Self-seeded Free-electron Laser Research Articles

Cascaded hard X-ray self-seeded free-electron laser at megahertz repetition rate

AbstractHigh-resolution X-ray spectroscopy in the sub-nanosecond to femtosecond time range requires ultrashort X-ray pulses and a spectral X-ray flux considerably larger than that presently available. X-ray free-electron laser (XFEL) radiation from hard X-ray self-seeding (HXRSS) setups has been demonstrated in the past and offers the necessary peak flux properties. So far, these systems could not provide high repetition rates enabling a high average flux. We report the results for a cascaded HXRSS system installed at the European XFEL, currently the only operating high-repetition-rate hard X-ray XFEL facility worldwide. A high repetition rate, combined with HXRSS, allows the generation of millijoule-level pulses in the photon energy range of 6–14 keV with a bandwidth of around 1 eV (corresponding to about 1 mJ eV–1 peak spectral density) at the rate of ten trains per second, each train including hundreds of pulses arriving at a megahertz repetition rate. At 2.25 MHz repetition rate and photon energies in the 6–7 keV range, we observed and characterized the heat-load effects on the HXRSS crystals, substantially altering the spectra of subsequent X-ray pulses. We demonstrated that our cascaded self-seeding scheme reduces this detrimental effect to below the detection level. This opens up exciting new possibilities in a wide range of scientific fields employing ultrafast X-ray spectroscopy, scattering and imaging techniques.

Self-seeded free-electron lasers with orbital angular momentum

X-ray beams carrying orbital angular momentum (OAM) are an emerging tool for probing matter. Optical elements, such as spiral phase plates and zone plates, have been widely used to generate OAM light. However, due to the high impinging intensities, these optics are challenging to use at X-ray free-electron lasers (XFELs). Here, we propose a self-seeded free-electron laser (FEL) method to produce intense X-ray vortices. Unlike passive filtering after amplification, an optical element will be used to introduce the helical phase to the radiation pulse in the linear regime, significantly reducing thermal load on the optical element. The generated OAM pulse is then used as a seed and significantly amplified. Theoretical analysis and numerical simulations demonstrate that the power of the OAM seed pulse can be amplified by more than two orders of magnitude, reaching peak powers of several tens of gigawatts. The proposed method paves the way for high-power and high-repetition-rate OAM pulses of XFEL light.

Reverse taper enhanced harmonic lasing for seeding an X-ray free-electron laser

The recent development of high repetition-rate free-electron laser (FEL) facility has brought new challenges for the self-seeding scheme, mainly the problems of heat load and radiation damage on the monochromator. In this paper, a simple technique is proposed to mitigate the effect of heat-load on the monochromator of a self-seeding FEL. We combine the reverse undulator taper with the harmonic lasing technique to enhance the spectral brightness of the radiation pulse. In this way, the required radiation power for the first stage of self-seeding can be significantly reduced. Theoretical analysis and numerical simulation at 2.86 nm are performed and the results demonstrate that the proposed method can decrease the heat-load on the monochromator by nearly one order of magnitude. At the same time, the peak power of final radiation can be enhanced and the total length of undulator can be reduced comparing with the conventional self-seeding. The proposed technique can be implemented at current existing FEL facilities with variable-gap undulators.

Enhanced Self-Seeding with Ultrashort Electron Beams.

We describe a new method to produce intensity stable, highly coherent, narrow-band x-ray pulses in self-seeded free electron (FEL) lasers. The approach uses an ultrashort electron beam to generate a single spike FEL pulse with a wide coherent bandwidth. The self-seeding monochromator then notches out a narrow spectral region of this pulse to be amplified by a long portion of electron beam to full saturation. In contrast to typical self-seeding where monochromatization of noisy self-amplified spontaneous emission pulses leads to either large intensity fluctuations or multiple frequencies, we show that this method produces a stable, coherent FEL output pulse with statistical properties similar to a fully coherent optical laser.

Laguerre-Gaussian Mode Laser Heater for Microbunching Instability Suppression in Free-Electron Lasers.

Microbunching instability (MBI) driven by beam collective effects is known to be detrimental to high-brightness storage rings, linacs, and free-electron lasers (FELs). One known way to suppress this instability is to induce a small amount of energy spread to an electron beam by a laser heater. The distribution of the induced energy spread greatly affects MBI suppression and can be controlled by shaping the transverse profile of the heater laser. Here, we present the first experimental demonstration of effective MBI suppression using a LG_{01} transverse laser mode and compare the improved results with respect to traditional Gaussian transverse laser mode at the Linac Coherent Light Source. The effects on MBI suppression are characterized by multiple downstream measurements, including longitudinal phase space analysis and coherent radiation spectroscopy. We also discuss the role of LG_{01} shaping in soft x-ray self-seeded FEL emission, one of the most advanced operation modes of a FEL for which controlled suppression of MBI is critical.

Statistical theory of a self-seeded free electron laser with noise pedestal growth

We study the impact of a spectral noise pedestal on the statistical properties of a self-seeded free electron laser (FEL). The broad pedestal is assumed to come from self amplified spontaneous emission (SASE) in the second stage of the self-seeding system and is uncorrelated with the narrowband amplified seed. An analytic description is developed based on the statistical theory of a one-dimensional FEL in the high gain linear regime. The theory shows good agreement with experimental data, which show that the presence of a SASE background can have a strong impact on the statistical behavior of self-seeding systems.

The seed energy fluctuation of hard X-ray self-seeding free electron laser

Self-seeding free electron lasers (FELs) are capable of generating fully coherent X-ray pulses. However, the stability of output pulse energy of hard X-ray self-seeding (HXRSS) FEL is poor. This letter reports the seed energy stability investigation of HXRSS FEL. For the purpose of a more stable HXRSS FEL, this work suggests a relatively broad bandwidth ρt of crystal monochromator, a relatively long electron bunch with energy jitter (r.m.s.) down to a quarter of FEL Pierce parameter ρ, and a larger Bragg angle θB to improve the seed energy stability. Moreover, the angle jitter (r.m.s.) between the SASE pulse incident direction and the crystal surface should be less than (ρ tan θB)/2, and the relative time jitter (r.m.s.) between the electron bunch and the seed should be less than half of the seed bump duration Tt.

BRIGHT: the three-dimensional X-ray crystal Bragg diffraction code

In pursuit of a fully coherent X-ray free-electron laser (FEL), highly reflective Bragg crystals are used and will be used as a highly selective spectral filter in hard X-ray self-seeding FELs and X-ray FEL oscillators (XFELO), respectively. However, currently, when simulating self-seeding and XFELO, the three-dimensional effect of Bragg diffraction is not fully considered. In this paper, we derive a comprehensive solution for the response function of the crystal in Bragg diffraction. A three-dimensional X-ray crystal Bragg diffraction code, named BRIGHT, is introduced, which can be combined with other FEL-related codes, e.g., GENESIS and OPC. Performance and feasibility are assessed using two numerical examples, namely a self-seeding experiment for the linac coherent light source and XFELO options for Shanghai high repetition rate XFEL. The results indicate that BRIGHT provides a new and useful tool for three-dimensional modeling of FEL.

Soft X-ray harmonic lasing self-seeded free electron laser at Pohang Accelerator Laboratory X-ray free electron laser

The demonstration of a harmonic lasing self-seeded free-electron laser (HLSS FEL) scheme in the soft X-ray range at the Pohang Accelerator Laboratory X-ray Free Electron Laser is presented. We report the experimental results of HLSS FEL radiation with the shortest wavelength of 1 nm by using the optimized phase shift of 2/3π. The key feature of the HLSS scheme is that the mode number is decreased (the longitudinal coherence length is enhanced) which is directly observed using a single-shot spectrometer. The spectral brightness is enhanced by a factor of 1.7 compared to the self-amplified spontaneous emission FEL because of the narrowed bandwidth. Our results show a good agreement with the theoretical expectation and simulations. The HLSS mode is a promising standard operation mode to generate a stable and high-brightness X-ray FEL that will provide more benefits to users for various applications.

Eliminating the microbunching-instability-induced sideband in a soft x-ray self-seeding free-electron laser

Soft x-ray self-seeding has been proved to be a feasible method to improve the longitudinal coherence of high gain free-electron laser. However, a pedestal-like sideband in the spectrum has been observed in the experiment, which generally limits the purity of the radiation pulse and the user’s application. The previous theoretical study indicates that the pedestal-like sideband is mainly induced by microbunching instability generated from LINAC. In this paper, three dimensional simulations have been performed to confirm the analytical results and show the formation process of the spectral sideband. A probable method is proposed to eliminate the pedestal-like sideband by simply inserting a magnetic chicane before the self-seeding FEL undulator. Theoretical and numerical simulations have been performed and the results show that the proposed method can efficiently eliminate the microbunching-instability-induced sideband in a soft x-ray self-seeding FEL.

Extending the photon energy coverage of an x-ray self-seeding FEL via the reverse taper enhanced harmonic generation technique

In this paper, a simple method is proposed to extend the photon energy range of a soft x-ray self-seeding free-electron laser (FEL). A normal monochromator is first applied to purify the FEL spectrum and provide a coherent seeding signal. This coherent signal then interacts with the electron beam in the following reverse tapered undulator section to generate strong coherent microbunchings while maintain the good quality of the electron beam. After that, the pre-bunched electron beam is sent into the third undulator section which resonates at a target high harmonic of the seed to amplify the coherent radiation at shorter wavelength. Three dimensional simulations have been performed and the results demonstrate that the photon energy gap between 1.5keV and 4.5keV of the self-seeding scheme can be fully covered and 100GW-level peak power can be achieved by using the proposed technique.

First operation of a harmonic lasing self-seeded free electron laser

Harmonic lasing is a perspective mode of operation of X-ray FEL user facilities that allows to provide brilliant beams of higher energy photons for user experiments. Another useful application of harmonic lasing is so called Harmonic Lasing Self-Seeded Free Electron Laser (HLSS FEL) that allows to improve spectral brightness of these facilities. In the past, harmonic lasing has been demonstrated in the FEL oscillators in infrared and visible wavelength ranges, but not in high-gain FELs and not at short wavelengths. In this paper we report on the first evidence of the harmonic lasing and the first operation of the HLSS FEL at the soft X-ray FEL user facility FLASH in the wavelength range between 4.5 nm and 15 nm. Spectral brightness was improved in comparison with Self-Amplified Spontaneous emission (SASE) FEL by a factor of six in the exponential gain regime. A better performance of HLSS FEL with respect to SASE FEL in the post-saturation regime with a tapered undulator was observed as well. The first demonstration of harmonic lasing in a high-gain FEL and at short wavelengths paves the way for a variety of applications of this new operation mode in X-ray FELs.

Self-seeded FEL wavelength extension with high-gain harmonic generation

We study a self-seeded high-gain harmonic generation (HGHG) free-electron laser (FEL) scheme to extend the wavelength of a soft X-ray FEL. This scheme uses a regular self-seeding monochromator to generate a seed laser at the wavelength of 1.52 nm, followed by a HGHG configuration to produce coherent, narrow-bandwidth harmonic radiations at the GW level. The 2nd and 3rd harmonic radiation is investigated with start-to-end simulations. Detailed studies of the FEL performance and shot-to-shot fluctuations are presented.

Generation of subterawatt-attosecond pulses in a soft x-ray free-electron laser

We propose a novel scheme to generate attosecond soft x rays in a self-seeded free-electron laser (FEL) suitable for enabling attosecond spectroscopic investigations. A time-energy chirped electron bunch with additional sinusoidal energy modulation is adopted to produce a short seed pulse through a self-seeding monochromator. This short seed pulse, together with high electron current spikes and a cascaded delay setup, enables a high-efficiency FEL with a fresh bunch scheme. Simulations show that using the Linac Coherent Light Source (LCLS) parameters, soft x-ray pulses with a FWHM of 260 attoseconds and a peak power of 0.5 TW can be obtained. This scheme also has the feature of providing a stable central wavelength determined by the self-seeding monochromator.

Experimental demonstration of a soft x-ray self-seeded free-electron laser.

The Linac Coherent Light Source has added a self-seeding capability to the soft x-ray range using a grating monochromator system. We report the demonstration of soft x-ray self-seeding with a measured resolving power of 2000-5000, wavelength stability of 10(-4), and an increase in peak brightness by a factor of 2-5 across the photon energy range of 500-1000 eV. By avoiding the need for a monochromator at the experimental station, the self-seeded beam can deliver as much as 50-fold higher brightness to users.

An analysis of undulator optimization in self-seeding free electron lasers

A simple analysis is given for the optimum length of undulator in a self-seeding free electron laser (FEL). The obtained relations show the correlation between the undulator length and the system parameters. The power required for the seeding in the second part of the undulator and the overall efficiency of monochromatizating the seeding determine the length of the first part of the undulator; the magnitude of seeding power dominates the length of the second part of the undulator; the whole length of the undulator in a self-seeding FEL is determined by the overall efficiency for getting coherent seed, and is about half as long again as that of SASE, not including the dispersion section. The requirement of the dispersion section strength is also analyzed.

Physical design of a wavelength tunable fully coherent VUV source using a self-seeding free electron laser

In order to meet the requirements of the synchrotron radiation users, a fully coherent VUV free electron laser (FEL) has been preliminarily designed. One important goal of this design is that the radiation wavelength can be easily tuned in a broad range (70–170 nm). In the light of the users' demand and our actual conditions, the self-seeding scheme is adopted for this proposal. Firstly, we attempted to fix the electron energy and only changed the undulator gap to vary the radiation wavelength; however, our analysis implies that this is difficult because of the great difference of the power gain length and FEL efficiency at different wavelengths. Therefore, we have considered dividing the wavelength range into three subareas. In each subarea, a constant electron energy is used and the wavelength tuning is realized only by adjusting the undulator gap. The simulation results show that this scheme has an acceptable performance.

Comparative study of nonideal beam effects in high gain harmonic generation and self-seeded free electron lasers

In this paper we investigate and compare the properties of two narrow-bandwidth free-electron laser (FEL) schemes, one using self-seeding and the other high gain harmonic generation (HGHG). The two systems have been thoroughly studied analytically and numerically in the past. The aim of this work is to compare their performances when the FEL is driven by an electron beam with nonideal properties, thus including effects such as shot-to-shot energy fluctuations and nonlinear energy chirp. In both cases nonlinearities produce a bandwidth larger than the Fourier transform limited value. However, our analysis indicates that, for approximately the same output power levels, the self-seeding scheme is less affected than the HGHG scheme by quadratic energy chirps in the electron beam longitudinal phase space. This is confirmed by a specific numerical example corresponding to SPARX parameters where the electron beam was optimized to minimize the FEL gain length. The work has been carried out with the aid of the time dependent FEL codes GENESIS 1.3 (3D) and PERSEO (1D).