Readout Of Spin States Research Articles

Photoelectrical imaging and coherent spin-state readout of single nitrogen-vacancy centers in diamond.

Nitrogen-vacancy (NV) centers in diamond have become an important instrument for quantum sensing and quantum information science. However, the readout of NV spin state requires bulky optical setups, limiting fabrication of miniaturized compact devices for practical use. Here we realized photoelectrical detection of magnetic resonance as well as Rabi oscillations on a single-defect level. Furthermore, photoelectrical imaging of individual NV centers at room temperature was demonstrated, surpassing conventional optical readout methods by providing high imaging contrast and signal-to-noise ratio. These results pave the way toward fully integrated quantum diamond devices.

Error corrected spin-state readout in a nanodiamond

Quantum state readout is a key component of quantum technologies, including applications in sensing, computation, and secure communication. Readout fidelity can be enhanced by repeating readouts. However, the number of repeated readouts is limited by measurement backaction, which changes the quantum state that is measured. This detrimental effect can be overcome by storing the quantum state in an ancilla qubit, chosen to be robust against measurement backaction and to allow error correction. Here, we protect the electronic-spin state of a diamond nitrogen-vacancy center from measurement backaction using a robust multilevel 14N nuclear-spin memory and perform repetitive readout, as demonstrated in previous work on bulk diamond devices. We achieve additional protection using error correction based on the quantum logic of coherent feedback to reverse measurement backaction. The repetitive spin readout scheme provides a 13-fold enhancement of readout fidelity over conventional readout and the error correction a 2-fold improvement in the signal. These experiments demonstrate full quantum control of a nitrogen-vacancy center electronic-spin coupled to its host 14N nuclear spin inside a ~25 nm nanodiamond, creating a sensitive and biologically compatible platform for nanoscale quantum sensing. Our error-corrected repetitive readout scheme is particularly useful for quadrupolar nuclear magnetic resonance imaging in the low magnetic field regime where conventional repetitive readout suffers from strong measurement backaction. More broadly, methods for correcting longitudinal (bit-flip) errors described here could be used to improve quantum algorithms that require non-volatile local memory, such as correlation spectroscopy measurements for high resolution sensing.

Nanoscale Spin Manipulation with Pulsed Magnetic Gradient Fields from a Hard Disc Drive Writer

The individual and coherent control of solid-state based electron spins is important covering fields from quantum information processing and quantum metrology to material research and medical imaging. Especially for the control of individual spins in nanoscale networks, the generation of strong, fast, and localized magnetic fields is crucial. Highly engineered devices that demonstrate most of the desired features are found in nanometer size magnetic writers of hard disk drives (HDD). Currently, however, their nanoscale operation in particular comes at the cost of excessive magnetic noise. Here, we present HDD writers as a tool for the efficient manipulation of single as well as multiple spins. We show that their tunable gradients of up to 100 μT/nm can be used to spectrally address individual spins on the nanoscale. Their gigahertz bandwidth allows one to switch control fields within nanoseconds, faster than characteristic time scales such as Rabi and Larmor periods, spin-spin couplings, or optical transitions, thus extending the set of feasible spin manipulations. We used the fields to drive spin transitions through nonadiabatic fast passages or to enable the optical readout of spin states in strong misaligned fields. Building on these techniques, we further apply the large magnetic field gradients for microwave selective addressing of single spins and show its use for the nanoscale optical colocalization of two emitters.

Enhanced readout of spin states in double quantum dot

We investigate a spin-to-charge conversion mechanism which maps the spin singlet and triplet states to two charge states differing by one electron mediated by an intermediate metastable charge state. This mechanism allows us to observe fringes in the spin-unblocked region beyond the triplet transition line in the measurement of the exchange oscillations between singlet and triplet states in a four-electron double quantum dot. Moreover, these fringes are amplified and π-phase shifted, compared with those in the spin blockade region. Unlike the signal enhancement mechanism reported before which produces similar effects, this mechanism only requires one dot coupling to the lead, which is a commonly encountered case especially in imperfect devices. Besides, the crucial tunnel rate asymmetry is provided by the dependence on spin state, not by the asymmetric couplings to the leads. We also design a scheme to control the amplification process, which enables us to extract the relevant time parameters. This mechanism will have potential applications in future investigations of spin qubits.

Vector Magnetometry Using Silicon Vacancies in4H-SiC Under Ambient Conditions

Point defects in solids promise precise measurements of various quantities. Especially magnetic field sensing using the spin of point defects has been of great interest recently. When optical readout of spin states is used, point defects achieve optical magnetic imaging with high spatial resolution at ambient conditions. Here, we demonstrate that genuine optical vector magnetometry can be realized using the silicon vacancy in SiC, which has an uncommon S=3/2 spin. To this end, we develop and experimentally test sensing protocols based on a reference field approach combined with multi frequency spin excitation. Our works suggest that the silicon vacancy in an industry-friendly platform, SiC, has potential for various magnetometry applications at ambient conditions.

Purcell-enhanced optical spin readout of nitrogen-vacancy centers in diamond

Nitrogen-vacancy (NV) color centers in diamond have emerged as promising quantum solid-state systems, with applications ranging from quantum information processing to magnetic sensing. One of the most useful properties of NVs is the ability to read their ground-state spin projection optically at room temperature. Using theoretical analysis of Purcell-enhanced NV optical coupling, we identify parameters for a significantly enhanced single-to-noise ratio (SNR) of the optical spin-state readout. We then demonstrate that a combined increase in spontaneous emission (through Purcell enhancement) and in optical excitation could significantly increase the readout SNR. Our combined analytical and numerical analysis, which is relevant for various optically active solid-state systems, differentiates between state-mixing processes and provides insights into the optimal light-matter coupling design.

Waveguide-coupled photonic crystal cavity for quantum dot spin readout

We present a waveguide-coupled photonic crystal H1 cavity structure in which the orthogonal dipole modes couple to spatially separated photonic crystal waveguides. Coupling of each cavity mode to its respective waveguide with equal efficiency is achieved by adjusting the position and orientation of the waveguides. The behavior of the optimized device is experimentally verified for where the cavity mode splitting is larger and smaller than the cavity mode linewidth. In both cases, coupled Q-factors up to 1600 and contrast ratios up to 10 are achieved. This design may allow for spin state readout of a self-assembled quantum dot positioned at the cavity center or function as an ultra-fast optical switch operating at the single photon level.

Measuring the Complex Admittance of a Carbon Nanotube Double Quantum Dot

We investigate radio-frequency (rf) reflectometry in a tunable carbon nanotube double quantum dot coupled to a resonant circuit. By measuring the in-phase and quadrature components of the reflected rf signal, we are able to determine the complex admittance of the double quantum dot as a function of the energies of the single-electron states. The measurements are found to be in good agreement with a theoretical model of the device in the incoherent limit. In addition to being of fundamental interest, our results present an important step forward towards noninvasive charge and spin state readout in carbon nanotube quantum dots.

Charge and Spin State Readout of a Double Quantum Dot Coupled to a Resonator

State readout is a key requirement for a quantum computer. For semiconductor-based qubit devices it is usually accomplished using a separate mesoscopic electrometer. Here we demonstrate a simple detection scheme in which a radio frequency resonant circuit coupled to a semiconductor double quantum dot is used to probe its charge and spin states. These results demonstrate a new noninvasive technique for measuring charge and spin states in quantum dot systems without requiring a separate mesoscopic detector.

Universal enhancement of the optical readout fidelity of single electron spins at nitrogen-vacancy centers in diamond

Precise readout of spin states is crucial for any approach toward physical realization of a spin-based quantum computer and for magnetometry with single spins. Here, we report a method to strongly improve the optical readout fidelity of electron spin states associated with single nitrogen-vacancy (NV) centers in diamond. The signal-to-noise ratio is enhanced significantly by performing conditional flip-flop processes between the electron spin and the nuclear spin of the NV center's nitrogen atom. The enhanced readout procedure is triggered by a short preparatory pulse sequence. As the nitrogen nuclear spin is intrinsically present in the system, this method is universally applicable to any nitrogen-vacancy center. Besides the readout method, our studies included coherent control over a single nitrogen nuclear spin for the first time.

Optical rotation of heavy hole spins by non-Abelian geometrical means

A non-Abelian geometric method is proposed for rotating of heavy hole spins in a singly positive charged quantum dot in Voigt geometry. The key ingredient is the delay-dependent non-Abelian geometric phase, which is produced by the nonadiabatic transition between the two degenerate dark states. We demonstrate, by controlling the pump, the Stokes and the driving fields, that the rotations about $y$- and $z$-axes with arbitrary angles can be realized with high fidelity. Fast initialization and heavy hole spin state readout are also possible.

Device fabrication and transport measurements of FinFETs built with 28Si SOI wafers toward donor qubits in silicon

We report on the fabrication of transistors in a FinFET geometry using isotopically purified silicon-28-on-insulator (28-SOI) substrates. Donor electron spin coherence in natural silicon is limited by spectral diffusion due to the residual 29Si nuclear spin bath, making isotopically enriched nuclear spin-free 28Si substrates a promising candidate for forming spin quantum bit devices. The FinFET architecture is fully compatible with single-ion implant detection for donor-based qubits and the donor spin-state readout through electrical detection of spin resonance. We describe device processing steps and discuss results on electrical transport measurements at 0.3 K.

Charge-to-spin conversion of electron entanglement states and spin-interaction-free solid-state quantum computation

Without resorting to spin-spin coupling, we propose a scalable spin quantum computing scheme assisted with a semiconductor multiple-quantum-dot structure. The techniques of single electron transitions and the nanostructure of quantum-dot cellular automata (QCA) are used to generate charge entangled states of two electrons, which are then converted into spin entanglement states using single-spin rotations only. Deterministic two-qubit quantum gates are also manipulated using only single-spin rotations with the help of QCA. A single-shot readout of spin states can be carried out by coupling the multiple dot structure to a quantum point contact. As a result, deterministic spin-interaction-free quantum computing can be implemented in semiconductor nanostructure.

Single-shot readout of electron spins in a semiconductor quantum dot

We report on a method for single-shot readout of spin states in a semiconductor quantum dot that is robust against charge noise and can be used even when the electron temperature exceeds the energy splitting between the states. The spin states are first correlated to different charge states using a spin dependence of the tunnel rates. A subsequent fast measurement of the charge on the dot then reveals the original spin state. The method is analyzed theoretically, and compared to a previously used method. We experimentally demonstrate the method by performing readout of the two-electron spin states, achieving a single-shot visibility of more than 80%. We find very long triplet-to-singlet relaxation times (up to several milliseconds), with a strong dependence on in-plane magnetic field.

Spin State Readout by Quantum Jump Technique: For the Purpose of Quantum Computing

Utilizing the Pauli-blocking mechanism we show that shining circular polarized light on a singly-charged quantum dot induces spin dependent fluorescence. Employing the quantum-jump technique we demonstrate that this resonance luminescence, due to a spin dependent optical excitation, serves as an excellent readout mechanism for measuring the spin state of a single electron confined to a quantum dot.