Simultaneous High-speed Imaging Research Articles

Laser-induced emission from iron oxide nanoparticles in spray-flame synthesis: in situ high-speed microscopy

Spray-flame synthesis uses low-cost precursors dissolved in organic solvents to produce functional metaloxide nanoparticles. In the spray flame, the precursor-laden droplets show frequent and intense thermally-induced disruption, so-called puffing and micro-explosion. This process is often correlated with high uniformity of particle sizes. Whether puffing and micro-explosion are also directly associated with the formation or release of iron oxide nanoparticles is not clear. Also, the spatiotemporal evolution of nanoparticles in the turbulent flow field of the flame is largely unknown from experiments. We performed simultaneous high-speed microscopic imaging of droplet shadowgraphs at 360 kHz as well as elastic light scattering (ELS) and laser-induced emission (LIE) of nanoparticles at 40 kHz. Comparing ELS and LIE images allows distinguishing signals from droplets, flame, and nanoparticles, as only the nanoparticles will appear in images from both methods. ELS and LIE show nanoparticles as thin narrow filaments, presumably following the local flow. Nanoparticle filaments are found at a height of 50 mm and more above the burner in the spray flame. The filaments show increasing LIE signal and higher confinement with increasing height above the burner. The appearance of LIE and thus nanoparticles does not directly correlate with the presence of droplets or their disruption.

Accelerated ignition-shock coupling and deflagration to detonation transition by ozone kinetic enhancement of dimethyl ether mixture

This study aims to understand the effect of kinetic enhancement by ozone addition on the Deflagration to Detonation Transition (DDT) and ignition-shock coupling in a microchannel using dimethyl ether (DME). Simultaneous high-speed chemiluminescence and shadowgraph imaging are carried out to analyze the flame front propagation, shock wave structures, autoignition, and ignition-shock coupling during the DDT process. The experimental results show that for all cases, with and without ozone kinetic enhancement, autoignition and DDT always occur in a reactivity gradient region with oblique shock cluster between the flame front and the flame acceleration-induced precursor shock. The observed DDT occurs via the Zeldovich hot spot gradient mechanism through the following stages: (1) Oblique shock cluster formation and acoustic compression between the flame front and the precursor shock, (2) autoignition initiation in the oblique shock cluster region, (3) spontaneous ignition wave propagation, and (4) ignition-shock coupling. It is found that autoignition location, oblique shock strength, induction zone length, ignition-shock coupling, and DDT onset flame velocity are very different from ozone kinetic enhancement. As the ozone addition is higher, the autoignition is advanced and the ignition location moves farther ahead of the flame front at a lower flame front propagation speed and weaker oblique shock clusters. Two different ignition-shock coupling modes are identified depending on ozone concentration. Without ozone kinetic enhancement, DDT occurs via ignition wave coupling with the precursor shock. However, ozone addition can accelerate the autoignition and initiate a direct ignition-shock coupling for DDT without interaction with the precursor shock. The present results show that kinetic enhancement in autoignition using an ignition enhancer such as ozone or plasma is critical and effective in accelerating and controlling DDT.

In vivo high-speed microscopy of microbubbles in the chorioallantoic membrane model.

Rationale: The acoustic stimulation of microbubbles within microvessels can elicit a spectrum of therapeutically relevant bioeffects from permeabilization to perfusion shutdown. These bioeffects ultimately arise from complex interactions between microbubbles and microvascular walls, though such interactions are poorly understood particularly at high pressure, due to a paucity of direct in vivo observations. The continued development of focused ultrasound methods hinges in large part on establishing links between microbubble-microvessel interactions, cavitation signals, and bioeffects. Methods: Here, a system was developed to enable simultaneous high-speed intravital imaging and cavitation monitoring of microbubbles in vivo in a chorioallantoic membrane model. Exposures were conducted using the clinical agent DefinityTM under conditions previously associated with microvascular damage (1 MHz, 0.5-3.5 MPa, 5 ms pulse length). Results: Ultrasound-activated microbubbles could be observed and were found to induce localized wall deformations that were more pronounced in smaller microvessels and increased with pressure. A central finding was that microbubbles could extravasate from microvessels (from 34% of vessels at 1 MPa to 79% at 3 MPa) during insonation (94% within 0.5 ms) and that this occurred more frequently and in progressively larger microvessels (up to 180 µm) as pressure was increased. Following microbubble extravasation, transient or sustained red blood cell leakage ensued at the extravasation site in 96% of cases for pressures ≥1 MPa. Conclusions: The results here represent the first high-speed in vivo investigation of high-pressure focused ultrasound-induced microbubble-microvessel interactions. This data provides direct evidence that the process of activated microbubble extravasation can occur in vivo and that it is linked to producing microvessel wall perforations of sufficient size to permit red blood cell leakage. The association of red blood cell leakage with microbubble extravasation provides mechanistic insight into the process of microvessel rupture, which has been widely observed in histology.

Development of Polyamine/Alkanolamine-based Hypergolics with hydrogen Peroxide: A new route to N-methylimidazole with MDEA as a promising green fuel

A novel non-ionic liquid fuel based on a mixture of N-methylimidazole (MIm) and N-methyldiethanolamine (MDEA) called PAHyp 2 which reacts hypergolically with hydrogen peroxide is presented in this work. To study the hypergolic behaviors, a drop test setup able of capturing simultaneous high-speed schlieren, infrared and visible imaging was used. While infrared images capture the temperature history of the ignition process, schlieren images offer advantages of capturing the pressure waves as well as providing better visualization of the morphological description of the liquid dynamics. PAHyp 2 with hydrogen peroxide has specific impulse 6% lower than hydrazine-based fuels but because of its higher density it requires smaller propellant tanks for a given mission. In order to meet the requirements of good chemical stability and low viscosity of<30 cP, the proportion of MIm should range between 40 and 50% (or 60 to 50% of MDEA) and the amount of catalyst should be no more than 3 wt%. FTIR spectra showed no chemical degradation. By adding 3 wt% catalyst, the shortest ignition delay time of 8.8 ms was recorded. Based on these preliminary results, we believe that just like the other polyamiane/akanolamine-based fuels recently reported by our group, this new recipe is also a promising candidate to replace conventional toxic propellants and as such should be further studied.

Chapman–Jouguet deflagration criteria and compressibility dynamics of turbulent fast flames for turbulence-induced deflagration-to-detonation transition

This work characterizes the compressibility dynamics in turbulent fast flames for a range of turbulent flame speeds. These turbulent fast flames experience increased effects of compressibility through the formation of strong shocks and may develop a runaway acceleration combined with a pressure buildup that leads to turbulence induced deflagration-to-detonation transition (tDDT). Simultaneous high-speed particle image velocimetry, OH* chemiluminescence, schlieren, and pressure measurements are used to examine the reacting flow field and flame dynamics. We examine flames with turbulent flame speeds ranging from 100 to 600 m/s. At lower turbulent flame speeds, the flame is not able to produce favorable background conditions for deflagration-to-detonation transition (DDT) onset, and thus flame compressibility and turbulence amplification are less dominant, resulting in a weaker acoustic coupling between the flame and compressed region. As the turbulent burning velocities exceed the Chapman–Jouguet deflagration speed, favorable background conditions are produced, as we observe flame-generated shocks and flame-generated turbulence with higher turbulent velocities and larger turbulent scales. At this regime, the flame is categorized to be at the runaway transition regime that leads to tDDT.

Simultaneous impact of droplet pairs on solid surfaces

This study investigates the dynamics of the simultaneous impact of two droplets on a dry substrate. We develop a new micro-controlled droplet generator that releases two equally sized water droplets simultaneously on-demand, with no trailing droplets. The impact Weber number, based on impact droplet size and velocity, and the inter-droplet spacing relative to the impact droplet size are varied in the ranges of 54 to 155 and 1.32 to 2.25, respectively, leading to the strong interaction of the spreading lamellae that form a central uprising sheet, which eventually deposits or breaks into tiny droplets. We analyse the impact processes for both deposition and splashing of the uprising sheets. Simultaneous high-speed imaging from two orthogonal views of the droplet impacts quantifies the three-dimensional structure of the sheet morphology, including the temporal evolution of the rim-bounded ‘semilunar’ shape, surface waves, rim corrugations and finger formation, and deposition or splashing of the liquid sheet. The characteristics of the sheet surface waves and the rim instabilities are quantified. Novel scaling is developed for the maximum sheet height, sheet width and thickness, which considers the geometrical constraints and mass balance of the interacting lamellae to describe the temporal evolution of a ‘semilunar’ uprising sheet and is in good agreement with the measurements. The uprising sheet splashing generates larger droplets than those from splashing of single-droplet impacts, and it occurs due to the end-pinching of sheet fingers and at conditions that single-droplet impacts lead only to liquid deposition.

High-speed low-light in vivo two-photon voltage imaging of large neuronal populations.

Monitoring spiking activity across large neuronal populations at behaviorally relevant timescales is critical for understanding neural circuit function. Unlike calcium imaging, voltage imaging requires kilohertz sampling rates that reduce fluorescence detection to near shot-noise levels. High-photon flux excitation can overcome photon-limited shot noise, but photobleaching and photodamage restrict the number and duration of simultaneously imaged neurons. We investigated an alternative approach aimed at low two-photon flux, which is voltage imaging below the shot-noise limit. This framework involved developing positive-going voltage indicators with improved spike detection (SpikeyGi and SpikeyGi2); a two-photon microscope ('SMURF') for kilohertz frame rate imaging across a 0.4 mm × 0.4 mm field of view; and a self-supervised denoising algorithm (DeepVID) for inferring fluorescence from shot-noise-limited signals. Through these combined advances, we achieved simultaneous high-speed deep-tissue imaging of more than 100 densely labeled neurons over 1 hour in awake behaving mice. This demonstrates a scalable approach for voltage imaging across increasing neuronal populations.

Experimental Investigation of a Cylindrical Air-Breathing Continuous Rotating Detonation Engine with Different Nozzle Throat Diameters

A continuous detonation engine with various exhaust nozzles, analogous to typical scramjet cavity combustors with variable rear-wall heights, was adopted to perform a succession of cylindrical air-breathing continuous rotating detonation experiments fueled by a non-premixed ethylene/air mixture. The results show that the detonation combustion was observed to self-sustain in the combustor through simultaneous high-speed imaging covering the combustor and isolator. A long test, lasting more than three seconds, was performed in this unique configuration, indicating that the cylindrical isolator–combustor engine exhibits potential for practical applications. Three distinct combustion modes were revealed with varied equivalent ratios (hybrid mode, sawtooth wave mode, and deflagration mode). The diameter of the nozzle throat was critical in the formation of rotating detonation waves. When the nozzle throat diameter was larger than the specific value, the detonation wave could not form and self-sustain. The upstream boundary of the shock train was supposed to be close to the isolator entrance in conditions of a high equivalence ratio and small nozzle throat diameter. In addition, it was verified that periodic high-frequency pressure oscillation could cause substantial impacts on the incoming flow as compared with the steady deflagration with the same combustor pressure.

Characterization of flow field and combustion dynamics in a novel pressurized side-wall quenching burner using high-speed PIV/OH-PLIF measurements

A novel, pressurized side-wall quenching (SWQ) burner test rig enabling investigations on flame-wall interactions (FWI) of a fully premixed V-shaped flame at conditions mimicking some characteristics of practical devices, e.g. increased pressures and Reynolds numbers, is introduced within this study. Two operating cases featuring turbulent flow conditions at atmospheric and 3 bar operating pressure are defined and characterized based on velocity fields and flame front positions provided by simultaneous high-speed particle image velocimetry (PIV) and planar laser-induced fluorescence of the OH radical (OH-PLIF). For non-reacting conditions, profiles of mean velocities and mean velocity fluctuations are measured in addition to near-wall flow fields at locations where FWI occurs for chemically reacting conditions. For reacting conditions, near-wall flows are characterized in the vicinity of the quenching zone. Based on measured fluctuations of the streamwise velocity component, the turbulent flame is classified at the transition from the wrinkled to the corrugated flamelet regime. Using the derived flame front positions, the instantaneous flame-wall interaction is classified into SWQ-like, head-on quenching (HOQ)-like and multi-zone quenching events and the transition between these scenarios is identified by means of OH-PLIF image sequences. A statistical analysis of the flame front topology is performed based on the flame brush and deduced frequency distributions. Statistically significant differences between both operating cases are confirmed by chi-squared homogeneity tests.

Simultaneous multiple laser beam intensity profile correction and its application to a vitiated bluff body combustor field.

Simultaneous high-speed stereo-particle image velocimetry, OH planar-laser-induced fluorescence (PLIF), and CH2O PLIF measurements in a vitiated bluff body combustor are considered. An ex situ, simultaneous, time-resolved laser sheet intensity profile correction procedure is introduced. This procedure is easily implemented experimentally and is capable of correcting multiple sheets at the same time. As a proof of concept, the procedure is applied to perform correction of the CH2O PLIF images in vitiated and unvitiated conditions. The challenges associated with CH2O PLIF under these combustor operating conditions are also discussed.

Spontaneous runaway of fast turbulent flames for turbulence-induced deflagration-to-detonation transition

One of the fundamental mechanisms for detonation initiation is deflagration-to-detonation transition (DDT). This research experimentally explores the runaway condition for highly turbulent fast flames before DDT, which are characterized by extremely high turbulent flame speeds. Such fast turbulent flames experience increased effects of compressibility and may develop a runaway acceleration combined with a pressure buildup that leads to a turbulence-induced DDT (tDDT) mechanism that has been recently reported. The flame dynamics and the associated reacting flow field are characterized using simultaneous high-speed particle image velocimetry, OH* chemiluminescence, pressure measurements, and schlieren imaging. We study the flow-field conditions for runaway acceleration of fast turbulent flames and effects of compressibility on the evolution of these flames. The locally measured turbulent flame speed is found to be greater than that of a Chapman–Jouguet deflagration speed, which places the flame in the runaway transition regime that would eventually lead to a detonation.

High-speed ultrasound imaging of laser-induced cavitation bubbles

While ultrasound and cavitation based therapies have mushroomed over the years, there is a lack of online monitoring of the cavitation bubble dynamics in biological tissue. Here, we demonstrate that with ultrasonic plane wave imaging, the fast dynamics of single cavitation bubbles can be resolved non-invasively in a tissue mimicking material. Due to the high contrast of bubbles, plane wave compounding is not necessary and the frame rates of up to 74 kHz can been achieved with a research grade ultrasound scanner. Comparison with simultaneous high-speed imaging demonstrates excellent agreement of both measurement modalities in water and in a tissue mimicking material.

Multi-parameter imaging of in-cylinder processes during transient engine operation for the investigation of soot formation

Transient engine operation of direct-injection spark ignition engines can result in high particulate number emissions. To investigate the causes of soot formation, an engine test rig was developed to perform detailed measurements of real transient operation. For this purpose, a single-cylinder full-metal engine with a real combustion chamber geometry was equipped with minimally invasive optical accesses. Simultaneous high-speed endoscopic PIV, spray visualization, and combustion imaging were applied to investigate the in-cylinder processes in detail. Endoscopic PIV was first compared in the central symmetry plane with classical PIV performed at the equivalent optical engine at steady-state operation for verification. Then the engine parameters of a tip-in performed by the corresponding four-cylinder engine, which led to high particle number emissions, were applied to the single-cylinder engine. The engine parameters were in a good agreement and particle number emissions due to the maneuver were within the same range of several 106 #/cm3. In total, 19 repetitions of the tip-in maneuver were analyzed with respect to the in-cylinder processes and repeatability of engine parameters. Furthermore, the in-cylinder flow field during the late compression stroke, flame propagation, and soot luminosity of single cycles during the tip-in indicated cause-and-effect chains for the formation of pool fire and soot at the injector tip. The direction of the flow below the spark plug influenced the direction of flame propagation. An early arrival of the flame enhanced the formation of soot from fuel films formed on the piston surface or at the injector. In engine applications, counter measures can be applied to reduce the particle number emissions when accounting for these indicated cause-and-effect chains.

Turbulence-Driven Blowout Instabilities of Premixed Bluff-Body Flames

Bluff-body flame instabilities are experimentally investigated under varying turbulence conditions during lean blowout. For all turbulence conditions, the blowout process is induced through a temporal reduction of the fuel flow rate to capture the flame-flow dynamics approaching blowout. Simultaneous high-speed particle image velocimetry (PIV), stereoscopic PIV, and C2*/CH* chemiluminescence imaging are employed, along with an independent CH* imaging system, to capture flame-flow instabilities. Proper orthogonal decomposition (POD) and dynamic mode decomposition (DMD) techniques are used to identify prominent flame oscillations and evaluate recurring spatiotemporal modes during blowout. The results reveal that the dominant flame oscillations and wrinkling characteristics are directly dependent on the turbulence conditions in the combustor. Specifically, the flame-flow oscillations are strongly coupled with the integral length scales, which were able to collapse the oscillation frequencies to a unified value. The turbulence-driven flame-flow oscillations are shown to largely impact the magnitude, temporal evolution, and oscillatory behavior of the flame strain rate. As the turbulence intensity is increased, the oscillation of the flame strain rate increases in frequency, making it more likely for localized extinctions to occur. Additionally, the magnitude of the flame strain rate increases at high turbulence intensities and accelerates the lean blowout process.

Airfoil flow receptivity to simulated tonal noise emissions

On airfoils at low to moderate Reynolds numbers, trailing edge sound can have a feedback effect on the development of instability waves resulting in strongly periodic vortex shedding and tonal noise. This complex problem is decoupled in this study to investigate the flow response to deterministic noise emissions. The flow receptivity and response to tonal noise are examined using controlled steady and transient acoustic excitation. Experiments are performed on a NACA 0018 airfoil at a Reynolds number of 1.15×105 and an angle of attack of 5°, with a separation bubble on the suction side. Controlled acoustic perturbations are introduced via a loudspeaker. A combination of mean and time-resolved surface pressure and simultaneous high-speed particle image velocimetry measurements provides insight into the response of the bubble to simulated acoustic forcing. Amplification of shear layer perturbations in the fore portion of the separation bubble is observed only after some time delay from the onset of acoustic forcing. This places the receptivity region within the boundary layer upstream of the separation bubble, extending from the leading edge to just downstream of the suction peak. The acoustically excited perturbations in the receptivity region attain higher amplitudes than natural disturbances and are amplified significantly in the separation bubble, leading to a transient reduction in the separation bubble size. Results elucidate the ensuing transient response of the separation bubble, illustrating the flow dynamics expected during the initiation of the acoustic feedback loop during natural tonal noise emissions on an airfoil.

The effects of turbulence and pressure gradients on vorticity transport in premixed bluff-body flames

The current study experimentally evaluates the effects of turbulence and pressure gradients on vorticity transport in premixed bluff-body flames. The flow field pressure gradient is modified using a variable-geometry test section. In tandem, a custom-designed turbulence generator is used to modulate the turbulence intensity in the test section. The objective of the combined pressure gradient and turbulence tailoring is to alter the balance between the individual terms of the vorticity transport equation and ultimately identify the subsequent impacts on the overall behavior of the flame and flow field. Simultaneous high-speed particle image velocimetry and CH* chemiluminescence are employed to measure the turbulent reacting flow field. The vorticity dynamics are analyzed using a mean, conditionally filtered, fluid element tracking method to calculate individual terms of the vorticity transport equation as fluid elements evolve across the flame front. The analysis shows that increasing the pressure gradient increases the reacting vorticity production for all vorticity terms. In contrast, the overall vorticity budget, or relative contribution of each vorticity term, is much more sensitive to turbulence effects. At low turbulence conditions, vorticity is dominated by baroclinic torque, regardless of the pressure gradient. As the turbulence intensity is increased, the exothermic effects of baroclinicity and dilatation are diminished, and the reacting flow field approaches that of a non-reacting turbulent flow. The relative balance of vorticity transport terms is shown to influence the overall flow field, as well as the structure and evolution of the flame front.

Transverse Acoustic Forcing of Gaseous Hydrogen/Liquid Oxygen Turbulent Shear Coaxial Flames

Gaseous hydrogen/liquid oxygen turbulent shear coaxial flames were subjected experimentally to both pressure antinode (PAN) and pressure node (PN) transverse acoustic forcing as a function of the gas-to-liquid momentum flux ratio. The response of the flow was recorded using simultaneous high-speed imaging of backlit shadowgraphs and chemiluminescence emission. It was observed that a wave amplification mechanism, defined in Sec. III, previously observed for unforced flows, remained present in the forced flows but was modified by the forcing. The response tended to be axisymmetric for PAN forcing, where the pressure fluctuations are symmetric, and asymmetric for PN forcing, where the velocity fluctuations are asymmetric. Additional analyses performed included dynamic mode decomposition (DMD) and an analysis of the wave trajectories as a function of time. Beyond the main observation that the wave amplification mechanism remained operative not only for unforced flows but also for both kinds of transverse forcing, secondary observations included a greater relative effect on the flow for PN forcing than for PAN forcing and a reduced general response of the flow to the acoustics at higher momentum flux ratios. The velocity of waves observed in the emission were found to depend mainly on the shear layer velocity and not directly on the acoustics.

Detailed measurements of transient two-stage ignition and combustion processes in high-pressure spray flames using simultaneous high-speed formaldehyde PLIF and schlieren imaging

This study investigates the low- and high-temperature ignition and combustion processes in a high-pressure spray flame of n-dodecane using simultaneous 50-kHz formaldehyde (HCHO) planar laser-induced fluorescence (PLIF) and 100-kHz schlieren imaging. The PLIF measurements were facilitated through the use of a pulse-burst-mode Nd:YAG laser, producing a 355-nm pulse-train with 300 pulses at 70 mJ/pulse, separated by 20-µs, in a 6-ms burst. The high-speed HCHO PLIF signal was imaged using a non-intensified CMOS camera with dynamic background emission correction. The acquisition rate of this HCHO PLIF diagnostic is unique to the research community, and when combined with high-speed schlieren imaging, provides unprecedented opportunity for analysis of the spatiotemporal evolution of fuel jet penetration and low- and high-temperature ignition processes relevant to internal combustion engine conditions. The present experiments are conducted in the Sandia constant-volume preburn vessel equipped with a new Spray A injector. The influences of ambient conditions are examined on the ignition delay times of the two-stage ignition events, HCHO structures, and lift-off length values. Consistent with past studies of traditional Spray A flames, the formation of HCHO is first observed in the jet peripheries where the equivalence ratio (Φ) is expected to be leaner and hotter and then grows in size and in intensity downstream into the jet core where Φ is expected to be richer and colder. The measurements demonstrate that the formation and propagation of HCHO from the leaner to richer region leads to high-temperature ignition events, supporting the identification of a phenomenon coined “cool-flame wave propagation” during the transient ignition process. Subsequent high-temperature ignition is found to consume the previously formed HCHO in the jet head, while the formation of HCHO persists in the fuel-rich zone near the flame base over the entire combustion period.

Turbulent flame-vortex dynamics of bluff-body premixed flames

Abstract To better understand the coupled dynamics of turbulence and premixed flames, this study experimentally investigates the effects of turbulence on reacting vorticity dynamics. In this investigation, a bluff-body stabilized, turbulent, premixed flame is analyzed in a high-speed combustor. A custom-designed turbulence generator is used to vary the inflow turbulence conditions and understand the subsequent impacts on the flame-flow field. The turbulent reacting flow-field is measured using simultaneous high-speed particle imaging velocimetry (PIV) and CH* chemiluminescence. A Lagrangian tracking method is implemented to study flame-vortex dynamics. Lagrangian fluid elements are tagged from the experimental data and are tracked as they convect through the flame, from reactants to products. The components of the vorticity transport equation are decomposed along the Lagrangian trajectories to determine their relative balance under various turbulence conditions. The results confirm that altering the turbulence intensity influences flame-vortex interactions and the relative balance of the vorticity components. At high turbulence intensities, the baroclinic torque and dilatation decrease, while the magnitude of viscous diffusion increases, and vortex stretching dominates the reacting flow field. These results suggest that increasing the turbulence intensity alters the dominant physical processes in the reacting domain as the combustion-driven phenomena become less significant.

Dual-camera high-speed imaging of the ignition modes of ethanol, methanol and n-hexane in a shock tube

Shock tubes are used as homogeneous batch reactors to measure ignition delay times, reaction rate coefficients and species time-histories of a variety of chemical systems. Any non-ideality or inhomogeneity in the shock tube experiment would affect the quality and usefulness of measured data. Experimental and computational efforts have previously been carried out to characterize the regimes of ideal operation of shock tubes. High-speed imaging has proven to be a highly useful tool to assess ignition homogeneity. In this work, a dual-camera setup has been used with an optical end-section in a circular shock tube to obtain simultaneous high-speed images from the shock tube endwall and sidewall, thus providing visualization of the ignition phenomenon in three dimensions. Two case studies are presented herein to demonstrate the quality of data and insights that are obtained using this diagnostic technique to study the ignition modes of different fuels. The first is a comparison of the ignition of two alternative fuels, methanol and ethanol, and the second is a study of the ignition dependence on the fuel concentration of a representative paraffinic fuel, n-hexane. The unique dual-camera imaging diagnostic enabled deeper insights into the ignition homogeneity, with all fuels exhibiting localized ignition at low temperatures. Methanol showed a higher propensity than ethanol to ignite far from the endwall, and the high concentration of n-hexane led to inhomogeneous ignition.