Subwavelength Light Confinement Research Articles

Polaritonic Hybrid-Epsilon-near-Zero Modes: Beating the Plasmonic Confinement vs Propagation-Length Trade-Off with Doped Cadmium Oxide Bilayers.

Polaritonic materials that support epsilon-near-zero (ENZ) modes offer the opportunity to design light-matter interactions at the nanoscale through extreme subwavelength light confinement, producing phenomena like resonant perfect absorption. However, the utility of ENZ modes in nanophotonic applications has been limited by a flat spectral dispersion, which leads to small group velocities and extremely short propagation lengths. Here, we overcome this constraint by hybridizing ENZ and surface plasmon polariton (SPP) modes in doped cadmium oxide epitaxial bilayers. This results in strongly coupled hybrid modes that are characterized by an anticrossing in the polariton dispersion and a large spectral splitting on the order of 1/3 of the mode frequency. These hybrid modes simultaneously achieve modal propagation and ENZ mode-like interior field confinement, adding propagation character to ENZ mode properties. We subsequently tune the resonant frequencies, dispersion, and coupling of these polaritonic-hybrid-epsilon-near-zero (PH-ENZ) modes by tailoring the modal oscillator strength and the ENZ-SPP spectral overlap. PH-ENZ modes ultimately leverage the most desirable characteristics of both ENZ and SPP modes, allowing us to overcome the canonical plasmonic trade-off between confinement and propagation length.

Strong Coupling of Epsilon-Near-Zero Phonon Polaritons in Polar Dielectric Heterostructures.

We report the first observation of epsilon-near-zero (ENZ) phonon polaritons in an ultrathin AlN film fully hybridized with surface phonon polaritons (SPhP) supported by the adjacent SiC substrate. Employing a strong coupling model for the analysis of the dispersion and electric field distribution in these hybridized modes, we show that they share the most prominent features of the two precursor modes. The novel ENZ-SPhP coupled polaritons with a highly propagative character and deeply subwavelength light confinement can be utilized as building blocks for future infrared and terahertz nanophotonic integration and communication devices.

Subwavelength light confinement and enhancement enabled by dissipative dielectric nanostructures.

Dissipative loss in optical materials is considered one of the major challenges in nano-optics. Here we show that, counter-intuitively, a large imaginary part of material permittivity contributes positively to subwavelength light enhancement and confinement. The Purcell factor and the fluorescence enhancement of dissipative dielectric bowtie nanoantennas, such as Si in ultraviolet (UV), are demonstrated to be orders of magnitude higher than their lossless dielectric counterparts, which is particularly favorable in deep UV applications where metals are plasmonically inactive. The loss-facilitated field enhancement is the result of a large material property contrast and an electric field discontinuity. These dissipative dielectric nanostructures can be easily achieved with a great variety of dielectrics at their Lorentz oscillation frequencies, thus having the potential to build a completely new material platform boosting light-matter interaction over broader frequency ranges, with advantages such as bio-compatibility, CMOS compatibility, and harsh environment endurance.

Infrared Fingerprints of Natural 2D Talc and Plasmon–Phonon Coupling in Graphene–Talc Heterostructures

Two-dimensional (2D) materials occupy noteworthy place in nanophotonics providing for subwavelength light confinement and optical phenomena dissimilar to those of their bulk counterparts. In the mid-infrared, graphene-based heterostructures and van der Waals crystals of hexagonal boron nitride (hBN) overwhelmingly concentrate the attention by exhibiting real-space nano-optics from plasmons, phonon-polaritons and hybrid plasmon phonon-polaritons quasiparticles. Here we present the mid-infrared nanophotonics of talc, a natural atomically flat layered material, and graphene-talc (G-talc) heterostructures using broadband synchrotron infrared nano-spectroscopy. We achieve wavelength tuning of the talc resonances, assigned to in- and out-of-plane vibrations by changing the thickness of the crystals, which serves as its infrared fingerprints. Moreover, we encounter coupling of the graphene plasmons polaritons with surface optical phonons of talc. As in the case of the G-hBN heterostructures, this coupling configures hybrid surface plasmon phonon-polariton modes causing 30 % increase in intensity for the out-of-plane mode, blue-shift for the in-plane mode and we have succeeded in altering the amplitude of such hybridization by varying the gate voltage. Therefore, our results promote talc and G-talc heterostructures as appealing materials for nanophotonics, like hBN and G-hBN, with potential applications for controllably manipulating infrared electromagnetic radiation at the subdiffraction scale.

Design and Simulation of a New Coaxial Probe for Near Field Scanning Optical Microscopy

Design of the new photonic devices having attractive optical properties such as subwavelength confinement of light has a numerous applications in developing nanoscale sensors, photonic integrated circuits, solar cells and etc. Abbe’s diffraction limit restricts the use of subwavelength scale photonic elements due to their size and therefore new approaches are required in order to achieve desirable nanometer scale properties of these devices. Delivering light energy to nanometer scale regions can be achieved by surface plasmon polariton (SPP) waves that propagate in metal-dielectric interface. The paper presents results in FDTD (finite-difference time domain) simulation of a new coaxial probe of nanometer-scale size.Based on FDTD simulations of the coaxial probe field localization and enhancement in the region around the tip of coaxial probe has been obtained. Configuration of the probe consists of the truncated Au cone as a core, truncated dielectric (SiO2) cone in the middle and outer metallic cladding. Simulations of the probe revealed that increasing the radius of Au core structure could lead to the enhanced field around the tip. Additionally, increasing radius of outer cladding layer doesn’t affect field enhancement around the tip. Different configurations of the probe have been analyzed in the range of visible spectrum of the source and as a result the most promising configuration has been selected

Design of a compact high-speed optical modulator based on a hybrid plasmonic nanobeam cavity

A hybrid plasmonic electro-optic modulator based on a polymer-filled one dimensional photonic crystal nanobeam (1D PhCNB) cavity is proposed here. In the proposed structure the optical intensity modulation is realized by shifting the resonant wavelength of the cavity through electrically tuning the refractive index of the electro-optic polymer in the hybrid plasmonic waveguide. As a result of the subwavelength light confinement in the hybrid plasmonic waveguide and the compact footprint of the 1D PhCNB cavity, the designed modulator has the small overall footprint of 3.6μm2 and the required wavelength shift can be achieved by applying very small actuating power. Three dimensional finite-difference time-domain (3D-FDTD) simulations show that the modulation depth of 10.9 dB, and insertion loss of 1.14 dB, along with very high modulation speed of 224 GHz can be achieved in the proposed modulator with very low modulation energy of 0.75 fJ/bit. A comparison between the performance parameters of the proposed modulator and those of previously reported PhCNB based modulators reveals the superior performance of the proposed structure in terms of modulation speed, energy consumption and overall footprint.

Transversely Divergent Second Harmonic Generation by Surface Plasmon Polaritons on Single Metallic Nanowires.

Coherently adding up signal wave from different locations are a prerequisite for realizing efficient nonlinear optical processes in traditional optical configurations. While nonlinear optical processes in plasmonic waveguides with subwavelength light confinement are in principle desirable for enhancing nonlinear effects, so far it has been difficult to improve the efficiency due to the large momentum mismatch. Here we demonstrate, using remotely excited surface plasmon polaritons (SPPs), axial collimated but transversely divergent second harmonic (SH) generation in a single silver nanowire-monolayer molybdenum disulfide hybrid system. Fourier imaging of the generated SH signal confirms the momentum conservation conditions between the incident and reflected SPPs and reveals distinct features inherent to the 1D plasmonic waveguides: (i) the SH photons are collimated perpendicular to the nanowire axis but are divergent within the perpendicular plane; (ii) the collimation (divergence) is inversely proportional to the length of the active region (lateral confinement of the SPPs); and (iii) the SH emission pattern resembles that of an aligned dipole chain on top of the substrate with an emission peak at the critical angle. Our results pave the way to generate and manipulate SH emission around subwavelength waveguides and open up new possibilities for realizing high efficiency on-chip nonlinear optics.

Low-loss nanowire and nanotube plasmonic waveguide with deep subwavelength light confinement and enhanced optical trapping forces

With the rapid development of the micro/nano fabrication technology, the semiconductor nanowires and nanotubes with size and dimensions controllable realize wide applications in nanophotonics. In this talk, we propose two kinds of hybrid plasmonics waveguides, one is consisting of nanowires, another is consisting of nanotubes. By employing the simulating with different geometric parameters, the basic waveguiding properties, including the effective mode area, the propagation length, the mode character and the optical trapping forces can be achieved. Compared with previous plasmonic waveguide with plane metal substrate, current plasmonics waveguides with ease of fabrication have the advantage of long propagation length and effectively optical trapping of nanoparticles with deep subwavelength light confinement, which may be very useful for nanophotonic integrated circuits, nanolasers and biosensing.

Photoswitchable Rabi Splitting in Hybrid Plasmon–Waveguide Modes

Rabi splitting that arises from strong plasmon-molecule coupling has attracted tremendous interests. However, it has remained elusive to integrate Rabi splitting into the hybrid plasmon-waveguide modes (HPWMs), which have advantages of both subwavelength light confinement of surface plasmons and long-range propagation of guided modes in dielectric waveguides. Herein, we explore a new type of HPWMs based on hybrid systems of Al nanodisk arrays covered by PMMA thin films that are doped with photochromic molecules and demonstrate the photoswitchable Rabi splitting with a maximum splitting energy of 572 meV in the HPWMs by controlling the photoisomerization of the molecules. Through our experimental measurements combined with finite-difference time-domain (FDTD) simulations, we reveal that the photoswitchable Rabi splitting arises from the switchable coupling between the HPWMs and molecular excitons. By harnessing the photoswitchable Rabi splitting, we develop all-optical light modulators and rewritable waveguides. The demonstration of Rabi splitting in the HPWMs will further advance scientific research and device applications of hybrid plasmon-molecule systems.

Impact of longitudinal fields on second harmonic generation in lithium niobate nanopillars

An optimized focused ion beam process is used to fabricate micrometer-long LiNbO3 nanopillars with diameters varying between 150 and 325 nm. Polarimetric mappings of second harmonic generation from a wavelength of 850 nm demonstrate the ability to modify the polarization features of the nonlinear response through a fine adjustment of the pillar size. The effect is ascribed to the non-negligible contribution of the longitudinal fields associated with sub-wavelength light confinement in the LiNbO3 nanopillars. The results also highlight the importance of a fine control over the nanopillar size in order to effectively engineer their nonlinear response.

Sub-Wavelength Dual Capillaries-Assisted Chalcogenide Optical Fibers: Unusual Modal Properties in Mid-IR (2–5 μm) Spectral Range

In this study, we apply the concept of sub-wavelength light confinement to achieve flat effective mode area ( $A_{{\rm eff}}$ ) characteristics over a wide wavelength range of 1400 nm in nano-sized dual capillary assisted chalcogenide core optical fibers. An unusual spectral behavior of $A_{{\rm eff}}$ is observed where the effective mode area increases, remains constant for a wide bandwidth, decreases and again increases with the increase in wavelength. The spectral region, in which this behavior is observed, can be tuned by varying the structural parameters of the fiber. Additionally, we noticed that the fiber exhibits four zero dispersion wavelengths for a particular polarization which suggests that sub-wavelength light localization can be an alternative solution for the dispersion engineering in order to attain multiple zero dispersion wavelengths. The fabrication tolerance of the dispersion profile has been found to fall within the current fabrication accuracies achievable. We believe that our findings might be useful in different applications such as light-matter interaction and spatial soliton propagation.

Photonic nanojet assisted enhancement in transmission of light through hollow pyramid shaped near field probes

We report the use of sub-wavelength confinement of light using dielectric microspheres for enhancing transmission through the cantilever-based hollow probes used in a near-field scanning optical microscope. With an appropriate choice of the dielectric microsphere, an order of magnitude enhancement was achieved in transmission through the probe. In addition, transmission through such a tip was also found to be less sensitive to the axial and lateral offset between the beam waist and symmetry axis of the probe tip.

Active hyperbolic metamaterials: enhanced spontaneous emission and light extraction

Hyperbolic metamaterials (HMMs) have recently garnered much attention because they possess the potential for broadband manipulation of the photonic density of states and subwavelength light confinement. These exceptional properties arise due to the excitation of electromagnetic states with high momentum (high-k modes). However, a major hindrance to practical applications of HMMs is the difficulty in coupling light out of these modes because they become evanescent at the surface of the metamaterial. Here we report the first demonstration, to our knowledge, of simultaneous spontaneous emission enhancement and outcoupling of high-k modes in an active HMM using a high-index-contrast bullseye grating. Quantum dots embedded inside the metamaterial are used for local excitation of high-k modes. This demonstration could pave the way for the development of photonic devices such as single-photon sources, ultrafast LEDs, and true nanoscale lasers.

Ultrastrong coupling in the near field of complementary split-ring resonators

The ultrastrong light-matter interaction regime was investigated in metallic and superconducting complementary split ring resonators coupled to the cyclotron transition of two dimensional electron gases. The sub-wavelength light confinement and the large optical dipole moment of the cyclotron transition yield record high normalized coupling rates of up to $\frac{\Omega_R}{\omega_c}=$ 0.87. We observed a blue-shift of both polaritons due to the diamagnetic term of the interaction Hamiltonian.

Integrated Grating-Nanoslot Probe Tip for Near-Field Subwavelength Light Confinement and Fluorescent Sensing

We demonstrate a near-field sub-wavelength light confinement probe tip comprised of compact embedded metallic focus grating (CEMFG) coupler and photonic crystal (PhC) based λ/4 nano-slot tip, in terms of its far-field radiation directivity and near-field sub-wavelength light enhancement. The embedded metallic grating coupler increases the free space coupling at tilted coupling angle of 25° with over 280 times light intensity enhancement for 10 μm coupler size. Further, 20 nm air slot embedded in single line defect PhC waveguide are designed, using the impedance matching concept of the λ/4 “air rod”, to form the TE mode light wave resonance right at the probe tip aperture opening. This leads to the light beam spot size reduction down to λ/20. The near-field center peak intensity is enhanced by 4.2 times from that of the rectangular waveguide input, with the total enhancement factor of 1185 from free space laser source intensity. The near-field fluorescence excitation and detection also demonstrate its single molecular enhanced fluorescence measurement capability.

Subwavelength light confinement and propagation: A numerical study of a two-layer silver film with perforated holes

Confinement and propagation of light under the diffraction limit is a substantial challenge for the development of waveguides as components in subwavelength optical devices. Light confinement and propagation at optical frequencies in a two-layer silver film with a periodic array of holes is investigated in a numerical study using the discrete dipole approximation method. Extraordinary subwavelength confinement and propagation of light can be obtained along an extremely subwavelength cross section of a region as small as 10 × 20 nm2 at a distance of over 10 μm. This study provides rational design of waveguides under subwavelength dimensions.

Analog of gravitational force in hyperbolic metamaterials

Subwavelength confinement of light in nonlinear hyperbolic metamaterials due to formation of spatial solitons has attracted much recent attention because of its seemingly counterintuitive behavior. In order to achieve self-focusing in a hyperbolic wire medium, a nonlinear self-defocusing Kerr medium must be used as a dielectric host. Here we demonstrate that this behavior finds a natural explanation in terms of the analog of gravity. A wave equation describing the propagation of extraordinary light inside hyperbolic metamaterials exhibits (2+1)-dimensional Lorentz symmetry. The role of time in the corresponding effective three-dimensional Minkowski space-time is played by the spatial coordinate aligned with the optical axis of the metamaterial. Nonlinear optical Kerr effect ``bends'' this space-time resulting in effective gravitational force between extraordinary photons. In order for the effective gravitational constant to be positive, a negative self-defocusing Kerr medium must be used as a host. If gravitational self-interaction is strong enough, the spatial soliton may collapse into a black hole analog.

Quantum interference in plasmonic circuits

Surface plasmon polaritons (plasmons) are a combination of light and a collective oscillation of the free electron plasma at metal/dielectric interfaces. This interaction allows subwavelength confinement of light beyond the diffraction limit inherent to dielectric structures. As a result, the intensity of the electromagnetic field is enhanced, with the possibility to increase the strength of the optical interactions between waveguides, light sources and detectors. Plasmons maintain non-classical photon statistics and preserve entanglement upon transmission through thin, patterned metallic films or weakly confining waveguides. For quantum applications, it is essential that plasmons behave as indistinguishable quantum particles. Here we report on a quantum interference experiment in a nanoscale plasmonic circuit consisting of an on-chip plasmon beamsplitter with integrated superconducting single-photon detectors to allow efficient single plasmon detection. We demonstrate a quantum-mechanical interaction between pairs of indistinguishable surface plasmons by observing Hong-Ou-Mandel (HOM) interference, a hallmark non-classical interference effect that is the basis of linear optics-based quantum computation. Our work shows that it is feasible to shrink quantum optical experiments to the nanoscale and offers a promising route towards subwavelength quantum optical networks.

Low-loss hybrid plasmonic modes guided by metal-coated dielectric wedges for subwavelength light confinement

The optical characteristics of a metal-coated dielectric wedge structure are investigated at a wavelength of 1550 nm. The effects of the metal/gap layers' thicknesses, as well as the dimension of the dielectric wedge on the guided modes' properties, are systematically analyzed. It is revealed that the characteristics of the fundamental quasi-TE and quasi-TM plasmonic modes supported by the configuration demonstrate similar trends against the variation of the metal layer thickness while exhibiting quite different behaviors with the change of the wedge size. By choosing appropriate physical dimensions, both modes could simultaneously achieve low modal loss and subwavelength field confinement, along with reasonable mode power inside the low-index gap region. Investigations on the directional coupling between adjacent identical waveguides indicate that ultralow crosstalk can be enabled by the quasi-TE mode, with the coupling length more than two orders of magnitude larger than that achieved by the plasmonic mode in conventional hybrid counterparts. The presented metal-coated dielectric wedge structures can be employed as important building blocks for a number of integrated nanophotonic components, and could also enable numerous applications at the subwavelength scale.

Manipulation of light in MIM plasmonic waveguide systems

Plasmonic waveguides that allow deeply subwavelength confinement of light provide an effective platform for the design of ultra-compact photonic devices. As an important plasmonic waveguide, metal-insulator-metal (MIM) structure supports the propagation of light in the nanoscale regime at the visible and near-infrared ranges. Here, we focus on our work in MIM plasmonic waveguide devices for manipulating light, and review some of the recent development of this topic. We introduce MIM plasmonic wavelength filtering and demultiplexing devices, and present the electromagnetic induced transparency (EIT)-like and Fano resonance effects in MIM waveguide systems. The slow-light and rainbow trapping effects are demonstrated theoretically. These results pave a way toward dynamic control of the special and useful optical responses, which actualize some new plasmonic waveguide-integrated devices such as nanoscale filters, demultiplexers, sensors, slow light waveguides, and buffers.