Single Neutral Atoms Research Articles

Quantum jump photodetector for narrowband photon counting with a single atom

Using a single neutral Rb87 atom held in an optical trap, and “quantum jump” detection of single-photon-initiated state changes, we demonstrate a single-photon quantum jump photodetector (QJPD) with intrinsically narrow bandwidth and strong rejection of out-of-band photons, of interest for detecting weak optical signals in the presence of a strong broadband background. By analyzing fluorescence photon count distributions for the bright and dark states with and without excitation, we measure quantum efficiency of 2.9(2)×10−3, a record for single-pass quantum jump production, and signal-photon-unprovoked “dark jump” rate—analogous to the dark count rate of other detectors —of 3(10)×10−3jumps/s during passive accumulation plus 4.0(4)×10−3 jumps per readout, orders of magnitude below those of traditional single-photon detectors. Available methods can substantially improve QJPD quantum efficiency, dark jump rate, bandwidth, and tunability. Published by the American Physical Society 2024

Direct generation of time-energy-entangled W triphotons in atomic vapor.

Entangled multiphoton sources are essential for both fundamental tests of quantum foundations and building blocks of contemporary optical quantum technologies. While efforts over the past three decades have focused on creating multiphoton entanglement through multiplexing existing biphoton sources with linear optics and postselections, our work presents a groundbreaking approach. We observe genuine continuous-mode time-energy-entangled W-class triphotons with an unprecedented production rate directly generated through spontaneous six-wave mixing (SSWM) in a four-level triple-Λ atomic vapor cell. Using electromagnetically induced transparency and coherence control, our SSWM scheme allows versatile narrowband triphoton generation with advantageous properties, including long temporal coherence and controllable waveforms. This advancement is ideal for applications like long-distance quantum communications and information processing, bridging single photons and neutral atoms. Most importantly, our work establishes a reliable and efficient genuine triphoton source, facilitating accessible research on multiphoton entanglement.

Fano resonance in excitation spectroscopy and cooling of an optically trapped single atom

Electromagnetically induced transparency (EIT) can be used to cool an atom in a harmonic potential close to the ground state by addressing several vibrational modes simultaneously. Previous experimental efforts focus on trapped ions and neutral atoms in a standing wave trap. In this work, we demonstrate EIT cooling of an optically trapped single neutral atom, where the trap frequencies are an order of magnitude smaller than in an ion trap and a standing wave trap. We resolve the Fano resonance feature in fluorescence excitation spectra and the corresponding cooling profile in temperature measurements. A final temperature of around 6 µK is achieved with EIT cooling, a factor of 2 lower than the previous value obtained using polarization gradient cooling. Published by the American Physical Society 2024

Simultaneous three-wave and six-wave mixing of microwave and optical fields in an atomic medium.

We experimentally investigate near-infrared optical field generation through simultaneous three-wave mixing (TWM) and six-wave mixing (SWM) processes in room-temperature 85Rb atoms. The nonlinear processes are induced using three hyperfine levels in the D1 manifold, which cyclically interact with pump optical fields and an idler microwave field. The simultaneous appearance of TWM and SWM signals in discrete frequency channels is made possible by breaking the three-photon resonance condition. This gives rise to coherent population oscillations (CPO), which are observed experimentally. We explain through our theoretical model the role of CPO in the generation of the SWM signal and its enhancement due to parametric coupling with the input seed field in contrast to the TWM signal. Our experiment proves that a single tone microwave can be converted to multiple optical frequency channels. The simultaneous existence of TWM and SWM processes can potentially enable various types of amplification to be achieved with a single neutral atom transducer platform.

Quantum jump spectroscopy of a single neutral atom for precise subwavelength intensity measurements

A single trapped neutral atom is used for precise subwavelength intensity measurements. Quantum jumps from a dark to a bright atomic state are used to boost signal-to-noise and avoid systematic errors.

Proposal for low-power atom trapping on a GaN-on-sapphire chip

The hybrid photon-atom integrated circuits, which include photonic microcavities and trapped single neutral atom in their evanescent field, are of great potential for quantum information processing. In this platform, the atoms provide the single-photon nonlinearity and long-lived memory, which are complementary to the excellent passive photonics devices in conventional quantum photonic circuits. In this work, we propose a stable platform for realizing the hybrid photon-atom circuits based on an unsuspended photonic chip. By introducing high-order modes in the microring, a feasible evanescent-field trap potential well $\sim0.3\,\mathrm{mK}$ could be obtained by only $10\,\mathrm{mW}$-level power in the cavity, compared with $100\,\mathrm{mW}$-level power required in the scheme based on fundamental modes. Based on our scheme, stable single atom trapping with relatively low laser power is feasible for future studies on high-fidelity quantum gates, single-photon sources, as well as many-body quantum physics based on a controllable atom array in a microcavity.

Single-Atom Trapping in a Metasurface-Lens Optical Tweezer

Optical metasurfaces of subwavelength pillars have provided new capabilities for the versatile definition of the amplitude, phase, and polarization of light. In this work, we demonstrate that an efficient dielectric metasurface lens can be used to trap and image single neutral atoms with a long working distance from the lens of 3 mm. We characterize the high-numerical-aperture optical tweezers using the trapped atoms and compare with numerical computations of the metasurface lens performance. We predict that future metasurfaces for atom trapping will be able to leverage multiple ongoing developments in metasurface design and enable multifunctional control in complex quantum information experiments with neutral-atoms arrays.

Motion induced excitation and radiation from an atom facing a mirror

We study quantum dissipative effects due to the nonrelativistic, bounded, accelerated motion of a single neutral atom in the presence of a planar perfect mirror, i.e., a perfect conductor at all frequencies. We consider a simplified model whereby a moving ``scalar atom'' is coupled to a quantum real scalar field, subjected to either Dirichlet or Neumann boundary conditions on the plane. We use an expansion in powers of the departure of the atom with respect to a static average position to compute the vacuum persistence amplitude and the resulting vacuum decay probability. We evaluate transition amplitudes corresponding to the excitation of the atom plus the emission of a particle, and show explicitly that the vacuum decay probabilities match the results obtained by integrating the transition amplitudes over the directions of the emitted particle. We also compute the spontaneous emission rate of an oscillating atom that is initially in an excited state.

Raman sideband cooling in optical tweezer arrays for Rydberg dressing

Single neutral atoms trapped in optical tweezers and laser-coupled to Rydberg states provide a fast and flexible platform to generate configurable atomic arrays for quantum simulation. The platform is especially suited to study quantum spin systems in various geometries. However, for experiments requiring continuous trapping, inhomogeneous light shifts induced by the trapping potential and temperature broadening impose severe limitations. Here we show how Raman sideband cooling allows one to overcome those limitations, thus, preparing the stage for Rydberg dressing in tweezer arrays.

Coherence of a dynamically decoupled single neutral atom

Long qubit coherence and efficient atom–photon coupling are essential for advanced applications in quantum communication. One technique to maintain coherence is dynamical decoupling (DD), where a periodic sequence of refocusing pulses is employed to reduce the interaction of the system with the environment. We experimentally study the implementation of DD on an optically trapped, spin-polarized 87 R b atom. We use the two magnetic-sensitive 5 S 1 / 2 Zeeman levels | F = 2 , m F = − 2 ⟩ and | F = 1 , m F = − 1 ⟩ as qubit states, motivated by the possibility of coupling | F = 2 , m F = − 2 ⟩ to 5 P 3 / 2 the excited state | F ′ = 3 , m F ′ = − 3 ⟩ via a closed optical transition. With more refocusing pulses in the DD technique, we manage to extend the coherence time from 38(3) µs to around 7 ms. We also observe a strong correlation between the motional states of the atom and the qubit coherence after the refocusing, which can be used as a measurement basis to resolve trapping parameters.

Supersymmetry-assisted high-fidelity ground-state preparation of a single neutral atom in an optical tweezer

Arrays of neutral-atom qubits in optical tweezers are a promising platform for quantum computation. Despite experimental progress, a major roadblock for realizing neutral-atom quantum computation is the qubit initialization. Here we propose that supersymmetry, a theoretical framework developed in particle physics, can be used for ultrahigh-fidelity initialization of neutral-atom qubits. We show that a single atom can be deterministically prepared in the vibrational ground state of an optical tweezer by adiabatically extracting all excited atoms to a supersymmetric auxiliary tweezer. The scheme works for both bosonic and fermionic atom qubits trapped in realistic Gaussian optical tweezers and may pave the way for realizing large-scale quantum computation, simulation, and information processing with neutral atoms.

Quantum Information Processing on the Basis of Single Ultracold Atoms in Optical Traps

A brief overview of experimental and theoretical studies on the use of single neutral atoms captured in arrays of optical dipole traps as qubits of a quantum computer is presented. Methods for loading and registering atoms in traps, and performing two-qubit quantum logic gates via dipole-dipole interaction during short-term laser excitation of atoms into Rydberg states are discussed.

Ground-state cooling of a single atom inside a high-bandwidth cavity

We report on vibrational ground-state cooling of a single neutral atom coupled to a high-bandwidth Fabry-P\'erot cavity. The cooling process relies on degenerate Raman sideband transitions driven by dipole trap beams, which confine the atoms in three dimensions. We infer a one-dimensional motional ground state population close to $90~\%$ by means of Raman spectroscopy. Moreover, lifetime measurements of a cavity-coupled atom exceeding 40 s imply three-dimensional cooling of the atomic motion, which makes this resource-efficient technique particularly interesting for cavity experiments with limited optical access.

Observation of the Dipole Blockade Effect in Detecting Rydberg Atoms by the Selective Field Ionization Method

The dipole blockade effect at laser excitation of mesoscopic ensembles of Rydberg atoms lies in the fact that the excitation of one atom to a Rydberg state blocks the excitation of other atoms due to the shift in the collective energy levels of interacting Rydberg atoms. It is used to obtain the entangled qubit states based on single neutral atoms in optical traps. In this paper, we present our experimental results on the observation of the dipole blockade for mesoscopic ensembles of 1-5 atoms when they are detected by the selective field ionization method. We investigated the spectra of the three-photon laser excitation $ 5S_{1/2} \to 5P_{3/2} \to 6S_{1/2} \to nP_{3/2} $ of cold Rb Rydberg atoms in a magneto-optical trap. We have found that for mesoscopic ensembles this method allows only a partial dipole blockage to be observed. This is most likely related to the presence of parasitic electric fields reducing the interaction energy of Rydberg atoms, the decrease in the probability of detecting high states, and the strong angular dependence of the interaction energy of Rydberg atoms in a single interaction volume.

Gray-Molasses Optical-Tweezer Loading: Controlling Collisions for Scaling Atom-Array Assembly

We show that with a purely blue-detuned cooling mechanism we can densely load single neutral atoms into large arrays of shallow optical tweezers. With this ability, more efficient assembly of larger ordered arrays will be possible - hence expanding the number of particles available for bottom-up quantum simulation and computation with atoms. Using Lambda-enhanced grey molasses on the D1 line of 87Rb, we achieve loading into a single 0.63 mK trap with 89% probability, and we further extend this loading to 100 atoms at 80% probability. The loading behavior agrees with a model of consecutive light-assisted collisions in repulsive molecular states. With simple rearrangement that only moves rows and columns of a 2D array, we demonstrate one example of the power of enhanced loading in large arrays.

Neutral-Atom Wavelength-Compatible 780 nm Single Photons from a Trapped Ion via Quantum Frequency Conversion

Quantum networks consisting of quantum memories and photonic interconnects can be used for entanglement distribution (L.-M.Duan and H. J. Kimble, PRL 90, 253601 (2003), H. J. Kimble, Nat. 453, 1023 EP (2008)), quantum teleportation (S.Pirandola et.al, Nat. Photon. 9, 641 (2015)), and distributed quantum computing (T.Spiller, et.al., New J. Phys. 8, 30 (2006). Remotely connected two-node networks have been demonstrated using memories of the same type: trapped ion systems (D.Hucul, et.al, Nat. Phys. 11, 37 (2014)), quantum dots (W. B. Gao et. al, Nat. Photon. 9, 363 (2015)), and nitrogen vacancy centers (W. B. Gao et. al, Nat. Photon. 9, 363 (2015), B. Hensen, et. al., Nat. 526, 682 (2015)). Hybrid systems constrained by the need to use photons with the native emission wavelength of the memory, have been demonstrated between a trapped ion and quantum dot (H.Meyer et.al PRL 114, 123001 (2015)) and between a single neutral atom and a Bose-Einstein Condensate (M.Lettner et. al, PRL 106, 210503 (2011)). Most quantum systems operate at disparate and incompatible wavelengths to each other so such two-node systems have never been demonstrated. Here, we use a trapped 138Ba$^{+}$ ion and a periodically poled lithium niobate (PPLN) waveguide, with a fiber coupled output, to demonstrate 19% end-to-end efficient quantum frequency conversion (QFC) of single photons from 493 nm to 780 nm. At the optimal signal-to-noise operational parameter, we use fluorescence of the ion to produce light resonant with the $^{87}$Rb $D_2$ transition. To demonstrate the quantum nature of both the unconverted 493 nm photons and the converted photons near 780 nm, we observe strong quantum statics in their respective second order intensity correlations. This work extends the range of intra-lab networking between ions and networking and communication between disparate quantum memories. A

Comparison of single-neutral-atom qubit between in bright trap and in dark trap**Project supported by the National Key Research and Development Program of China (Grant No. 2017YFA0304502) and the National Natural Science Foundation of China (Grant Nos. 11634008, 11674203, 11574187, and 61227902), and the Fund for Shanxi “1331 Project” Key Subjects Construction, Shanxi Province, China.

A single neutral atom is one of the most promising candidates to encode a quantum bit (qubit). In a real experiment, a single neutral atom is always confined in a micro-sized far off-resonant optical trap (FORT). There are generally two types of traps: red-detuned trap and blue-detuned trap. We experimentally compare the qubits encoded in “clock states” of single cesium atoms confined separately in either 1064-nm red-detuned (bright) trap or 780-nm blue-detuned (dark) trap: both traps have almost the same trap depth. A longer lifetime of 117 s and a longer coherence time of about 10 ms are achieved in the dark trap. This provides a direct proof of the superiority of the dark trap over the bright trap. The measures to further improve the coherence are discussed.

编码于单个中性原子的单量子比特的量子层析

编码于单个中性原子的单量子比特的量子层析

Experimental progress of quantum computation based on trapped single neutral atoms

As an important candidate for quantum simulation and quantum computation, a microscopic array of single atoms confined in optical dipole traps is advantageous in controlled interaction, long coherence time, and scalability of providing thousands of qubits in a small footprint of less than 1 mm<sup>2</sup>. Recently, several breakthroughs have greatly advanced the applications of neutral atom system in quantum simulation and quantum computation, such as atom-by-atom assembling of defect-free arbitrary atomic arrays, single qubit addressing and manipulating in two-dimensional and three-dimensional arrays, extending coherence time of atomic qubits, controlled-NOT (C-NOT) gate based on Rydberg interactions, high fidelity readout, etc.In this paper, the experimental progress of quantum computation based on trapped single neutral atoms is reviewed, along with two contributions done by single atom group in Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences. First, a magic-intensity trapping technique is developed and used to mitigate the detrimental decoherence effects which are induced by light shift and substantially enhance the coherence time to 225 ms which is 100 times as large as our previous coherence time thus amplifying the ratio between coherence time and single qubit operation time to 10<sup>5</sup>. Second, the difference in resonant frequency between the two atoms of different isotopes is used to avoid crosstalking between individually addressing and manipulating nearby atoms. Based on this heteronuclear single atom system, the heteronuclear C-NOT quantum gate and entanglement of an Rb-85 atom and an Rb-87 atom are demonstrated via Rydberg blockade for the first time. These results will trigger the quests for new protocols and schemes to use the double species for quantum computation with neutral atoms. In the end, the challenge and outlook for further developing the neutral atom system in quantum simulation and quantum computation are also reviewed.

Controlled doping of a bosonic quantum gas with single neutral atoms

We report on the experimental doping of a 87Rubidium (Rb) Bose–Einstein condensate (BEC) with individual neutral 133Cesium (Cs) atoms. We discuss the experimental tools and procedures to facilitate Cs-Rb interaction. First, we use degenerate Raman side-band cooling of the impurities to enhance the immersion efficiency for the impurity in the quantum gas. We identify the immersed fraction of Cs impurities from the thermalization of Cs atoms upon impinging on a BEC, where elastic collisions lead to a localization of Cs atoms in the Rb cloud. Second, further enhancement of the immersion probability is obtained by localizing the Cs atoms in a species-selective optical lattice and a subsequent transport into the Rb cloud. Here, impurity-BEC interaction is monitored by position and time-resolved three-body loss of Cs impurities immersed into the BEC. This combination of experimental methods allows for the controlled doping of a BEC with neutral impurity atoms, paving the way to impurity aided probing and coherent impurity-quantum bath interaction.