ABSTRACTThe fracture toughness properties, in terms of stress intensity factor KIc and strain energy release rate GIc, of hemp fibre mat-reinforced sheet moulding compound (H-SMC) are measured using the compact tension (CT) method and compared with those of glass fibre-reinforced SMC (G-SMC). Three material parameters were considered for composite optimisation: fibre volume fraction, CaCO3 filler content and hemp fibre surface treatments using either alkaline, silane or a combination of these two treatments. The highest fracture toughness for H-SMC composites was obtained at a fibre loading of around 30 vol.-%, while it was also shown that the fracture toughness properties of H-SMC are sensitive to mineral filler content. Surface treatment of the hemp fibres using a combined alkaline-silane treatment resulted in a significant improvement in fracture toughness of H-SMC composites. Optimised H-SMC composites exhibited fracture toughness properties similar to those of G-SMC at fibre contents of 20 vol.-%, with KIc values of around 6 MPa.m−1/2.