Modern communications have created a great demand of magneto-dielectric functional materials having low loss and high permeability properties under the sub-6 GHz band. CoZn-18H planar hexagonal ferrites with strong magnetic anisotropy are more promising in meeting these requirements than that of traditional ferrites. The textured CoZn-18H hexagonal ferrites were synthesized by the reactive templated grain growth (RTGG) method to obtain high magnetic resonance frequency without sacrificing permeability. The layered texture composed of flaky hexagonal particles with a high aspect ratio played an important role in obtaining high permeability and high magnetic resonance frequency. The permeability μ′, magnetic loss tangent tan δμ, and performance factor (PF) of the textured CoZn-18H hexagonal ferrite with the highest Snoek’s product (SP = 6.99 GHz) under 3.41 GHz were 1.66, 0.10, and 56.61 GHz, respectively. Compared with the traditional pure dielectric substrate, a planar inverted F antenna (PIFA) working at 3.0 GHz with a miniaturization rate of 18.1 % was simulated based on the textured CoZn-18H hexagonal ferrite. These results demonstrated that the method of preparing textured CoZn-18H hexagonal ferrites without the application of a magnetic field was effective and revealed the potential of textured planar hexagonal ferrites synthesized by the RTGG method of high-frequency and low-loss applications.
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