The support structure of deep buried tunnel often encountered bias load of during construction in weak layered strata. This paper studied the support structure failure behavior and surrounding rock deformation mechanism with Wuduxi Tunnel as an engineering case. The tunnel presents the damge phenomenons such as primary support cracking, steel arch distortion, secondary lining sidewall extrusion under asymmetrical load and high geostress. Firstly, the laboratory test was producted to research the engineering characteristics of the broken phyllite. The field test results show that the surrounding rock pressure is unevenly distributed around the tunnel, the primary support is all under pressure and the secondary lining is partial in tension. The surrounding rock pressure distribution shows an ellipsoidal distribution consistent with the trend of the rock stratum. The maximum vault settlement and horizontal convergence are 165.58 mm and 282.56 mm, respectively, and the convergence rate is far more than the stable deformation rate in the specification, which proves that the existing specification is not applicable to the large deformation deep buried bias highway tunnel with soft rock. Furthermore, the construction methods of “double primary support-secondary lining” are proposed to control the large deformation of surrounding rock. The field test is carried out to verify the feasibility of the double layer primary support. The field test show that the large deformation can be effectively controlled, and the support structure was stable without crack and damage, which ensured the construction safety of the deep buried bias tunnel in broken phyllite.