Target Normal Sheath Acceleration Regime Research Articles

Proton acceleration from optically tailored high-density gas jet targets

Laser-driven ion acceleration is well established using solid targets mainly in the target normal sheath acceleration regime. To follow the increasing repetition rate available on high-intensity lasers, the use of high-density gas targets has been explored in the past decade. When interacting with targets reaching densities close to the critical one, the laser pulse can trigger different acceleration mechanisms such as Collisionless Shock Acceleration (CSA) or hole boring. Particle-in-cell simulations using ideal target profiles show that CSA can accelerate a collimated, narrow energy spread and few hundreds of megaelectronvolts ion beam on the laser axis. Nevertheless, in real experiments, the laser will not only interact with an overcritical, thin plasma slab with sharp density gradients, but also with lower density regions surrounding the core of the gas jet, extending to several hundreds of micrometres. The interaction of the laser with these lower density wings will lead to nonlinear effects that will reduce the available energy to drive the shock in the high-density region of the target. Optically tailoring this target could mitigate that issue. Recent experiments conducted on different laser facilities aimed at testing several tailoring configurations. We first tested a scheme with a copropagating picosecond prepulse to create a lower density plasma channel to facilitate the propagation of the main pulse, while the second one was a transverse tailoring driven by nanosecond laser pulses to generate blast waves and form a high-density plasma slab. The main results will be presented here and the methods compared.

Real-time bremsstrahlung detector as a monitoring tool for laser–plasma proton acceleration

Abstract Real-time evaluation of laser-driven byproducts is crucial for state-of-the-art facilities operating at high repetition rates. This work presents real-time measurements of hard X-rays (bremsstrahlung radiation) generated from the interaction of high-intensity laser pulses with solid targets in the target normal sheath acceleration regime using a scintillator stack detector. The detector offers insights into the effectiveness of laser–plasma interaction through measured fluctuations in bremsstrahlung radiation temperature and scintillation light yield on a shot-to-shot basis. Moreover, a strong correlation of the bremsstrahlung measurements (i.e., temperature and yield) with the cutoff energy of laser-driven protons was observed. The scintillator stack detector serves not only as a diagnostic for online monitoring of the laser–plasma interaction but also as a promising tool for estimating proton energy fluctuations in a non-disruptive manner, which is particularly important when direct proton source characterization is impractical, for example, during experiments aimed at irradiating user samples with the accelerated proton beam.

Optically tunable proton acceleration with a controlled prepulse in ultrashort intense laser double-foil target interaction

Competition and transition of the dominated mechanisms for proton acceleration were investigated in experiments by optically tuning the preplasma density profile using an additional femtosecond pre-ablation laser beam. Two groups of proton beams with angular separation were measured along the laser propagation axis and target normal direction from a vacuum-gapped double-foil target. A transition of proton acceleration from a target normal sheath acceleration regime to relativistically induced transparency (RIT) domination was observed when increasing the prepulse intensity. Two-dimensional particle-in-cell simulations qualitatively verify the experimental observations that a proton component along the laser axis is mainly generated by the RIT induced breakout afterburner from the tailored pre-expanded ultrathin front-layer foil with spatial-intensity distribution improvement by the second-layer foil. Our method can be popularized in manipulating the laser-driven proton acceleration and beam spatial quality for wide applications.

Advantages to use graphene oxide thin targets in forward ion acceleration using fs lasers

AbstractAdvanced targets based on thin foils of graphene oxide (GO) covered by metallic layers show many advantages with respect to others because permit high proton and light ion acceleration using high intensity pulsed lasers in Target‐Normal Sheath‐Acceleration (TNSA) regime. GO foils contain parallel micrometric graphene sheets, have low density, show high penetration, and low scattering by energetic electrons accelerated by laser, inducing electron channelling effects. They contain high concentrations of hydrogen, water, and functional oxygen groups, can be realized as thin films with high mechanical resistance, and show high photon absorbance for laser beams. In this work, we present experimental results obtained by our research group using thin GO targets covered by thin gold films, prepared in our laboratories. Advanced targets have been irradiated in TNSA regime with 40 fs laser pulses at the intensity of the order of 1019 W/cm2, using a laser spot of about 10 microns diameter, permitting to accelerate ions at energies of the order of 6 MeV per charge state. The electric field of ion acceleration can be increased by optimizing the irradiation conditions and the GO and Au film thicknesses. The novel findings of this work concern the high forward ion acceleration obtained using thin targets containing GO which induces the effect of electron channelling and production of high‐density forward plasma. The plasma diagnostics are developed with fast SiC semiconductor detectors connected in time‐of‐flight (TOF) configuration. The fast semiconductor detector response permits to optimize the ion acceleration conditions by changing the distance of the laser focus with respect to the target surface, the incidence angle and the laser parameters.

A laser parameter study on enhancing proton generation from microtube foil targets

The interaction of an intense laser with a solid foil target can drive sim TV/m electric fields, accelerating ions to MeV energies. In this study, we experimentally observe that structured targets can dramatically enhance proton acceleration in the target normal sheath acceleration regime. At the Texas Petawatt Laser facility, we compared proton acceleration from a 1, {upmu }hbox {m} flat Ag foil, to a fixed microtube structure 3D printed on the front side of the same foil type. A pulse length (140–450 fs) and intensity ((4–10) times 10^{20} W/cm^2) study found an optimum laser configuration (140 fs, 4 times 10^{20} W/cm^2), in which microtube targets increase the proton cutoff energy by 50% and the yield of highly energetic protons (>10 MeV) by a factor of 8times. When the laser intensity reaches 10^{21} W/cm^2, the prepulse shutters the microtubes with an overcritical plasma, damping their performance. 2D particle-in-cell simulations are performed, with and without the preplasma profile imported, to better understand the coupling of laser energy to the microtube targets. The simulations are in qualitative agreement with the experimental results, and show that the prepulse is necessary to account for when the laser intensity is sufficiently high.

Intensity scaling limitations of laser-driven proton acceleration in the TNSA-regime

We report on experimental results on laser-driven proton acceleration using high-intensity laser pulses. We present power law scalings of the maximum proton energy with laser pulse energy and show that the scaling exponent $\ensuremath{\xi}$ strongly depends on the scale length of the preplasma, which is affected by the temporal intensity contrast. At lower laser intensities, a shortening of the scale length leads to a transition from a square root toward a linear scaling. Above a certain threshold, however, a significant deviation from this scaling is observed. Two-dimensional particle-in-cell simulations show that, in this case, the electric field accelerating the ions is generated earlier and has a higher amplitude. However, since the acceleration process starts earlier as well, the fastest protons outrun the region of highest field strength, ultimately rendering the acceleration less effective. Our investigations thus point to a principle limitation of the proton energy in the target normal sheath acceleration regime, which would explain why a significant increase of the maximum proton energy above the limit of $100\phantom{\rule{0.16em}{0ex}}\mathrm{MeV}$ has not yet been achieved.

Analysis of laser-proton acceleration experiments for development of empirical scaling laws

Numerous experiments on laser-driven proton acceleration in the MeV range have been performed with a large variety of laser parameters since its discovery around the year 2000. Both experiments and simulations have revealed that protons are accelerated up to a maximum cut-off energy during this process. Several attempts have been made to find a universal model for laser proton acceleration in the target normal sheath acceleration regime. While these models can qualitatively explain most experimental findings, they can hardly be used as predictive models, for example, for the energy cut-off of accelerated protons, as many of the underlying parameters are often unknown. Here we analyze experiments on laser proton acceleration in which scans of laser and target parameters were performed. We derive empirical scaling laws from these parameter scans and combine them in a scaling law for the proton energy cut-off that incorporates the laser pulse energy, the laser pulse duration, the focal spot radius, and the target thickness. Using these scaling laws, we give examples for predicting the proton energy cut-off and conversion efficiency for state-of-the-art laser systems.

Laser-plasma proton acceleration with a combined gas-foil target

Laser-plasma proton acceleration was investigated in the target normal sheath acceleration regime with a target composed of a gas layer and a thin foil. The laser’s shape, duration, energy and frequency are modified as it propagates in the gas, altering the laser-solid interaction leading to proton acceleration. The modified properties of the laser were assessed by both numerical simulations and by measurements. The 3D particle-in-cell simulations have shown that a nearly seven-fold increase in peak intensity at the foil plane is possible. In the experiment, maximum proton energies showed high dependence on the energy transmission of the laser through the gas and a lesser dependence on the size and shape of the pulse. At high gas densities, where high intensity was expected, laser energy depletion and pulse distortion suppressed proton energies. At low densities, with the laser focused far behind the foil, self-focusing was observed and the gas showed a positive effect on proton energies. The promising results of this first exploration motivate further study of the target.

Assessment of Angular Spectral Distributions of Laser Accelerated Particles for Simulation of Radiation Dose Map in Target Normal Sheath Acceleration Regime of High Power Laser-Thin Solid Target Interaction—Comparison with Experiments

An adequate simulation model has been used for the calculation of angular and energy distributions of electrons, protons, and photons emitted during a high-power laser, 5-µm thick Ag target interaction. Their energy spectra and fluencies have been calculated between 0 and 360 degrees around the interaction point with a step angle of five degrees. Thus, the contribution of each ionizing species to the total fluency value has been established. Considering the geometry of the experimental set-up, a map of the radiation dose inside the target vacuum chamber has been simulated, using the Geant4 General Particle Source code, and further compared with the experimental one. Maximum values of the measured dose of the order of tens of mGy per laser shot have been obtained in the direction normal to the target at about 30 cm from the interaction point.

Investigation of the effect of plasma waves excitation on target normal sheath ion acceleration using fs laser‐irradiating hydrogenated structures

Measurements of ion acceleration in polymethylmethacrylate foils covered by a thin copper film irradiated by fs laser in target normal sheath acceleration regime are presented. The ion acceleration depends on the laser parameters, such as the pulse energy; depends on the irradiation conditions, such as the focal point position of the laser with respect to the target surface; and depends on the target properties, such as the metallic film thickness. The proton acceleration increases in the presence of the metallic film enhancing the plasma electron density, reaching about 1.6 MeV energy for a focal position on the target surface. The plasma diagnostics uses SiC detectors, absorber foils, Faraday cups, and gafchromic films. Employing p‐polarized laser light and a suitable oblique incidence, it is possible to increase the proton acceleration up to about 2.0 MeV thanks to the effects of laser absorption resonance due to plasma waves excitation.

Protons accelerated in the target normal sheath acceleration regime by a femtosecond laser

Advanced targets based on thin films of graphene oxide covered by metallic layers have been irradiated at high laser intensity ($\ensuremath{\sim}{10}^{19}\text{ }\text{ }\mathrm{W}/{\mathrm{cm}}^{2}$) with 40 fs laser pulses to investigate the forward ion acceleration in the target normal sheath acceleration regime. A time-of-flight technique was employed with silicon-carbide detectors and ion collectors as fast on-line plasma diagnostics. At the optimized conditions of the laser focus position with respect to the target surface was measured the maximum proton energy using Au metallic films. A maximum proton energy of 2.85 MeV was measured using the Au metallization of 200 nm. The presence of graphene oxide facilitates the electron crossing of the foil minimizing the electron scattering and increasing the electric field driving the ion acceleration. The effect of plasma electron density control using the graphene oxide is presented and discussed.

Proton acceleration measurements using fs laser irradiation of foils in the target normal sheath acceleration regime

We present experimental results obtained at the CELIA laboratory using the laser ECLIPSE to study proton acceleration from ultra-intense laser pulses. Several types of targets were irradiated with different laser conditions (focusing and prepulse level). Proton emission was characterized using time-of-flight detectors (SiC and diamond) and a Thomson parabola spectrometer. In all cases, the maximum energy of observed protons was of the order of 260 keV with a large energy spectrum. Such characteristics are typical of protons emitted following the target normal sheath acceleration mechanism for low-energy short-pulse lasers like ECLIPSE.

Laser-ablation-based ion source characterization and manipulation for laser-driven ion acceleration

For laser-driven ion acceleration from thin foils (∼10 μm–100 nm) in the target normal sheath acceleration regime, the hydro-carbon contaminant layer at the target surface generally serves as the ion source and hence determines the accelerated ion species, i.e. mainly protons, carbon and oxygen ions. The specific characteristics of the source layer—thickness and relevant lateral extent—as well as its manipulation have both been investigated since the first experiments on laser-driven ion acceleration using a variety of techniques from direct source imaging to knife-edge or mesh imaging. In this publication, we present an experimental study in which laser ablation in two fluence regimes (low: F ∼ 0.6 J cm−2, high: F ∼ 4 J cm−2) was applied to characterize and manipulate the hydro-carbon source layer. The high-fluence ablation in combination with a timed laser pulse for particle acceleration allowed for an estimation of the relevant source layer thickness for proton acceleration. Moreover, from these data and independently from the low-fluence regime, the lateral extent of the ion source layer became accessible.

Rise time of proton cut-off energy in 2D and 3D PIC simulations

The Target Normal Sheath Acceleration regime for proton acceleration by laser pulses is experimentally consolidated and fairly well understood. However, uncertainties remain in the analysis of particle-in-cell simulation results. The energy spectrum is exponential with a cut-off, but the maximum energy depends on the simulation time, following different laws in two and three dimensional (2D, 3D) PIC simulations so that the determination of an asymptotic value has some arbitrariness. We propose two empirical laws for the rise time of the cut-off energy in 2D and 3D PIC simulations, suggested by a model in which the proton acceleration is due to a surface charge distribution on the target rear side. The kinetic energy of the protons that we obtain follows two distinct laws, which appear to be nicely satisfied by PIC simulations, for a model target given by a uniform foil plus a contaminant layer that is hydrogen-rich. The laws depend on two parameters: the scaling time, at which the energy starts to rise, and the asymptotic cut-off energy. The values of the cut-off energy, obtained by fitting 2D and 3D simulations for the same target and laser pulse configuration, are comparable. This suggests that parametric scans can be performed with 2D simulations since 3D ones are computationally very expensive, delegating their role only to a correspondence check. In this paper, the simulations are carried out with the PIC code ALaDyn by changing the target thickness L and the incidence angle α, with a fixed a0 = 3. A monotonic dependence, on L for normal incidence and on α for fixed L, is found, as in the experimental results for high temporal contrast pulses.

Advanced polymer targets for TNSA regime producing 6 MeV protons at 1016 W/cm2 laser intensity

High intensity laser pulses, at an intensity of the order of 1016 W/cm2, are employed to irradiate in vacuum polyethylene terephthalate thin foils in the target normal sheath acceleration (TNSA) regime. The plasma obtained in the forward emission is investigated using ion collectors and semiconductor detectors connected in a time-of-flight configuration, Thomson parabola spectrometer, and X-ray streak camera. The results indicate that the foil thickness of 1 micron is optimal to accelerate protons of up to 6.5 MeV. The high ion acceleration can be due to different effects such as the high absorption in the advanced semicrystalline polymer containing spherulite centers, the high resonant absorption in gold nanoparticles embedded in the polymer, the optimal thickness of the used polymer to enhance the electron density in the forward plasma, and the self-focusing effect induced by preplasma created in front of the irradiated target.

Acceleration of high charge-state target ions in high-intensity laser interactions with sub-micron targets

We have studied laser acceleration of ions from Si3N4 and Al foils ranging in thickness from 1800 to 8 nm with particular interest in acceleration of ions from the bulk of the target. The study includes results of experiments conducted with the HERCULES laser with pulse duration 40 fs and intensity 3 × 1020 W cm−2 and corresponding two-dimensional particle-in-cell simulations. When the target thickness was reduced the distribution of ion species heavier than protons transitioned from being dominated by carbon contaminant ions of low ionization states to being dominated by high ionization states of bulk ions (such as Si12+) and carbon. Targets in the range 50–150 nm yielded dramatically greater particle number and higher ion maximum energy for these high ionization states compared to thicker targets typifying the Target Normal Sheath Acceleration (TNSA) regime. The high charge states persisted for the thinnest targets, but the accelerated particle numbers decreased for targets 35 nm and thinner. This transition to an enhanced ion TNSA regime, which more efficiently generates ion beams from the bulk target material, is also seen in the simulations.

Electron emission from laser irradiating target normal sheath acceleration (TNSA)

ABSTRACTA study of the electron emission from laser-generated plasma in target normal sheath acceleration regime is presented for different targets. The used laser has an intensity of about 1016 W/cm2 and a pulse duration of 300 ps. Electrons were detected using SiC detectors and plastic scintillators employed in time-of-flight configuration and a Thomson parabola spectrometer (TPS). Measurements indicated the presence of hot electrons with a kinetic energy of the order of some MeVs. SiC and scintillators detect electrons up to about 400 keV while TPS electrons up to about 5 MeV energy. Electrons yield emitted in the forward direction is proportional to the effective atomic number of the target and is inversely proportional to the target thickness.

Ion acceleration in the transparent regime and the critical influence of the plasma density scale length

The influence of a plasma density gradient on ions accelerated along the specular (back reflection) direction in the transparent Target Normal Sheath Acceleration regime is investigated. Enhanced acceleration of ions is experimentally observed in this regime using high-intensity and ultra-high contrast laser pulses and extremely thin foils of few nanometer thicknesses. The experimental trend for the maximum proton energy appeared quite different from the already published numerical results in this regime where an infinitely steep plasma gradient was assumed. We showed that for a realistic modelling, a finite density gradient has to be taken into account. By means of particle-in-cell (PIC) simulations, we studied for the first time the influence of the plasma density scale length on ion acceleration from these nanofoil targets. Through a qualitative agreement between our numerical particle-in-cell simulations and our experiments, the main conclusion with regard to the experimental requirements is that, in the transparent regime evidenced with nanofoils as compared to the opaque regime, the plasma expansion has to be taken into account and both the pulse contrast and the damage threshold of the material are essential parameters.

Generation of heavy ion beams using femtosecond laser pulses in the target normal sheath acceleration and radiation pressure acceleration regimes

Theoretical study of heavy ion acceleration from sub-micron gold foils irradiated by a short pulse laser is presented. Using two dimensional particle-in-cell simulations, the time history of the laser pulse is examined in order to get insight into the laser energy deposition and ion acceleration process. For laser pulses with intensity 3×1021 W/cm2, duration 32 fs, focal spot size 5 μm, and energy 27 J, the calculated reflection, transmission, and coupling coefficients from a 20 nm foil are 80%, 5%, and 15%, respectively. The conversion efficiency into gold ions is 8%. Two highly collimated counter-propagating ion beams have been identified. The forward accelerated gold ions have average and maximum charge-to-mass ratio of 0.25 and 0.3, respectively, maximum normalized energy 25 MeV/nucleon, and flux 2×1011 ions/sr. An analytical model was used to determine a range of foil thicknesses suitable for acceleration of gold ions in the radiation pressure acceleration regime and the onset of the target normal sheath acceleration regime. The numerical simulations and analytical model point to at least four technical challenges hindering the heavy ion acceleration: low charge-to-mass ratio, limited number of ions amenable to acceleration, delayed acceleration, and high reflectivity of the plasma. Finally, a regime suitable for heavy ion acceleration has been identified in an alternative approach by analyzing the energy absorption and distribution among participating species and scaling of conversion efficiency, maximum energy, and flux with laser intensity.

Resonant absorption effects induced by polarized laser light irradiating thin foils in the TNSA regime of ion acceleration

Thin foils were irradiated by short pulsed lasers at intensities of 1016−19W/cm2 in order to produce non-equilibrium plasmas and ion acceleration from the target-normal-sheath-acceleration (TNSA) regime. Ion acceleration in forward direction was measured by SiC detectors and ion collectors used in the time-of-flight configuration. Laser irradiations were employed using p-polarized light at different incidence angles with respect to the target surface and at different focal distances from the target surface. Measurements demonstrate that resonant absorption effects, due to the plasma wave excitations, enhance the plasma temperature and the ion acceleration with respect to those performed without to use of p-polarized light. Dependences of the ion flux characteristics on the laser energy, wavelength, focal distance and incidence angle will be reported and discussed.