Spallation Research Articles

The ESS Test and Instruments Cryoplant – First test results and operation experiences

The European Spallation Source (ESS) is a neutron-scattering facility being built with extensive international collaboration in Lund, Sweden. The world’s most powerful linear proton accelerator shoots protons against a rotating tungsten target where neutrons are knocked off (“spallate”) and are guided to the neutron instrument suites. Three cryogenic plants and a vast cryogenic distribution system serve the cooling needs of the superconducting RF cavities in the accelerator, the cold hydrogen moderators in the target, a cryomodule test stand and the sample environments for neutron instruments. The project’s demand of schedule and economic feasibility requires a high degree of parallel work for installation and commissioning of the cryogenic and auxiliary systems. The first of the three plants, the Test and Instrumentation Cryoplant (TICP) has been installed, commissioned and acceptance tested in 2018 by Air Liquide Advanced Technologies (ALAT). The plant consists not only of a standard compressor system and coldbox but also of a process vacuum system for 2K operation, internal and external helium purifiers, liquid helium tank, filling and boil of station and a helium recovery system. It is heavily integrated in the overall cryogenic installations at ESS. The paper describes some project challenges, acceptance test results and first operation experience.

The Multi-Blade Boron-10-based neutron detector performance using a focusing reflectometer

The Multi-Blade is a Boron-10-based neutron detector designed for neutron reflectometers and developed for the two instruments (Estia and FREIA) planned for the European Spallation Source in Sweden. A demonstrator has been installed at the AMOR reflectometer at the Paul Scherrer Institut (PSI—Switzerland). AMOR exploits the Selene guide concept and can be considered a scaled-down demonstrator of Estia. The results of these tests are discussed. It will be shown how the characteristics of the Multi-Blade detector are features that allow the focusing reflectometry operation mode. Additionally the performance of the Multi-Blade, in terms of rate capability, exceeds current state-of-the-art technology. The improvements with respect to the previous prototypes are also highlighted; from background considerations to the linear and angular uniformity response of the detector.

Physics potential of the ESSnu SB

The ESSnu SB project proposes to base a neutrino “Super Beam” of unprecedented luminosity at the European Spallation Source. The original proposal identified the second peak of the oscillation probability as the optimal to maximize the discovery potential to leptonic CP violation. However this choice reduces the statistics at the detector and penalizes other complementary searches such as the determination of the atmospheric oscillation parameters, particularly the octant of theta _{23} as well as the neutrino mass ordering. We explore how these shortcomings can be alleviated by the combination of the beam data with the atmospheric neutrino sample that would also be collected at the detector. We find that the combination not only improves very significantly these drawbacks, but also enhances both the CP violation discovery potential and the precision in the measurement of the CP violating phase, for which the facility was originally optimized, by lifting parametric degeneracies. We then reassess the optimization of the ESSnu SB setup when the atmospheric neutrino sample is considered, with an emphasis in performing a measurement of the CP violating phase as precise as possible. We find that for the presently preferred value of delta sim -pi /2, shorter baselines and longer running time in neutrino mode would be optimal. In these conditions, a measurement better than 14^circ would be achievable for any value of the theta _{23} octant and the mass ordering. Conversely, if present and next generation facilities were not able to discover CP violation, longer baselines and more even splitting between neutrino and neutrino modes would be preferable. These choices would allow a 5 sigma discovery of CP violation for around a 60% of the possible values of delta and to determine its value with a precision around 6^circ if it is close to 0 or pi .

Helium Management of ESS Cryoplants with Common Safety Relief Header and Recovery System

The European Spallation Source (ESS) is a neutron-scattering facility being built with extensive international collaboration in Lund, Sweden. Three cryogenic plants with a vast cryogenic distribution system meet the cooling requirements of the superconducting RF cavities in the accelerator (ACCP), the cold hydrogen moderators in the target (TMCP), a cryomodule test stand and the sample environments for neutron instruments (TICP). The first of the three plants, the TICP has been successfully installed, commissioned and acceptance tested in 2018 by Air Liquide Advanced Technologies. Meanwhile the other two cryoplants (ACCP and TMCP) are under commissioning and testing by Linde Kryotechnik AG. The cryoplants share common helium buffer tanks, safety relief headers and helium recovery system due to historical, economical and architectural reasons. The helium recovery strategy and system configuration will be described in the paper. Resulting challenges, risks and safety relevant events that happened during, especially parallel, commissioning activities will be presented. The measures implemented to mitigate major risk and lessons learned are addressed as well.

Progress and simulations for intranuclear neutron-antineutron transformations in Ar1840

With the imminent construction of the Deep Underground Neutrino Experiment (DUNE) and Hyper-Kamiokande, nucleon decay searches as a means to constrain beyond Standard Model (BSM) extensions are once again at the forefront of fundamental physics. Abundant neutrons within these large experimental volumes, along with future high-intensity neutron beams such as the European Spallation Source, offer a powerful, high-precision portal onto this physics through searches for $\mathcal{B}$ and $\mathcal{B}-\mathcal{L}$ violating processes such as neutron--antineutron transformations ($n\rightarrow\bar{n}$), a key prediction of compelling theories of baryogenesis. With this in mind, this paper discusses a novel and self-consistent intranuclear simulation of this process within ${}^{40}_{18} Ar$, which plays the role of both detector and target within DUNE's gigantic liquid argon time projection chambers. An accurate and independent simulation of the resulting intranuclear annihilation respecting important physical correlations and cascade dynamics for this large nucleus is necessary to understand the viability of such rare searches when contrasted against background sources such as atmospheric neutrinos. Recent theoretical improvements to our model, including the first calculation of ${}^{40}_{18} Ar$'s $\bar{n}$-intranuclear suppression factor, and Monte Carlo simulation comparisons to another publicly available $n\rightarrow\bar{n}$ generator within GENIE, are also discussed.

Coherent elastic neutrino-nucleus scattering at the European Spallation Source

The European Spallation Source (ESS), presently well on its way to completion, will soon provide the most intense neutron beams for multi-disciplinary science. Fortuitously, it will also generate the largest pulsed neutrino flux suitable for the detection of Coherent Elastic Neutrino-Nucleus Scattering (CEνNS), a process recently measured for the first time at ORNL’s Spallation Neutron Source. We describe innovative detector technologies maximally able to profit from the order-of-magnitude increase in neutrino flux provided by the ESS, along with their sensitivity to a rich particle physics phenomenology accessible through high-statistics, precision CEνNS measurements.

Neutrino CP Violation with the European Spallation Source neutrino Super Beam project

After measuring in 2012 a relatively large value of the neutrino mixing angle θ 13, the door is now open to observe for the first time a possible CP violation in the leptonic sector. The measured value of θ 13 also privileges the 2nd oscillation maximum for the discovery of CP violation instead of the usually used 1st oscillation maximum. The sensitivity at this 2nd oscillation maximum is about three times higher than for the 1st oscillation maximum inducing a lower influence of systematic errors. Going to the 2nd oscillation maximum necessitates a very intense neutrino beam with the appropriate energy. The world’s most intense pulsed spallation neutron source, the European Spallation Source (ESS), will have a proton linac with 5 MW power and 2 GeV energy. This linac, under construction, also has the potential to become the proton driver of the world’s most intense neutrino beam with very high potential to discover a neutrino CP violation. The physics performance of that neutrino Super Beam in conjunction with a megaton underground Water Cherenkov neutrino detector installed at a distance of about 500 km from ESS has been evaluated. In addition, the choice of such detector will extent the physics program to proton–decay, atmospheric neutrinos and astrophysics searches. The ESS proton linac upgrades, the accumulator ring needed for proton pulse compression, the target station optimization and the physics potential are described. In addition to neutrinos, this facility will also produce at the same time a copious number of muons which could be used by a muon collider. The ESS neutron facility will be fully ready by 2023 at which moment the upgrades for the neutrino facility could start.

Neutron activation properties of PE-B4C-concrete assessed by measurements and simulations

The neutron activation properties of the PE-B4C-concrete recently developed for the European Spallation Source (ESS) ERIC (European Spallation Source, https://europeanspallationsource.se/about ) were investigated. On the one hand the concrete activat

Neutron radiation shielding with sintered lunar regolith

Lunar regolith simulant is exposed to a fast neutron flux of a spallation source. The samples consisted of a set of as-received, traditionally sintered, and solar sintered JSC-2A lunar regolith simulant. Aluminium samples were also irradiated for comparison. The ChipIr beamline of the ISIS neutron and muon source was used to provide a flux of atmospheric-like neutrons. The shielding properties of the different samples were measured for transmission, by counting neutrons before and after the samples using fast neutron detectors. Monte-Carlo simulations were carried out concurrently. The simulations are in good agreement with measurements. Aluminium simulations have shown to be in better accordance with the experimental results, probably because less affected by systematic errors. As for regolith shielding, a sensitivity analysis showed the low impact of the variations in regolith composition on the shielding properties. The benchmark of the simulations has allowed an independent estimate of the required level of regolith shielding needed to cope with primary and secondary radiation emissions. For galactic cosmic rays a value > 200 g/cm2 is estimated to give >50% reduction in transmission. For solar particle events a few 10s of g/cm2 can reduce the dose by more than an order of magnitude.

High-rate measurements of the novel BAND-GEM technology for thermal neutron detection at spallation sources

Thermal neutron detection technologies alternative to 3He, featuring a rate capability matching the high flux expected at the European Spallation Source (ESS), are one of the main present challenges of neutron science. A new thermal neutron detection technology was recently developed named the BAND-GEM, a Gas Electron Multiplier (GEM)-based detector provided with a borated 3D converter to reach high efficiency. In this paper the results of a count rate test performed on the BAND-GEM at the ORPHEE reactor are presented. The results show that the detector can easily reach a neutron count rate of 2 MHz/cm2 while maintaining a good linearity and it is able to reach 8 MHz/cm2 with a measurable loss of linearity η and with no sign of instability.

The instrument suite of the European Spallation Source

An overview is provided of the 15 neutron beam instruments making up the initial instrument suite of the European Spallation Source (ESS), and being made available to the neutron user community. The ESS neutron source consists of a high-power accelerator and target station, providing a unique long-pulse time structure of slow neutrons. The design considerations behind the time structure, moderator geometry and instrument layout are presented.The 15-instrument suite consists of two small-angle instruments, two reflectometers, an imaging beamline, two single-crystal diffractometers; one for macromolecular crystallography and one for magnetism, two powder diffractometers, and an engineering diffractometer, as well as an array of five inelastic instruments comprising two chopper spectrometers, an inverse-geometry single-crystal excitations spectrometer, an instrument for vibrational spectroscopy and a high-resolution backscattering spectrometer. The conceptual design, performance and scientific drivers of each of these instruments are described.All of the instruments are designed to provide breakthrough new scientific capability, not currently available at existing facilities, building on the inherent strengths of the ESS long-pulse neutron source of high flux, flexible resolution and large bandwidth. Each of them is predicted to provide world-leading performance at an accelerator power of 2 MW. This technical capability translates into a very broad range of scientific capabilities. The composition of the instrument suite has been chosen to maximise the breadth and depth of the scientific impact of the early years of the ESS, and provide a solid base for completion and further expansion of the facility.

Tritium in urine from members of the general public and occupationally exposed workers in Lund, Sweden, prior to operation of the European Spallation Source

A powerful neutron source, the European Spallation Source (ESS), is currently under construction in Lund, Sweden (~90 000 inhabitants). Levels of tritium (3H) in urine were estimated in members of the public in Lund and employees at the ESS using liquid scintillation counting, to obtain baseline levels before the start of operation of the ESS. These were compared with levels in other occupationally exposed radiation workers. Both the spallation reaction in the ESS tungsten target and the activation of various materials by the protons produced by the 5 MW linear accelerator will generate tritium, which will be released into the atmosphere mainly as tritiated water (HTO). Urinary HTO activity concentrations were determined in a total of 55 individuals belonging to four different categories: ESS employees, neighbours of the ESS, members of the general public in Lund and exposed workers from other facilities. The participants were asked to provide information on their beverage intake the day before urine sampling. The urine samples were filtered on activated charcoal and distilled before analysis. The effect of sample preparation on the isotope fractionation of urine samples was investigated by isotope ratio mass spectrometry (IRMS) of 2H/1H, which showed no influence. IRMS was also used to investigate if the ratio between the stable hydrogen isotopes (2H/1H) could provide useful data of the origin, and hence the tritium concentration, of various types of drinking water. Urinary HTO activity concentrations determined using liquid scintillation counting (LSC) were found to be below the minimum detectable activity (MDA) of 2.1 Bq⋅L−1 for most of the participants. Five of the workers actively handling organic tritiated material were found to have activity concentrations between 3.5 and 11 Bq⋅L−1, which were higher than the average value in local tap water of 1.5 ± 0.6 Bq⋅L−1. The results will be used to evaluate the radiological impact on the population from future releases of tritium resulting from the operation of the ESS.

Dose Measurements around Spallation Neutron Sources

Neutron dose measurements and calculations around spallation sources are of importance for an appropriate shielding study. Two spallation sources, consisted of Pb target, have been irradiated by high-energy proton beams, delivered by the Nuclotron accelerator (JINR), Dubna. Dose measurements of the neutrons produced by the two spallation sources were performed using Solid State Nuclear Track Detectors (SSNTDs). In addition, the neutron dose after polyethylene and concrete was calculated using phenomenological model based on empirical relations applied in high energy Physics. Analytical and experimental neutron benchmark analysis has been performed using the transmission factor. A comparison of experimental results with calculations is given.

Application of ADVANTG variance reduction parameters with MCNP6 at ESS

Monte Carlo radiation transport codes have become the primary tool for shielding and activation analysis at high-powered spallation neutron sources. However, use of these codes to model facilities that have large amounts of shielding requires the use of variance reduction methods. This paper presents examples that apply ADVANTG generated variance reduction parameters to analyses performed at ESS using MCNP6. This requires some limitations in ADVANTG to be overcome and little-known features to be used. The focus of this paper is to describe how these limitations were overcome so other analyst at spallation sources can benefit from these methods as well.

First steps toward the development of SONATE, a Compact Accelerator driven Neutron Source

Facilities providing bright thermal neutron beams are of primary importance for various research topics such as condensed matter experiments, neutron-imaging or medical applications. Currently these are mainly spallation sources and nuclear reactors. However, these later facilities are ageing and the political context does not favor the building of new ones. This is the case in CEA-Saclay (France), where the Orphee reactor is planned to shutdown in 2019. Therefore, another local facility, affordable by one country, able to provide high brilliance neutron beams has to be built. At CEA-Saclay, a compact accelerator driven neutron source, SONATE, is investigated in taking advantage of the IPHI accelerator able to deliver a 3 MeV proton beam with an intensity up to 100 mA. In the future, SONATE is foreseen to operate with 20 MeV protons to increase the neutron brightness. In addition to the difficulties to operate such high intensity accelerators, the other challenges regard the target-moderator-reflector (TMR) design which is crucial to maximize the neutron flux at the detector location. At CEA-Saclay, several experiments were performed between 2016 and 2019 with the IPHI accelerator. Geant4 simulations were also developed. They demonstrate the feasibility of such concept and enable to find the best TMR configuration for the future SONATE facility. These developments are reported in this article.

Mechanical engineering, design and structural health monitoring at the ESS facility to enable science

The European Spallation Source (ESS), which is established as a European Research Infrastructure Consortium (ERIC), is a multi-disciplinary research facility that is currently under construction. ESS has as vision to develop to a world class facility, enabling scientific breakthroughs in research related to materials, energy, health and the environment. The ESS facility is built by a collaboration of some 100 research institutes and universities. With its 5 MW average beam power, its linac will be the most powerful linac of all neutron spallation sources. Neutrons are obtained by delivering 2 GeV protons at a repetition rate of 14 Hz to the He-cooled solid tungsten rotating target. The Accelerator is built with a high percentage of In-Kind Contributions (IKC) with major accelerator systems being designed, prototyped and built outside ESS. The first major accelerator elements are now being assembled and tested with their first parts being installed. Future similar large-scale projects could likely be IKC-based, which is a powerful model. Within ESS, the Mechanical Engineering & Technology (MET) section is responsible for developing and maintaining mechanical engineering and design throughout the facility. The mechanical design is consolidated in the master model and available under the ESS Plant Layout, including all In-Kind Contributions as well as other related mechanical engineering content. Consequently, the MET section is also responsible for the design, development and supervision of the proton accelerator and tungsten target in terms of civil and infrastructure design for the physical plant. In parallel, ESS has set stringent goals for high availability and reliability on the machines during operations. In order to deliver these goals and monitor the aging status of critical parts of the machines, prototypes and one-of-a-kinds, the MET section has developed and currently implements Structural Health Monitoring (SHM) program on the accelerator primarily and other machines for Operations. The innovative strategy and application of Non-Destructive Testing for Machines (NDTM) is under development by the MET section with the leading benefit of utilizing the technology of Resonant Ultrasound Spectroscopy (RUS). Both reference and irradiated samples undergo RUS measurements to obtain spectral responses of the dedicated materials, for machine reliability and operations availability purposes.

Neutron macromolecular crystallography at the European spallation source.

The long-pulse spallation source of the European Spallation Source-a facility under construction in Lund, Sweden-is well suited for macromolecular crystallography experiments. We review briefly the particular properties of the long-pulse source and the associated high-brilliance moderators from the point of view of instrument design. We then outline the design philosophy and current design of the NMX macromolecular diffractometer. We also briefly describe the supporting facilities available for users and finish by an evaluation of the expected performance.

Low-dimensional moderators at ESS and compact neutron sources

Low-dimensional moderators were designed for the European Spallation Source (ESS), and the same concepts can be applied to compact sources. At ESS, quasi two-dimensional (2D) high-brightness moderators will serve all the instruments of the initial suite. The design of the moderators is influenced by several factors, such as the layout of the facility, the requirements for beam extraction, and the number of instruments; these constraints led to the choice of the 2D “butterfly” moderator for ESS. In an accelerator-based compact source, such moderators can be designed in an even more efficient way than for high-power sources, taking advantage of the lower heat loads and of the more compact arrangement of the target-moderator system, which gives more freedom in the optimization of the geometrical setup. Some promising design options have been explored.

Impact of crystallite size on the performance of a beryllium reflector

Beryllium reflectors are used at spallation neutron sources in order to enhance the low-energy flux of neutrons emanating from the surface of a cold and thermal moderator. The design of such a moderator/reflector system is typically carried out using detailed Monte-Carlo simulations, where the beryllium reflector is assumed to behave as a poly-crystalline material. In reality, however, inhomogeneities in the beryllium could lead to discrepancies between the performance of the actual system when compared to the modeled system. The dependence of the total cross-section in particular on crystallite size, in the Bragg scattering region, could influence the reflector performance, and if such an effect is significant, it should be taken into account in the design of the moderator/reflector system. In this paper, we report on the preliminary results of using cross-section libraries, which include corrections for the crystallite size effect, in spallation source neutronics calculations.

Design of the third-generation neutron spallation target for the CERN’s n_TOF facility

The neutron Time-Of-Flight (n_TOF) facility at the European Laboratory for Particle Physics (CERN) is a pulsed white-spectrum neutron spallation source producing neutrons for two experimental areas: EAR1, located 185 m downstream of the spallation target, and EAR2, located 20 m above the target. The facility is based on a lead target impacted by a high-intensity 20 GeV/c proton beam. It is designed to study neutron-nucleus interactions for neutron kinetic energies from a few meV to several GeV, with applications in nuclear astrophysics, nuclear technology, and medical research. The facility is undergoing a major upgrade in 2019–2020, which will include the installation of the new third-generation target. The second-generation target consists in a water-cooled lead cylinder, while the new target will be cooled by nitrogen to avoid erosion-corrosion phenomena and contamination of the cooling water with radioactive lead spallation products. The new design will be optimized also for the vertical flight path. The operation of the new spallation target will start in 2021. This paper presents an overview on the evolution of the design and on the related R&D activities (including beam irradiation tests) carried out to ensure the best performance for both experimental areas and avoid the contamination issues of the previous targets.