The contactless micromanipulation capability and microgravity environment provided by the acoustic levitation technology have excellent application prospects in many fields, such as droplet dynamics, solidification state physics, life sciences, etc. However, the applications are severely constrained by the limitation of the transducer power. In this paper, we explore an array geometry optimization framework to improve the levitation capability. First, the acoustic pressure attenuation and directional characteristics of commercial transducers are analyzed to uncover the mechanism of the array geometry affecting the acoustic radiation force (ARF). Second, based on the Gor'kov potential theory, the array geometry form of N-elements is derived, and the arrangement in the spherical ring (ASR) method is proposed to obtain the element coordinates. Then, spherical radius and array height are adjusted to obtain the optimal array geometry. On this basis, the directional angle of each transducer is further optimized. Finally, simulation and physical verification are carried out. The simulation results indicate that the ARF increases and then decreases with the spherical radius and array height, which are the existing maximum values. Directional angle optimization (DAO) can improve the ARF, particularly when the array height exceeds the sphere diameter. These findings are consistent with the analytical results. Notably, we built a prototype physical system, and the physical experiments showed that the optimized array improved the axial ARF by 201.2% and the radial ARF by 115.9% over the conventional array. The works presented in this paper offer a valuable design approach for acoustic levitation arrays, thereby contributing to the advancement and application of ultrasonic array levitation technology.