Abstract Delamination is a typical failure mode in multilayered materials, which may potentially threaten the safety and reliability of the materials if not detected promptly. This paper proposes a novel quantitative detection method for delamination in multilayered materials based on laser-generated Lamb waves with improved wavenumber analysis. First, a three-dimensional(3D) finite element model is established to simulate the interaction between delamination and laser-generated Lamb waves. The propagation characteristics of Lamb waves in multilayered materials without defects and with delamination of three different shapes, i.e., rectangular, circular and triangular are analyzed. And the mechanism that delamination can lead to the appearance of scattered wave and new wavenumber components is investigated, facilitating the quantitative detection of delamination. Then, an improved wavenumber analysis method for quantitative detection of delamination is proposed. The new wavenumber components caused by delamination are extracted by broadband adaptive wavenumber filtering to reduce imaging interference and artifacts caused by irrelevant components, and the spatial wavenumber spectrum is obtained by fast broadband local wavenumber estimation algorithm to enhance the delamination imaging accuracy and spatial resolution. The experimental results indicate that, across various experimental scenarios, the proposed method achieves superior imaging precision compared to traditional wavenumber filtering or local wavenumber estimation methods, and can quantitatively identify delamination defects of various shapes and sizes.