industrialization, total emissions experienced soaring increases. The emission inventories provide robust, self-consistent, transparent and comparable data support for identifying spatial–temporal emission characteristics, developing low-carbon policies, monitoring mitigation progress in GBA cities as well as further emissions-related studies at a city-level. The low-carbon roadmaps designed for GBA cities and their surroundings also provide a benchmark for other developing countries/cities to adapting changing climate and achieve sustainable development.

Energy transfer networks: Quasicontinuum photoluminescence linked to high densities of defects

In a series of studies related to laser-induced damage of optical materials and deposition of plastics, we discovered a broadly emitting photoluminescence with fast lifetimes that we termed quasicontinuum photoluminescence (QC-PL). Here, we suggest that a high density of optically active defects leads to QC-PL, where interactions between defects affect the temporal and spectral characteristics of both excitation and emission. We develop a model that predicts the temporal characteristics of QC-PL, based on energy transfer interactions between high densities of defects. Our model does not explain all spectral broadening and redshifts found in QC-PL, since we do not model spectral changes in defects due to proximity to other defects. However, we do provide an example of a well-defined system that exhibits the QC-PL characteristics of a distribution in shortened lifetimes and broadened, redshifted energy levels: an organic chromophore (fluorescein) that has been dried rapidly on a fused silica surface. Recently, we showed that regions of fused silica exposed to up to 1 billion high-fluence laser shots at 351 rm nm at subdamage fluences exhibit significant transmission losses at the surface. Here, we find that these laser-exposed regions also exhibit QC-PL. Increases in the density of induced defects on these laser-exposed surfaces, as measured by the local transmission loss, lead to decreases in the observed lifetime and redshifts in the spectrum of the QC-PL, consistent with our explanation for QC-PL. We have found QC-PL in an increasing variety of situations and materials, and we believe it is a phenomenon commonly found on surfaces and nanostructured materials.

Eigen-analysis reveals components supporting super-resolution imaging of blinking fluorophores

This paper presents eigen-analysis of image stack of blinking fluorophores to identify the components that enable super-resolved imaging of blinking fluorophores. Eigen-analysis reveals that the contributions of spatial distribution of fluorophores and their temporal photon emission characteristics can be completely separated. While cross-emitter cross-pixel information of spatial distribution that permits super-resolution is encoded in two matrices, temporal statistics weigh the contribution of these matrices to the measured data. The properties and conditions of exploitation of these matrices are investigated. Con-temporary super-resolution imaging methods that use blinking for super-resolution are studied in the context of the presented analysis. Besides providing insight into the capabilities and limitations of existing super-resolution methods, the analysis shall help in designing better super-resolution techniques that directly exploit these matrices.

Optical Signatures of Quantum Emitters in Suspended Hexagonal Boron Nitride

Hexagonal boron nitride (h-BN) is rapidly emerging as an attractive material for solid-state quantum engineering. Analogously to three-dimensional wide-band-gap semiconductors such as diamond, h-BN hosts isolated defects exhibiting visible fluorescence at room temperature, and the ability to position such quantum emitters within a two-dimensional material promises breakthrough advances in quantum sensing, photonics, and other quantum technologies. Critical to such applications is an understanding of the physics underlying h-BN's quantum emission. We report the creation and characterization of visible single-photon sources in suspended, single-crystal, h-BN films. With substrate interactions eliminated, we study the spectral, temporal, and spatial characteristics of the defects' optical emission. Theoretical analysis of the defects' spectra reveals similarities in vibronic coupling to h-BN phonon modes despite widely varying fluorescence wavelengths, and a statistical analysis of the polarized emission from many emitters throughout the same single-crystal flake uncovers a weak correlation between the optical dipole orientations of some defects and h-BN's primitive crystallographic axes, despite a clear misalignment for other dipoles. These measurements constrain possible defect models and, moreover, suggest that several classes of emitters can exist simultaneously throughout free-standing h-BN, whether they be different defects, different charge states of the same defect, or the result of strong local perturbations.

Effect of different central interacting positions on the radiated power and spatial distribution characteristics

According to the classical theory of backwards Thomson scattering, if an electron is encountered with an intense multi-cycle circularly polarized laser pulse, the radiated power is produced in the propagation of the laser pulse. The spatial and temporal emission characteristics of radiation have been investigated theoretically and numerically using a single electron model. The motion of an electron is highly relativistic and the radiated power produced by head-on collision transits from two peaks to single peak finally. This interesting phenomenon can be attributed to acceleration of the single electron on the z axis and has been studied in detail in this treatise.

Assessing greenhouse gas emissions from electric vehicle operation in Australia using temporal vehicle charging and electricity emission characteristics

ABSTRACTSignificant interest exists in the potential for electric vehicles (EVs) to be a source of greenhouse gas (GHG) abatement. In order to establish the extent to which EVs will deliver abatement, however, a realistic understanding of the electricity and transport sector GHG emissions impacts arising from different approaches to integrating EVs into the power system is required. A key issue in this regard is the extent to which GHG emissions are a function of where and when EV charging will be enabled (or disabled) by the provision of recharging infrastructure and implementation of charging management strategies by the electricity industry. This article presents an investigation of the GHG emissions arising from electricity and gasoline consumption by plug-in hybrid EVs under a range of standard EV-power system integration scenarios. An assessment framework is presented, and GHG emissions from EV use are assessed for the New South Wales (NSW) and South Australian (SA) pools of the Australian National Electricity Market (NEM) using retrospective electricity system generation data for 2011. Results highlight that there is a range of possible outcomes depending on the integration scenario and emissions accounting approach used. This range illustrates value of a temporally explicit assessment approach in capturing the temporal alignment of electricity sector emission intensity and EV charging. Results also show the importance of a clean electricity generation mix in order for EVs to provide a GHG abatement benefit beyond what would be achieved by a hybrid (but non-plug-in) vehicle. The extent to which overnight charging in NSW is observed to produce higher emissions relative to unmanaged charging also illustrates a possible trade-off between GHG emissions and benefits for electricity industry from EV charging at times of low demand.

AN EXTRAORDINARY OUTBURST OF THE MAGNETAR SWIFT J1822.3–1606

The 2011 outburst of Swift J1822.3–1606 was extraordinary; periodic modulations at the spin period of the underlying neutron star were clearly visible, remarkably similar to what is observed during the decaying tail of magnetar giant flares. We investigated the temporal characteristics of X-ray emission during the early phases of the outburst. We performed a periodicity search with the spectral hardness ratio (HR) and found a coherent signal near the spin period of the neutron star, but with a lag of about 3 radians. Therefore, the HR is strongly anti-correlated with the X-ray intensity, which is also seen in the giant flares. We studied the time evolution of the pulse profile and found that it evolves from a complex morphology to a much simpler shape within about a month. Pulse profile simplification also takes place during the giant flares, but on a much shorter timescale of about a few minutes. We found that the amount of energy emitted during the first 25 days of the outburst is comparable to what was detected in minutes during the decaying tail of giant flares. Based on these similarities, we suggest that the triggering mechanisms of the giant flares and the magnetar outbursts are likely the same. We propose that the trapped fireball that develops in the magnetosphere at the onset of the outburst radiates away efficiently in minutes in magnetars exhibiting giant flares, while in other magnetars, such as Swift J1822.3–1606, the efficiency of radiation of the fireball is not as high and, therefore, lasts much longer.

Generation of hard X-ray emission by the electron beam in plasma focus facilities

The results of measurements of the temporal characteristics of hard X-ray emission generated at plasma focus (PF) facilities are presented. Mechanisms of electron beam generation in the PF pinch are analyzed. On the basis of the known mechanisms and experimental data on the measured temporal characteristics of hard X-ray pulses, a mechanism of fast electron generation that takes into account both the effect of the anomalous pinch resistance and the current redistribution in the near-pinch region is proposed. The processes occurring in the pinch plasma are simulated on the basis of the proposed mechanism by using the MicroCap code. It is shown that only a small fraction of the discharge current (1–10%) can be transformed into the electron beam current.

Spectral and temporal characteristics of hydrogen emission during femtosecond optical breakdown on a water surface

Spectral and time characteristics of a hydrogen HI 656 nm emission line are experimentally investigated during optical breakdown generated by pulses of the first harmonics of a femtosecond Ti:Sapphire laser on the water surface. The electron density of the generated plasma is estimated.

Spatial, temporal and spectral emission characteristics from electron oscillation driven by an intense circularly polarized few-cycle laser pulse

The spatial, temporal and spectral emission characteristics of radiation generated from electron oscillations driven by an intense circularly polarized few-cycle laser pulse have been investigated theoretically and numerically using a single electron model. For a femtosecond driving laser pulse with duration of one optical cycle, the maximal radiation emitted by the electron comprises only one electromagnetic pulse having durations much shorter than the optical cycle and belonging to the attosecond range. It is discovered that the influence of the initial phase on the process of full spatial characteristics of the radiation is apparent for intense few-cycle laser pulse. The characteristics can be used to measure the initial phase of intense circularly polarized few-cycle laser pulse in experiments.

Synthesis and cathodoluminescence characteristics of europium-doped Ca-sialons

Using solid-state reactions and a combination of carbothermal reduction-nitridation with solgel processing, we have synthesized a number of oxynitride phases: Eu2+-doped Ca-sialons. We have measured the pulsed cathodoluminescence spectra of the synthesized powders under pulsed electron beam excitation and determined their emission parameters, including temporal emission characteristics.

Temporally and spatially resolved imaging of laser-nucleated bubble cloud sonoluminescence

Imaging techniques have been used to capture the temporal and spatial evolution of light emissions from collapsing bubble clouds at high static pressures. Emission events lasting up to 70 ns with peak diameters nearing 1 mm have been observed. Observations of the cloud evolution before and after emission events have been made. Photomultiplier tube monitoring has been employed in conjunction with imaging to study the temporal characteristics of light emission.

TRLFS Evidence for Precipitation of Uranyl Phosphate on the Surface of Alumina: Environmental Implications

We studied the ligand-enhanced sorption of uranyl ions (1-12 μM) on α-alumina colloids suspended in (and pre-equilibrated with) solutions at various concentrations of phosphate ions (P(T) = 0-900 μM). A highly sensitive technique, time resolved laser-induced fluorescence spectroscopy (TRLFS), was used to examine the chemical speciation of uranyl sorbed at trace concentrations (0.4-4 μmol U·g⁻¹). The suspensions with P(T) ≥ 100 μM exhibited high uranyl adsorption, and a very high intensity of fluorescence that increased with the sorbed amounts of phosphate and uranyl. These samples exhibited similar spectral and temporal characteristics of fluorescence emission, evidencing a uniform speciation pattern and a single coordination environment for sorbed U, despite large variation in parameters such as aqueous uranyl speciation, U loading, and extent of coverage of alumina by secondary Al phosphates precipitating on the surface. The results pointed formation of surface precipitates of uranyl phosphates, which are characterized by high quantum yield, peak maxima at positions similar to those of U(VI) phosphate minerals and four lifetimes indicating distortions, in-homogeneities or varying number of water molecules in the lattice. The findings have major implications for our understanding of the mechanisms of immobilization of U at trace levels on surfaces of oxides submitted to phosphated solutions in soils with low pH.

Comparison of the spectral and temporal emission characteristics of homoepitaxial and heteroepitaxial ZnO nanowires

Using metalorganic chemical vapor deposition, we have grown ZnO nanowires (NWs) on ZnO(0001) as well as on Al2O3(0001) and Si(111) substrates. The optical properties of these NWs are studied by continuous-wave and time-resolved photoluminescence spectroscopy. Both the spectral and the temporal characteristics of the NWs are found to be virtually identical despite the different substrates and the different morphology of the NWs. This study thus provides strong experimental evidence for the hypothesis that NWs remove the constraints introduced by the substrate.

Directional and Dynamic Modulation of the Optical Emission of an Individual GaAs Nanowire Using Surface Acoustic Waves

We report on optical experiments performed on individual GaAs nanowires and the manipulation of their temporal emission characteristics using a surface acoustic wave. We find a pronounced, characteristic suppression of the emission intensity for the surface acoustic wave propagation aligned with the axis of the nanowire. Furthermore, we demonstrate that this quenching is dynamical as it shows a pronounced modulation as the local phase of the surface acoustic wave is tuned. These effects are strongly reduced for a surface acoustic wave applied in the direction perpendicular to the axis of the nanowire due to their inherent one-dimensional geometry. We resolve a fully dynamic modulation of the nanowire emission up to 678 MHz not limited by the physical properties of the nanowires.

Spatial and temporal characteristics of X-ray emission from hot plasma driven by a relativistic femtosecond laser pulse

AbstractWe present the temporal and spatial characterization of X-ray sources (at ~1 keV) driven by a 200 TW, 30 fs, 800 nm laser pulse on SILEX-I laser facility at Research Center of Laser Fusion. For laser copper foil interaction with laser intensity between 6 × 1018 W/cm2and 3 × 1019 W/cm2, the X-ray images show cone-like jet structures. While the yield of X-rays is strongly dependent on the laser intensity, the plasma expansion length is weakly dependent on the laser intensity, and the open angle of the cone-like jet is not correlated to the laser intensity. The formation of the jet structure is attributed to the plasma transverse confine by the self-induced quasi-static magnetic field. An X-ray pedestal 4 ns preceding the main pulse was observed. The correlation between X-ray pedestal and collimated proton beam generation was found.

Accelerated electrons and hard X-ray emission from X-pinches

The generation of accelerated electrons in the X-pinch minidiode is studied experimentally. It is well known that the explosion of an X-pinch consisting of two or more wires is accompanied by the formation of a minidiode, in which electrons are accelerated. The subsequent slowing down of electrons in the products of wire explosion causes the generation of hard X-ray (HXR) emission with photon energies higher than 10 keV. In this work, the spatial and temporal characteristics of X-pinch HXR emission are studied, the specific features of HXR generation are discussed, and the capability of applying this radiation to point-projection X-ray imaging of various plasma and biological objects is considered. The parameters of the electron beam produced in the X-pinch are measured using a Faraday cup and X-ray diagnostics. The experiments were performed with the XP generator (550 kA, 100 ns) at Cornell University (United States) and the BIN generator (270 kA, 150 ns) at the Lebedev Physical Institute (Russia).

Time-resolved spectroscopy and imaging diagnostics of single pulse and collinear double pulse laser induced plasma from a glass sample

The characterization of laser-induced plasma from a glass sample was performed in the single- and double-pulse excitation regimes. The detailed information about density distributions of excited atoms and ions in the expanding plasma was obtained by using the imaging detection system providing measurements of the spatial, temporal, and spectral plasma emission characteristics. The expansion dynamics was shown to differ strongly between two excitation regimes. The enhancement factors of the line emissions in the double-pulse mode were found to be spatial dependent and to differ for the different elements in the plasma plume. The obtained results are useful for a better understanding of the main physical processes leading to the analytical improvement achieved by the use of double-pulse laser-induced breakdown spectroscopy (LIBS).

Temporal characteristics of X-ray emission from X-pinches

The temporal characteristics of X-ray emission from X-pinches have been studied experimentally on the XP facility (with a 100-ns current pulse duration and 470-kA current amplitude) at Cornell University. The experiments were performed with X-pinches made of Al, Ti, Mo, and W wires. Radiation in the photon energy range 1–10 keV was recorded using diamond and silicon photodiodes with a subnanosecond time resolution and X-ray streak cameras with a picosecond time resolution. It is shown that, for high-Z elements, the duration of the X-ray pulse in the short-wavelength part of the spectral range under study does not exceed 5–10 ps.