Soft X-ray Measurements Research Articles

Heterogeneous Online Computational Platform for GEM-Based Plasma Impurity Monitoring Systems

The fusion energy research field presents many intricate challenges that require resolution. Many diagnostic systems employed in experiments are approaching the limits of current technology. Implementing efficient measurements requires using an appropriate set of tools to facilitate the optimal utilization of hardware. Fusion energy measurements must provide low latency processing with the capacity for future improvements and the ability to handle complex data flows efficiently. The presented work addresses these requirements and describes the implementation of a high-performance, low-latency software platform with convenient development for soft X-ray (SXR) plasma impurities emission tracing—the Asynchronous Complex Computation Platform (AC2P). This article presents the architectural design, implementation details, and performance and latency measurements based on the raw data acquired from the WEST tokamak and laboratory tests. AC2P provides the tools to develop low-latency, multi-core, multi-device complex data flow graph scale-up solutions for measuring impurities in hot plasmas. The system has been designed to operate online during experiments, calculate the energy distribution, position and occurrence time of SXR photons, monitor the data stream’s quality and archive any abnormalities for subsequent offline verification and algorithm improvement. This article presents AC2P, which operates as part of the SXR measurement system on the WEST tokamak.

Hanle Effect for Lifetime Determinations in the Soft X-Ray Regime.

By exciting a series of 1s^{2} ^{1}S_{0}→1snp^{1}P_{1} transitions in heliumlike nitrogen ions with linearly polarized monochromatic soft x rays at the Elettra facility, we found a change in the angular distribution of the fluorescence sensitive to the principal quantum number n. In particular it is observed that the ratio of emission in directions parallel and perpendicular to the polarization of incident radiation increases with higher n. We find this n dependence to be a manifestation of the Hanle effect, which served as a practical tool for lifetime determinations of optical transitions since its discovery in 1924. In contrast to traditional Hanle effect experiments, in which one varies the magnetic field and considers a particular excited state, we demonstrate a "soft x-ray Hanle effect" which arises in a static magnetic field but for a series of excited states. By comparing experimental data with theoretical predictions, we were able to determine lifetimes ranging from hundreds of femtoseconds to tens of picoseconds of the 1snp^{1}P_{1} levels, which find excellent agreement with atomic-structure calculations. We argue that dedicated soft x-ray measurements could yield lifetime data that are beyond current experimental reach and cannot yet be predicted with sufficient accuracy.

Table-Top Ultrafast Soft X-Ray Spectroscopy Toward Synchrotron-like in-Situ Photoelectrochemical Measurements

Advancements in in-situ X-ray capabilities have enabled the measurement of electrochemical systems in more realistic operating conditions. While these measurements have progressed our understanding of electrochemical reactions from carrier dynamics to reaction mechanisms to degradation processes, they have mostly been limited to synchrotron facilities. However, performing in-situ table-top measurements has remained a challenge in the field. Table-top XUV spectrometers based on high-harmonic generation (HHG) are powerful tools for measuring ultrafast electronic and structural properties of photoelectrocatalysts ex-situ. However, extending the accessible energy range of HHG-based spectrometers beyond 300 eV is difficult due to inherent physical scaling laws. Laser-produced plasma sources can extend into the soft X-ray range to cover the water window. This capability could enable in-situ studies of photocatalysts, but their inherent source fluctuations have prevented ultrafast studies in the past. In this work, we employ methods pioneered by HHG-based setups to create a novel laser-produced plasma technique for table-top time-resolved measurements in the soft X-ray regime (200 – 1000 eV). We combine EMCCD detection, background-free self-referencing, edge-referencing analysis, amongst other advances, to reduce shot-to-shot noise so that sub-mOD signals are detectable. This presentation will also describe the technical advances pioneered at synchrotron sources that have enabled in-situ X-ray measurements of electrochemical systems. These advancements have inspired the effort to achieve the first table-top soft X-ray measurements in device-relevant liquid environments, enabling the correlation of photocatalyst properties, such as electron and hole energies and polarons, with photoelectrochemical product formation.

Estimation of the Radial Tungsten Concentration Profiles from Soft X-ray Measurements at WEST with Bayesian Integrated Data Analysis

Estimation of the Radial Tungsten Concentration Profiles from Soft X-ray Measurements at WEST with Bayesian Integrated Data Analysis

High-Performance FPGA Streaming Data Concentrator for GEM Electronic Measurement System for WEST Tokamak

The paper presents developments and significant improvements of the soft X-ray measurement system installed at the WEST tokamak. In the introduction, a brief discussion is carried out in the scope of energy shortage, fusion energy as a remedy, and the necessity of impurities monitoring in the scope of stable and long plasma discharge. This requires high-speed and accurate measurement systems due to the intense data streams that need to be processed online. For that reason, the SXR GEM FPGA-based system was designed by the Institute of Electronic Systems of the Warsaw University of Technology, the Institute of Plasma Physics and Laser Microfusion from Warsaw, and installed at the WEST tokamak in collaboration with the Institute for Magnetic Fusion Research, Commissariat à l’Énergie Atomique. It is the second-generation system, whereas the first was installed at JET tokamak. The article describes the architecture of the designed electronic part of the system. The paper presents an entirely new approach for the data concentration module implemented in FPGA. The main premise is to select only active data and send them chronologically to the embedded computer with high throughput. It is the essential component for long-term plasma operations, about 1 min, now carried out at WEST tokamak during the C3 campaign. The paper describes the laboratory tests under the exploitation of various radiation sources and the implementation of the solution and measurements during tokamak plasmas. Previous and current data acquisition methods are compared. The results show that implementing a new local trigger has significantly improved the system performance compared to the global trigger-based acquisition. The results are approximately 17 times better in the scope of performance and more than 20 times better in terms of data compression. The described design was successfully applied during the most recent 2023 experimental campaign at the WEST tokamak.

Development of soft X-ray ptychography and fluorescence microscopy system using total-reflection wolter mirror and application to measurement of drug-treated mammalian cells

We developed a soft X-ray microscopic imaging system, CARROT, that combines ptychography and fluorescence X-ray microscopy using a total-reflection Wolter mirror illumination system. The system offers advantages such as achromaticity and long working distances, enabling seamless application to a wide wavelength range. We demonstrated high-resolution imaging of cellular structures and sub-micrometer-scale changes induced by drug administration in mammalian cells. We further showcased the capability to seamlessly switch from ptychography measurements to X-ray fluorescence measurements at different wavelengths to map elemental distributions within cells. Our findings suggest that this system can be used for investigating the correlation between intracellular structures and elemental distribution, as well as for multimodal measurements of visible light fluorescence, Raman scattering, and soft X-rays to provide valuable insights into understanding intracellular dynamics.

Development of a detection system for gas-phase aromatics and other molecules ionizable by soft X-rays demonstrated using methyl salicylate

In the present study, we developed the detection method for gas-phase aromatics and other molecules ionizable by soft X-rays demonstrated using methyl salicylate which is one of the chemical warfare agent simulants by using soft X-ray and aerosol measurement techniques. The aromatic chemical compounds which have the benzene ring are well detected by the soft X-ray assisted detection method which converts gas vapors to nanoparticles through the photochemical processes. The present study reports on the formation of nanoparticles by describing the stage change during the soft X-ray irradiation: particle-free mode; nucleation mode; transition mode; accumulation mode; and stable mode. In a controlled environment, the empirical calibration curves can predict ppbv-level methyl salicylate vapor concentrations using particle number or volume concentration data obtained from the real-time aerosol detection instrument. We expect that this technology can be utilized for calibrating or intercomparing other instruments that measure methyl salicylate concentrations.

Parametric study of the kinematic evolution of coronal mass ejection shock waves and their relation to flaring activity

Context.Coronal and interplanetary shock waves produced by coronal mass ejections (CMEs) are major drivers of space-weather phenomena, inducing major changes in the heliospheric radiation environment and directly perturbing the near-Earth environment, including its magnetosphere. A better understanding of how these shock waves evolve from the corona to the interplanetary medium can therefore contribute to improving nowcasting and forecasting of space weather. Early warnings from these shock waves can come from radio measurements as well as coronagraphic observations that can be exploited to characterise the dynamical evolution of these structures.Aims.Our aim is to analyse the geometrical and kinematic properties of 32 CME shock waves derived from multi-point white-light and ultraviolet imagery taken by the Solar Dynamics Observatory (SDO), Solar and Heliospheric Observatory (SoHO), and Solar-Terrestrial Relations Observatory (STEREO) to improve our understanding of how shock waves evolve in 3D during the eruption of a CME. We use our catalogue to search for relations between the shock wave’s kinematic properties and the flaring activity associated with the underlying genesis of the CME piston.Methods.Past studies have shown that shock waves observed from multiple vantage points can be aptly reproduced geometrically by simple ellipsoids. The catalogue of reconstructed shock waves provides the time-dependent evolution of these ellipsoidal parameters. From these parameters, we deduced the lateral and radial expansion speeds of the shocks evolving over time. We compared these kinematic properties with those obtained from a single viewpoint by SoHO in order to evaluate projection effects. Finally, we examined the relationships between the shock wave and the associated flare when the latter was observed on the disc by considering the measurements of soft and hard X-rays.Results.We find that at around 25 solar radii (R⊙), the shape of a shock wave is very spherical, with a ratio between the lateral and radial dimensions (minor radii) remaining at aroundb/a ≈ 1.03 and a radial to lateral speed ratio (VR/VL)≈1.44. The CME starts to slow down a few tens of minutes after the first acceleration and then propagates at a nearly constant speed. We revisit past studies that show a relation between the CME speed and the soft X-ray emission of the flare measured by the Geostationary Operational Environmental Satellite (GOES) and extend them to higher flare intensities and shock speeds. The time lag between the peak of the flare and of the CME speed is up to a few tens of minutes. We find that for several well-observed shock onsets, a clear correlation is visible between the derivative of the soft X-ray flux and the acceleration of the shock wave.

Self-Prepared Hyaluronic Acid/Alkaline Gelatin Composite with Nano-Hydroxyapatite and Bone Morphogenetic Protein for Cranial Bone Formation.

New bone-forming substitute materials are highly useful in dental implantology. The purpose of this study was to prepare cross-linked hyaluronic acid (cHLA)/cross-linked alkaline gelatin (cAG)/nano-hydroxyapatite (nHAp)/bone morphogenic protein (BMP) constructs; and evaluate their bone-forming capabilities in rat cranial bone defects. The cHLA and cAG liquids processed with an epoxy cross-linker were blended with a 3:1 volume ratio, followed by freeze-drying. The dry composites were further infiltrated with water containing nHAp only (BMP (-)) or with water containing nHAp and BMP (BMP (+)). Prepared wet constructs (BMP (-) and BMP (+)) were implanted in rat cranial bone defects, while defects only were also made, and animals were fed for 8 weeks, followed by subsequent soft X-ray measurements and histological observations. The X-ray results showed that BMP (+) constructs disappeared, though caused inward extension of peripherical bone from defect edges with an increase in length of approximately 24%, larger than those of BMP (-) constructs and defect only with approximately 17% and 8% increments, respectively (p < 0.05). Histological observations of BMP (+) construct samples clearly indicated active bone extension consisting of an array of island-like bones. It was concluded that cHLA/cAG/nHAp/BMP could be used as novel bone-substitute materials.

Preparation of Collagen/Hydroxyapatite Composites Using the Alternate Immersion Method and Evaluation of the Cranial Bone-Forming Capability of Composites Complexed with Acidic Gelatin and b-FGF.

Bone-substitute materials are essential in dental implantology. We prepared collagen (Col)/hydroxyapatite (Hap)/acidic gelatin (AG)/basic fibroblast growth factor (b-FGF) constructs with enhanced bone-forming capability. The Col/Hap apatite composites were prepared by immersing Col sponges alternately in calcium and phosphate ion solutions five times, for 20 and 60 min, respectively. Then, the sponges were heated to 56 °C for 48 h. Scanning electron microscopy/energy-dispersive X-ray spectroscopy, Fourier-transform infrared spectroscopy, and X-ray diffraction analyses showed that the Col/Hap composites contained poorly crystalline Hap precipitates on the Col matrix. Col/Hap composite granules were infiltrated by AG, freeze-dried, and immersed in b-FGF solution. The wet quaternary constructs were implanted in rat cranial bone defects for 8 weeks, followed by soft X-ray measurements and histological analysis. Animal studies have shown that the constructs moderately increase bone formation in cranial bone defects. We found that an alternate immersion time of 20 min led to the greatest bone formation (p < 0.05). Constructs placed inside defects slightly extend the preexisting bone from the defect edges and lead to the formation of small island-like bones inside the defect, followed by disappearance of the constructs. The combined use of Col, Hap, AG, and b-FGF might bring about novel bone-forming biomaterials.

Fast characterization of plasma states in W7-X with permutation entropy

Detecting changes in plasmas is compulsory for control and the detection of novelties. Moreover, automated novelty detection allows one to investigate large data sets to substantially enhance the efficiency of data mining approaches. To this end we introduce permutation entropy (PE) for the detection of changes in plasmas. PE is an information-theoretic complexity measure based in fluctuation analysis that quantifies the degree of randomness (resp. disorder, unpredictability) of the ordering of time series data. This method is computationally fast and robust against noise, which allows the evaluation of large data sets in an automated procedure. PE is applied on electron cyclotron emission and soft x-ray measurements in different Wendelstein 7-X low-iota configuration plasmas. A spontaneous transition to high core-electron temperature () was detected, as well as a localized low-coherent intermittent oscillation which ceased when increased in the transition. The results are validated with spectrogram analysis and provide evidence that a complexity measure such as PE is a method to support in-situ monitoring of plasma parameters and for novelty detection in plasma data. Moreover, the acceleration in processing time offers implementations of plasma-state-detection that provides results fast enough to induce control actions even during the experiment.

Comparative Study of Electric Currents and Energetic Particle Fluxes in a Solar Flare and Earth Magnetospheric Substorm

Abstract Magnetic field line reconnection is a universal plasma process responsible for the conversion of magnetic field energy to plasma heating and charged particle acceleration. Solar flares and Earth's magnetospheric substorms are two of the most investigated dynamical systems where global magnetic field reconfiguration is accompanied by energization of plasma populations. Such a reconfiguration includes formation of a long-living current system connecting the primary energy release region and cold dense conductive plasma of the photosphere/ionosphere. In both flares and substorms the evolution of this current system correlates with the formation and dynamics of energetic particle fluxes (although energy ranges can be different for these systems). Our study is focused on the similarity between flares and substorms. Using a wide range of data sets available for flare and substorm investigations, we qualitatively compare the dynamics of currents and energetic particle fluxes for one flare and one substorm. We show that there is a clear correlation between energetic particle precipitations (associated with energy release due to magnetic reconnection seen from riometer and hard X-ray measurements) and magnetic field reconfiguration/formation of the current system, whereas the long-term current system evolution correlates better with hot plasma fluxes (seen from in situ and soft X-ray measurements). We then discuss how data sets of in situ measurements of magnetospheric substorms can help interpret solar flare data.

Bolometer tomography on Wendelstein 7-X for study of radiation asymmetry

The algorithm for bolometer tomography at Wendelstein 7-X (W7-X) has been recently improved using a novel regularization functional, based on relative gradient smoothing of the sought radiation profile. It has been validated using radiation patterns provided by 3D modeling under real plasma conditions as phantoms and then applied to bolometer measurements performed during the first divertor operation phase of W7-X. The following results are presented: (1) edge-localized 2D radiation patterns with clearly resolved magnetic island radiation structures, (2) an up-down asymmetry in the impurity radiation that is not captured by the 3D edge plasma transport modeling, (3) reversal of the asymmetry with reversed magnetic field direction. Further analysis reveals a poloidal variation of the emissivity in the outer confined plasma region with a field-direction dependent asymmetry, also supported by the soft x-ray measurements. This asymmetry is considered to be related to asymmetric impurity distributions, driven by the pronounced ion-impurity friction force at the plasma edge where the collisionality of the W7-X plasma is sufficiently high to develop impurity asymmetry as predicted by neoclassical theory of parallel impurity transport.

Robust analysis of space-, time-, and energy-resolved soft x-ray measurements of magnetically confined fusion plasmas (invited).

A novel compact multi-energy soft x-ray (ME-SXR) diagnostic based on the PILATUS3 100K x-ray detector has been developed in collaboration between the Princeton Plasma Physics Laboratory and the University of Wisconsin-Madison and tested on the Madison Symmetric Torus (MST) reversed-field pinch. This solid-state photon-counting detector consists of a two-dimensional array of ∼100 000 pixels for which the lower photon absorption cutoff energy can be independently set, allowing it to be configured for a unique combination of simultaneous spatial, spectral, and temporal resolution of ∼1cm, 100eV, and 500Hz, respectively. The diagnostic is highly versatile and can be readily adapted to diverse plasma operating conditions and scientific needs without any required downtime. New results from improved-confinement and quasi-single helicity plasmas in the MST demonstrate how the detector can be applied to study multiple aspects of the evolution of magnetically confined fusion-grade plasmas. These include observing the evolution of thermal emissivity, characterizing the energy of mid-Z excitation lines, extracting the Te profile, and observing the evolution of non-thermal populations. A technique for integrating the ME-SXR diagnostic into an integrated data analysis framework based on Bayesian inference is also presented. This allows ME-SXR measurements to be combined with data for complementary diagnostics in order to simultaneously infer Te and nZ from all available information.

Time-dependent soft and hard x-ray measurements using streak and x-ray diode array diagnostic systems.

High-temperature, high-density experiments require a simultaneous understanding of temporal and spectral regions. The spectral x-ray streak camera (SXSC) is a new high-temporal-resolution spectral x-ray diagnostic system that allows researchers to differentiate between soft and hard x-ray regions. The diagnostic offers three spectral channels with a wide spectral range, one direct channel that includes a filter and two indirect channels that include both mirrors and filters. The opto-mechanical design positions the filtered radiation at three different locations along the streak photo-cathode (PC) slit to provide time-dependent spectral channels with pico-second temporal resolution. A moderate spatial resolution (150-700 μm) is achieved using slits perpendicular to the PC slit, while the slit width is optimized according to the central channel wavelength (for each channel). The diagnostic system covers a spectral range of 30-500eV for the mirror channels and >1300eV for the direct channel. The temporal and spatial axes of the streak camera are calibrated with respect to a sequence of x-ray pulses. The SXSC diagnostic system is tested and analyzed using Marshak-wave emission from an SiO2 foam that was heated by a laser-beam irradiated halfraum. The SXSC results are compared to measurements from an x-ray diode array with similar spectral channels.

Solar Energetic Particle Event occurrence prediction using Solar Flare Soft X-ray measurements and Machine Learning

The prediction of the occurrence of Solar Energetic Particle (SEP) events has been investigated over many years, and multiple works have presented significant advances in this problem. The accurate and timely prediction of SEPs is of interest to the scientific community as well as mission designers, operators, and industrial partners due to the threat SEPs pose to satellites, spacecrafts, and crewed missions. In this work, we present a methodology for the prediction of SEPs from the soft X-rays of solar flares associated with SEPs that were measured in 1 AU. We use an expansive dataset covering 25 years of solar activity, 1988–2013, which includes thousands of flares and more than two hundred identified and catalogued SEPs. Neural networks are employed as the predictors in the model, providing probabilities for the occurrence or not of a SEP, which are converted to yes/no predictions. The neural networks are designed using current and state-of-the-art tools integrating recent advances in the machine learning field. The results of the methodology are extensively evaluated and validated using all the available data, and it is shown that we achieve very good levels of accuracy with correct SEP occurrence prediction higher than 85% and correct no-SEP predictions higher than 92%. Finally, we discuss further work towards potential improvements and the applicability of our model in real-life conditions.

Measurement Capabilities Upgrade of GEM Soft X-ray Measurement System for Hot Plasma Diagnostics

Measurement Capabilities Upgrade of GEM Soft X-ray Measurement System for Hot Plasma Diagnostics

Metamagnetic transitions and magnetoelectric responses in the chiral polar helimagnet Ni2InSbO6

Magnetic-field effect on the magnetic and electric properties in a chiral polar ordered corundum Ni$_2$InSbO$_6$ has been investigated. Single-crystal soft x-ray and neutron diffraction measurements confirm long-wavelength magnetic modulation. The modulation direction tends to align along the magnetic field applied perpendicular to the polar axis, suggesting that the nearly proper-screw type helicoid should be formed below 77\,K. The application of a high magnetic field causes a metamagnetic transition. In a magnetic field applied perpendicular to the polar axis, a helix-to-canted antiferromagnetic transition takes place through the intermediate soliton lattice type state. On the other hand, a magnetic field applied along the polar axis induces a first-order metamagnetic transition. These metamagnetic transitions accompany a change in the electric polarization along the polar axis.

Dependence of the impurity transport on the dominant turbulent regime in ELM-y H-mode discharges on the DIII-D tokamak

Laser blow-off injections of aluminum and tungsten have been performed on the DIII-D tokamak to investigate the variation of impurity transport in a set of dedicated ion and electron heating scans with a fixed value of the external torque. The particle transport is quantified via the Bayesian inference method, which, constrained by a combination of a charge exchange recombination spectroscopy, soft x-ray measurements, and vacuum ultraviolet spectroscopy provides a detailed uncertainty quantification of transport coefficients. Contrasting discharge phases with a dominant electron and ion heating reveal a threefold drop in the impurity confinement time and order of magnitude increase in midradius impurity diffusion, when additional electron heating is applied. Furthermore, the calculated stationary aluminum density profiles reverse from peaked in electron heated to hollow in the ion heated case, following a similar trend to electron and carbon density. Comparable values of a core diffusion have been observed for W and Al ions, while differences in the propagation dynamics of these impurities are attributed to pedestal and edge transport. Modeling of the core transport with non-linear gyrokinetics code CGYRO [J. Candy and E. Belly, J. Comput. Phys. 324, 73 (2016)], significantly underpredicts the magnitude of the variation in Al transport. Diffusion increases three-times steeper with additional electron heat flux, and 10-times lower diffusion is observed in ion heated case than predicted by the modeling. The CGYRO model quantitatively matches the increase in the Al diffusion when approaching the linear threshold for the transition from the ion temperature gradient to trapped electron mode.

Soft X-ray measurements with a gas detector coupled to microchips in laser-plasma experiments at VEGA-2

This work presents an innovative usage of the GEMpix detector for soft X-rays (SXR) measurements aimed to make an estimate of the electron temperature of a Laser Produced Plasma (LPP). The GEMpix is a proportional gas detector based on three Gas Electron Multipliers (GEMs) with a Front-End Electronics (FEE) based on four Timepix chips. This FEE provides the Time over Threshold (ToT) acquisition mode pixel by pixel and then a digital measure of the released charge in the gas mixture. In addition, the charge can be amplified through the GEM foils with 4 orders of magnitude spanning gain offering, in this way, a big dynamic range and adjustable sensitivity. Chip design provides a threshold for each channel. All the thresholds are set in order to cut electronic noise and detect X-rays. In this configuration, a cut on the low amplitude signals is set, but the gain has been tuned in order to observe the main signal due to the soft X-rays reaching the detector. This detector works in an energy range between 2 to 15 keV . It offers good imaging properties, high efficiency and absolute calibration. It offers a good immunity to Electromagnetic Pulse (EMP), as checked at VEGA-2 laser facility (hundreds of TW in about 30 fs). In these experiments, where the formation of warm dense matter produced by blast waves has been studied, a measure of the plasma temperature was required. This measurement was realized applying some filters on the active area of the detector, in correspondence of three chips. With this configuration a study of the GEMpix response due to the photons coming from the coronal plasma produced by the laser on the target has been done for each single shot. GEMpix revealed innovative and attractive features, compared to the state of the art where passive films or detectors based on indirect conversion are used, for SXR imaging and spectral analysis to infer the electron temperature.