With the increasing penetration rate of distributed power supply, the interaction between grid-connected inverters and power grid is prone to harmonic oscillation, which will seriously threaten the stable operation of power grid. At present, impedance analysis has been proved to be an effective tool to study the stability of grid-connected systems. However, few studies have considered the influence of frequency coupling effect on the output impedance characteristics of grid-connected inverters. To solve this problem, the sequence impedance model of a three-phase grid-connected inverter controlled by a virtual synchronous generator is established by harmonic linearization method based on the frequency coupling effect. In addition, an improved method of sequence impedance modeling based on grid impedance is proposed to effectively eliminate the influence of coupling terms. Finally, the correctness and practicability of the proposed simplified sequence impedance model are verified by simulation and experiment.