Single Photons Research Articles

Mid-infrared characterization of NbTiN superconducting nanowire single-photon detectors on silicon-on-insulator

Superconducting nanowire single-photon detectors are widely used for detecting individual photons across various wavelengths from ultraviolet to near-infrared range. Recently, there has been increasing interest in enhancing their sensitivity to single photons in the mid-infrared spectrum, driven by applications in quantum communication, spectroscopy, and astrophysics. Here, we present our efforts to expand the spectral detection capabilities of U-shaped NbTiN-based superconducting nanowire single-photon detectors, fabricated in a 2-wire configuration on a silicon-on-insulator substrate, into the mid-infrared range. We demonstrate saturated internal detection efficiency extending up to a wavelength of 3.5 μm for a 5 nm thick and 50 nm wide NbTiN nanowire with a dark count rate less than 10 counts per second at 0.9 K and a rapid recovery time of 4.3 ns. The detectors are engineered for integration on waveguides in a silicon-on-insulator platform for compact, multi-channel device applications.

High-dimensional spin-orbital single-photon sources.

Hybrid integration of solid-state quantum emitters (QEs) into nanophotonic structures opens enticing perspectives for exploiting multiple degrees of freedom of single-photon sources for on-chip quantum photonic applications. However, the state-of-the-art single-photon sources are mostly limited to two-level states or scalar vortex beams. Direct generation of high-dimensional structured single photons remains challenging, being still in its infancy. Here, we propose a general strategy to design highly entangled high-dimensional spin-orbital single-photon sources by taking full advantage of the spatial freedom to design QE-coupled composite (i.e., Moiré/multipart) metasurfaces. We demonstrate the generation of arbitrary vectorial spin-orbital photon emission in high-dimensional Hilbert spaces, mapping the generated states on hybrid-order Bloch spheres. We further realize single-photon sources of high-dimensional spin-orbital quantum emission and experimentally verify the entanglement of high-dimensional superposition states with high fidelity. We believe that the results obtained facilitate further progress in integrated solutions for the deployment of next-generation high-capacity quantum information technologies.

Superconducting quasiparticle-amplifying transmon: A qubit-based sensor for meV-scale phonons and single terahertz photons

With great interest from the quantum computing community, an immense amount of R&D effort has been invested into improving superconducting qubits. The technologies developed for the design and fabrication of these qubits can be directly applied to applications for ultralow-threshold particle detectors, e.g., low-mass dark matter and far-infrared photon sensing. We propose a novel energy-resolving sensor based on the transmon qubit architecture combined with a signal-enhancing superconducting quasiparticle amplification stage. We refer to these sensors as SQUATs: superconducting quasiparticle-amplifying transmons. We detail the operating principle and design of this new sensor and predict that, with minimal R&D effort, solid-state-based detectors patterned with these sensors can achieve sensitivity to single terahertz photons, and sensitivity to 1meV phonons in the detector absorber substrate on the microsecond timescale. Published by the American Physical Society 2024

Highly Efficient Single Photon Coupling via Surface Plasmons into Single-Mode Optical Fiber

Quanta of light (single photon) play as one of the building blocks of photonic based quantum computations, sensing, and communications. This makes a necessity to develop practical approaches for tuning, guiding, and coupling of single photons in photonic circuits for viable applications. Interaction and coupling efficiency of single photon into optical fibers is a technical bottleneck of quantum optics and should be addressed by novel design and materials. Here, we introduce a fiber-based micro-photonic design to directly coupling of the emitted single-photon to the core of a single mode fiber (SMF). The results of the simulation indicate that the emission of single photon source on a D-shaped SMF coated by a thin plasmonic film, provide remarkable amplifying of the evanescent field by confined surface plasmons into the SMF. The numerical analysis of different types and thicknesses of plasmonic materials by finite element method (FEM) is conducted to study the propagation vectors along the SMF as a function of the emission angle and wavelength of the single photon source. The results revealed that by the optimum thickness of the tantalum layer as novel plasmonic material, the best record of coupling efficiency can be achieved in the fiber optics communication region (λ ∼ 1550 nm). This approach sheds light on novel plasmonic-assisted coupling and promises a functional strategy for single photon manipulation in various fields of quantum optics.

Cavity-enhanced induced coherence without induced emission

This paper presents a theoretical study of the enhancement of Zou-Wang-Mandel (ZWM) interferometry through cavity-enhanced spontaneous parametric down-conversion (SPDC) processes producing frequency-entangled biphotons. The ZWM interferometry shows the capability to generate interference effects between single signal photons via indistinguishability between the entangled idler photons. This paper extends the foundational principles of ZWM interferometry by integrating cavity-enhanced SPDCs, aiming to narrow photon bandwidths for improved coherence and photon pair generation efficiency, which is critical for applications in quantum information technologies, quantum encryption, and quantum imaging. This work explores the theoretical implication of employing singly resonant optical parametric oscillators within the ZWM interferometer to produce narrow-band single photons. By combining cavity-enhanced SPDCs with ZWM interferometry, this study fills a gap in current theoretical proposals, offering significant advancements in quantum cryptography and network applications that require reliable, narrow-band single photons.

Implementation of controlled unitary gates and its application in a remote-controlled quantum gate

Recently, remote-controlled quantum information processing has been proposed for its applications in secure quantum processing protocols and distributed quantum networks. For remote-controlled quantum gates, the experimental realization of controlled unitary (CU) gates between any quantum gates is an essential task. Here, we propose and experimentally demonstrate a scheme for implementing CU gates between any pair of unitary gates using the polarization and time-bin degrees of freedom of single photons. Then, we experimentally implement remote-controlled single-qubit unitary gates by controlling either the state preparation or measurement of the control qubit with high process fidelities. We believe the proposed remote-controlled quantum gate model can pave the way for secure and efficient quantum information processing.

Semi‐Quantum Signature Protocol Using EPR Steering and Single Photons

AbstractThis study tackles critical issues in semi‐quantum signature (SQS) protocols to enhance security and efficiency. It revisits Xia et al.’s SQS protocol, which uses EPR steering for security but introduces inconsistencies in a semi‐quantum environment. Xia et al. assume that both the signatory and arbitrator have full quantum capabilities, while the verifier only has partial capabilities, making them a classical participant. However, their protocol requires the verifier to perform eavesdropping checks, necessitating quantum storage, which is not aligned with a semi‐quantum environment. The study proposes a novel SQS protocol using EPR steering and single photons, with pre‐shared keys to determine photon arrangements to address this. This ensures that only the communicating parties know the inspection and message transmission locations, solving the quantum storage issue and enabling efficient eavesdropper detection and identity authentication. This new protocol adheres to semi‐quantum principles and sets a foundation for future advancements in quantum cryptography and secure communication.

Heralded Generation of Correlated Photon Pairs from CdS/CdSe/CdS Quantum Shells.

Quantum information processing demands efficient quantum light sources (QLS) capable of producing high-fidelity single photons or entangled photon pairs. Single epitaxial quantum dots (QDs) have long been proven to be efficient sources of deterministic single photons; however, their production via molecular-beam epitaxy presents scalability challenges. Conversely, colloidal semiconductor QDs offer scalable solution processing and tunable photoluminescence, but suffer from broader linewidths and unstable emissions. This leads to spectrally inseparable emission from exciton (X) and biexciton (XX) states, complicating the production of single photons and triggered photon pairs. Here, we demonstrate that colloidal semiconductor quantum shells (QSs) achieve significant spectral separation (∼75-80 meV) and long temporal stability of X and XX emissive states, enabling the observation of exciton-biexciton bunching in colloidal QDs. Our low-temperature single-particle measurements show cascaded XX-X emission of single photon pairs for over 200 s, with minimal overlap between X and XX features. The X-XX distinguishability allows for an in-depth theoretical characterization of cross-correlation strength, placing it in perspective with photon pairs of epitaxial counterparts. These findings highlight a strong potential of semiconductor quantum shells for applications in quantum information processing.

Dynamic quantum secret sharing with identity verification based on quantum walks

Abstract A dynamic quantum secret sharing protocol with authentication is proposed based on quantum walks. The protocol can share specific secrets and also update the secret information periodically based on the existing quantum walks structure. Participants can be added or removed while keeping the original secret unchanged. This is more flexible in practical applications. Before the secrets are shared, each participant is authenticated to ensure the legitimacy of all participants' identities. In addition, the protocol uses single photons as quantum resources, avoiding the complex preparation of entangled states, which makes the protocol more advantageous and potential in practical applications. Security analyses show that the protocol is resistant to collusion attack and other common attacks.

Continuously tunable single-photon level nonlinearity with Rydberg state wave-function engineering

Extending optical nonlinearity into the extremely weak light regime is at the heart of quantum optics, since it enables the efficient generation of photonic entanglement and implementation of photonic quantum logic gate. Here, we demonstrate the capability for continuously tunable single-photon level nonlinearity, enabled by precise control of Rydberg interaction over two orders of magnitude, through the use of microwave-assisted wave-function engineering. To characterize this nonlinearity, light storage and retrieval protocol utilizing Rydberg electromagnetically induced transparency is employed, and the quantum statistics of the retrieved photons are analyzed. As a first application, we demonstrate our protocol can speed up the preparation of single photons in low-lying Rydberg states by a factor of up to∼40. Our work holds the potential to accelerate quantum operations and to improve the circuit depth and connectivity in Rydberg systems, representing a crucial step towards scalable quantum information processing with Rydberg atoms.

Single and entangled photon pair generation using atomic vapors for quantum communication applications

Significant progress has been achieved in leveraging atomic systems for the effective operation of quantum networks, which are essential for secure and long-distance quantum communication protocols. The key elements of such networks are quantum nodes that can store or generate both single and entangled photon pairs. The primary mechanisms leading to the production of single and entangled photon pairs revolve around established techniques such as parametric down-conversion, four-wave mixing, and stimulated Raman scattering. In contrast to solid-state platforms, atomic platforms offer a more controlled approach to the generation of single and entangled photon pairs, owing to the progress made in atom manipulation techniques such as trapping, cooling, and precise excitation schemes facilitated by the use of lasers. This review article delves into the techniques implemented for generating single and entangled photon pairs in atomic platforms, starting with a detailed discussion of the fundamental concepts associated with single and entangled photons and their characterization techniques. The aim is to evaluate the strengths and limitations of these methodologies and offer insights into potential applications. Additionally, the article will review the extent to which these atomic-based systems have been integrated into operational quantum communication networks.

First observation of single photons in a CRESST detector and new dark matter exclusion limits

The main goal of the CRESST-III experiment is the direct detection of dark matter particles via their scattering off target nuclei in cryogenic detectors. In this work we present the results of a silicon-on-sapphire (SOS) detector with a mass of 0.6 g and an energy threshold of (6.7±0.2) eV with a baseline energy resolution of (1.0±0.2) eV. This allowed for a calibration via the detection of single luminescence photons in the eV-range, which could be observed in CRESST for the first time. We present new exclusion limits on the spin-independent and spin-dependent dark matter-nucleon cross section that extend to dark matter particle masses of less than 100 MeV/c2. Published by the American Physical Society 2024

Comment on “quantum identity authentication with single photon”

A few years ago Hong et al. (Quantum Inf Process 16:236, 2017) proposed a quantum identity authentication protocol using single photons and executable on currently available quantum hardware. Zawadzki later published two attacks on this protocol, and suggested a mitigation in the same work. In this comment we point out an additional vulnerability that causes the prover Alice to leak a percentage of her secret key at every authentication attempt. The latter is due to a problematic policy in the generation and management of decoy states. We conclude by showing a simple mitigation that addresses the issue.

Mie metasurfaces for enhancing photon outcoupling from single embedded quantum emitters

Abstract Solid-state quantum emitters (QE) can produce single photons required for quantum information processing. However, their emission properties often exhibit poor directivity and polarisation definition resulting in considerable loss of generated photons. Here we propose and numerically evaluate Mie metasurface designs for outcoupling photons from an embedded and randomly-positioned QE. These Mie metasurface designs can provide over one order of magnitude enhancement in photon outcoupling with only several percent of photons being lost. Importantly, the Mie metasurfaces provide the enhancement in photon outcoupling without the need for strict QE position alignment and without affecting the intrinsic QE emission rate (Purcell enhancement). Electric dipole modes are key for achieving the enhancement and they offer a path for selective outcoupling for photons emitted with specific polarisation, including the out-of-plane polarisation. Mie metasurfaces can provide an efficient, polarisation-selective and scalable platform for QEs.

Efficient, high-fidelity single-photon switch based on waveguide-coupled cavities

We demonstrate theoretically that waveguide-coupled cavities with embedded two-level emitters can act as a highly efficient, high-fidelity single-photon switch. The photon switch is an optical router triggered by a classical signal—the propagation direction of single input photons in the waveguide is controlled by changing the emitter-cavity coupling parameters , for example, using applied fields. The switch reflects photons in the weak emitter-cavity coupling regime and transmits photons in the strong coupling regime. By calculating transmission and reflection spectra using the input-output formalism of quantum optics and the transfer matrix approach, we obtain the fidelity and efficiency of the switch with a single-photon input in both regimes. We find that a single waveguide-coupled cavity can route input photon wave packets with near-unity efficiency and fidelity if the wave packet width is smaller than the cavity mode linewidth. We also find that using multiple waveguide-coupled cavities increases the switching bandwidth, allowing wider wave packets to be routed with high efficiency and fidelity. For example, an array of three waveguide-coupled cavities can reflect an input Gaussian wave packet with a full width at half-maximum of 1 nm (corresponding to a few-picosecond pulse) with an efficiency Er=96.4% and a fidelity Fr=97.7%, or transmit the wave packet with an efficiency Et=99.7% and a fidelity Ft=99.8%. Such efficient, high-fidelity single-photon routing is essential for scalable photonic quantum technologies. Published by the American Physical Society 2024

High-dimensional quantum key distribution using orbital angular momentum of single photons from a colloidal quantum dot at room temperature

High-dimensional quantum key distribution (HDQKD) is a promising avenue to address the inherent limitations of basic quantum key distribution (QKD) protocols. However, experimental realizations of HDQKD to date have relied on indeterministic photon sources that limit the achievable key rate. In this paper, we demonstrate a full emulation of a HDQKD system using a single colloidal giant quantum dot (gQD) as a deterministic, compact, and room-temperature single-photon source (SPS). We demonstrate a practical protocol by encoding information in a high-dimensional space (d = 3) of the orbital angular momentum of the photons. Our experimental configuration incorporates two spatial light modulators for encoding and decoding the spatial information carried by individual photons. Our experimental demonstration establishes the feasibility of utilizing high radiative quantum yield gQDs as practical SPSs for HDQKD. We also experimentally demonstrate surpassing the traditional d = 2 QKD capacity with comparable error rates, indicating a significant improvement in performance while maintaining reliability.

Purifying quantum-dot light in a coherent frequency interface

Abstract Quantum networks typically operate in the telecom wavelengths to take advantage of low-loss transmission in optical fibres. However, bright quantum dots (QDs) emitting highly indistinguishable quantum states of light, such as InGaAs QDs, often emit photons in the near infrared thus necessitating frequency conversion (FC) to the telecom band. Furthermore, the signal quality of quantum emissions is crucial for the effective performance of these networks. In this work we report a method for simultaneously implementing spectral purification and frequency shifting of single photons from QD sources to the c-band in a periodically poled lithium niobate waveguide. We consider difference frequency generation in the counter-propagating configuration to implement FC with the output emission bandwidth in units of GHz. Our approach establishes a clear path to integrating high-performance single-emitter sources in a hybrid quantum network.

Efficient coupling of single photons from chromium-vacancy centers in nanodiamonds into end-to-end aligned optical nanowires

Abstract We report a numerical simulation on the coupling of chromium-vacancy centers in nanodiamond (CrV-ND) with end-to-end aligned optical nanowires (ONWs) structure. The structure is designed using finite-difference time-domain simulations to maximize the bidirectional coupling of spontaneous emission from a CrV-ND into ONW-guided modes. We systematically analyze the dependence of spontaneous emission characteristics on the ONW and CrV-ND dimension, quantum emitter (QE) position, and polarization. We show that coupling efficiency as high as 62% can be achieved into the guided modes from a CrV-ND placed at the center of ONWs, which is twice as compared to a CrV-ND placed on an ONW surface. The degree of polarization of single photons from CrV-ND is also estimated to be as high as 64%. This simple device can be reconfigured for various QEs. This present fiber inline platform may open new avenues in quantum photonics.

Effects of chromatic dispersion on single-photon temporal wave functions in quantum communications

In this study, we investigate the effects of chromatic dispersion on single-photon temporal wave functions (TWFs) in the context of quantum communications. Departing from classical beam analysis, we focus on the temporal shape of single photons, specifically exploring generalized Gaussian modes. From this foundation, we introduce chirped and unchirped Gaussian TWFs, demonstrating the impact of the chirp parameter in mitigating chromatic dispersion effects. Furthermore, we extend our investigation to time-bin qubits, a topic of ongoing research relevance. By exploring the interplay of dispersion effects on qubit interference patterns, we contribute essential insights to quantum information processing. This comprehensive analysis considers various parameters, introducing a level of complexity not previously explored in the context of dispersion management. We demonstrate the relationships between different quantities and their impact on the spreading of TWFs. Our results not only deepen the theoretical understanding of single-photon TWFs but also offer practical guidelines for system designers to optimize symbol rates in quantum communications.

Interference of single photons with ultralong coherence time

Interference of single photons with ultralong coherence time