Spontaneous Emission Free-electron Laser Research Articles

Generation of Ultrashort Pulses in XUV and X-ray FELs via an Excessive Reverse Undulator Taper

The pulse duration in short-pulse schemes for Self-Amplified Spontaneous Emission Free Electron Lasers (SASE FELs) is limited by the FEL coherence time. A recently proposed concept allows to overcome the coherence time barrier and to obtain much shorter pulses. When the lasing part of an electron bunch is much shorter than the coherence time, one can suppress the radiation in the long main undulator while preserving microbunching within that short lasing slice. Then, a short radiation pulse is produced in a relatively short radiator. A possible suppression method, an excessive reverse undulator taper, is discussed and illustrated numerically in this paper. We also performed the first experimental tests of this method at the soft X-ray FEL user facility FLASH. The measured pulse duration approaches 1 fs (FWHM) at the wavelength of 5 nm.

Differential Measurement of Electron Ejection after Two-Photon Two-Electron Excitation of Helium.

We report the measurement of the photoelectron angular distribution of two-photon single-ionization near the 2p^{2} ^{1}D^{e} double-excitation resonance in helium, benchmarking the fundamental nonlinear interaction of two photons with two correlated electrons. This observation is enabled by the unique combination of intense extreme ultraviolet pulses, delivered at the high-repetition-rate free-electron laser in Hamburg (FLASH), ionizing a jet of cryogenically cooled helium atoms in a reaction microscope. The spectral structure of the intense self-amplified spontaneous emission free-electron laser pulses has been resolved on a single-shot level to allow for post selection of pulses, leading to an enhanced spectral resolution, and introducing a new experimental method. The measured angular distribution is directly compared to state-of-the-art theory based on multichannel quantum defect theory and the streamlined R-matrix method. These results and experimental methodology open a promising route for exploring fundamental interactions of few photons with few electrons in general.

Application of a modified chirp-taper scheme for generation of attosecond pulses in extreme ultraviolet and soft x-ray free electron lasers

Typically, in Self-Amplified Spontaneous Emission Free Electron Laser (SASE FEL) based short-pulse schemes, pulse duration is limited by FEL coherence time. For hard X-ray FELs, coherence time is in a few hundred attosecond range while for XUV and soft X-ray FELs it is in the femtosecond regime. In this paper the modification of so-called chirp-taper scheme is developed that allows to overcome the coherence time barrier. Numerical simulations for XUV and soft X-ray FEL user facility FLASH demonstrate that one can generate a few hundred attosecond long pulses in the wavelength range 2 - 10 nm with peak power reaching hundreds of megawatts. With several thousand pulses per second this can be a unique source for attosecond science.

Construction and commissioning of mid-infrared self-amplified spontaneous emission free-electron laser at compact energy recovery linac.

The mid-infrared range is an important spectrum range where materials exhibit a characteristic response corresponding to their molecular structure. A free-electron laser (FEL) is a promising candidate for a high-power light source with wavelength tunability to investigate the nonlinear response of materials. Although the self-amplification spontaneous emission (SASE) scheme is not usually adopted in the mid-infrared wavelength range, it may have advantages such as layout simplicity, the possibility of producing a single pulse, and scalability to a short-wavelength facility. To demonstrate the operation of a mid-infrared SASE FEL system in an energy recovery linac (ERL) layout, we constructed an SASE FEL setup in cERL, a test facility of the superconducting linac with the ERL configuration. Despite the adverse circumstance of space charge effects due to the given boundary condition of the facility, we successfully established the beam condition at the undulators and observed FEL emission at a wavelength of 20 μm. The results show that the layout of cERL has the potential for serving as a mid-infrared light source.

Beam dynamic studies at accelerator system of gun for a self-amplified spontaneous emission free electron laser project

One of the important factors in high radiation generation facilities is the production of a high quality electron beam. To do that, the requirements of an optical electron source, such as current, radiation emission, etc. must be met. For this purpose, cavity beam dynamics studies of 1.4, 1.5, 1.6 and 1.8-cell SRF gun were performed. In addition, detailed studies have been made on the solenoid design and the location of the solenoid along the beam path. A design with the most optimized cavity geometry and RF fields for the gun cavity was posed. The injector system was designed for the Turkish SASE-FEL project with cavities of many different geometrical sizes. The most efficient high energy cavity system is determined as 1.6-cell cavity. The emittance value of the beam was achieved as 1.76±0.42π mm mrad and the beam energy reached at the end of cavity was obtained as 3.5MeV.

Revision of optical klystron enhancement effects in self-amplified spontaneous emission free electron lasers

We review the theory of optical klystrons, with its applications for self-amplified spontaneous emission free electron lasers in mind. We show that previous theories miss terms in the power gain factor that cannot be neglected, and we illustrate differences between the previously known analytical expressions, new ones found in this paper, and numerical calculations. We then consider the use of optical klystrons for electron energy-spread and radiation coherence-time diagnostics purposes.

Wigner distribution of self-amplified spontaneous emission free-electron laser pulses and extracting its autocorrelation.

The emerging concept of `beam by design' in free-electron laser (FEL) accelerator physics aims for accurate manipulation of the electron beam to tailor spectral and temporal properties of the radiation for specific experimental purposes, such as X-ray pump/X-ray probe and multiple wavelength experiments. `Beam by design' requires fast, efficient, and detailed feedback on the spectral and temporal properties of the generated X-ray radiation. Here a simple and cost-efficient method to extract information on the longitudinal Wigner distribution function of emitted FEL pulses is proposed. The method requires only an ensemble of measured FEL spectra and is rather robust with respect to accelerator fluctuations. The method is applied to both the simulated SASE spectra with known radiation properties as well as to the SASE spectra measured at the European XFEL revealing underlying non-linear chirp of the generated radiation. In the Appendices an intuitive understanding of time-frequency representations of chirped SASE radiation is provided.

Refractive Guide Switching a Regenerative Amplifier Free-Electron Laser for High Peak and Average Power Hard X Rays.

We present an x-ray regenerative amplifier free-electron laser design capable of producing fully coherent hard x-ray pulses across a broad tuning range at a high steady state repetition rate. The scheme leverages a strong undulator taper and an apertured diamond output-coupling cavity crystal to produce both high peak and average spectral brightness radiation that is 2 to 3 orders of magnitude greater than conventional single-pass self-amplified spontaneous emission free-electron laser amplifiers. Refractive guiding in the postsaturation regime is found to play a key role in passively controlling the stored cavity power. The scheme is explored both analytically and numerically in the context of the Linac Coherent Light Source II High Energy upgrade.

Slice collective dynamics, projected emittance deterioration and free electron laser performances detrimental effects

Self-amplified spontaneous emission (SASE) free electron laser (FEL) devices have disclosed an unexpected interplay between the laser intensity growth and regions of the electron bunch of the order of the coherence length. They are usually identified with the bunch slice and contribute to the laser dynamics with their own characteristics. The dynamical effects inducing geometrical and phase space misalignment of bunch slice in X-ray operating FELs can be traced back to a plethora of phenomena, both in the Linac accelerating section or inside the beam transport optic magnet. They are responsible for spoiling of the beam projected qualities and, if not corrected properly, induce an increase of the saturation length and a decreasing of the output power. We discuss the inclusion of these effects in models employing scaling formulae.

Design of an online spectrometer for the diagnosis of free-electron lasers.

A self-amplified spontaneous emission free-electron laser (FEL) is under construction at the Shanghai Soft X-ray Free-Electron Facility. Therefore, it is necessary to develop a suitable diagnostic tool capable of resolving the natural emission band of each FEL pulse. Thus, an online spectrometer with a plane mirror and plane variable-line-spacing grating at grazing incidence to monitor each single FEL pulse during the propagation of FEL radiation has been designed and is presented in this work. The method of ray tracing is used for monitoring incident radiation in order to understand spectral characteristics, and SHADOW, an X-ray optics simulation tool, and SRW, an X-ray optics wavefront tool, are applied to study the resolving power and focusing properties of the grating. The designed resolving power is ∼3 × 104 at 620 eV. Meanwhile, the effect of the actual slope error of mirrors on the ray-tracing results is also discussed. In order to provide further optimization for the choice of grating, a comparison of resolving powers between 2000 lines mm-1 and 3000 lines mm-1 gratings at different energies is analyzed in detail and radiation damage of mirrors as well as parameters such as the first-order diffraction angle β, the exit-arm length r2, and the tilt angle θ between the focal plane and the diffraction arm are studied and optimized. This work has provided comprehensive designing methods and detailed data for the design of diagnostic spectrometers in soft X-ray FELs and will be favorable to the design of other similar instruments.

A hard X-ray self-amplified spontaneous emission free-electron laser optimizationusing evolutionary algorithms for dedicated user applications

Accelerator-based fourth-generation light sources are utilized in a wide range of interdisciplinary applications such as nanotechnology, materials science, biosciences, and medicine. A hard X-ray free-electron laser (FEL), as a state-of-the-art light source, was optimized using evolutionary algorithms for dedicated user applications such as X-ray Raman scattering (XRS), resonant inelastic X-ray scattering (RIXS), and X-ray emission spectroscopies (XES). Optimal parameter sets were obtained for an in-vacuum planar undulator driven by an 8 GeV electron beam. Performance parameters of self-amplified spontaneous emission (SASE) operation (i.e. optimized SASE performance parameters through evolutionary algorithms) were found to be consistent with operating X-ray FEL facilities around the world. It is shown that FEL characteristics for specific user experiments can be optimized by finding several evolutionary algorithm solutions within the range of 5 keV to 10 keV.

The detuning effect of crystal monochromator in self-seeding and oscillator free electron laser.

Self-amplified spontaneous emission (SASE) free electron laser (FEL) is capable of generating ultra-short, high power and high brightness X-ray pulses, but its temporal coherence is poor. Self-seeding scheme is an approach to improve the temporal coherence by employing a crystal monochromator. The crystal detuning effect is the phenomenon that the Bragg angle deviates from the middle of the reflection domain due to the refraction effect, and can affect the seed power of hard X-ray self-seeding (HXRSS) FEL. In this paper, we introduce a novel idea to maximize the seed power by tuning the incident angle off the Bragg condition where the Bragg photon energy is corresponding to the central photon energy of the input X-ray pulse. We present the numerical analysis of the detuning effect in different reflecting atomic planes and different asymmetry angles of diamond crystal. Moreover, we analyze how the detuning affects the seed efficiency of HXRSS FEL, and discuss the application to X-ray FEL oscillator (XFELO). We find when the detuning is much smaller than the bandwidth of input X-ray pulse, we can neglect the detuning effect. However, if the detuning is much larger than or comparable with the bandwidth of input X-ray pulse, the detuning effect can not be ignored. This work can give a guidance to HXRSS FEL and XFELO commissioning for high efficiency FEL output.

Generating attosecond x-ray pulses through an angular dispersion enhanced self-amplified spontaneous emission free electron laser

We propose a scheme that can generate attosecond x-ray pulses through an angular dispersion enhanced self-amplified spontaneous emission (ESASE) free electron laser (FEL). In this scheme, an angular dispersion section is implemented into a conventional ESASE set-up, together with a few cycle laser pulse to manipulate the electron beam effectively. During the procedure, the transverse-longitudinal phase space coupling is introduced into the electron beam in addition to the energy modulation and momentum compaction processes. As a result, the peak current of the electron beam will be strengthened significantly within a narrow width of the electron bunch, which can be used to generate ultrashort FEL pulses. Comparing to a conventional ESASE scheme, the proposed scheme can reduce the required modulation laser power by at least one order of magnitude. The signal-to-noise ratio of the final FEL radiation pulses can also be improved. In addition, we discuss the possibility of using this scheme to generate two-pulse two-color x-ray FEL with tunable central wavelengths and time delays for a conceivable x-ray pump/x-ray probe experiment.

Generation of Coherent Radiation in the Near X-Ray Band by a Cascade FEL with a Two-Frequency Undulator

Generation of X-ray radiation in a cascade self-amplified spontaneous emission free-electron laser (SASE FEL) using the harmonics of a two-frequency undulator is studied. The advanced phenomenological model of a one-pass FEL that accounts for the main losses in real FELs is presented: the electron energy spread in the beam, the beam divergence, diffraction, and the fact that emission losses are greater at higher harmonics than in the main frequency range. The FEL mathematical model was performed using the Mathematica software and calibrated within the experiment carried out at the operating SPARC facility via complex three-dimensional numerical simulations. The phenomenological model is used to analyze FEL dynamics for generation of a high-energy X-ray emission at a relatively short length. It is proposed to use a two-frequency undulator for the initial electron grouping and subsequent frequency multiplication in a cascade FEL with higher harmonic amplification (HGHG). The advantages of the two-frequency undulator are presented for electron grouping at higher harmonics of the undulator radiation (UR). The operation of several types of FEL is simulated with amplification of the seed laser wave frequency in two and three cascades to generate the soft X-ray radiation. A seed laser with a wavelength of 11.43 nm corresponding to the peak reflectivity of mirror coatings with MoRu/Be is proposed for generating the intensive X-ray laser radiation with λ ~ 1.27–3.37 nm. Here, the intensive radiation power reaches 50 MW at a length of only 35 meters; the radiation shows good temporal coherence corresponding to the performance of a low-power seed laser with a lower frequency.

Dispersion-Based Fresh-Slice Scheme for Free-Electron Lasers.

The fresh-slice technique improved the performance of several self-amplified spontaneous emission free-electron laser schemes by granting selective control on the temporal lasing slice without spoiling the other electron bunch slices. So far, the implementation has required a special insertion device to create the beam yaw, called a dechirper. We demonstrate a novel scheme to enable fresh-slice operation based on electron energy chirp and orbit dispersion that can be implemented at any free-electron laser facility without additional hardware.

High-Power Femtosecond Soft X Rays from Fresh-Slice Multistage Free-Electron Lasers.

We demonstrate a novel multistage amplification scheme for self-amplified spontaneous-emission free electron lasers for the production of few femtosecond pulses with very high power in the soft x-ray regime. The scheme uses the fresh-slice technique to produce an x-ray pulse on the bunch tail, subsequently amplified in downstream undulator sections by fresh electrons. With three-stages amplification, x-ray pulses with an energy of hundreds of microjoules are produced in few femtoseconds. For single-spike spectra x-ray pulses the pulse power is increased more than an order of magnitude compared to other techniques in the same wavelength range.

Soft X-ray generation in cascade SASE FEL with two-frequency undulator

The generation of soft X-ray radiation in cascade self-amplified spontaneous emission free electron laser (SASE FEL) using harmonics of a two-frequency undulator is studied. An advanced phenomenological model of SASE FEL, accounting for the properties of the undulator and of the electron beam, including major losses, is employed. The account for the beam energy spread, divergence and diffraction is harmonic dependent, which is a step forward from the previous models and phenomenological approach, which consider all the losses independent of the harmonic number. The model is validated with the experimental measurements of the FEL harmonic generation and with relevant three-dimensional numerical simulations. The model is adopted for the description of cascading SASE FELs. With its help the dynamics of high-gain harmonic generation (HGHG) SASE FEL cascades is analyzed to obtain the maximum high harmonic power in the X-ray band with the lowest possible seed frequency and the shortest FEL length. The advantages of the two-frequency undulator for SASE FEL in this context are demonstrated and the possibility of its usage in cascading HGHG SASE FEL is shown. Several types of cascade FELs with two-frequency undulators are simulated. Frequency multiplication in two, three and four stage cascades is introduced to obtain soft X-ray radiation. The possibility of the generation of a powerful radiation, 75 MW at and a lower intensity 3rd harmonic, 100 kW at , is demonstrated in multi-cascade FELs at just 20–35 meters with the seed wavelengths and .

Two-frequency undulator usage in compact self-amplified spontaneous emission free electron laser in Roentgen range

AbstractThe generation of harmonics in two-frequency undulator in a self-amplified spontaneous emission free electron laser (SASE FEL) is studied in order to produce Roentgen radiation in a relatively compact sized installation. The dynamics of SASE FEL is analyzed with the help of the phenomenological model to obtain the maximum of the X-ray high-harmonic power. The model accounts for the properties of the undulator magnetic field and of the electron beam and includes the major sources of losses, such as the electron energy spread, etc. It is compared and calibrated with the existing data on a FEL experiment. The advantages of the two-frequency undulator for Roentgen SASE FEL are demonstrated and the possibility to generate powerful mild Roentgen radiation at already ~25 m length is shown. The evolution of the bunching coefficients for high harmonics is studied together with the evolution of the FEL-induced energy spread. The linear and non-linear regimes are explored for common and for two-frequency undulators The usage of the two-frequency undulator for cascade SASE FEL with high X-ray harmonic power and high-harmonic bunching coefficients with low-induced energy spread is proposed.

Optical Klystron Enhancement to Self Amplified Spontaneous Emission at FERMI

The optical klystron enhancement to a self-amplified spontaneous emission free electron laser has been studied in theory and in simulations and has been experimentally demonstrated on a single-pass high-gain free electron laser, the FERMI FEL-1, in 2014. The main concept consists of two undulators separated by a dispersive section that converts the energy modulation induced in the first undulator in density modulation, enhancing the coherent harmonic generation in the first part of the second undulator. This scheme could be replicated in a multi-stage: the bunching is enhanced after each dispersive section, consistently reducing the saturation length. We have applied the multi-stage optical klystron (OK) scheme on the FEL-2 line at FERMI, whose layout includes three dispersive sections. Optimizing the strength of the dispersions allowed a significant increase of the self-amplified spontaneous emission (SASE) intensity in comparison to a single-stage OK and extending to the soft-X rays the OK enhanced SASE previously demonstrated on FEL-1.

Statistical properties of a free-electron laser revealed by Hanbury Brown–Twiss interferometry

We present a comprehensive experimental analysis of statistical properties of the self-amplified spontaneous emission (SASE) free-electron laser (FEL) FLASH at DESY in Hamburg by means of Hanbury Brown and Twiss (HBT) interferometry. The experiments were performed at the FEL wavelengths of 5.5 nm, 13.4 nm, and 20.8 nm. We determined the 2-nd order intensity correlation function for all wavelengths and different operation conditions of FLASH. In all experiments a high degree of spatial coherence (above 50%) was obtained. Our analysis performed in spatial and spectral domains provided us with the independent measurements of an average pulse duration of the FEL that were below 60 fs. To explain complicated behaviour of the 2-nd order intensity correlation function we developed advanced theoretical model that includes the presence of multiple beams and external positional jitter of the FEL pulses. By this analysis we determined that in most experiments several beams were present in radiating field and in one of the experiments external positional jitter was about 25% of the beam size. We envision that methods developed in our study will be used widely for analysis and diagnostics of the FEL radiation.