The morphology and material characteristics of uranium dendrites that have been electrochemically separated in a LiCl-KClUCl3 (1 wt% U) molten salt system—by varying (1) an applied overpotential to the electrolytic cell, (2) a submerged cathode area, and (3) an allotted time for dendrite growth—are being investigated. By applying cyclic voltammetry (CV) and open-circuit potentiometry (OCP) techniques, the submerged cathode area in the molten salt system and the equilibrium potential of the electrolytic cell were found, respectively. A scanning electron microscope with energy dispersive x-ray spectroscopy (SEM-EDS) capability was used to study the morphological growth patterns and analyze the surface elemental composition of the samples for each parameter. Portions of the samples were used to perform inductively coupled plasma mass spectrometry (ICP-MS) to analyze for volumetric elemental composition for occulated salt impurities in the uranium dendrites carried over by the electrochemical separation technique. Any remaining sample material from SEMEDS and ICP-MS was used to perform x-ray diffraction (XRD) to study crystallography effects of impurities. In brief, the morphologies found at the lowest overpotential of 25 mV exhibit a coarse, rhomboidal, leaf-like geometry with severe porosity and pitting. At 50 mV, the pitting appears to have decreased and the morphology exhibits stem-and-leaf or stem-and-bulb orientations. The morphology of the higher overpotentials (100 mV, 200 mV) are very similar to that of the 50 mV, but also seem to be much more random and chaotic in orientation, with an increase in pitting and porosity from the 50 mV samples. Preliminary results also show that residual ternary salt does not play a factor in the impurity of the uranium dendrite crystals.