Spontaneous Parametric Down-conversion Process Research Articles

Selective tuning of Hilbert spaces in states encoded with spatial modes of light

Spatial modes of light directly give the most easily accessible degree of freedom that span an infinite dimensional Hilbert space. The higher dimensional spatial mode entanglement realized using spontaneous parametric down conversion (SPDC) process is generally restricted to the subspace defined by a single spatial mode in pump. Access to other modal subspaces can be realized by pumping beams carrying several easily tunable transverse modes. As a proof of principle experiment, we generate twin-photon states in an SPDC process with pump as a superposition of first order Laguerre–Gaussian (or Hermite–Gaussian) modes. We show that the generated states can be easily tuned between different subspaces by controlling the respective modal content in the pump superposition.

Amplification of polarization correlations in Compton scattering of hard x-ray Bell states

The theoretical cross section for Compton scattering of maximally entangled Bell photons has yet to be rigorously confirmed by experiments. Test cases of Bell states for use in Compton scattering experiments can now be expanded given reports of creating all 4 Bell states in the hard x-ray regime by the process of spontaneous parametric down-conversion. We outline an experiment and apply a matrix method to parameterize Compton scattering theory using the phase matching angles. When the azimuths of two hypothetical photon counters are recorded at angles of 0 degrees and 90 degrees, and the ratio of their counting rates determined, azimuthal ratios are expected to be 600 times larger compared to 511 keV Bell photons.

Generation of narrowband counterpropagating polarization-entangled photon pairs based on thin-film lithium niobate on insulator

We propose a scheme for the generation of counterpropagating polarization-entangled photon pairs from a periodically poled lithium niobate on insulator waveguide. The waveguide is designed to enable a special dispersion relationship between the T M 00 and T E 00 modes that allows two concurrent counterpropagating quasi-phase-matching type-II spontaneous parametric downconversion processes with a single reciprocal wave vector. Due to the counterpropagating phase-matching geometry, the source has a narrow bandwidth in the order of several gigahertz. The compact source opens up a new method for integrated photonic technologies.

Experimental demonstration of hidden nonlocality with local filters.

The violation of the Bell inequalities implies that quantum mechanics cannot be interpreted using any local hidden variable theory. However, particular quantum states that can originally be described using a local hidden variable model surprisingly exhibit nonlocality by employing local filters before a standard Bell test is performed. This is referred to as hidden nonlocality. In this study, we provide the experimental demonstration of hidden nonlocality through linear optics towards the local states which are put forword by Hirsch et al., PRL 111, 160402 (2013). A class of local states is generated through a spontaneous parametric down-conversion process, and the violation of the Clauser-Horne-Shimony-Holt (CHSH)-Bell inequality is observed by applying local filters. Our experimental results confirm the superiority of local filters, and throw light on deep understanding the intriguing phenomena of hidden nonlocality and local states.

Continuous-variable Bell nonlocality with biphotons produced by spontaneous parametric down-conversion

We revisit a continuous-variable version of the Clauser-Horne-Shimony-Holt inequality with sign binning, first proposed by Bell [J. S. Bell, Speakable and Unspeakable in Quantum Mechanics, 1st ed. (Cambridge University, New York, 1987); Ann. N.Y. Acad. Sci. 480, 263 (1986)]. To explore Bell nonlocality, we use a biphoton effective wave function resulting from a type-I spontaneous parametric down-conversion process. After reviewing the approximations involved in the production and time evolution of such biphotons, we judiciously choose a series expansion for the sinc function part of the biphoton wave function in order to integrate the Wigner function. We conclude that we can qualitatively achieve Bell nonlocality within a regime in which the twin photons are described.

Characterization of spectrally filtered heralded single photons

One method to produce pure heralded single photons (HSP) when using the optical process of spontaneous parametric down-conversion (SPDC) is by modifying the joint spectrum of the photon pairs by means of spectral filters. In this work, we characterize the dependence, with the bandwidth of such filters, of the spectral purity and heralding efficiency of the HSP generated in a bulk SPDC. The values we report for the purity and heralding efficiency are obtained from measurements of the joint spectrum. Our results are in agreement with the theoretical model that predicts a trade-off between the purity and heralding efficiency, and they complement similar measurements that have been done for HSP produced by other types of sources.

Inherent resolution limit on nonlocal wavelength-to-time mapping with entangled photon pairs.

Nonlocal wavelength-to-time mapping between frequency-entangled photon pairs generated with the process of spontaneous parametric down-conversion is theoretically analyzed and experimentally demonstrated. The spectral filtering pattern experienced by one photon in the photon pair will be non-locally mapped into the time domain when the other photon propagates inside a dispersion-compensation fiber with large group velocity dispersion. Our work, for the first time, points out that the spectral bandwidth of the pump laser will become the dominated factor preventing the improvement of the spectral resolution when the involved group velocity dispersion is large enough, which provides an excellent tool for characterizing the resolution of a nonlocal wavelength-to-time mapping for further quantum information applications.

Pancharatnam-Berry geometric phase memory based on spontaneous parametric down-conversion.

Phase memory is an effect in which the interaction between a coherent pump beam and a nonlinear crystal generates photon pairs via the spontaneous parametric down-conversion process, then the down-converted photons (signal and idler) can carry the phase information of the pump beam. There has been much research on the memory of the dynamic phase so far; however, there is no report on the memory of non-dynamic phase, to the best of our knowledge. Here we acquire a Pancharatnam-Berry (PB) geometric phase in a physical system when light travels along a trajectory in polarization-state space. Induced coherence occurs in a cascaded scheme composed of two nonlinear crystals, when the idler photons in both crystals are aligned to be indistinguishable. A NOON ($N\; = \;{2}$N=2) state is established when blocking the two idler photons. We explore the PB geometric phase memory of the NOON state and induced coherence. We find that the first-order interference of the two-photon state or signal photons can be controlled by introducing the PB geometric phase to the pump light. This may facilitate precise control of the phase of the down-converted photons.

Compact polarization-entangled photon-pair source based on a dual-periodically-poled Ti:LiNbO3 waveguide.

We present an experimental realization of a compact and reliable way to build a nondegenerate polarization-entangled photon-pair source based on a dual-periodically-poled $ {\rm Ti}:{{\rm LiNbO}_3} $Ti:LiNbO3 waveguide, which is in the telecommunication window and compatible with the fiber quantum networks. The dual-periodic structure allows two inherently concurrent quasiphase-matching spontaneous parametric down-conversion processes pumped by a single laser beam, hence enabling our source to be compact and stable. We show that our source has a high brightness of $ B = 1.22{\rm } \times {\rm }{10^7}\;{\rm pairs}/(\rm s \times mW \times nm) $B=1.22×107pairs/(s×mW×nm). With quantum state tomography, we estimate an entanglement fidelity of $ 0.945 \pm 0.003 $0.945±0.003. A violation of Clauser-Horne-Shimony-Holt inequality with $ S = 2.75 \pm 0.03 $S=2.75±0.03 is also demonstrated.

A simple technique for measuring the spatial correlation of photon pairs for complete interference in the Michelson interferometer

In this research, a simple technique for measuring the spatial correlation or angular correlation of photon pairs was developed. The system consisted of two aluminium rails which had the same pivot at the position of a nonlinear crystal. The rails were manually moved to find the position of the correlated photon pairs. At this position, the photon pairs were collected by the collimators attached at the end of the rails. The pairs were produced by type I spontaneous parametric down-conversion process using a 405 nm diode laser and a BBO crystal. The crystal was specifically cut for emitting the photon pairs at an angle of 3° with respect to the direction of the pump laser. These pairing photons were correlated and interfered in the Michelson interferometer, then, the correlated photons were demonstrated. It was found that the visibilities in the case of perfect alignment, near perfect alignment and misalignment were V = 1.0000 ± 0.0004, 0.869 ± 0.002, 0.591 ± 0.002 and 0.168 ± 0.002, respectively.

Experimental observation of quantum contextuality beyond Bell nonlocality

Bell nonlocality and quantum contextuality are two important resources which, however, behave very differently in many tasks where the quantum correlation has an edge over its classical counterpart. In this work, we directly compare these two behaviors, which via the Cabello-Severini-Winter graph-theoretical approach, can be associated with a same exclusivity graph. In particular, we consider the exclusivity graph that leads to ${I}_{3322}$-type inequalities in the Bell and the contextual scenarios, respectively. We find that maximal violation of Bell inequality is around 6.251, and maximal violation of the noncontextuality inequality is around 6.588 for a five-dimensional system and 6.571 for a four-dimensional system, respectively. The results predict a gap of $\mathrm{\ensuremath{\Delta}}\ensuremath{\approx}0.32$ between quantum contextuality and Bell nonlocality. We then present an experimental observation of the gap by employing both the maximally entangled photon pairs from the spontaneous parametric down-conversion process and the single photons encoded into qudits from an intrinsic defect in gallium nitride. Our results will further deepen the understanding of different types of quantum correlations.

Temporally Correlated Narrowband Biphoton Interference Based on Mach–Zehnder Interferometer

AbstractSince early 1990s, Mach–Zehnder interferometer has been used to investigate the interference of biphoton wave packets. Due to subpicosecond time coherence of biphoton generated by spontaneous parametric downconversion process, some physical processes are ignored in the interferometer, most likely the biphoton time‐domain interference. Here, the two‐photon interference phenomenon based on the Mach–Zehnder interferometer is theoretically studied, where the correlated photon pairs are produced by the four‐wave mixing in atomic system. In particular, the quantum interference effect to effectively control the coherent time of two‐photon by adjusting the input delay is used. In the damped Rabi oscillation regime, two‐photon bunching and antibunching effects are observed. In addition, in the group‐delay regime, the interference between biphoton precursor, slow‐light wave packets and also in between the precursor and the slow‐light wave packets is observed, which had never been reported before. These results may have potential applications in the fields of biphoton shaping and quantum information processing.

Storage of telecom-C-band heralded single photons with orbital-angular-momentum encoding in a crystal

A memory-based quantum repeater architecture provides a solution to distribute quantum information to an arbitrary long distance. Practical quantum repeaters are likely to be built in optical-fiber networks which take advantage of the low-loss transmission between quantum memory nodes. Most quantum memory platforms have characteristic atomic transitions away from the telecommunication band. A nondegenerate photon pair source is therefore useful for connection of a quantum memory to optical fibers. Here, we report a high-brightness narrowband photon-pair source which is compatible with a rare-earth-ion-doped crystal Pr3+:Y2SiO5. The photon-pair source is generated through a cavity-enhanced spontaneous parametric down-conversion process with the signal photon at 606 nm and the idler photon at 1540 nm. Moreover, using the telecom C-band idler photons for heralding, we demonstrate the reversible transfer of orbital-angular-momentum qubit between the signal photon and the quantum memory based on Pr3+:Y2SiO5.

CNOT-based quantum swapping of polarization and modal encoded qubits in photonic Ti:LiNbO3 channel waveguides

A photonic circuit aimed at implementing a CNOT-based quantum swapping of the modal and polarization qubits, is designed and simulated, using Ti:LiNbO3 indiffused channel waveguides. A few on-chip optical elements such as the polarization-sensitive odd-mode analyzers and combiners, along with the electrically controllable directional couplers and polarization converters, are incorporated within the circuit and together serve to realize the operation of a deterministic single-photon quantum swap gate. Entanglement generation is realized on-chip by means of two concurrent spontaneous parametric down-conversion processes in the twice periodically poled Ti:LiNbO3 waveguide, placed at the input section of the circuit. The constituent elements of the circuit are characterized separately using numerical beam propagation method in RSoft program package. Two poling periods of $$\varLambda_{1} = 11.762\,\upmu{\text{m}}$$ and $$\varLambda_{2} = 23.667\,\upmu{\text{m}}$$ are calculated for the dual periodically perturbed structure in the circuit. The directional couplers operate at $$V_{DC} = 31.6$$ V. Maximum polarization conversion efficiency is achieved by applying a constant switching voltage of $$V_{EO} = 4.52$$ V.

Spatial control of spontaneous parametric down-conversion photon pairs through the use of apertured Bessel-Gauss pump beams

We demonstrate, both experimentally and theoretically, a method that allows us to modify the spatial properties of photon pairs produced by the process of spontaneous parametric down-conversion (SPDC) with an apertured, zeroth-order Bessel-Gauss beam. Concentrating on the use of a half-plane aperture, we show that the phase-matching conditions for non-paraxial pump beams can be controlled by simply changing the aperture orientation. Partially blocking the pump beam, leads to a selection of either one of two individual cones that form a dual-cone SPDC angular spectrum, or a portion of both of them. We can likewise determine the shape and orientation of the conditional angular spectrum. This control of the SPDC spatial properties could be useful for quantum information processing protocols.

Engineering quantum correlations for m×n spatially encoded two-photons states

Discretizing transverse linear momentum of photon pairs, generated by spontaneous parametric down conversion (SPDC), is one of the simplest methods for producing bipartite entangled states in high dimensions. So far, it has been employed only to prepare states in dimensions $m\ifmmode\times\else\texttimes\fi{}m$. In this work, we study the generalization for engineering entangled states in dimensions $m\ifmmode\times\else\texttimes\fi{}n$. Our approach relies on the manipulation of the pump beam transverse profile and the phase-matching function of the SPDC process to prepare, behind an $m$- and $n$-slit aperture, different $m\ifmmode\times\else\texttimes\fi{}n$ spatial entangled states. We demonstrate the technique experimentally for some $2\ifmmode\times\else\texttimes\fi{}3$ states. Compared to previous approaches in producing $2\ifmmode\times\else\texttimes\fi{}n$ photonic entanglement, which require either more than two photons or hybrid entanglement, our scheme is less demanding and simpler since we employ only two photons and a single degree of freedom to encode the states.

Experimental realization of more quantum randomness generation based on non-projective measurement

Quantum random numbers are fundamental resources (Rev. Mod. Phys. 89 015004) for the fields of communications and information security. Usually, projective measurements can be applied on a two-qubit entangled state to generate quantum random numbers. However, it cannot certify more than one bit of randomness for one set of measurements. On contrast, non-projective measurements in-principle may be able to generate more random bits, and therefore show some merits among present methods. Here, we report the implementation of a quantum random number generator based on a symmetric informationally complete positive operator-valued measure. In our experiment, we prepare a maximally entangled state of two-qubits through spontaneous parametric down-conversion processes, and observe the violation of Gisin’s elegant Bell inequality with the value of 6.8138 ± 0.0822, exceeding the classical bound of 6. Through randomness extractors, including a Toeplitz extractor and a parallel linear feedback shift register based extractor, we finally extract a random string with an autocorrelation coefficient below 10−3 and the string can pass all randomness tests of the National Institute of Science and Technology (NIST).

Interference effects in quantum-optical coherence tomography using spectrally engineered photon pairs

Optical-coherence tomography (OCT) is a technique that employs light in order to measure the internal structure of semitransparent, e.g. biological, samples. It is based on the interference pattern of low-coherence light. Quantum-OCT (QOCT), instead, employs the correlation properties of entangled photon pairs, for example, generated by the process of spontaneous parametric downconversion (SPDC). The usual QOCT scheme uses photon pairs characterised by a joint-spectral amplitude with strict spectral anti-correlations. It has been shown that, in contrast with its classical counterpart, QOCT provides resolution enhancement and dispersion cancellation. In this paper, we revisit the theory of QOCT and extend the theoretical model so as to include photon pairs with arbitrary spectral correlations. We present experimental results that complement the theory and explain the physical underpinnings appearing in the interference pattern. In our experiment, we utilize a pump for the SPDC process ranging from continuous wave to pulsed in the femtosecond regime, and show that cross-correlation interference effects appearing for each pair of layers may be directly suppressed for a sufficiently large pump bandwidth. Our results provide insights and strategies that could guide practical implementations of QOCT.

Spatially entangled photon-pair generation using a partial spatially coherent pump beam

We demonstrate experimental generation of spatially-entangled photon-pairs by spontaneous parametric down conversion (SPDC) using a partial spatially coherent pump beam. By varying the spatial coherence of the pump, we show its influence on the downconverted photon's spatial correlations and on their degree of entanglement, in excellent agreement with theory. We then exploit this property to produce pairs of photons with a specific degree of entanglement by tailoring of the pump coherence length. This work thus unravels the fundamental transfer of coherence occuring in SPDC processes, and provides a simple experimental scheme to generate photon-pairs with a well-defined degree of spatial entanglement, which may be useful for quantum communication and information processing

Multi-Path Ghost Imaging by Means of an Additional Time Correlation**Supported by the National Key R&D Program of China under Grant Nos 2017YFA0303800 and 2017YFA0303700, the National Natural Science Foundation of China under Grant Nos 11534006, 11774183 and 11674184, and the Collaborative Innovation Center of Extreme Optics.

Ghost imaging functions achieved by means of the spatial correlations between two photons is a new modality in imaging systems. With a small number of photons, ghost imaging is usually realized based on the position correlation of photon pairs produced from the spontaneous parametric down-conversion process. Here we demonstrate a way to realize multi-path ghost imaging by introducing an additional time correlation. Different delays of paths will induce the shift of the coincidence peak, which carries the information about objects. By choosing the suitable coincidence window, we obtain images of three objects simultaneously, with a visibility of 87.2%. This method provides insights and techniques into multi-parameter ghost imaging. It can be applied to other correlated imaging systems, for example, quantum spiral imaging.