Single-photon Measurements Research Articles

Detection efficiency characterization for free-space single-photon detectors: Measurement facility and wavelength-dependence investigation

In this paper, we present an experimental apparatus for the measurement of the detection efficiency of free-space single-photon detectors based on the substitution method. We extend the analysis to account for the wavelength dependence introduced by the transmissivity of the optical window in front of the detector's active area. Our method involves measuring the detector's response at different wavelengths and comparing it to a calibrated reference detector. This allows us to accurately quantify the efficiency variations due to the optical window's transmissivity. The results provide a comprehensive understanding of the wavelength-dependent efficiency, which is crucial for optimizing the performance of single-photon detectors in various applications, including quantum communication and photonics research. This characterization technique offers a significant advancement in the precision and reliability of single-photon detection efficiency measurements.

Multi-party quantum key distribution protocol in quantum network

This study proposes a measurement property of graph states and applies it to design a mediated multiparty quantum key distribution (M-MQKD) protocol for a repeater-based quantum network in a restricted quantum environment. The protocol enables remote classical users, who cannot directly transmit qubits, to securely distribute a secret key with the assistance of potentially dishonest quantum repeaters. Classical users only require two quantum capabilities, while quantum repeaters handle entanglement transmission through single-photon measurements. The one-way transmission approach eliminates the need for additional defenses against quantum Trojan horse attacks, reducing maintenance costs compared to round-trip or circular transmission methods. As a result, the M-MQKD protocol is lightweight and easy to implement. The study also evaluates the security of the protocol and demonstrates its practicality through quantum network simulations.

High-dimensional quantum correlation measurements with an adaptively gated hybrid single-photon camera

Efficient measurement of high-dimensional quantum correlations, especially spatial ones, is essential for quantum technologies. We propose and demonstrate an adaptively gated hybrid intensified camera (HIC) that combines the information from a high spatial resolution sensor and a high temporal resolution detector, offering precise control over the number of photons detected within each frame. The HIC facilitates spatially resolved single-photon counting measurements. We study the measurement of momentum correlations of photon pairs generated in type-I spontaneous parametric downconversion with the HIC and demonstrate the possibility of time-tagging the registered photons. With a spatial resolution of multi-megapixels and nanosecond temporal resolution, this system allows for the realization of previously infeasible quantum optics experiments.

Bayesian neuromorphic imaging for single-photon LiDAR.

This paper proposes a Bayesian approach to enable single photon avalanche diode (SPAD) arrays to be used as pseudo event cameras that report changes in the scene. Motivated by the working principle of event cameras, which produce sparse events associated with light flux changes, we adopt a changepoint detection strategy to generate intensity and depth change event streams from direct time-of-flight (dToF) sequences measured by SPAD arrays. Although not our main goal, the algorithm also produces as a by-product, intensity and depth estimates. Unlike the output of passive event cameras that only correspond to light flux changes, the change events detected from the sequential dToFs can relate to changes in light flux and/or depth. The integration of the proposed Bayesian approach with single-photon LiDAR (SPL) systems provides a novel solution to achieve active neuromorphic 3D imaging that offers the advantages of significantly reduced output redundancy and in particular the capacity to report scene depth changes. For each pixel of the SPAD array, asynchronous events are generated by performing online Bayesian inference to detect changepoints and estimate the model parameters simultaneously from individual single-photon measurements. Experiments are conducted on synthetic data and real dToF measurements acquired by a 172×126 pixel SPAD camera to demonstrate the feasibility and efficiency of the proposed Bayesian approach.

Front-end electronics development of large-area SiPM arrays for high-precision single-photon time measurement

TRopIcal DEep-sea Neutrino Telescope (TRIDENT) plans to incorporate silicon photomultipliers (SiPMs) with superior time resolution in addition to photomultiplier tubes (PMTs) into its detection units, namely hybrid Digital Optical Modules (hDOMs), to improve its angular resolution. However, the time resolution significantly degrades for large-area SiPMs due to the large detector capacitance, posing significant challenges for the readout electronics of SiPMs in hDOM. We analyzed the influences of series and parallel connections when constructing a large-area SiPM array and designed a series-parallel connection SiPM array with differential output. We also designed a high-speed pre-amplifier based on transformers (MABA-007159) and radio frequency amplifiers (BGA2803), and an analog multi-channel summing circuit based on operational amplifiers (LMH6629). We measured the single photon time resolution (SPTR) of a 4 × 4 SiPM (Hamamatsu S13360-3050PE) array (12 × 12 mm2) of approximately 300 ps FWHM. This front-end readout design enables the large-area SiPM array to achieve high-precision single photon time measurement in one readout channel.

A novel quantum dialogue without information leakage based on single photons in both polarization and spatial-mode degrees of freedom

This paper puts forward a novel quantum dialogue (QD) protocol without information leakage based on single photons in both polarization and spatial-mode degrees of freedom. In this protocol, the receiver sends his private message to the sender in the way of quantum secure direct communication; and the receiver decodes out the private message of the sender with the help of auxiliary single photons in two degrees of freedom, double controlled-not (CNOT) operations and an auxiliary classical bit sequence sent from the sender. As a result, no information leakage takes place. Moreover, this protocol is proven to defeat the intercept-resend attack, the measure-resend attack, the entangle-measure attack and the Trojan horse attack from an outside eavesdropper. This protocol only employs single photons in two degrees of freedom as quantum resource and needs single-photon measurements. The qubit efficiency of this protocol is as high as 66.7%.

Adaptive quantum state estimation for two optical point sources

In classical optics, there is a well-known resolution limit called Rayleigh's curse in the separation of two incoherent optical sources in close proximity. Recently, Tsang [] revealed that this difficulty may be circumvented in the framework of quantum theory. Following their work, various estimation methods have been proposed to overcome Rayleigh's curse, but none of them enables us to estimate the positions of two point sources simultaneously based on single-photon measurements with high accuracy. In this study, we propose a method to estimate the positions of two point sources with the highest accuracy using an adaptive quantum state estimation scheme. ©2024 American Physical Society 2024 American Physical Society

Chiral-Induced Spin Selectivity Modulated Time-Correlated Single-Photon Counting for DNA Hybridization Detection.

The chiral-induced spin selectivity (CISS) effect can distinguish between the spin of electrons as they pass through chiral molecules by backscattering one of the spin components. Herein, we explore the role of the CISS effect in time-correlated single-photon counting measurements to detect DNA hybridization. We observe that the average lifetime of optical excited states of quantum dots attached to double-stranded DNA (dsDNA) varies with directions of the applied magnetic field. Specifically, the difference in the nonradiative average decay lifetime for the two orientations of the applied magnetic field is 2.21 ns in the case of hybridized strands, which is 130 times higher than that observed with quantum dots attached to single-strand DNA. Additionally, we investigate the application of Fourier transform infrared (FTIR) spectroscopy for detecting double-stranded DNA in the presence of a magnetic field, establishing a theoretical framework to substantiate the experimental evidence of magnetic field-dependent FTIR spectroscopy for dsDNA.

Single-photon sub-Rayleigh precision measurements of a pair of incoherent sources of unequal intensity

Interferometric methods have been recently investigated to achieve sub-Rayleigh imaging and precision measurements of faint incoherent sources up to the ultimate quantum limit. Here we consider single-photon imaging of two point-like emitters of unequal intensity. This is motivated by the fact that pairs of natural emitters typically have unequal brightness, for example, binary star systems and exoplanets. We address the problem of estimating the transverse separation d or the relative intensity . Our theoretical analysis shows that the associated statistical errors are qualitatively different from the case of equal intensity. We employ multi-plane light conversion technology to implement Hermite–Gaussian (HG) spatial-mode demultiplexing (SPADE), and demonstrate sub-Rayleigh measurement of two emitters with a Gaussian point-spread function. The experimental errors are comparable with the theoretical bounds. The latter are benchmarked against direct imaging, yielding an improvement in the signal-to-noise ratio, which may be significant when the primary source is much brighter than the secondary one, for example, as for imaging of exoplanets.

Towards Precision Muonic X-ray Measurements of Charge Radii of Light Nuclei

We, the QUARTET Collaboration, propose an experiment to measure the nuclear charge radii of light elements with up to 20 times higher accuracy. These are essential both for understanding nuclear physics at low energies, and for experimental and theoretical applications in simple atomic systems. Such comparisons advance the understanding of bound-state quantum electrodynamics and are useful for searching for new physics beyond the Standard Model. The energy levels of muonic atoms are highly susceptible to nuclear structure, especially to the mean square charge radius. The radii of the lightest nuclei (with the atomic number, Z=1,2) have been determined with high accuracy using laser spectroscopy in muonic atoms, while those of medium mass and above were determined using X-ray spectroscopy with semiconductor detectors. In this communication, we present a new experiment, aiming to obtain precision measurements of the radii of light nuclei 3≤Z≤10 using single-photon energy measurements with cryogenic microcalorimeters; a quantum-sensing technology capable of high efficiency with outstanding resolution for low-energy X-rays.

Single-photon level ultrafast time-resolved measurement using two-color dual-comb-based asynchronous linear optical sampling

We demonstrated an ultrafast time-resolved measurement method operating at the single-photon level and employing a two-color comb-based asynchronous optical sampling (ASOPS) setup. We harnessed the two-color ASOPS photon counting approach to achieve long-term averaging of the ultralow intensity signal with a synchronized optical trigger signal, which minimizes residual timing jitter between the two combs. A pulse-width limited picosecond cross-correlation signal was successfully obtained with a power level of <1 photon/pulse. This approach enables the thorough study of ultrafast time-resolved detection of entangled photon pairs, quantum mechanical correlations in the time-frequency domain and finds wide use in optical quantum technology.

Secure communication based on sensing of undetected photons

In this paper, we introduce a secure optical communication protocol that harnesses quantum correlation within entangled photon pairs. A message written by acting on one of the photons can be read by measuring exclusively the other photon of the pair. In this scheme, a bright, meaningless optical beam hides the message, rendering it inaccessible to potential eavesdroppers. Unlike traditional methods, our approach only affects unauthorized users, fundamentally limiting their access to the communication channel. We demonstrate the effectiveness of our protocol by achieving secure communication through both amplitude and phase modulation, relying on single-photon measurements, as opposed to most approaches which rely on coincidence measurements. We successfully demonstrate the resilience of the data transfer to noise up to 105 times greater than the signal, and we employ this technique for the secure transfer of an image.

The hyperentanglement-based quantum secure direct communication protocol with single-photon measurement

The hyperentanglement-based quantum secure direct communication protocol with single-photon measurement

Orange Pomace-Derived Fluorescent Carbon Quantum Dots: Detection of Dual Analytes in the Nanomolar Range.

Green-emissive carbon quantum dots (CQDs) with exclusive chemosensing aspects were synthesized from orange pomace as a biomass-based precursor via a facile microwave method without using any chemicals. The synthesis of highly fluorescent CQDs with inherent nitrogen was confirmed through X-ray diffraction, X-ray photoelectron, Fourier transform infrared, Raman, and transmission electron microscopic techniques. The average size of the synthesized CQDs was found to be 7.5 nm. These fabricated CQDs displayed excellent photostability, water solubility, and outstanding fluorescent quantum yield, i.e., 54.26%. The synthesized CQDs showed promising results for the detection of Cr6+ ions and 4-nitrophenol (4-NP). The sensitivity of CQDs toward Cr6+ and 4-NP was found up to the nanomolar range with the limit of detection values of 59.6 and 14 nM, respectively. Several analytical performances were thoroughly studied for high precision of dual analytes of the proposed nanosensor. Various photophysical parameters of CQDs (quenching efficiency, binding constant, etc.) were analyzed in the presence of dual analytes to gain more insights into the sensing mechanism. The synthesized CQDs exhibited fluorescence quenching toward incrementing the quencher concentration, which was rationalized by the inner filter effect through time-correlated single-photon counting measurements. The CQDs fabricated in the current work exhibited a lower detection limit and a wide linear range through the simple, eco-friendly, and rapid detection of Cr6+ and 4-NP ions. To evaluate the feasibility of the detection approach, real sample analysis was conducted, demonstrating satisfactory recovery rates and relative standard deviations toward the developed probes. This research paves the way for developing CQDs with superior characteristics utilizing orange pomace (biowaste precursor).

Multi-party simultaneous quantum identity authentication based on Greenberger-Horne-Zeilinger states

A successful implementation of any secure communication protocols requires the identity authentication as a prerequisite. Quantum identity authentication (QIA) can ensure the unconditional security of identity code. In this paper, we propose a multi-party simultaneous quantum identity authentication (MSQIA) protocol based on the Greenberger-Horne-Zeilinger (GHZ) state. In the protocol, N certified users can directly send their identity codes to the authenticator Alice simultaneously through quantum channels without classical communication, which enables Alice to authenticate their identity at the same time. Our protocol only requires Alice to perform the single-photon measurement. In theory, this protocol is unconditionally secure and one pair of (N + 1)-photon GHZ state can transmit N bits of identity codes. Our MSQIA protocol has application potential in the quantum communication field in the near future.

Comparative study of lidars for measuring atmospheric temperature and wind.

The uncertainty of lidar measured atmospheric temperature T or line-of-sight (LOS) wind V is inversely proportional to the signal-to-noise ratio (SNR) of the received photocounts. We term the proportionality constant, which depicts the efficacy of the measurement method, the single-photon (or unity SNR) measurement uncertainty for T and/or V measurement. In this study, we use the single-photon measurement uncertainty as the figure of merit to compare and understand the practical differences between Cabannes scattering (CS), Rayleigh inversion (RI), rotational Raman (RR), and laser induced fluorescence (LIF) lidars for atmospheric temperature and wind measurements, and to optimize the choice and receiver design of a lidar system for a potential application.

Evaluating strain and doping of Janus MoSSe from phonon mode shifts supported by ab initio DFT calculations.

With the study of Janus monolayer transition metal dichalcogenides, in which one of the two chalcogen layers is replaced by another type of chalcogen atom, research on two-dimensional materials is advancing into new areas. Yet only little is known about this new kind of material class, mainly due to the difficult synthesis. In this work, we synthesize MoSSe monolayers from exfoliated samples and compare their Raman signatures with density functional theory calculations of phonon modes that depend in a nontrivial way on doping and strain. With this as a tool, we can infer limits for the possible combinations of strain and doping levels. This reference data can be applied to all MoSSe Janus samples in order to quickly estimate their strain and doping, providing a reliable tool for future work. In order to narrow down the results for our samples further, we analyze the temperature-dependent photoluminescence spectra and time-correlated single-photon counting measurements. The lifetime of Janus MoSSe monolayers exhibits two decay processes with an average total lifetime of 1.57 ns. Moreover, we find a strong trion contribution to the photoluminescence spectra at low temperature which we attribute to excess charge carriers, corroborating our ab initio calculations.

Utilizing broadband wavelength-division multiplexing capabilities of hollow-core fiber forquantum communications.

One of the major challenges in the deployment of quantum communications (QC) over solid-core silica optical fiber is the performance degradation due to the optical noise generated with co-propagating classical optical signals. To reduce the impact of the optical noise, research teams are turning to new and novel architectures of solid-core and hollow-core optical fiber. We studied the impact when co-propagating a single-photon level (850nm) and two classical optical signals (940nm and 1550nm) while utilizing a nested antiresonant nodeless fiber (NANF) with two low-loss windows. The 940nm signal was shown to impact the single-photon measurement due to the silicon detector technology implemented; however, multiplexing techniques and filtering could reduce the impact. The 1550nm signal was shown to have no detrimental impact. The results highlight that both high bandwidth optical traffic at 1550nm and a QC channel at 850nm could co-propagate without degradation to the QC channel.

Measuring space-time curvature using maximally path-entangled quantum states

The authors describe an experimental scheme capable of simultaneously demonstrating signatures of quantum theory and general relativity by using entangled multiphoton states to measure space-time curvature. The setup allows for curvature measurements at altitudes smaller than those required for classical or single-photon measurements.

Multi-party deterministic secure quantum communication using d-dimension GHZ state

Quantum direct communication (QDC) uses the basic principle of quantum mechanics to realize the secure communication between legal parties. Deterministic secure quantum communication (DSQC), as a branch of QDC, is a way to transmit secret message with the aid of classical bits. In this paper, a multi-party DSQC based on [Formula: see text]-dimension [Formula: see text]-particles GHZ states is proposed, in which unitary operation is not required. On the basis of [Formula: see text]-dimension single-photon measurement results, the communication parties encode and decode the message through performing modulo addition and subtraction. In addition, the scheme uses the added [Formula: see text]-dimension single photon for eavesdropping detection. The scheme has expansibility and universality. It can scale to as many parties in any dimension as required. Based on the star-shaped communication structure, it can be extended to a network to achieve the rapid communication of secret message across regions.